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Coherent Excitation Of The Optic Phonon In Si: Transiently Stimulated Raman Scattering With Afinite-Lifetime Electronic Excitation, D. Mark Riffe, A. J. Sabbah

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Using 28-fs, 800-nm laser pulses we have coherently excited and subsequently probed, with time-dependent reflectivity, the Si zone-center optic phonon. The phonon-induced reflectivity change ΔR∕R is well described by the response of an underdamped oscillator: ΔR∕R∝ exp(−t∕τ_ph) cos(2πt∕T_ph+ϕ). The measured phase ϕ indicates that transiently stimulated Raman scattering (TSRS) is responsible for the coherent-phonon generation: our results are in good agreement with a recent theory of TSRS for opaque materials [ T. E. Stevens et al. Phys. Rev. B 65 144304 (2002)] when we extend the theory to include the finite lifetime of the excited charge …