Physical Sciences and Mathematics Commons^™

Intracavity Phase Interferometry Based Fiber Sensors, Luke Jameson Horstman

Optical Science and Engineering ETDs

Intracavity Phase Interferometry (IPI) is a detection technique that exploits the inherent sensitivity of a laser's frequency to the parameters of its cavity. Intracavity interferometry is orders of magnitude more sensitive than its extracavity alternatives. This dissertation improves on previous free-space proof-of-concept designs. By implementing the technique in fiber optics, using optical parametric oscillation, and investigating non-Hermitian quantum mechanics and dispersion tailoring enhancement techniques, IPI has become more applicable and sensitive. Ring and linear IPI configurations were realized in this work, both operating as bidirectional fiber optical parametric oscillators. The benefit of using externally pumped synchronous optical parametric oscillation is …

Effects Of Anharmonicity In A Dual-Sagnac Interferometer, Stephen Thomas

Honors College Theses

A recent experiment implemented a dual Sagnac atom interferometer (AI) for rotation sensing using a Bose-Einstein condensate (BEC) confined in a TOP-trap potential. The BEC is split twice by laser light to create two pairs of counter-orbiting clouds in a lowest-order harmonic potential with each pair acting as a separate Sagnac interferometer. After one orbit the two overlapping cloud pairs are split again and the interference patterns are inferred from the population of atoms in the zero-momentum state. We have simulated the impact of the presence of anharmonic terms in the potential on the performance of the AI as measured …

Development Of A Magnetic Confinement Attachment For Enhanced Signal In Handheld Laser Induced Breakdown Spectroscopy Soil Analysis, Alfred C. Anderson

Theses and Dissertations

Field techniques for characterizing low levels of heavy elements of less than 100 parts per million in soils tend to be unreliable because of the relatively weak signal of these elements and the large, variable background inherent to analyzing soils with minimal sample preparation. To enhance the detection and analysis capability of a handheld laser-induced breakdown spectroscopy (LIBS) instrument, this work investigates the effects of a unique magnetic confinement apparatus on signal intensities, focusing on five iron lines as well as those from actinides in 11 soil samples. The proposed magnetic confinement apparatus achieved over 0.8 T but did not …

Sigesn Light-Emitting Devices: From Optical To Electrical Injection, Yiyin Zhou

Graduate Theses and Dissertations

Si photonics is a fast-developing technology that impacts many applications such as data centers, 5G, Lidar, and biological/chemical sensing. One of the merits of Si photonics is to integrate electronic and photonic components on a single chip to form a complex functional system that features compact, low-cost, high-performance, and reliability. Among all building blocks, the monolithic integration of lasers on Si encountered substantial challenges. Si and Ge, conventional epitaxial material on Si, are incompetent for light emission due to the indirect bandgap. The current solution compromises the hybrid integration of III-V lasers, which requires growing on separate smaller size substrates …

Ultrafast Magnetic Entropy Dynamics With Time-Resolved Pump-Probe Magneto-Optical Technique., Sahar Goharshenasanesfahani

Electronic Theses and Dissertations

It has been observed that ultrathin films, multilayers, or magnetic nanostructures indicate novel magnetic phenomena that differ profoundly from the respective bulk properties. Besides, because of the broad applications of these magnetic materials in the industry, they are an exciting research area. Hence, investigating the low-dimensional magnetic systems is one of the most active fields in experimental condensed matter physics. Magnetization dynamics can occur over a wide range of time scales (from seconds to femtoseconds). Some of these processes even occur on time scales as short as a few picoseconds (10^-12s) or femtoseconds (10^-15s). Measurement of …

Parity-Time Symmetry In A Coherent Atomic Medium, Jingliang Feng

Graduate Theses and Dissertations

Parity-time (PT) symmetry has attracted considerable attention since optics was realized with the ability to provide a fertile platform for the exploration of PT symmetry. Although many of the previous researches on PT symmetry have been conducted in solid-state system and the network of fiber loops, coherent atomic medium offers another platform for the exploration of PT symmetry due to its easy reconfigurability and flexible tunability in parameters.

