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Full-Text Articles in Physical Sciences and Mathematics
Ultrafast Intense-Field Photoionization And Photofragmentation Of Systematic Series Of Substituted Organic Molecules, Timothy D. Scarborough
Ultrafast Intense-Field Photoionization And Photofragmentation Of Systematic Series Of Substituted Organic Molecules, Timothy D. Scarborough
Department of Physics and Astronomy: Dissertations, Theses, and Student Research
The abundance and relevance of organic molecules similar to benzene makes their study important. Studying the interactions of such molecules with intense light fields has implications for the generation of short-wavelength radiation, attosecond science, high-harmonic generation, and many other fields. However, the computing power necessary to complete fully ab initio calculations describing molecules of this size does not exist; this leaves theoretical studies to rely on assumptions and approximations just to calculate the energies of the ground state. Including any sort of dynamics in these calculations is prohibitively complicated, and this makes experimental observations important. Since many organic molecules are …
In Situ Measurement Of Three-Dimensional Ion Densities In Focused Femtosecond Pulses, James Strohaber, Cornelis J. Uiterwaal
In Situ Measurement Of Three-Dimensional Ion Densities In Focused Femtosecond Pulses, James Strohaber, Cornelis J. Uiterwaal
Department of Physics and Astronomy: Dissertations, Theses, and Student Research
We image spatial distribution of xenon ions in the focus of a laser beam of ultrashort, intense pulses in all three dimensions, with a resolution of three by twelve microns in the two transverse directions. This allows for studying ionization processes without spatially averaging ion yields. Our in situ ion imaging is also useful to analyze focal intensity profiles and to investigate the transverse modal purity of tightly focused beams of complex light. As an example, the intensity profile of a Hermite-Gaussian beam mode HG recorded with ions is found to be in good agreement with optical images.