Physical Sciences and Mathematics Commons^™

Spectroscopy Of 88Y By The (P,Dγ) Reaction, T. J. Ross, C. W. Beausang, R. O. Hughes, N. D. Scielzo, J. T. Burke, J. M. Allmond, C. Angell, M. S. Basunia, D. L. Bleuel, R. J. Casperson, J. Escher, P. Fallon, R. Hatarik, J. Munson, S. Paschalis, M. Petri, L. Phair, J. J. Ressler

Physics Faculty Publications

Low-spin, high-excitation energy states in ⁸⁸Y have been studied using the ⁸⁹Y(p,dγ) reaction. For this experiment a 25 MeV proton beam was incident upon a monoisotopic ⁸⁹Y target. A silicon telescope array was used to detect deuterons, and coincident γ rays were detected using a germanium clover array. Most of the known low-excitation-energy low-spin states populated strongly via the (p,d) reaction mechanism are confirmed. Two states are seen for the first time and seven new transitions, including one which bypasses the two low-lying isomeric states, are observed.

Stress-Lifetime Joint Distribution Model For Performance Degradation Failure, Quan Sun, Yanzhen Tang, Jing Feng, Paul Kvam

Department of Math & Statistics Faculty Publications

The high energy density self-healing metallized film pulse capacitor has been applied to all kinds of laser facilities for their power conditioning systems under several stress levels, such as 23kV, 30kV and 35kV, whose reliability performance and maintenance costs are affected by the reliability of capacitors. Due to the costs and time restriction, how to assess the reliability of highly reliable capacitors under a certain stress level as soon as possible becomes a challenge. Accelerated degradation test provides a way to predict its lifetime and reliability effectively. A model called stress-lifetime joint distribution model and an analysis method based on …

Triaxial Deformation And Nuclear Shape Transition In 192Au, Y. Oktem, D. L. Balabanski, B. Akkus, L. Amon Susam, L. Atanasova, C. W. Beausang, R. Cakirli, R. F. Casten, M. Danchev, M. Djongolov, E. Ganioglu, K. A. Gladnishki, J. Tm. Goon, D. J. Hartley, A. A. Hecht, R. Krucken, J. R. Novak, G. Rainovski, L. L. Riedinger, T. Venkova, I. Yigitoglu, N. V. Zamfir, O. Zeidan

Physics Faculty Publications

Background: Nuclei in the A≈190 mass region show gradual shape changes from prolate through nonaxial deformed shapes and ultimately towards spherical shapes as the Pb region is approached. Exploring how this shape evolution occurs will help us understand the evolution of collectivity in this region.

Purpose: The level scheme of the ¹⁹²Au nucleus in A ≈ 190 region was studied in order to deduce its deformations.

Methods: High-spin states of ¹⁹²Au have been populated in the ¹⁸⁶W(¹¹B, 5n) reaction at a beam energy of 68 MeV and their γ decay was studied …

"Tuning Hole Mobility In Inp Nanowires", Mariama Rebello Sousa Dias, A. Picinin, V. Lopez-Richard, S. E. Ulloa, L. K. Castelano, J. P. Rino, G. E. Marques

Physics Faculty Publications

Transport properties of holes in InP nanowires (NWs) were calculated considering electron-phonon interaction via deformation potentials, the effect of temperature, and strain fields. Using molecular dynamics, we simulate NW structures, the longitudinal optical phonon (LO-phonon) energy renormalization, and lifetime. The valence band ground state changes between light- and heavy-hole character, as the strain fields and the NW size vary. Drastic changes in the mobility arise with the onset of resonance between the LO-phonons and the separation between valence subbands.

