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Full-Text Articles in Physical Sciences and Mathematics

Real-Time Observation Of Molecular Spinning With Angular High-Harmonic Spectroscopy, Lixin He, Pengfei Lan, Anh-Thu Le, Baoning Wang, Bincheng Wang, Xiaosong Zhu, Peixiang Lu, C. D. Lin Oct 2018

Real-Time Observation Of Molecular Spinning With Angular High-Harmonic Spectroscopy, Lixin He, Pengfei Lan, Anh-Thu Le, Baoning Wang, Bincheng Wang, Xiaosong Zhu, Peixiang Lu, C. D. Lin

Physics Faculty Research & Creative Works

We demonstrate an angular high-harmonic spectroscopy method to probe the spinning dynamics of a molecular rotation wave packet in real time. With the excitation of two time-delayed, polarization-skewed pump pulses, the molecular ensemble is impulsively kicked to rotate unidirectionally, which is subsequently irradiated by another delayed probe pulse for high-order harmonic generation (HHG). The spatiotemporal evolution of the molecular rotation wave packet is visualized from the time-dependent angular distributions of the HHG yields and frequency shift measured at various polarization directions and time delays of the probe pulse. The observed frequency shift in HHG is demonstrated to arise from the …


Search For Tensor, Vector, And Scalar Polarizations In The Stochastic Gravitational-Wave Background, Benjamin P. Abbott, Marco Cavaglia, For Full List Of Authors, See Publisher's Website. May 2018

Search For Tensor, Vector, And Scalar Polarizations In The Stochastic Gravitational-Wave Background, Benjamin P. Abbott, Marco Cavaglia, For Full List Of Authors, See Publisher's Website.

Physics Faculty Research & Creative Works

The detection of gravitational waves with Advanced LIGO and Advanced Virgo has enabled novel tests of general relativity, including direct study of the polarization of gravitational waves. While general relativity allows for only two tensor gravitational-wave polarizations, general metric theories can additionally predict two vector and two scalar polarizations. The polarization of gravitational waves is encoded in the spectral shape of the stochastic gravitational-wave background, formed by the superposition of cosmological and individually unresolved astrophysical sources. Using data recorded by Advanced LIGO during its first observing run, we search for a stochastic background of generically polarized gravitational waves. We find …


First Search For Nontensorial Gravitational Waves From Known Pulsars, Benjamin P. Abbott, Marco Cavaglia, For Full List Of Authors, See Publisher's Website. Jan 2018

First Search For Nontensorial Gravitational Waves From Known Pulsars, Benjamin P. Abbott, Marco Cavaglia, For Full List Of Authors, See Publisher's Website.

Physics Faculty Research & Creative Works

We present results from the first directed search for nontensorial gravitational waves. While general relativity allows for tensorial (plus and cross) modes only, a generic metric theory may, in principle, predict waves with up to six different polarizations. This analysis is sensitive to continuous signals of scalar, vector, or tensor polarizations, and does not rely on any specific theory of gravity. After searching data from the first observation run of the advanced LIGO detectors for signals at twice the rotational frequency of 200 known pulsars, we find no evidence of gravitational waves of any polarization. We report the first upper …


Gravitational Correction To Vacuum Polarization, Ulrich D. Jentschura Feb 2015

Gravitational Correction To Vacuum Polarization, Ulrich D. Jentschura

Physics Faculty Research & Creative Works

We consider the gravitational correction to (electronic) vacuum polarization in the presence of a gravitational background field. The Dirac propagators for the virtual fermions are modified to include the leading gravitational correction (potential term) which corresponds to a coordinate-dependent fermion mass. The mass term is assumed to be uniform over a length scale commensurate with the virtual electron-positron pair. The on-mass shell renormalization condition ensures that the gravitational correction vanishes on the mass shell of the photon, i.e., the speed of light is unaffected by the quantum field theoretical loop correction, in full agreement with the equivalence principle. Nontrivial corrections …