This dissertation mainly focuses on the investigations of the phenomena related to PT-symmetric optical lattice in a coherent atomic medium. First, a controllable photonic crystal with periodic Raman gain was constructed in …

Variational Energies For The Rydberg P States Of Helium, Cody Mcleod

Electronic Theses and Dissertations

The aim of this work is to solve the quantum mechanical three-body problem for helium, and to obtain high precision eigenvalues for the higher-lying Rydberg states where previous methods have been of limited accuracy. A variational method in correlated Hylleraas coordinates is used involving three distinct distance scales, called a triple basis set. The eigenvalues and matrix elements of other operators are computed for P states of helium up to n = 15 using the varational method with a triple basis set in Hylleraas coordinates. The construction of the wave functions, as well as the behaviour of the asymptotic, intermediate …

Neutron Energy Tuning Assemblies For Nuclear Weapon Environment Applications At The National Ignition Facility, Nicholas J. Quartemont

Theses and Dissertations

An energy tuning assembly was developed to spectrally shape the National Ignition Facility deuterium-tritium fusion neutron source to a notional thermonuclear and prompt fission neutron spectrum to fulfill neutron source capability gaps. The experimental neutron environment was characterized with activation dosimetry, neutronics and covariance models, and unfolded to determine the as-fielded neutron spectrum. The first energy tuning assembly was demonstrated to create synthetic spectrally accurate post-detonation fission products, enhancing U.S. technical nuclear forensics capabilities. ATHENA, a second-generation energy tuning assembly, was also optimized to meet similar objectives, but the new platform neutron fluence efficiency was increased by a factor of …

Nonlinear Optical Studies Of Interfacial Ferroelectricity And Strain Distribution In Perovskite Dielectric Films, Tony Le

Dissertations, Theses, and Capstone Projects

Dielectric and ferroelectric perovskite films have been model energy storage structures for their low-dielectric loss, extremely high charge-discharge speed, and good temperature stability, yet there is still much to understand about the material’s limitations. This dissertation presents a detailed understanding of the strain-induced ferroelectricity at the boundary between a strontium titanate (SrTiO₃) ultrathin film epitaxially grown on a germanium (Ge) substrate through optical second harmonic generation (SHG), and the polydomain distribution in the Zr-doped BaTiO₃ (BZT) films by time-resolved pump-probe spectroscopy.

First, SHG measurements were performed to reveal interfacial ferroelectricity in the epitaxial SrTiO₃/Ge (100) …

Fabrication Of Specialized Scintillators For Nuclear Security Applications, Cordell James Delzer

Doctoral Dissertations

Radiation detectors are important for a variety of fields including medical imaging, oil drilling, and nuclear security. Within nuclear security, they can serve a multitude of purposes whether that be imaging, localization, isotopic identification, or even just activity measurement. Even without directly seeing a nuclear material it is often able to notice their existence without a detector. Scintillators make up an important part of these detectors due to their large intrinsic efficiency, low cost, large volume, and relatively low upkeep. Due to the importance of the large number of purposes these scintillators may be used for, it can often be …

Modeling Of Argon Bombardment And Densification Of Low Temperature Organic Precursors Using Reactive Md Simulations And Machine Learning, Kwabena Asante-Boahen

MSU Graduate Theses

In this study, an important aspect of the synthesis process for a-BxC:Hy was systematically modeled by utilizing the Reactive Molecular Dynamics (MD) in modeling the argon bombardment from the orthocarborane molecules as the precursor. The MD simulations are used to assess the dynamics associated with the free radicals that result from the ion bombardment. By applying the Data Mining/Machine Learning analysis into the datasets generated from the large reactive MD simulations, I was able to identify and quality the kinetics of these radicals. Overall, this approach allows for a better understanding of the overall mechanism at the atomistic level of …

Fabrication And Characterization Of Photodetector Devices Based On Nanostructured Materials: Graphene And Colloidal Nanocrystals, Wafaa Gebril

Graduate Theses and Dissertations

Photodetectors are devices that capture light signals and convert them into electrical signals. High performance photodetectors are in demand in a variety of applications, such as optical communication, security, and environmental monitoring. Among many appealing nanomaterials for novel photodetection devices, graphene and semiconductor colloidal nanocrystals are promising candidates because of their desirable and unique properties compared to conventional materials.