One-Pot Synthesis Of (Z)-B-Sulfonyl Enoates From Ethyl Propiolate, C. Wade Downey, Smaranda Craciun, Ana M. Neferu, Christina A. Vivelo, Carly J. Mueller, Brian C. Southall, Stephanie Corsi, Eric W. Etchill, Ryan J. Sault

Chemistry Faculty Publications

B-Sulfonyl enoates may be synthesized through a one-pot two-step sequence from ethyl propiolate with good to excellent selectivity for the Z isomer. Trialkylamines catalyze thioconjugate additions of aryl thiols, and alkoxides catalyze the addition of aliphatic thiols. Addition of meta-chloroperbenzoic acid (mCPBA) and LiClO₄ to the reaction mixture provides rapid access to the sulfonyl enoates. Yields of the pure Z isomer range from 51 – 90%.

One-Pot Three-Step Thioconjugate Addition-Oxidation-Diels–Alder Reactions Of Ethyl Propiolate, C. Wade Downey, Smaranda Craciun, Christina A. Vivelo, Ana M. Neferu, Carly J. Mueller, Stephanie Corsi

Chemistry Faculty Publications

Ethyl propiolate undergoes one-pot three-step thioconjugate addition-oxidation-Diels–Alder cycloaddition when treated with a variety of thiols in the presence of catalytic base, meta-chloroperbenzoic acid, lithium perchlorate, and cyclopentadiene. The reaction of S‑aryl thiols is catalyzed by trialkylamines, and the reaction of aliphatic thiols requires catalytic alkoxide base. Yields of the major diastereomer of the conveniently functionalized bicyclic products range from 47 to 81% depending upon the thiol reactant, which compares favorably to yields observed when the entire synthesis is performed step by step.

A Modular Fibrinogen Model That Captures The Stress-Strain Behavior Of Fibrin Fibers, Rodney D. Averett, Bryant Menn, Eric H. Lee, Christine C. Helms, Thomas Barker, Martin Guthold

Physics Faculty Publications

We tested what to our knowledge is a new computational model for fibrin fiber mechanical behavior. The model is composed of three distinct elements: the folded fibrinogen core as seen in the crystal structure, the unstructured α-C connector, and the partially folded α-C domain. Previous studies have highlighted the importance of all three regions and how they may contribute to fibrin fiber stress-strain behavior. Yet no molecular model has been computationally tested that takes into account the individual contributions of all these regions. Constant velocity, steered molecular dynamics studies at 0.025 Å/ps were conducted on the folded fibrinogen …

Energizing Liberal Education, Mary Finley-Brook, Megan Zanella-Litke, Kyle Ragan, Breana Coleman

Geography and the Environment Faculty Publications

The article examines how liberal arts colleges in the U.S. offer opportunities for developing and expanding the use of renewable energy and for promoting educational initiatives associated with community projects. Swarthmore College bought Renewable Energy Credits (RECs) from Direct Energy Renewable Choice. A team from Middlebury College designed a solar-powered farmhouse.

Experimental Study Of The P11(1440) And D13(1520) Resonances From The Clas Data On Ep→E′Π+Π−P′, V. I. Mokeev, Gerard P. Gilfoyle, Et. Al.

Physics Faculty Publications

The transition helicity amplitudes from the proton ground state to the P₁₁(1440) and D₁₃(1520) excited states (v_γpN* electrocouplings) were determined from the analysis of nine independent one-fold differential π⁺π⁻p electroproduction cross sections off a proton target, taken with CLAS at photon virtualities of 0.25 < Q² < 0.60 GeV². The phenomenological reaction model was employed for separation of the resonant and nonresonant contributions to the final state. The P₁₁(1440) and D₁₃(1520) electrocouplings were obtained from the resonant amplitudes parametrized within the framework of a unitarized …

Comparison Of Forward And Backward Pp Pair Knockout In 3He(E,E′Pp)N, H. Baghdasaryan, Gerard P. Gilfoyle, Et. Al.

