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Graphene Cryogel Papers With Enhanced Mechanical Strength For High Performance Lithium Battery Anodes, Kewei Shu, Caiyun Wang, Meng Wang, Chen Zhao, Gordon G. Wallace

Faculty of Science, Medicine and Health - Papers: part A

A porous graphene paper was prepared by pressing a graphene cryogel, followed by thermal reduction at 220 °C. The cryogel was formed by freeze-drying a solution containing chemically reduced graphene and graphene oxide (CRG/GO). The formed graphene cryogel papers deliver a much higher discharge capacity and rate capability than that from conventional graphene papers fabricated by filtration. These new structures have a discharge capacity higher than 400 mA h g−1 at a current density of 2000 mA g−1 in sharp contrast to 229 mA h g−1 at 50 mA g−1 obtained from conventional graphene papers. These greatly improved electrochemical properties …