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Full-Text Articles in Physical Sciences and Mathematics
Anisotropic Softening Of Magnetic Excitations In Lightly Electron-Doped Sr2Iro4, X. Liu, M. P. M. Dean, Z. Y. Meng, M. H. Upton, T. Qi, T. Gog, Y. Cao, J. Q. Lin, D. Meyers, H. Ding, Gang Cao, J. P. Hill
Anisotropic Softening Of Magnetic Excitations In Lightly Electron-Doped Sr2Iro4, X. Liu, M. P. M. Dean, Z. Y. Meng, M. H. Upton, T. Qi, T. Gog, Y. Cao, J. Q. Lin, D. Meyers, H. Ding, Gang Cao, J. P. Hill
Center for Advanced Materials Faculty Publications
The magnetic excitations in electron-doped (Sr1−xLax)2IrO4 with x = 0.03 were measured using resonant inelastic x-ray scattering at the Ir L3 edge. Although much broadened, well defined dispersive magnetic excitations were observed. Comparing with the magnetic dispersion from the undoped compound, the evolution of the magnetic excitations upon doping is highly anisotropic. Along the antinodal direction, the dispersion is almost intact. On the other hand, the magnetic excitations along the nodal direction show significant softening. These results establish the presence of strong magnetic correlations in electron-doped (Sr1−xLax …
Investigations Of Metastable Ca2Iro4 Epitaxial Thin-Films: Systematic Comparison With Sr2Iro4 And Ba2Iro4, Maryam Souri, John H. Gruenewald, Jsaminka Terzic, Joseph W. Brill, Gang Cao, Sung S. Ambrose Seo
Investigations Of Metastable Ca2Iro4 Epitaxial Thin-Films: Systematic Comparison With Sr2Iro4 And Ba2Iro4, Maryam Souri, John H. Gruenewald, Jsaminka Terzic, Joseph W. Brill, Gang Cao, Sung S. Ambrose Seo
Physics and Astronomy Faculty Publications
We have synthesized thermodynamically metastable Ca2IrO4 thin-films on YAlO3 (110) substrates by pulsed laser deposition. The epitaxial Ca2IrO4 thin-films are of K2NiF4-type tetragonal structure. Transport and optical spectroscopy measurements indicate that the electronic structure of the Ca2IrO4 thin-films is similar to that of Jeff = 1/2 spin-orbit-coupled Mott insulator Sr2IrO4 and Ba2IrO4, with the exception of an increased gap energy. The gap increase is to be expected in Ca2IrO4 due to its increased octahedral rotation …
X-Ray Absorption Spectroscopy Study Of The Effect Of Rh Doping In Sr2Iro4, C. H. Sohn, Deok-Yong Cho, C. -T. Kuo, L. J. Sandilands, Tongfei Qi, Gang Cao, T. W. Noh
X-Ray Absorption Spectroscopy Study Of The Effect Of Rh Doping In Sr2Iro4, C. H. Sohn, Deok-Yong Cho, C. -T. Kuo, L. J. Sandilands, Tongfei Qi, Gang Cao, T. W. Noh
Center for Advanced Materials Faculty Publications
We investigate the effect of Rh doping in Sr2IrO4 using X-ray absorption spectroscopy (XAS). We observed appearance of new electron-addition states with increasing Rh concentration (x in Sr2Ir1−xRhxO4) in accordance with the concept of hole doping. The intensity of the hole-induced state is however weak, suggesting weakness of charge transfer (CT) effect and Mott insulating ground states. Also, Ir Jeff = 1/2 upper Hubbard band shifts to lower energy as x increases up to x = 0.23. Combined with optical spectroscopy, these results suggest a hybridisation-related mechanism, in …
Isotropic And Anisotropic Regimes Of The Field-Dependent Spin Dynamics In Sr2Iro4: Raman Scattering Studies, Y. Gim, A. Sethi, Q. Zhao, J. F. Mitchell, Gang Cao, S. L. Cooper
Isotropic And Anisotropic Regimes Of The Field-Dependent Spin Dynamics In Sr2Iro4: Raman Scattering Studies, Y. Gim, A. Sethi, Q. Zhao, J. F. Mitchell, Gang Cao, S. L. Cooper
Physics and Astronomy Faculty Publications
A major focus of experimental interest in Sr2IrO4 has been to clarify how the magnetic excitations of this strongly spin-orbit coupled system differ from the predictions of an isotropic 2D spin-1/2 Heisenberg model and to explore the extent to which strong spin-orbit coupling affects the magnetic properties of iridates. Here, we present a high-resolution inelastic light (Raman) scattering study of the low-energy magnetic excitation spectrum of Sr2IrO4 and Eu-doped Sr2IrO4 as functions of both temperature and applied magnetic field. We show that the high-field (H > 1.5 T) in-plane spin dynamics …