Physical Sciences and Mathematics Commons^™

Radiative Double Electron Capture In Collisions Of Fully-Stripped Fluorine Ions With Thin Carbon Foils, Tamer Mohammad Samy Elkafrawy

Dissertations

Radiative double electron capture (RDEC) is a one-step process in ion-atom collisions occurring when two target electrons are captured to a bound state of the projectile simultaneously with the emission of a single photon. The emitted photon has approximately double the energy of the photon emitted due to radiative electron capture (REC), which occurs when a target electron is captured to a projectile bound state with simultaneous emission of a photon. REC and RDEC can be treated as timereversed photoionization (PI) and double photoionization (DPI), respectively, if loosely-bound target electrons are captured. This concept can be formulated with the principle …

Novel Production Techniques Of Radioisotopes Using Electron Accelerators, Daniel Robert Lowe

UNLV Theses, Dissertations, Professional Papers, and Capstones

Non-traditional radioisotope production techniques using a compact, high power linear electron accelerator have been demonstrated and characterized for the production of 18F, 47Sc, 147Pm, and 99mTc from a variety of target candidates. These isotopes are used extensively in the medical field as diagnostic and therapy radioisotopes, as well as the space industry as RTG's. Primary focus was placed on 99mTc as it constitutes approximately 80% of all diagnostic procedures in the medical community that use radioactive tracers. It was also the prime focus due to recent events at the Chalk River nuclear reactor, which caused global shortages of this isotope …

Evaluation Of Tagging Techniques Gamma-Decay Probabilities Using The Surrogate Method, Timothy Lee Reed

Masters Theses

A detailed analysis of the statistical and discrete [gamma]-decay tagging techniques was conducted using the absolute surrogate and surrogate ratio method (SRM) to obtain the 92Mo(n,[gamma]) cross section in an equivalent neutron energy range of 80 to 880 keV. Excited 93Mo and 95Mo nuclei were populated using (d,p) reactions on 92Mo and 94Mo targets, respectively. The absolute surrogate 92Mo(n,[gamma]) cross sections disagreed with evaluated neutron capture cross section data by as much as a factor of 4 using the statistical tagging approach, whereas the discrete [gamma]-decay tag absolute surrogate cross section disagreed with the evaluated neutron capture cross section by …

Testing A Novel Technique To Improve Aluminum-26 Accelerator Mass Spectrometry Measurements For Earth Science Applications, Meghan Sarah Janzen

Masters Theses

The measurement of cosmogenic ²⁶Al [aluminum-26] in geological samples by accelerator mass spectrometry (AMS) is typically conducted on Al₂O₃ [aluminum oxide] targets. However, Al₂O₃ is not an ideal source material because it does not form a prolific beam of Al^- [negative atomic aluminum ions] required for measuring low-levels of ²⁶Al. This thesis presents the performance of AlN [aluminum nitride], AlF₃ [aluminum fluoride] and mixed AlN + Al₂O₃ as novel alternative source materials for the analysis of ²⁶Al. A negative ion cesium sputtering source at the Holifield …

Mapping Nuclear Fallout Using The Weather Research & Forecasting (Wrf) Model, Joseph C. Schofield

Theses and Dissertations

There are many models that attempt to predict transport & dispersion (T&D) of particulate matter in the sensible atmosphere. The majority of these existing models are unable to incorporate atmospheric processes such wet deposition through scavenging and cloud condensation nuclei (CCN) formation. To this end, the numerical weather prediction (NWP) model known as the Weather Research & Forecasting with Chemistry (WRF/Chem) Model is studied to determine its suitability as a potential tool for predicting particulate T&D following an atmospheric nuclear detonation. This is done by modifying relevant modules, originally designed to predict the settling of volcanic ash, such that a …

Secondary Light Particle Data Base Development Using A Thermodynamic Coalescence Model, Mahmoud Pourarsalan

Doctoral Dissertations

ABSTRACT

As heavy ions are transported through shielding and interact with shielding materials accurate values of total, elastic scattering, reactions cross sections and angular distributions of the emitted nucleons, light high energy particles such as deuteron, triton, helion, alpha particles and other heavy ions are required in order to design appropriate and adequate shielding to protect the human crews and instruments from ionizing radiations during long duration space missions. Double-differential (energy and angle) light energetic particle production cross sections must be known for ion energies from tens of MeV/nucleon to tens of GeV/nucleon for all emitted light energetic particles for …

