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Nonlinear Optical Studies Of Bulk And Thin Film Complex Materials, Joel E. Taylor
Nonlinear Optical Studies Of Bulk And Thin Film Complex Materials, Joel E. Taylor
LSU Doctoral Dissertations
Nonlinear optical studies of bulk and thin film materials provide a vast playground for physical and dynamical characterization. In this thesis, we have implemented experimental methods to probe novel phase transitions in single crystals using rotational anisotropic second harmonic generation (RASHG) and carrier dynamics in thin films with time-resolved pump-probe reflectivity. Furthermore, a novel low temperature ultra-high vacuum system coupled to nonlinear optics has been developed to extend lab capabilities. Doping (Bi1-xSbx)2Se3 with antimony, the surface electronic reconstruction near x=80% was identified with RASHG by deviations in the six-fold and three-fold polarization anisotropic …
Evolution Of Structural And Physical Properties Of Transition Metal Oxide Sr₃(Ru₁₋Xmnx)₂O₇ (0 <̲ X >̲ 0.7) With Mn Concentration, Biao Hu
LSU Doctoral Dissertations
Correlated Electron Materials (CEMs) have attracted the attention of the materials community because the strong coupling between charge, lattice, orbital, and spin degrees of freedom produces exotic phenomena. Transition metal oxide series Srn+1RunO3n+1 (n = 1 to ∞) is a prototype of CEMs. The n = 2 member of this family Sr3Ru2O7 is the subject of this dissertation. It has a paramagnetic (PM) metallic ground state, which can be driven into an antiferromagnetic (AFM) insulator with a partial substitution of Ru by Mn. The focus of this research is to understand the role of chemical doping as the driving force …