Physical Sciences and Mathematics Commons^™

Simulating Strongly Coupled Many-Body Systems With Quantum Algorithms, Manqoba Qedindaba Hlatshwayo

Dissertations

The complexity of the nuclear many-body problem is a severe obstacle to finding a general and accurate numerical approach needed to simulate medium-mass and heavy nuclei. Even with the advent of exascale classical computing, the impediment of exponential growth of the Hilbert space renders the problem intractable for most classical calculations. In the last few years, quantum algorithms have become an attractive alternative for practitioners because quantum computers are more efficient in simulating quantum physics than classical computers. While a fully fault-tolerant universal quantum computer will not be realized soon, this dissertation explores quantum algorithms for simulating nuclear physics suitable …

Probing The Equation Of State Of Neutron Stars With Heavy Ion Collisions, Om Bhadra Khanal

Dissertations

The equation of state (EOS) is a fundamental property of nuclear matter, important for studying the structure of systems as diverse as the atomic nucleus and the neutron star. Nuclear reactions, especially heavy-ion collisions in the laboratories, can produce the nuclear matter similar to those contained in neutron stars. The density and the momentum dependence of the EOS of asymmetric nuclear matter, especially the symmetry energy term, is widely unconstrained. Finding appropriate constrains, especially at higher densities of the nuclear matter, requires the development of new devices, new experimental measurements as well as advances in theoretical understanding of nuclear collisions …

Time-Dependent Photoionization Modeling Of Warm Absorbers In Active Galactic Nuclei, Dev Raj Sadaula

Dissertations

Warm absorber spectra are bound-bound and bound-free absorption features, seen in the X-ray and UV spectra from many active galactic nuclei (AGN). The widths and centroid energies of these features indicate they occur in outflowing gas moving with hundreds to thousands of km/s. Depending upon the energy and momentum of the outflow, it can affect the gas within the host galaxy. Thus, warm absorbers’ mass and energy budgets are of great interest. Estimates for these properties depend on models that connect the absorption features' observed strengths with the density, composition, and ionization state of the absorbing gas. Such models assume …

Studying The Synthesis Of 196Hg At Astrophysically Relevant Energies Through The Measurement Of Capture Reaction Cross-Sections Of (P, Γ) (P, N) And (P, Α) Reactions, Khushi Bhatt

Dissertations

Understanding the origin of all the chemical elements is an important question for the nuclear-astrophysics community. There are many unanswered questions like: What astrophysical events are responsible for the synthesis of what particular chemical elements? How many different elements were made in total? What is the abundance of each synthesized element? etc. Currently, scientists are largely depending upon theory and simulations to define nuclear and astrophysical reaction. This makes it critical to have accurate experimental nuclear physics data to input in astrophysical theoretical models. However, out of more than 20000 reactions involved in these calculations, only a very few are …

Novel Low Temperature Properties Of Filled And Unfilled Single Crystal Irsb3, Matthew Cook

Dissertations

The skutterudite family of materials has garnered a lot of attention in the condensed matter community and it persists to be an important system for exploring the fundamental physics of solids. The initial interest into compounds with this common structure was due to their promising thermoelectric properties giving the possibility of efficient energy harvesting. Since, there has been a huge effort to systematically synthesize new filled skutterudite compounds, as nearly every type of strongly correlated behavior has been found within this family. As the field of topological materials has gained momentum, these materials have also been given a renewed interest …

Enhancement Of Critical Current In High-Temperature Superconductors By Ion Beam Irradiation Induced Defects, Prashanta Mani Niraula

Dissertations

Particle irradiation is used to induce defects in high-temperature superconducting Y₁Ba₂Cu₃O_7-x (YBCO) coated conductors, containing predominantly c-axis oriented barium zirconate (BZO) nanorods as pre-existing vortex pinning defects. Samples are irradiated with 50.0 MeV Cu ions with doses of 2.5 x 10¹², 2.0 x 10¹², 1.5 x 10¹², 1.0 x 10¹², 0.75 x 10¹², 0.5 x 10¹², 0.05 x 10¹² ions/cm². The dose of 0.5 x 10¹² ions/cm² is found to be the optimal dose with a …