Microscopic Description Of Nuclear Fission At Finite Temperature, Jordan David Mcdonnell

Doctoral Dissertations

While a predictive, microscopic theory of nuclear fission has been elusive, advances in computational techniques and in our understanding of nuclear structure are allowing us to make significant progress. Through nuclear energy density functional theory, we study the fission of thorium and uranium isotopes in detail. These nuclides have been thought to possess hyperdeformed isomers in the third minima of their potential energy surfaces, but microscopic theories tend to estimate either shallow or non- existent third minima in these nuclei. We seek an explanation in terms of neutron shell effects. We study how the fission pathways, the symmetry, and the …

An Extension To Particle Polarizability To Predict Coupling Behavior In Periodic Nanoplasmonic Arrays, Drew Dejarnette

Graduate Theses and Dissertations

Plasmonic nanoparticles organized in arrays interact to create spectral patterns which are amplified by individual particle polarizability. It was hypothesized that particle polarizability could be used as a predictor of spectral behavior from far-field interactions within the array. Inter-particle coupling produced an extraordinary peak in extinction efficiency at wavelengths equal to or larger than the single particle plasmon resonance peak. Interactions that produced constructive coupling were found to mimic changes in the particle polarizability model. Testing of the hypothesis was performed using the coupled dipole approximation with parametric characterization of array geometries, giving specific particle size and lattice constant combinations …

Phase Control In Atomic Coherence, Utsab Khadka

Graduate Theses and Dissertations

In this thesis, atomic coherence is used to enhance nonlinear optical processes in multi-level atoms. The multi-photon transitions are driven resonantly, and at the same time without absorptive losses, by using electromagnetically induced transparency (EIT), thereby allowing the study of χ⁽³⁾ and χ⁽⁵⁾ nonlinearities using weak driving fields. The coherently modified probe beam(s) and the atom-radiated signal fields arising from four- and six- wave- mixing (FWM and SWM) processes are measured in the spectral, temporal and spatial domains.

In a three-level ladder-type atomic system, multiple peaks having spectral asymmetries are observed in the EIT window as well as …

Evaluating Actinide Sorption To Graphite With Regards To Triso Repository Performance, Corey Christopher Keith

UNLV Theses, Dissertations, Professional Papers, and Capstones

Graphite has the potential for inclusion in nuclear waste for disposal in waste repository settings. Implementation of High Temperature Gas-cooled Reactors contributes to this potential through use of TRISO fuel, if direct disposal of the graphite matrix surrounding the fuel is employed. The inclusion of the large mass and volume in the TRISO fuel waste form differs significantly from used light water reactor fuel waste forms, requiring new performance models to describe the behavior in a repository setting. The purpose of this study is to evaluate the potential for the graphite to improve actinide, specifically uranium and neptunium, retardation from …

Higher-Order Corrections In Effective Theory Of Deformed Nuclei, Jialin Zhang

Masters Theses

The low-energy excitation bands of open-shell heavy nuclei have been accounted for by collective motion of the constituting nucleons. Macroscopically, heavy nuclei can be looked upon as deformed rotors undergoing surface vibration and rotation. Traditionally, deformed nuclei are described within the Bohr-Mottelson geometric model or the interacting boson model. An effective theory that exploits spontaneous symmetry breaking has recently been developed for axially deformed nuclei. It describes the rotational and vibrational degrees of freedom in terms of Nambu-Goldstone bosons and quadrupole phonons respectively, with a power counting based on their different energy scales. A systematic way to construct the rotationally …

Calibration Of A Silver Detector Using A Pube Source, Melanie E. Mace

Theses and Dissertations

During the initial design of the Field Reversed Compression and Heating Experiment (FRCHX), magnetohydrodynamic simulations performed by Los Alamos National Laboratory using MACH2 predicted a neutron yield on the order of 10¹² neutrons. However, Air Force Research Laboratory (AFRL) measurements indicate a total of 10⁷-10⁸ neutrons are generated from the FRCHX. A PuBe source was used to create a burst of neutrons to calibrate an AFRL silver detector based on distance to determine if the four order of magnitude discrepancy was cause by an improperly calibrated detector. It was determined that the calibration equation in use …