Physics Faculty Publications

Measuring nucleon-nucleon short range correlations (SRCs) has been a goal of the nuclear physics community for many years. They are an important part of the nuclear wave function, accounting for almost all of the high-momentum strength. They are closely related to the EMC effect. While their overall probability has been measured, measuring their momentum distributions is more difficult. In order to determine the best configuration for studying SRC momentum distributions, we measured the ³He(e,e’ pp)n reaction, looking at events with high-momentum protons (p_p > 0.35 GeV/c) and a low-momentum neutron ( …

Flux And Photon Spectral Index Distributions Of Fermi-Lat Blazars And Contribution To The Extragalactic Gamma-Ray Background, Jack Singal, V. Petrosian, M. Ajello

Physics Faculty Publications

We present a determination of the distributions of the photon spectral index and gamma-ray flux—the so-called log N–log S relation—for the 352 blazars detected with a greater than approximately 7σ detection threshold and located above ±20◦ Galactic latitude by the Large Area Telescope of the Fermi Gamma-ray Space Telescope in its first year catalog. Because the flux detection threshold depends on the photon index, the observed raw distributions do not provide the true log N–log S counts or the true distribution of the photon index. We use the non-parametric methods developed by Efron and Petrosian to reconstruct the intrinsic distributions …

Measurement Of The Entry-Spin Distribution Imparted To The High Excitation Continuum Region Of Gadolinium Nuclei Via (P,D) And (P,T) Reactions, T. J. Ross, C. W. Beausang, R. O. Hughes, J. M. Allmond, C. Angell, M. S. Basunia, D. L. Bleuel, J. T. Burke, R. J. Casperson, J. Escher, P. Fallon, R. Hatarik, J. Munson, S. Paschalis, M. Petri, L. Phair, J. J. Ressler, N. D. Scielzo, I. Thompson

Physics Faculty Publications

Over the last several years, the surrogate reaction technique has been successfully employed to extract (n,f) and (n,γ) cross sections in the actinide region to a precision of ∼5% and ∼20%, respectively. However, attempts to apply the technique in the rare earth region have shown large (factors of 2–3) discrepancies between the directly measured (n,γ) and extracted surrogate cross sections. One possible origin of this discrepancy lies in differences between the initial spin-parity population distribution in the neutron induced and surrogate reactions. To address this issue, the angular …

Statistical Γ Rays In The Analysis Of Surrogate Nuclear Reactions, N. D. Scielzo, J. Escher, J. M. Allmond, M. S. Basunia, C. W. Beausang, L. A. Bernstein, D. L. Bleuel, J. T. Burke, R. M. Clark, F. S. Dietrich, P. Fallon, J. Gibelin, B. L. Goldblum, S. R. Lesher, M. A. Mcmahan, E. B. Norman, L. Phair, E. Rodriguez-Vieitez, S. A. Sheets, I. Thompson, M. Wiedeking

Physics Faculty Publications

The surrogate nuclear reaction method is being applied in many efforts to indirectly determine neutron-induced reaction cross sections on short-lived isotopes. This technique aims to extract accurate (n,γ) cross sections from measured decay properties of the compound nucleus of interest (created using a different reaction). The advantages and limitations of a method that identifies the γ-ray decay channel by detecting any high-energy (“statistical”) γ ray emitted during the relaxation of the compound nucleus were investigated. Data collected using the Silicon Telescope Array for Reaction Studies and Livermore-Berkeley Array for Collaborative Experiments silicon and germanium detector arrays were used …

Challenging Disciplinary Boundaries In The First Year: A New Introductory Integrated Science Course For Stem Majors, Lisa Gentile, Lester Caudill, Mirela Fetea, April L. Hill, Kathy Hoke, Barry Lawson, Ovidiu Z. Lipan, Michael Kerckhove, Carol A. Parish, Krista J. Stenger, Doug Szajda

Department of Math & Statistics Faculty Publications

To help undergraduates make connections among disciplines so they are able to approach, evaluate, and contribute to the solutions of important global problems, our campus has been focused on interdisciplinary research and education opportunities across the science, technology, engineering, and mathematics (STEM) disciplines. This paper describes the mobilization, planning, and implementation of a first-year interdisciplinary course for STEM majors that integrates key concepts found in traditional first-semester biology, chemistry, computer science, mathematics, and physics courses. This team-taught course, Integrated Quantitative Science (IQS), is half of a first-year student’s schedule in both semesters and is composed of a double lecture and …