Photodetector devices based on different types of nanostructured materials including graphene and colloidal nanocrystals were investigated. First, graphene layers were mechanically exfoliated and characterized for device fabrication. Self-powered few layers graphene phototransistors were studied. At zero drain voltage bias and room …

Self-Contained Photon Coincidence Counting With Ni Myrio Ecosystem, Georges Oates Larsen, Andres H. La Rosa

University Honors Theses

Digital coincidence counting units (CCU) have made experimental verification of fundamental quantum mechanical principles financially accessible to undergraduate level teaching programs. However, recent implementations of these systems are not easily ported to National Instruments (NI) FPGAs, making them unsuitable for physics departments that have heavily invested in the NI ecosystem. Therefore, there is clear need for a detailed implementation based on an NI FPGA. We present a formal description of one such implementation, based on the NI myRIO (NI's lower-cost, student-oriented offering) which achieves 6.9 ns minimum guaranteed-distinguishable delay and 32.2 MHz peak coincidence counting rate with four input channels …

Correlated Positron-Electron Orbital (Cpeo): A Novel Method That Models Positron-Electron Correlation In Virtual Ps At The Mean-Field Level, Kevin E. Blaine

Theses and Dissertations

The Correlated Positronic-Electronic Orbital (CPEO) method was developed and implemented to capture correlation effects at between the positron and electron in the modeling of systems that involve a bound positron. Methods that effectively model these systems require many hundred basis functions and use a mean field approach as the beginning step. CPEO builds an orbital for virtual Positronium (Ps) that contains a positron in a bound state along with an accompanying electron to the larger system. Assigning the virtual Ps orbital allows for the two particle variational optimization in conjunction with the other particles that compose the whole system. This …

Design And Characterization Of Standard Cell Library Using Finfets, Phanindra Datta Sadhu

Master's Theses

The processors and digital circuits designed today contain billions of transistors on a small piece of silicon. As devices are becoming smaller, slimmer, faster, and more efficient, the transistors also have to keep up with the demands and needs of the daily user. Unfortunately, the CMOS technology has reached its limit and cannot be used to scale down due to the transistor's breakdown caused by short channel effects. An alternative solution to this is the FinFET transistor technology, where the gate of the transistor is a three dimensional fin that surrounds the transistor and prevents the breakdown caused by scaling …

A Theoretical Study Of Synchronous Proton Transfer In (Hf)N, (H2O) N, And (Hcl) N Where N = 3, 4, 5, Johnny Yang

Honors Theses

For (HF)_n, (H₂O)_n, and (HCl)_n (n = 3 − 5), we have rigorously characterized the structures for the minima and transition states for synchronous proton transfer (SPT) with the CCSD(T) method and aug-cc-pVTZ basis set. The electronic barrier heights (∆E^†) associated with these transition states have also been computed with the explicitly correlated CCSD(T)-F12 method and the aug-cc-pVQZ-F12 basis set (abbreviated aQZ-F12). (HCl)_n (n = 3 − 5) SPT transition states have not been previously identified to the best of our knowledge, and they have been found …

Can Parallel Gravitational Search Algorithm Effectively Choose Parameters For Photovoltaic Cell Current Voltage Characteristics?, Alan Kirkpatrick

Honors Projects

This study asks the question “Can parallel Gravitational Search Algorithm (GSA) effectively choose parameters for photovoltaic cell current voltage characteristics?” These parameters will be plugged into the Single Diode Model to create the IV curve. It will also investigate Particle Swarm Optimization (PSO) and a population based random search (PBRS) to see if GSA performs the search better and or more quickly than alternative algorithms

Simulating Many Body Localization With Rydberg Atoms, Alicia Handian

Physics and Astronomy Honors Papers

In thermodynamics, interacting systems are expected to achieve equilibrium with one another over the course of time. However, there are exceptions to this rule. When systems localize, or fail to reach equilibrium, information about the initial state of the system is preserved and locally observable after long periods of time. Many-body localization focuses on systems of interacting particles that fail to thermalize. We have developed a simulation that models the behavior of a many-body quantum system. The simulation is inspired by experiments conducted by Liu, et al., in their recent publication “Time Dependence of Few Body Forster Interactions Among Ultracold …

Investigation Of G Protein-Coupled Receptor Quaternary Structure Through Fluorescence Micro-Spectroscopy And Theoretical Modeling: Interdependence Between Receptor-Receptor And Receptor-Ligand Interactions, Joel David Paprocki