Mri-Based Attenuation Correction In Emission Computed Tomography, Harry R. Marshall

Electronic Thesis and Dissertation Repository

The hybridization of magnetic resonance imaging (MRI) with positron emission tomography (PET) or single photon emission computed tomography (SPECT) enables the collection of an assortment of biological data in spatial and temporal register. However, both PET and SPECT are subject to photon attenuation, a process that degrades image quality and precludes quantification. To correct for the effects of attenuation, the spatial distribution of linear attenuation coefficients (μ-coefficients) within and about the patient must be available. Unfortunately, extracting μ-coefficients from MRI is non-trivial. In this thesis, I explore the problem of MRI-based attenuation correction (AC) in emission tomography.

In particular, I …

Experimental Studies Of Nuclei Near Doubly Magic 100sn And 78ni, Lucia Cartegni

Doctoral Dissertations

The experimental study of exotic nuclei is very important for our understanding of nuclear structure. In this work the nuclei near doubly magic nuclei 100Sn and 78Ni were studied in two separate experiments. The first one was performed at the Holifield Radioactive Ion Beam Facility (HRIBF) at Oak Ridge National Laboratory. This experiment searched for the alpha decay of 112Cs, in order to establish the proton separation energy of 104Sb. Although the alpha decay of 112Cs was not observed, the upper limit of the alpha branching ratio was set at 0.26%. The improved statistics enabled an improved half-lives measurement of …

A High-Energy Neutron Flux Spectra Measurement Method For The Spallation Neutron Source, Nicholas Patrick Luciano

Masters Theses

The goal of this work was to develop a foil activation method to measure high-energy (∼1-100 MeV) neutron flux spectra at the Spallation Neutron Source by researching the scientific literature, assembling an experimental apparatus, performing experiments, analyzing the results, and refining the technique based on experience. The primary motivation for this work is to provide a benchmark for the neutron source term used in target station and shielding simulations Two sets of foil irradiations were performed, one at the ARCS beamline and one at the POWGEN beamline. The gamma radiation of the foil activation products was measured with a high …

Single And Double Spin Asymmetries For Pion Electro-Production From The Deuteron In The Resonance Region, Sharon L. Careccia

Physics Theses & Dissertations

The single and double spin asymmetries A_t and A_et have been measured in π^- electro-production off the deuteron using a longitudinally polarized electron beam and a polarized ND₃ target. The electron beam was polarized using a strained GaAs cathode and the target was polarized using Dynamic Nuclear Polarization. The data were collected at beam energies of 1.6, 1.7, 2.5 and 4.2 GeV in Hall B at Jefferson Lab in the spring of 2001. The final state particles were detected in the CEBAF Large Acceptance Spectrometer (CLAS). The d(e,e'π-p)p exclusive channel was identified using the missing mass …

Positron Lifetime Modulation By Electric Field Induced Positronium Formation On A Gold Surface, Daniel J. Higgins

Theses and Dissertations

The purpose of this project is to study the lifetime and annihilation mode of positrons, the antimatter counterpart to electrons, and the formation rate of positronium on a gold surface modified by gold nanoparticles under the influence of radial electric fields measured using two independent systems. The positron annihilation photon pair/triplet spectroscopy system uses a sodium iodide ring detector segmented into six detection regions providing rough position sensitivity to measure the ratio of two to three photon positron annihilation events. An increased rate of three photon annihilation events and a decreased rate of two photon annihilation events are observed when …

Design And Characterization Of A Three-Dimensional Positron Annihilation Spectroscopy System Using A Low-Energy Positron Beam, Stephen M. Jimenez

Theses and Dissertations

Previous forays by AFIT into positron research have resulted in the development of a new positron annihilation spectroscopy (PAS) technique and the procurement of a low-energy positron beam system. The primary purpose of this research was to design and build a state-of-the-art PAS laboratory at AFIT capable to address a myriad of DoD solid-state and surface physics questions. The main objectives were to acquire and assemble utilities to operate a positron beam, assemble and configure an ultra-high vacuum (UHV) system for samples, design and build an interface with a magnetic field to propagate positrons onto samples, and create a new …

Durability Of Mwcnt Composites Under Electron And Neutron Irradiation, Quan-Hai T. Lu