Challenging Disciplinary Boundaries In The First Year: A New Introductory Integrated Science Course For Stem Majors, Lisa Gentile, Lester Caudill, Mirela Fetea, April L. Hill, Kathy Hoke, Barry Lawson, Ovidiu Z. Lipan, Michael Kerckhove, Carol A. Parish, Krista J. Stenger, Doug Szajda

Biology Faculty Publications

To help undergraduates make connections among disciplines so they are able to approach, evaluate, and contribute to the solutions of important global problems, our campus has been focused on interdisciplinary research and education opportunities across the science, technology, engineering, and mathematics (STEM) disciplines. This paper describes the mobilization, planning, and implementation of a first-year interdisciplinary course for STEM majors that integrates key concepts found in traditional first-semester biology, chemistry, computer science, mathematics, and physics courses. This team-taught course, Integrated Quantitative Science (IQS), is half of a first-year student’s schedule in both semesters and is composed of a double lecture and …

Measurement Of The Neutron F2 Structure Function Via Spectator Tagging With Clas, N. Baillie, Gerard P. Gilfoyle, Et. Al.

Physics Faculty Publications

We report on the first measurement of the F₂ structure function of the neutron from semi-inclusive scattering of electrons from deuterium, with low-momentum protons detected in the backward hemisphere. Restricting the momentum of the spectator protons to ≲ 100° MeV/c and their angles to ≳ 100° relative to the momentum transfer allows an interpretation of the process in terms of scattering from nearly on-shell neutrons. The Fⁿ₂ data collected cover the nucleon-resonance and deep-inelastic regions over a wide range of Bjorken x for 0.65 < Q² < 4.52 GeV², with uncertainties from nuclear corrections estimated to be less than …

Measurement Of The Generalized Form Factors Near Threshold Via Γ*P→Nπ+ At High Q2, K. Park, Gerard P. Gilfoyle, Et. Al.

Physics Faculty Publications

We report the first extraction of the pion-nucleon multipoles near the production threshold for the nπ⁺ channel at relatively high momentum transfer (Q² up to 4.2 GeV²). The dominance of the s-wave transverse multipole (E₀₊), expected in this region, allowed us to access the generalized form factor G₁ within the light-cone sum-rule (LCSR) framework as well as the axial form factor G_A. The data analyzed in this work were collected by the nearly 4π CEBAF Large Acceptance Spectrometer (CLAS) using a 5.754-GeV electron beam on a proton …

Utilizing (P,D) And (P,T) Reactions To Obtain (N,F) Cross Sections In Uranium Nuclei Via The Surrogate-Ratio Method, R. O. Hughes, C. W. Beausang, T. J. Ross, J. T. Burke, N. D. Scielzo, M. S. Basunia, C. M. Campbell, R. J. Casperson, H. L. Crawford, J. Escher, J. Munson, L. Phair, J. J. Ressler

Physics Faculty Publications

The surrogate ratio method has been tested for (p,d) and (p,t) reactions on uranium nuclei. ²³⁶U and ²³⁸U targets were bombarded with 28-MeV protons and the light ion recoils and fission fragments were detected using the Silicon Telescope Array for Reaction Studies detector array at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. The (p,df) reaction channels on ²³⁶U and ²³⁸U targets were used as a surrogate to determine the σ[²³⁶U(n,f)]/σ[²³⁴U(n, …

Upper Limits For The Photoproduction Cross Section For The Φ−−(1860) Pentaquark State Off The Deuteron, H. Egiyan, Gerard P. Gilfoyle, Et. Al.