One-Loop Dominance In The Imaginary Part Of The Polarizability: Application To Blackbody And Noncontact Van Der Waals Friction, Ulrich D. Jentschura, Grzegorz Lach, Maarten Dekieviet, Krzysztof Pachucki Jan 2015

One-Loop Dominance In The Imaginary Part Of The Polarizability: Application To Blackbody And Noncontact Van Der Waals Friction, Ulrich D. Jentschura, Grzegorz Lach, Maarten Dekieviet, Krzysztof Pachucki

Physics Faculty Research & Creative Works

Phenomenologically important quantum dissipative processes include blackbody friction (an atom absorbs counterpropagating blueshifted photons and spontaneously emits them in all directions, losing kinetic energy) and noncontact van der Waals friction (in the vicinity of a dielectric surface, the mirror charges of the constituent particles inside the surface experience drag, slowing the atom). The theoretical predictions for these processes are modified upon a rigorous quantum electrodynamic treatment, which shows that the one-loop "correction" yields the dominant contribution to the off-resonant, gauge-invariant, imaginary part of the atom's polarizability at room temperature, for typical atom-surface interactions. The tree-level contribution to the polarizability dominates …


Theoretical And Experimental (E, 2e) Study Of Electron-Impact Ionization Of Laser-Aligned Mg Atoms, Sadek Amami, Andrew J. Murray, Al Stauffer, Kate Nixon, Gregory Armstrong, James Colgan, Don H. Madison Dec 2014

Theoretical And Experimental (E, 2e) Study Of Electron-Impact Ionization Of Laser-Aligned Mg Atoms, Sadek Amami, Andrew J. Murray, Al Stauffer, Kate Nixon, Gregory Armstrong, James Colgan, Don H. Madison

Physics Faculty Research & Creative Works

We have performed calculations of the fully differential cross sections for electron-impact ionization of magnesium atoms. Three theoretical approximations, the time-dependent close coupling, the three-body distorted wave, and the distorted wave Born approximation, are compared with experiment in this article. Results will be shown for ionization of the 3s ground state of Mg for both asymmetric and symmetric coplanar geometries. Results will also be shown for ionization of the 3p state which has been excited by a linearly polarized laser which produces a charge cloud aligned perpendicular to the laser beam direction and parallel to the linear polarization. Theoretical and …


Spectral Induced Polarization (Sip) Response Of Biodegraded Oil In Porous Media, Gamal Z. Abdel Aal, Estella A. Atekwana Feb 2014

Spectral Induced Polarization (Sip) Response Of Biodegraded Oil In Porous Media, Gamal Z. Abdel Aal, Estella A. Atekwana

Geosciences and Geological and Petroleum Engineering Faculty Research & Creative Works

Laboratory experiments were conducted to investigate the effect of different oil saturation (0.2- 0.8), wetting conditions (water-wet and oil-wet), and the addition of asphaltene on the spectral induced polarization (SIP) response of biodegraded and fresh crude oil in sand columns. In the water-wet case, no significant differences were observed for both the fresh and biodegraded oil and both displayed an increase in the magnitude of the phase (φ) and decrease in the magnitudes of the real (σ′) and imaginary (σ″) conductivity components with increasing oil saturation. In this instance the SIP response is most likely controlled by the conduction and …


A New Model For The Spectral Induced Polarization Signature Of Bacterial Growth In Porous Media, Andre Revil, Estella A. Atekwana, C. Zhang, Abderrahim Jardani, Schaun M. Smith Sep 2012

A New Model For The Spectral Induced Polarization Signature Of Bacterial Growth In Porous Media, Andre Revil, Estella A. Atekwana, C. Zhang, Abderrahim Jardani, Schaun M. Smith

Geosciences and Geological and Petroleum Engineering Faculty Research & Creative Works