Embedded Gold Nanoparticles For Metal Enhanced Photoluminescence, Hasna Alali

Dissertations

Noble metal nanoparticles (MNPs) have attracted great attention in electronics, solar cells and catalysis. Their unique optical properties and biocompatibility makes them useful in biological applications like imaging, drug delivery, therapy and diagnostic. At the surface of MNPs the collective oscillation of free electrons resonates with a particular wavelength of incident light, generating the Localized Surface Plasmons Resonance (LSPR). LSPR results in absorption and scattering of incident light. Scattering results in reflecting photons and absorption leads to enhanced photoluminescence and quenching of fluorophores, if the fluorophore is in the vicinity of MNPs.

Most of the studies in this regard have …

Investigation Of Finite Temperature And Continuum Effects On Nuclear Excitations, Herlik Wibowo

Dissertations

The low-energy nuclear response at finite-temperature significantly affects the radiative neutron capture reaction rates of the r-process nucleosynthesis. In order to address this topic, the first part of this study focuses on the response of compound nuclei or nuclei at finite temperature. The thermal nuclear response satisfies the Bethe-Salpeter equation (BSE) with the static and dynamical kernels of different origins. While the origin of the static kernel is the nearly instantaneous nucleon-meson interaction, the dynamical kernel is induced by the coupling between nucleons and phonons. The presence of singularities in the dynamical kernel makes the BSE unsolvable, however, a time …

Embedded Silver Nanoparticles For Metal Enhanced Photoluminescence, Shahid Iqbal

Dissertations

Imaging of biologically significant molecules using plasmons of Metal Nanoparticles (MNPs) is gaining attention in the research community. Localized Surface Plasmon Resonance (LSPR) is the coherent oscillation of conduction electrons of MNPs. The biologically significant molecule is labeled with the fluorophore molecule to get the image. This approach is widely used in clinical practices, however, low intensity light emission from the labeled molecule makes it difficult to image the biologically significant material. One way to improve the weak intensities of fluorophore is to enhance the brightness using a process called Metal Enhanced Photoluminescence (MEP). This phenomenon occurs in the close …

Simultaneous X-Ray Emission Accompanying Two Electron Capture For Fluorine On Gas Targets, David S. La Mantia

Dissertations

The collision between a charged ion and an atom resulting in the capture of two electrons, simultaneous with the emission of a single photon is referred to as radiative double electron capture (RDEC). For ion-atom collisions, this process can be considered the inverse of double photoionization. The study of either process, where just two electrons are involved without influence from neighboring electrons, promises new insight into electron correlation and the role it plays in quantum mechanics. Such a study for photoionization has not yet been done experimentally for two-electron ions because the only target system for which two electrons are …

Investigation Of Structural, Optical And Electronic Properties Of Modified Methylammonium Lead Iodide Perovskites, Rasanjali Jayathissa

Dissertations

Owing to their high-power conversion efficiency (PCE), easy processability, and low fabrication cost, organic lead halide perovskites (OLHP) are emerging as a most promising photovoltaic technology. However, toxicity of lead (Pb) is a major concern for further development. Therefore, it is essential to explore nontoxic metals to replace lead in these materials. In the current research work, nontoxic Mn²⁺, Na⁺ and Ba²⁺ are doped at 1, 5 and 10% mole concentrations to partially substitute Pb²⁺ in methyl ammonium lead iodide (CH₃NH₃PbI₃ or MAPbI₃) perovskite systems, and the effects …

Sensitivity Of The Theoretical Electron Capture Shape And Comparisons To Experiment, Katrina E. Koehler

Dissertations

The direct neutrino mass is a fundamental physics quantity with far-reaching implications for the physics community. Current experimental limits put the direct neutrino mass at less than 2 eV. The neutrino mass can be explored through an end-point measurement of tritium beta decay, which is currently underway in the KArlsruhe TRItium Neutrino experiment (KATRIN). KATRIN has a lower limit of 0.2 eV, at which point there will be either a mass measurement or another upper bound. In either case, an alternative experiment with different systematics is needed to verify the results and/or push the upper bound lower. The end point …