Theses and Dissertations

Electromagnetic interference shielding effectiveness and conductive properties of carbon nanotube containing composites intended for use as satellite surface materials have been investigated following electron and neutron irradiation. The MWCNT composites were irradiated to fluence levels of 10¹⁶ electrons/cm² with 500 keV electrons. Increase in EMI-SE and conductivity was observed following electron irradiation in two of the samples. The sample with alternating layers of MWCNT and glass had a decrease in conductivity and an increase in EMI-SE post irradiation. This would suggest that the different layered configuration does play a role in the durability of the composite. Having multiple …

Neutron Detection Using Amorphous Boron-Carbide Hetero-Junction Diodes, Thomas P. Mcquary

Theses and Dissertations

The high energy products of the ¹⁰B(n,α)⁷Li neutron capture reaction were explored as a means of thermal neutron detection in thin film amorphous boron carbide (a--B₅C:H_x) on n-type silicon hetero-junction diodes. Pulse height spectroscopy was conducted on the diodes while they were subjected to a moderated plutonium-beryllium (PuBe) source. Neutron capture could not be confirmed experimentally in any of the devices tested. Device modeling was performed to investigate the cause for the diode detector's negative response. A 1.47 MeV α particle produced transient current of 10^-7 A and the induced was 4.7 …

Measurement Of Single And Double Spin Asymmetries In P(E, E' Pi(+/-,0))X Semi-Inclusive Deep-Inelastic Scattering, Sucheta Shrikant Jawalkar

Dissertations, Theses, and Masters Projects

Measurements in the late 1980s at CERN revealed that quark spins account for a small fraction of the proton's spin. This so-called spin crisis spurred a number of new experiments to identify the proton's silent spin contributors, namely, the spin of the gluons, which hold the quarks together, and the orbital angular momentum of both quarks and gluons. One such experiment was eg1-dvcs at the Thomas Jefferson National Accelerator Facility in Newport News, Va., which ran in 2009 and collected approximately 19 billion electron triggers for hydrogen. I will present new measurements of the single and double-spin asymmetries ALU, AUL …

The First Direct Measurement Of The Weak Charge Of The Proton, John Poague Leckey Iv

Dissertations, Theses, and Masters Projects

Qweak is an experiment currently running at the Thomas Jefferson National Accelerator Facility that uses parity-violating elastic electron-proton scattering to measure the weak charge of the proton QPweak . Longitudinally polarized electrons are scattered off a liquid hydrogen target and pass through a toroidal-field magnetic spectrometer. This experiment is a sensitive test for physics beyond the Standard Model, as QPweak is well predicted in the Standard Model. This dissertation describes the first direct measurement of QPweak . The precision that will be generated by the final 4% measurement will allow the probing of certain classes of new physics up to …

Dark Matter In The Heavens And At Colliders: Models And Constraints, Reinard Primulando

Dissertations, Theses, and Masters Projects

In this dissertation, we investigate various aspects of dark matter detection and model building. Motivated by the cosmic ray positron excess observed by PAMELA, we construct models of decaying dark matter to explain the excess. Specifically we present an explicit, TeV-scale model of decaying dark matter in which the approximate stability of the dark matter candidate is a consequence of a global symmetry that is broken only by instanton-induced operators generated by a non-Abelian dark gauge group. Alternatively, the decaying operator can arise as a Planck suppressed correction in a model with an Abelian discrete symmetry and vector-like states at …

Parity-Violating Asymmetry In The Nucleon To Delta Transition: A Study Of Inelastic Electron Scattering In The G0 Experiment, Carissa Lee Capuano

Dissertations, Theses, and Masters Projects

The parity-violating asymmetry arising from inelastic electron scattering at backward angle (∼ 95??) near the Delta resonance has been measured for both hydrogen and deuterium targets as part of the G 0 experiment. For Q2 = 0.34 (GeV/c) 2 and W = 1.18 GeV, the asymmetries were found to be AHinel=-33.4+/-5 .3stat+/-5 .1sysppm, ADinel=-43.6+/-1 4.6stat+/- 6.2sysppm. .;From the hydrogen asymmetry, the axial transition form factor, GAND , can be extracted. GAND is related to probability of the quark spin-flip that occurs as the proton transitions to the Delta. From the measured asymmetry, the form factor is found to be GAND=-0.046+/- …