The complex conductivity of porous materials and colloidal suspensions comprises two components: an in-phase conductivity associated with electromigration of the charge carriers and a quadrature conductivity associated with the reversible storage of the charges at some polarization length scales. We developed a quantitative model to investigate the frequency domain induced polarization response of suspensions of bacteria and bacteria growth in porous media. Induced polarization of bacteria (α polarization) is related to the properties of the electrical double layer of the bacteria. Surface conductivity and α polarization are due to the Stern layer of counterions occurring in a brush of polymers …


Artificially Disordered Birefringent Optical Fibers, Sumudu Herath, N. P. Puente, Elena I. Chaikina, Alexey Yamilov Feb 2012

Artificially Disordered Birefringent Optical Fibers, Sumudu Herath, N. P. Puente, Elena I. Chaikina, Alexey Yamilov

Physics Faculty Research & Creative Works

We develop and experimentally verify a theory of evolution of polarization in artificially-disordered multi-mode optical fibers. Starting with a microscopic model of photo-induced index change, we obtain the first and second order statistics of the dielectric tensor in a Ge-doped fiber, where a volume disorder is intentionally inscribed via UV radiation transmitted through a diffuser. A hybrid coupled-power & coupled-mode theory is developed to describe the transient process of de-polarization of light launched into such a fiber. After certain characteristic distance, the power is predicted to be equally distributed over all co-propagating modes of the fiber regardless of their polarization. …


Thermal Correction To The Molar Polarizability Of A Boltzmann Gas, Ulrich D. Jentschura, Mariusz Puchalski, Peter J. Mohr Dec 2011

Thermal Correction To The Molar Polarizability Of A Boltzmann Gas, Ulrich D. Jentschura, Mariusz Puchalski, Peter J. Mohr

Physics Faculty Research & Creative Works

Metrology in atomic physics has been crucial for a number of advanced determinations of fundamental constants. In addition to very precise frequency measurements, the molar polarizability of an atomic gas has recently also been measured very accurately. Part of the motivation for the measurements is due to ongoing efforts to redefine the International System of Units (SI), for which an accurate value of the Boltzmann constant is needed. Here we calculate the dominant shift of the molar polarizability in an atomic gas due to thermal effects. It is given by the relativistic correction to the dipole interaction, which emerges when …


Relativistic Reduced-Mass And Recoil Corrections To Vacuum Polarization In Muonic Hydrogen, Muonic Deuterium, And Muonic Helium Ions, Ulrich D. Jentschura Jul 2011

Relativistic Reduced-Mass And Recoil Corrections To Vacuum Polarization In Muonic Hydrogen, Muonic Deuterium, And Muonic Helium Ions, Ulrich D. Jentschura

Physics Faculty Research & Creative Works

The reduced-mass dependence of relativistic and radiative effects in simple muonic bound systems is investigated. The spin-dependent nuclear recoil correction of order (Zα)4μ3/m2N is evaluated for muonic hydrogen and deuterium and muonic helium ions (μ is the reduced mass and mN is the nuclear mass). Relativistic corrections to vacuum polarization of order α(Zα)4μ are calculated, with a full account of the reduced-mass dependence. The results shift theoretical predictions. The radiative-recoil correction to vacuum polarization of order α(Zα)5-ln2(Zα) μ2/mN is obtained in leading logarithmic approximation. …


Blackbody-Radiation Correction To The Polarizability Of Helium, Mariusz Puchalski, Ulrich D. Jentschura, Peter J. Mohr Apr 2011

Blackbody-Radiation Correction To The Polarizability Of Helium, Mariusz Puchalski, Ulrich D. Jentschura, Peter J. Mohr