Radiative Double Electron Capture (Rdec) By Fully-Stripped Fluorine Ions In Collisions With Nitrogen, Nuwan Sisira Kumara

Dissertations

Radiative double electron capture (RDEC) by highly-stripped ions in collisions with atomic targets is a fundamental process that can be used to study electron-electron correlation, the interaction between two electrons, in the vicinity of the Coulomb field of a bare ion. In this process two electrons from the target are captured to bound states of the projectile with the simultaneous emission of a single photon. RDEC is closely related to the well-known one-step atomic process of radiative electron capture (REC), in which a target electron is captured to the projectile and a photon is simultaneously emitted. REC and RDEC can …

A 3d Simulation Of Leukocyte Adhesion In Blood Flow, Tai-Hsien Wu

Dissertations

It has been widely acknowledged that further understanding about the dynamics between blood cells and blood flow can help us gain more knowledge about the causes of diseases and discover more effective treatments. Examples of such dynamics include red blood cell (RBC, or erythrocyte) aggregation, white blood cell (WBC, or leukocyte) margination, and WBC extravasation. WBC extravasation is an important multiple-step process in the inflammatory response and therefore has drawn considerable attention over the past two decades. In this multiple-step process, a WBC undergoes at least four steps, including capture, rolling, firm adhesion, and transmigration, and each step is influenced …

Dielectronic Recombination Calculations For Silicon-Like Ions And The S2+ Orion Nebula Abundance Conundrum, Jagjit Kaur

Dissertations

Modern astronomical spectroscopy and imaging data are of an unprecedented quality, and span the full electromagnetic spectrum. To take full advantage of these data and successfully model the physical conditions in and elemental abundances of astrophysical plasmas, an accurate and complete description of relevant atomic processes occurring in a wide range of cosmic environments is required. The primary focus of this project is to investigate one of the atomic processes, dielectronic recombination (DR), for the entire silicon-like isoelectronic sequence. Dielectronic recombination is generally the most important contribution to the total recombination rate of atomic ions. This study will serve as …

Time-Dependent Photoionization Of Gaseous Nebulae, Ehab Elsayed Elhoussieny Ahmed

Dissertations

We study time-dependent photoionization of gaseous nebulae, i.e. the physical conditions and spectra of astronomical plasmas photoionized by a time-dependent source of ionizing radiation. Our study proceeds in two chief steps: First, we start with a simplified model of plasmas of pure H. Second, we develop a more realistic model of plasmas composed of a mixture of chemical elements. For the first step, we wrote a time-dependent photoionization code (TDP) that solves the coupled system of equations for ionization, energy balance, and radiation transfer in their full time-dependent forms For the second step, we developed a more realistic code (TDXSTAR) …

Crystallography And Magnetism Of Magnetocalorically Important Ni-Mn-X Based Heusler Alloys, Amila S. B. Madiligama

Dissertations

Ni-Mn-X Heusler alloys, demonstrating strong coupling between crystalline structure and magnetic state, were studied. They undergo field-induced, first-order transformations from a low symmetry martensite to a high-symmetry austenitic phase around room temperature. The substantial difference between the entropies of the two phases results in a large adiabatic temperature change, called “Giant Magnetocaloric Effect (GMCE)”. Consequently, these alloys are promising refrigerants for near-room temperature cooling systems. This magnetic cooling is an energy-efficient and eco-friendly technology.

Crystalline structures and magnetic states of these alloys, which determine their magnetocaloric performances, highly depend on their composition. To examine new paths to optimize their magnetocaloric …

An R-Matrix, Quantum Defect Theory Approach To The Photoionization Of Molecular Nitrogen, Gaetan L. Vangyseghem

Dissertations

No abstract provided.

