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Articles 1 - 5 of 5
Full-Text Articles in Physical Sciences and Mathematics
Retrieving Photorecombination Cross Sections Of Atoms From High-Order Harmonic Spectra, Shinichiro Minemoto, Toshihito Umegaki, Yuichiro Oguchi, Toru Morishita, Anh-Thu Le, Shinichi Watanabe, Hirofumi Sakai
Retrieving Photorecombination Cross Sections Of Atoms From High-Order Harmonic Spectra, Shinichiro Minemoto, Toshihito Umegaki, Yuichiro Oguchi, Toru Morishita, Anh-Thu Le, Shinichi Watanabe, Hirofumi Sakai
Physics Faculty Research & Creative Works
We observe high-order harmonic spectra generated from a thin atomic medium, Ar, Kr, and Xe, by intense 800-nm and 1300-nm femtosecond pulses. A clear signature of a single-atom response is observed in the harmonic spectra. Especially in the case of Ar, a Cooper minimum, reflecting the electronic structure of the atom, is observed in the harmonic spectra. We successfully extract the photorecombination cross sections of the atoms in the field-free condition with the help of an accurate recolliding electron wave packet. The present protocol paves the way for exploring ultrafast imaging of molecular dynamics with attosecond resolution.
Reexamining Blackbody Shifts For Hydrogenlike Ions, Ulrich D. Jentschura, Martin K. Haas
Reexamining Blackbody Shifts For Hydrogenlike Ions, Ulrich D. Jentschura, Martin K. Haas
Physics Faculty Research & Creative Works
We investigate blackbody-induced energy shifts for low-lying levels of atomic systems, with a special emphasis on transitions used in current and planned high-precision experiments on atomic hydrogen and ionized helium. Fine-structure- and Lamb-shift-induced blackbody shifts are found to increase with the square of the nuclear charge number, whereas blackbody shifts due to virtual transitions decrease with increasing nuclear charge as the fourth power of the nuclear charge. We also investigate the decay width acquired by the ground state of atomic hydrogen, due to interaction with blackbody photons. The corresponding width is due to an instability against excitation to higher excited …
Efimov States Embedded In The Three-Body Continuum, Nirav P. Mehta, Seth T. Rittenhouse, J P. D’Incao, Chris H. Greene
Efimov States Embedded In The Three-Body Continuum, Nirav P. Mehta, Seth T. Rittenhouse, J P. D’Incao, Chris H. Greene
Physics and Astronomy Faculty Research
We present analytical solutions for the three-body problem with multichannel interactions and identify a class of quasibound Efimov states that can be viewed as three-body Fano-Feshbach resonances. Our method employs a multichannel generalization of the Fermi pseudopotential to model low-energy atom-atom interactions near a magnetically tunable Fano-Feshbach resonance. We discuss the conditions under which quasibound Efimov states may be supported and identify the interaction parameters that limit the lifetimes of these states. We speculate that it may be possible to observe these states using spectroscopic methods, perhaps allowing for the measurement of multiple Efimov resonances.
Extraction Of The Species-Dependent Dipole Amplitude And Phase From High-Order Harmonic Spectra In Rare-Gas Atoms, Anh-Thu Le, Toru Morishita, C. D. Lin
Extraction Of The Species-Dependent Dipole Amplitude And Phase From High-Order Harmonic Spectra In Rare-Gas Atoms, Anh-Thu Le, Toru Morishita, C. D. Lin
Physics Faculty Research & Creative Works
Based on high-order harmonic generation (HHG) spectra obtained from solving the time-dependent Schrödinger equation for atoms, we established quantitatively that the HHG yield can be expressed as the product of a returning electron wave packet and photorecombination cross sections, and the shape of the returning wave packet is shown to be largely independent of the species. By comparing the HHG spectra generated from different targets under identical laser pulses, accurate structural information, including the phase of the recombination amplitude, can be retrieved. This result opens up the possibility of studying the target structure of complex systems, including their time evolution, …
Potential For Ultrafast Dynamic Chemical Imaging With Few-Cycle Infrared Lasers, Toru Morishita, Anh-Thu Le, Zhangjin Chen, C. D. Lin
Potential For Ultrafast Dynamic Chemical Imaging With Few-Cycle Infrared Lasers, Toru Morishita, Anh-Thu Le, Zhangjin Chen, C. D. Lin
Physics Faculty Research & Creative Works
We studied the photoelectron spectra generated by an intense few cycle infrared laser pulse. By focusing on the angular distributions of the back rescattered high energy photoelectrons, we show that accurate differential elastic scattering cross-sections of the target ion by free electrons can be extracted. Since the incident direction and the energy of the free electrons can be easily changed by manipulating the laser's polarization, intensity and wavelength, these extracted elastic scattering cross-sections, in combination with more advanced inversion algorithms, may be used to reconstruct the effective single-scattering potential of the molecule, thus opening up the possibility of using few-cycle …