Physics Faculty Research & Creative Works

The correction to the polarizability of helium due to blackbody radiation is calculated near room temperature. A precise theoretical determination of the blackbody radiation correction to the polarizability of helium is essential for dielectric gas thermometry and for the determination of the Boltzmann constant. We find that the correction, for not too high temperature, is roughly proportional to a modified hyperpolarizability (two-color hyperpolarizability), which is different from the ordinary hyperpolarizability of helium. Our explicit calculations provide a definite numerical result for the effect and indicate that the effect of blackbody radiation can be excluded as a limiting factor for dielectric …


Quantum Electrodynamic Corrections To The Hyperfine Structure Of Excited S States, Ulrich D. Jentschura, Vladimir A. Yerokhin Jun 2006

Quantum Electrodynamic Corrections To The Hyperfine Structure Of Excited S States, Ulrich D. Jentschura, Vladimir A. Yerokhin

Physics Faculty Research & Creative Works

State-dependent quantum electrodynamic corrections are evaluated for the hyperfine splitting of nS states for arbitrary principal quantum number n. The calculations comprise both the self-energy and the vacuum-polarization correction of order α(Zα) 2 EF and the recoil correction of order (Zα)2 (m/M) EF. Higher-order corrections are summarized and partly reevaluated as well. Accurate predictions for hydrogen hyperfine splitting intervals of nS states with n=2,...,8 are presented. The results obtained are important due to steady progress in hydrogen spectroscopy for transitions involving highly excited S states.


Induced-Polarization Measurements On Unconsolidated Sediments From A Site Of Active Hydrocarbon Biodegradation, Gamal Z. Abdel Aal, Lee D. Slater, Estella A. Atekwana Mar 2006

Induced-Polarization Measurements On Unconsolidated Sediments From A Site Of Active Hydrocarbon Biodegradation, Gamal Z. Abdel Aal, Lee D. Slater, Estella A. Atekwana

Geosciences and Geological and Petroleum Engineering Faculty Research & Creative Works

To investigate the potential role that indigenous microorganisms and microbial processes may play in altering low frequency electrical properties, induced-polarization (IP) measurements in the frequency range of 0.1 to 1000 Hz were acquired from sediment samples retrieved from a site contaminated by hydrocarbon undergoing intrinsic biodegradation. Increased imaginary conductivity and phase were observed for samples from the smear zone (contaminated with residual-phase hydrocarbon), exceeding values obtained for samples contaminated with dissolved-phase hydrocarbons, and in turn, exceeding values obtained for uncontaminated samples. Real conductivity, although generally elevated for samples from the smear zone, did not show a strong correlation with contamination. …


(±)-1-Methyl-1,3,6-Triphenyl-7-(2-Phenylpropenyl)-1, 2-Dihydronaphthalene, Yongqiang Sui, Charles Leslie Barnes, Rainer Glaser Feb 2006

(±)-1-Methyl-1,3,6-Triphenyl-7-(2-Phenylpropenyl)-1, 2-Dihydronaphthalene, Yongqiang Sui, Charles Leslie Barnes, Rainer Glaser

Chemistry Faculty Research & Creative Works

The crystal structure of the title compound, C38H32, presents a novel framework that combines the functionalities of a 1,6-diarene-substituted 1,2-dihydronaphthalene (DHN) with a 1,4-distyrylbenzene (DSB) to form a crossed bis-diarene. The lamellar crystal structure is held together by arene-arene interactions. While the orientations of the phenyl rings of the DSB units alternate within both the R and the S substructures, the homochiral substructures feature opposing polarity along the long axes of the DHN-based diarenes.