Deposition And Characterization Of Carbon Nanotubes (Cnts) Based Films For Sensing Applications, Amila C. Dissanayake

Dissertations

The advent of carbon nanotubes (CNTs) has opened up lot of novel applications because of their unique electrical and mechanical properties. CNTs are well known material for its exceptional electrical, mechanical, optical, thermal and chemical properties. A single-wall nanotube (SWNT) can be either semiconducting, metallic or semi-metallic, based on its chirality and diameter. SWNTs can be used in transistor device as active channels due to high electron mobility (~10000 cm2/(V s), electrical interconnects, nano-scale circuits, field-emission displays, light-emitting devices and thermal heat sinks due to low resistivity, high current density (~109A cm-2) and high thermal conductivity (~3500 W m-1). Further, …

Electron Transmission Through Micrometer Sized Funnelshaped Tapered Glass Capillaries And Electron Micro-Beam Production, Samanthi Jayamini Wickramarachchi

Dissertations

The prime motivation of this work is to understand the fundamental transmission process of an electron beam through a funnel-shaped capillary taking into account its shape together with the energy, angular and time dependence of the transmitted electrons produce a microsized electron beam. The utilized capillaries had inlet/outlet diameters of 800/16 μm, 800/100 μm and lengths of 35 mm. Considerable transmission of 800 and 1000 eV electrons for tilt angles up to 1.5^o and only small transmission for 500 eV electrons was observed for the capillary with the smaller outlet diameter of 16 μm. Incident electrons with energies of …

Integrating Formative Assessment Into Physics Instruction: The Effect Of Formative Vs. Summative Assessment On Student Physics Learning And Attitudes, Chaiphat Plybour

Dissertations

Of many instructional strategies used to improve teaching and learning in science, formative assessment is potentially one of the most effective. A central feature is timely feedback during learning, giving students the opportunity to benefit and improve while also enabling teachers to adjust instruction to learner needs. By contrast, conventional assessment tends to be mostly summative, assigning point scores, grading and ranking students, and providing extrinsic motivation. For maximum effectiveness in enhancing learning, formative assessment should be designed into instruction from the start rather than being an add-on. This project comprised development, teaching, and research aspects. Two physics topic modules, …

The Experiences Of Women In Post Graduate Physics And Astronomy Programs: The Roles Of Support, Career Goals, And Gendered Experiences, Ramón S. Barthelemy

Dissertations

In physics and astronomy the low representation of women is obvious at every stage of the educational pathway from undergraduate students to full professors. These low numbers perpetuate themselves by failing to create new mentors to foster the next generation of women. Women and men also have different experiences as they traverse into physics and astronomy careers. Women often experience chilly climates, discrimination, and challenges coordinating the demands of young families with their careers. In the literature exploring this topic, little focus is put on the experiences of women graduate students in physics and no focus is put on women …

Studies Of The Quantum Phase Transition In Chromium Using Inelastic X-Ray Scattering And Ab Initio Methods, Chengyang Li

Dissertations

In this project, inelastic x-ray scattering (IXS) was used to measure the phonon dispersion in chromium at high pressure and low temperature, and an ab initio method was used to simulate the phonon dispersion with different lattice constants and magnetic orders. The IXS measurements were carried out in Sector 30 at the Advanced Photon Source at Argonne National Laboratory. Data were taken at room temperature with pressures of 1.29 GPa, 8.15 GPa, 10.6 GPa, and at 5 K with a pressure of 18.36 GPa. The data shows similar phonon behavior in the antiferromagnetism (AFM) and the spin density wave (SDW) …

Development Of Polarization Analysis Of Resonant Inelastic X-Ray Scattering, Xuan Gao

Dissertations

Resonant inelastic x-ray scattering (RIXS) is a powerful technique in condensed matter physics for studying the electronic excitations in novel materials of interest. In currently operating hard x-ray RIXS instruments the energy and momentum transfers are measured while the outgoing polarization is not measured due to significant technical challenges. But the outgoing polarization of the scattered photons provides valuable information (excitation symmetry) about the states involved in the scattering which is difficult to determine without polarization analysis. Polarization analysis has proved extremely valuable in soft x-ray RIXS, and so a polarization analysis system is being developed to fill the technical …