Physics Faculty Publications

We searched for the Φ^--(1860) pentaquark in the photoproduction process off the deuteron in the Ξ^-π^--decay channel using CLAS. The invariant-mass spectrum of the Ξ^-π^- system does not indicate any statistically significant enhancement near the reported mass M = 1.860 GeV. The statistical analysis of the sideband-subtracted mass spectrum yields a 90%-confidence-level upper limit of 0.7 nb for the photoproduction cross section of Φ^--(1860) with a consecutive decay into Ξ^-π^- in the photon-energy range 4.5 GeV < E_γ < 5.5 GeV.

Α−Α Cross-Links Increase Fibrin Fiber Elasticity And Stiffness, Christine C. Helms, Robert A.S. Ariens, S. Uitte De Willige, Kristina F. Standeven, Martin Guthold

Physics Faculty Publications

Fibrin fibers, which are ∼100 nm in diameter, are the major structural component of a blood clot. The mechanical properties of single fibrin fibers determine the behavior of a blood clot and, thus, have a critical influence on heart attacks, strokes, and embolisms. Cross-linking is thought to fortify blood clots; though, the role of α–α cross-links in fibrin fiber assembly and their effect on the mechanical properties of single fibrin fibers are poorly understood. To address this knowledge gap, we used a combined fluorescence and atomic force microscope technique to determine the stiffness (modulus), extensibility, and elasticity of …

Bad Boundary Behavior In Star Invariant Subspaces Ii, William T. Ross, Andreas Hartmann

Department of Math & Statistics Faculty Publications

We continue our study begun in [HR11] concerning the radial growth of functions in the model spaces (IH²)^⊥.

Unitary Equivalence To A Truncated Toeplitz Operator: Analytic Symbols, William T. Ross, Stephan Ramon Garcia, Daniel E. Poore

Department of Math & Statistics Faculty Publications

Unlike Toeplitz operators on H², truncated Toeplitz operators do not have a natural matricial characterization. Consequently, these operators are difficult to study numerically. In this note we provide criteria for a matrix with distinct eigenvalues to be unitarily equivalent to a truncated Toeplitz operator having an analytic symbol. This test is constructive and we illustrate it with several examples. As a byproduct, we also prove that every complex symmetric operator on a Hilbert space of dimension < 3 is unitarily equivalent to a direct sum of truncated Toeplitz operators.

Boundary Values In Range Spaces Of Co-Analytic Truncated Toeplitz Operator, William T. Ross, Andreas Hartmann

Department of Math & Statistics Faculty Publications

Functions in backward shift invariant subspaces have nice analytic continuation properties outside the spectrum of the inner function defining the space. Inside the spectrum of the inner function, Ahern and Clark showed that under some distribution condition on the zeros and the singular measure of the inner function, it is possible to obtain non-tangential boundary values of every function in the backward shift invariant subspace as well as for their derivatives up to a certain order. Here we will investigate, at least when the inner function is a Blaschke product, the non-tangential boundary values of the functions of the backward …

Connected Inverse Limits With A Set-Valued Function, Van C. Nall

Department of Math & Statistics Faculty Publications

In this paper we provide techniques to build set-valued functions whose resulting inverse limits will be connected.

To The Continuum And Beyond: Structure Of U Nuclei, R. O. Hughes, C. W. Beausang, T. J. Ross, J. T. Burke, N. D. Scielzo, M. S. Basunia, C. M. Campbell, R. J. Casperson, H. L. Crawford, J. Munson, L. Phair, J. J. Ressler

Physics Faculty Publications

An experiment was performed at the 88-inch cyclotron at LBNL to investigate the structure of uranium isotopes and concurrently test the so-called surrogate ratio method. A 28 MeV proton beam was used to bombard ²³⁶U and ²³⁸U targets and the outgoing light ions were detected using the STARS silicon telescope allowing isotopic assignments and the excitation energy of the compound nucleus to be measured. A fission detector was placed at backward angles to give particle-fission coincidences, while the six clover germanium detectors of the LIBERACE array were used for particle-γ coincidences. The (p,d) reaction channels on ²³⁶U …