Laser-Dressed Vacuum Polarization In A Coulomb Field, A. I. Milstein, Ivan S. Terekhov, Ulrich D. Jentschura, Christoph H. Keitel Nov 2005

Laser-Dressed Vacuum Polarization In A Coulomb Field, A. I. Milstein, Ivan S. Terekhov, Ulrich D. Jentschura, Christoph H. Keitel

Physics Faculty Research & Creative Works

We investigate quantum electrodynamic effects under the influence of an external, time-dependent electromagnetic field, which mediates dynamic modifications of the radiative corrections. Specifically, we consider the quantum electrodynamic vacuum-polarization tensor under the influence of two external background fields: a strong laser field and a nuclear Coulomb field. We calculate the charge and current densities induced by a nuclear Coulomb field in the presence of a laser field. We find the corresponding induced scalar and vector potentials. The induced potential, in first-order perturbation theory, leads to a correction to atomic energy levels. The external laser field breaks the rotational symmetry of …


Positronium Formation In Positron-Li And Positron-Na Collisions At Low Energies, Anh-Thu Le, M. W. J. Bromley, C. D. Lin Mar 2005

Positronium Formation In Positron-Li And Positron-Na Collisions At Low Energies, Anh-Thu Le, M. W. J. Bromley, C. D. Lin

Physics Faculty Research & Creative Works

We present the positronium formation cross sections for a positron colliding with lithium and sodium for the collision energies from 0.01 eV up to 20 eV by the hyperspherical close-coupling method. For Li, our results agree with the experimental data and with other calculations. Our results for Na remain in agreement with previous close-coupling calculations, but do not support the latest experimental data for Na below 1 eV. To validate our model potentials and method in the low-energy regime, the binding energies of positronic lithium and positronic sodium as well as the s-wave scattering lengths for positronium scattering from Li⁺ …


Nonrelativistic Qed Approach To The Bound-Electron G Factor, Krzysztof Pachucki, Ulrich D. Jentschura, Vladimir A. Yerokhin Oct 2004

Nonrelativistic Qed Approach To The Bound-Electron G Factor, Krzysztof Pachucki, Ulrich D. Jentschura, Vladimir A. Yerokhin

Physics Faculty Research & Creative Works

Within a systematic approach based on nonrelativistic quantum electrodynamics, we derive the one-loop self-energy correction of order α ( Z α )4 to the bound-electron g factor. In combination with numerical data, this analytic result improves theoretical predictions for the self-energy correction for carbon and oxygen by an order of magnitude. Basing on one-loop calculations, we obtain the logarithmic two-loop contribution of order α2 ( Z α )4 ln [ ( Z α )- 2 ] and the dominant part of the corresponding constant term. The results obtained improve the accuracy of the theoretical predictions for …


Polarized Neutron Diffraction And Mössbauer Spectral Study Of Short-Range Magnetic Correlations In The Ferrimagnetic Layered Compounds (Pph₄) [FeIiFeIii(Ox)₃] And (Nbu₄) [FeIiFeIii(Ox)₃], Simon G. Carling, Dirk W. Visser, Dimitri Hautot, Ian D. Watts, Peter Day, Jürgen Ensling, Phillip Gütlich, Gary J. Long, Fernande Grandjean Sep 2002

Polarized Neutron Diffraction And Mössbauer Spectral Study Of Short-Range Magnetic Correlations In The Ferrimagnetic Layered Compounds (Pph₄) [FeIiFeIii(Ox)₃] And (Nbu₄) [FeIiFeIii(Ox)₃], Simon G. Carling, Dirk W. Visser, Dimitri Hautot, Ian D. Watts, Peter Day, Jürgen Ensling, Phillip Gütlich, Gary J. Long, Fernande Grandjean

Chemistry Faculty Research & Creative Works

Short-range antiferromagnetic correlations have been studied in the layered compounds (PPh4) [FeIIFeIII(ox)3] and (NBu4) [FeIIFeIII(ox)3] by neutron polarization analysis and Mössbauer spectroscopy. Polarized neutron diffraction profiles obtained between 2 and 50 K on (d20-Pph4) [FeIIFeIII(ox)3] show no magnetic Bragg scattering; the lack of such scattering indicates the absence of long-range magnetic order. However, a broad asymmetric feature observed at a Q of ca. 0.8 Å-1 is attributed to two-dimensional short-range magnetic correlations, which …