Organic Solar Cells Based On High Dielectric Constant Materials: An Approach To Increase Efficiency, Khalil Jumah Tawfiq Hamam

Dissertations

The efficiency of organic solar cells still lags behind inorganic solar cells due to their low dielectric constant which results in a weakly screened columbic attraction between the photogenerated electron-hole system, therefore the probability of charge separating is low. Having an organic material with a high dielectric constant could be the solution to get separated charges or at least weakly bounded electron-hole pairs. Therefore, high dielectric constant materials have been investigated and studied by measuring modified metal-phthalocyanine (MePc) and polyaniline in pellets and thin films. The dielectric constant was investigated as a function of temperature and frequency in the range …

Compositional And Structural Analysis Of Nitrogen Incorporated And Ion Implanted Diamond Thin Films, Elias James Garratt

Dissertations

Significant progress in area of nano-structured thin film systems has taken place in recent decades. In particular, diamond thin film systems are being widely studied for their wear resistant, optical and electronic properties. Of the various methods researchers use to modify the structure of such films, three techniques in particular are of interest due to their versatility: modification of the growth atmosphere, growth on metalized substrates, providing an interfacial layer, and modification through post-growth ion implantation. The aim of this study is to investigate the effects each has to the structure and composition of elements. Different techniques are applied in …

Engineered Interfaces And Nano-Scale Thin Films For Solid Oxide Fuel Cell Electrolytes, Manjula I. Nandasiri

Dissertations

Solid state electrolytes with high oxygen ionic conductivity at low temperatures are required to develop cost effective and efficient solid oxide fuel cells. This study investigates the influence of engineered interfaces on the oxygen ionic conductivity of nano-scale multilayer thin film electrolytes. The epitaxial Sm₂O₃ doped C_eO₂ (SDC) and Sc₂O₃ stabilized ZrO₂ (ScSZ) are selected as the alternative layers for the proposed multilayer thin film electrolyte based on the optimum structural, chemical, and electrical properties reported in the previous studies. The epitaxial SDC(111)/ScSZ(111) multilayer thin films are grown on high …

Localized Surface Plasmon Resonance Induced Structure-Property Relationships Of Metal Nanostructures, Subramanian Vilayurganapathy

Dissertations

The confluence of nanotechnology and plasmonics has led to new and interesting phenomena. The industrial need for fast, efficient and miniature devices which constantly push the boundaries on device performance tap into the happy marriage between these diverse fields. Designing devices for real life application that give superior performance when compared with existing ones are enabled by a better understanding of their structure-property relationships. Among all the design constraints, without doubt, the shape and size of the nanostructure along with the dielectric medium surrounding it has the maximum influence on the response and thereby the performance of the device. Hence …

Radiative Double Electron Capture In Collisions Of Fully-Stripped Fluorine Ions With Thin Carbon Foils, Tamer Mohammad Samy Elkafrawy

Dissertations

Radiative double electron capture (RDEC) is a one-step process in ion-atom collisions occurring when two target electrons are captured to a bound state of the projectile simultaneously with the emission of a single photon. The emitted photon has approximately double the energy of the photon emitted due to radiative electron capture (REC), which occurs when a target electron is captured to a projectile bound state with simultaneous emission of a photon. REC and RDEC can be treated as timereversed photoionization (PI) and double photoionization (DPI), respectively, if loosely-bound target electrons are captured. This concept can be formulated with the principle …

Modeling Transmission Of Photonic Crystal Waveguide Modes Enhanced By Kerr Nonlinearity, Buddhi M. Rai

Dissertations

Nonlinear modes of electromagnetic fields propagating in photonic crystal systems have been studied by implementing various computer simulation techniques using electromagnetic theory. The fundamentals of simulation of photonic crystals are analyzed using general purpose methodologies such as the FDTD or PWE methods. Information derived from the underlying physical insights into the systems could be utilized to describe the control mechanisms over the propagation of the modes around impurities in the photonic crystal lattice. The impurities trap the resonantly localized electromagnetic modes having a frequency in a stop band of the photonic crystal, suggesting novel optical controls in the photonic crystal …