Theses and Dissertations

Proteins are of high interest in biophysics research due to the important roles they play within cells, such as sensing of chemical (ions and small molecules) and physical (e.g., light) stimuli, providing structure, transporting ions/molecules, signaling, and intercellular communication. The studies described in this dissertation focus on a particular type of membrane proteins known as G protein-coupled receptors (GPCR), which play a key role in cellular response to external stimuli. We used the sterile 2 α-factor mating pheromone receptor (Ste2), a prototypical class D GPCR present within Saccharomyces cerevisiae (baker’s yeast). Ste2 is responsible for initiating the second messenger signal …

Non-Gaussian Measurements Of Coherent States Of Light For Metrology And Communication, Matthew Dimario

Physics & Astronomy ETDs

Conventional measurement technology is unable to extract the most amount of information possible from coherent states of light. Non-Gaussian measurements which can count individual photons can surpass the sensitivity limits of ideal conventional strategies, and approach the ultimate limits achievable given by quantum mechanics. This thesis presents investigations and demonstrations of these unconventional measurements, which utilize coherent operations and single photon counting. This thesis shows that non-Gaussian measurements can outperform conventional strategies in estimation tasks as well as a variety of communication problems. This thesis also investigates novel approaches and algorithms for building robustness to static and dynamic noise which …

Progress Towards Electromagnetic Manipulation And Trapping Of Micro-Particles, Andrew John Beling

Undergraduate Honors Theses

This thesis describes research to investigate the electromagnetic manipulation of microspheres and microrings. The work consists of three main thrusts: 1) the use of an electric field gradient to move dielectric microspheres, 2) the use of an AC magnetic field to move a conducting ring, and 3) the preparation of substrates for a microwave atom chip. The electrostatic movement of dielectric polyethylene microspheres was observed and recorded with a CCD imaging system. The microspheres were suspended in various liquids and placed on top of a microstrip transmission line, which consists of a conducting copper trace separated from a ground plate …

Structural Origin Of Thermal, Mechanical Properties And Morphological Behaviors Of Semiconducting Polymers, Song Zhang

Dissertations

The past decades have witnessed a surging exploration of semiconducting polymers for the application of wearable and flexible organic electronic devices. Despite the increased amounts of molecular engineered polymers and their much-improved electrical performances, a systematic study of the structure-thermal/mechanical property-morphology relationship of semiconducting polymers is still less investigated.

To understand the thin-film mechanical properties, a pseudo-free standing tensile tester was self-built and utilized to obtain their real-time stress-strain behaviors through uniaxial stretching on top of the water surface. It also enables the first quantitative measurement of fracture energy on ultrathin polymeric films. Through multiple mechanical testing methods (i.e., strain-rate …

Quantum Dynamical Phenomena In Non-Hermitian And Magnomechanical Systems, Saeid Vashahri Ghamsari

Graduate Theses and Dissertations

In this dissertation, we have investigated quantum dynamics via three case studies. First, we studied a system of two coupled waveguides respectively carrying optical damping and optical gain in addition to squeezing elements in one or both waveguides. Such a system is expected to generate highly entangled light fields in the two waveguides. We, however, show that the degree of the created entanglement is significantly affected by the quantum noises associated with the amplification and dissipation. Because of the noise effect, one can only have nonzero entanglement for a limited time interval. Second, we generalized the first project by considering …

Toward Improving Understanding Of The Structure And Biophysics Of Glycosaminoglycans, Elizabeth K. Whitmore

Electronic Theses and Dissertations

Glycosaminoglycans (GAGs) are the linear carbohydrate components of proteoglycans (PGs) that mediate PG bioactivities, including signal transduction, tissue morphogenesis, and matrix assembly. To understand GAG function, it is important to understand GAG structure and biophysics at atomic resolution. This is a challenge for existing experimental and computational methods because GAGs are heterogeneous, conformationally complex, and polydisperse, containing up to 200 monosaccharides. Molecular dynamics (MD) simulations come close to overcoming this challenge but are only feasible for short GAG polymers. To address this problem, we developed an algorithm that applies conformations from unbiased all-atom explicit-solvent MD simulations of short GAG polymers …

Smart Quantum Technologies Using Photons, Narayan Bhusal

LSU Doctoral Dissertations

The technologies utilizing quantum states of light have been in the spotlight for the last two decades. In this regard, quantum metrology, quantum imaging, quantum-optical communication are some of the important applications that exploit fascinating quantum properties like quantum superposition, quantum correlations, and nonclassical photon statistics. However, the state-of-art technologies operating at the single-photon level are not robust enough to truly realize a reliable quantum-photonic technology.