A Shell Model Study Of The High Spin States Of 88Y, M. Bunce, P. H. Regan, V. Werner, A. Anagnostatou, C. W. Beausang, M. Bowry, R. J. Casperson, D. Chen, N. Cooper, P. Goddard, R. O. Hughes, G. Ilie, P.J.R. Mason, B. Pauerstein, M. W. Reed

Physics Faculty Publications

Experiments were carried out at the Wright Nuclear Structure Laboratory at Yale University using the 21MV ESTU Tandem Van de Graaff accelerator with the purpose of studying ⁸⁸Y. A beam of ¹⁸O impinged at laboratory energies of 60, 65 and 70 MeV on a 600 μg/cm ^{2 74}Ge target with a thick (10mg/cm ²) ¹⁹⁷Au backing. This experiment was performed with the specific aim of accessing medium spin states of the nucleus of interest. A second experiment was undertaken to populate the nucleus of interest in higher spin states by impinging the same ^{18 …}

Comment On “Observation Of A Narrow Structure In 1H(Γ,KS0)X Via Interference With Φ-Meson Production”, M. Anghinolfi, Gerard P. Gilfoyle, Et. Al.

Physics Faculty Publications

In Ref. [1], the authors claim to observe a narrow structure in the mass spectrum constructed from the (pKL) system using data from the CLAS detector. The interpretation of this narrow structure given in Ref. [1] is as follows: “It may be due to the photoproduction of the Θ⁺pentaquark or some unknown Σ* resonance.” The authors go on to say that “it is unlikely for the observed structure to be due to a Σ* resonance.”

Cbe5e− (E = Al, Ga, In, Tl): Planar Pentacoordinate Carbon In Heptaatomic Clusters, Abril C. Castro, Gerarso Martinez-Guajardo, Thomas Johnson, Jesus M. Ugalde, Yan-Bo Wu, Jose M. Mercero, Thomas Heine, Kelling J. Donald, Gabriel Merino

Chemistry Faculty Publications

A series of clusters with the general formula CBe₅E^- (E = Al, Ga, In, Tl) are theoretically shown to have a planar pentacoordinate carbon atom. The structures show a simple and rigid topological framework—a planar EBe4 ring surrounding a C center, with one of the ring Be–Be bonds capped in-plane by a fifth Be atom. The system is stabilized by a network of multicenter σ bonds in which the central C atom is the acceptor, and π systems as well by which the C atom donates charge to the Be and E atoms that encircle it.

Plane And Simple: Planar Tetracoordinate Carbon Centers In Small Moleculesw, Chad Crigger, Bernard K. Wittmaack, Marina Tawfik, Gabriel Merino, Kelling J. Donald

Chemistry Faculty Publications

A class of neutral 18-electron molecules with planar tetracoordinate carbon (ptC) centers is introduced. We show computationally that when n = 3 the neutral singlet molecule C(BeH)_n(BH₂)_4-n and other isoelectronic (18-valence electron) molecules of main group elements collapse from locally tetrahedral arrangements at the C-center to (near) planar tetracoordinate structures. For C(BeH)₃BH₂ and C(CH₃)(BH₂)Li₂, for example, the tetrahedral type conformation is not even a minimum on the potential energy surface at the B3PW91, MP2(full), or CCSD levels of theory. The Mg analogue C(MgH)₃BH_{2 …}

Grts And Graphs: Monitoring Natural Resources In Urban Landscapes, Todd R. Lookingbill, John Paul Schmit, Shawn L. Carter

Geography and the Environment Faculty Publications

Environmental monitoring programs are an important tool for providing land managers with a scientific basis for management decisions. However, many ecological processes operate on spatial scales that transcend management boundaries (Schonewald-Cox 1988). For example, adjacent lands may influence protected-area resources via edge effects, source-sink dynamics, or invasion processes (Jones et al. 2009). Hydrologic alterations outside management units also may have profound effects on the integrity of resources being managed (Pringle 2000). The impacts of climate change are presenting challenges to resource management at local-to-global scales (Karl et al. 2009). This potential disparity between ecological and political boundaries presents an interesting …