Mantle Deformation Beneath Southern Africa, Paul G. Silver, Stephen S. Gao, Kelly H. Liu, Kaapvaal Seismic Group Jul 2001

Mantle Deformation Beneath Southern Africa, Paul G. Silver, Stephen S. Gao, Kelly H. Liu, Kaapvaal Seismic Group

Geosciences and Geological and Petroleum Engineering Faculty Research & Creative Works

Seismic anisotropy from the southern African mantle has been inferred from shear-wave splitting measured at 79 sites of the Southern African Seismic Experiment. These data provide the most dramatic support to date that Archean mantle deformation is preserved as fossil mantle anisotropy. Fast polarization directions systematically follow the trend of Archean structures and splitting delay times exhibit geologic control. The most anisotropic regions are Late-Archean in age (Zimbabwe craton, Limpopo belt, western Kaapvaal craton), with delay times reduced dramatically in off-craton regions to the southwest and Early-Archean regions to the southeast. While thin lithosphere can account for weak off-craton splitting, …


Separation Of Recollision Mechanisms In Nonsequential Strong Field Double Ionization Of Ar: The Role Of Excitation Tunneling, Bernold Feuerstein, Daniel Fischer, Alexander Dorn, Claus Dieter Schroter, J. Deipenwisch, Jose R. Crespo Lopez-Urrutia, C. Hohr, Paul B. Neumayer, Horst Rottke, Christoph Trump, M. Wittmann, Georg Korn, Wolfgang Sandner, Robert Moshammer, Joachim Hermann Ullrich Jul 2001

Separation Of Recollision Mechanisms In Nonsequential Strong Field Double Ionization Of Ar: The Role Of Excitation Tunneling, Bernold Feuerstein, Daniel Fischer, Alexander Dorn, Claus Dieter Schroter, J. Deipenwisch, Jose R. Crespo Lopez-Urrutia, C. Hohr, Paul B. Neumayer, Horst Rottke, Christoph Trump, M. Wittmann, Georg Korn, Wolfgang Sandner, Robert Moshammer, Joachim Hermann Ullrich

Physics Faculty Research & Creative Works

Vector momentum distributions of two electrons created in double ionization of Ar by 25 fs, 0.25PW/cm2 laser pulses at 795 nm have been measured using a “reaction microscope.” At this intensity, where nonsequential ionization dominates, distinct correlation patterns are observed in the two-electron momentum distributions. A kinematical analysis of these spectra within the classical “recollision model” revealed an (e,2e)-like process and excitation with subsequent tunneling of the second electron as two different ionization mechanisms. This allows a qualitative separation of the two mechanisms demonstrating that excitation-tunneling is the dominant contribution to the total double ionization yield.


S K S Splitting Beneath Continental Rift Zones, Stephen S. Gao, Paul M. Davis, Kelly H. Liu, Philip D. Slack, Andrew W. Rigor, Yu A. Zorin, Valentina V. Mordvinova, Vladimir M. Kozhevnikov, Nikolai A. Logatchev Oct 1997

S K S Splitting Beneath Continental Rift Zones, Stephen S. Gao, Paul M. Davis, Kelly H. Liu, Philip D. Slack, Andrew W. Rigor, Yu A. Zorin, Valentina V. Mordvinova, Vladimir M. Kozhevnikov, Nikolai A. Logatchev

Geosciences and Geological and Petroleum Engineering Faculty Research & Creative Works

We present measurements of S K S splitting at 28 digital seismic stations and 35 analog stations in the Baikal rift zone, Siberia, and adjacent areas, and at 17 stations in the East African Rift in Kenya and compare them with previous measurements from the Rio Grande Rift of North America. Fast directions in the inner region of the Baikal rift zone are distributed in two orthogonal directions, NE and NW, approximately parallel and perpendicular to the NE strike of the rift. In the adjacent Siberian platform and northern Mongolian fold belt, only the rift-orthogonal fast direction is observed. In …