In Chapter 1, I present a historical account of photon-based technologies. Furthermore, I discuss recent efforts and encouraging developments in the field of quantum-photonic technologies, and major challenges for the experimental realization of reliable …

Computational Electromagnetic Modeling Of Metasurface Optical Devices With Defect Study, Carlos D. Diaz

Theses and Dissertations

One of the first fabricated metasurface optical devices, the in-plane V-antenna lenses, were plagued by a fundamental transmission limit (<25 >). Two distinct sets of Out-of-Plane phase elements were designed with improved transmission (~60 ). These were fabricated as beamsteerers and characterized in terms of their Bidirectional Transmittance Distribution Function measured as a function of scatter angle. Experimental data from the beamsteerers was analyzed via simulations using a finite element method (FEM). The measurements showed the designed beamsteering, but also a strong zero-order diffraction not present in the simulations, which motivated this study to understand what was causing these differences. …

Ab Initio Spectroscopy Of Natural And Artificial Fire Contaminants For V/W Band Frequency Signal Absorbance, Matthew B. Husk

Theses and Dissertations

The rotation and vibration spectral properties including frequencies and intensities for highly concentrated molecules present in wildland and artificial fires have been studied. These properties were used to determine absorption and its effect in a link budget analysis. Absorption in link budget analyses is commonly accounted for via line-by-line methodology aided by HITRAN documented intensities. Limited, if any, customization of spectral properties is available with HITRAN and other spectral databases. Ab initio calculations with different atomic basis sets were employed to obtain structures, dipole moments, rotational-vibrational frequencies and intensities, as well as various coupling parameters. Anharmonic corrections to the vibrational …

Error Reduction For The Determination Of Transverse Moduli Of Single-Strand Carbon Fibers Via Atomic Force Microscopy, Joshua D. Frey

Theses and Dissertations

The transverse modulus of single strand carbon fibers is measured using PeakForce Atomic Force Microscopy - Quantitative Nanomechanical Measurement to less than 5 percent error for 11 types of carbon fiber with longitudinal moduli between 924-231 GPA, including export-controlled fibers. Statistical methods are employed to improve the quality of data to exclude outliers within an measurement and within the sample set. A positive linear correlation between the longitudinal and transverse modulus with an R²=0.76 is found. Pitch-based fibers exhibit lower measurement error than PAN-based fibers, while PAN fibers exhibited no apparent modulus correlation when the Pitch fibers are …

Lithium Compound Characterization Via Laser Induced Breakdown Spectroscopy And Raman Spectroscopy, James T. Stofel

Theses and Dissertations

Industries such as lithium-ion battery producers and the nuclear industry community seek to produce and store lithium in pure chemical forms. However, these lithium compounds are reactive with the atmosphere and quickly degrade into less desirable forms. Therefore, industry desires a fast and effective quality control approach to quantify the ingrowth of these secondary lithium chemical forms. This research presents a novel approach using Laser-Induced Breakdown Spectroscopy (LIBS) and Raman spectroscopy in tandem to enhance lithium compound characterization beyond what is achieved by either technique alone. The resulting spectral data are aggregated using data fusion and analyzed using chemometrics for …

Data Driven Investigation Into The Off-Axis Brdf To Develop An Algorithm To Classify Anisotropicity, Anne W. Werkley

Theses and Dissertations

The Bi-directional Reflectance Distribution Function (BRDF) is used to describe reflectances of materials by calculating the ratio of the reflected radiance to the incident irradiance. While it was found that isotropic BRDF microfacet models maintained symmetry about ɸ_s = π, such symmetry was not maintained about the θ_s = θ_i axis, except for close to the specular peak. This led to development of a novel data-driven metric for how isotropic a BRDF measurement is. Research efforts centered around developing an algorithm that could determine material anisotropy without having to fit to models. The algorithm developed here successfully …