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Full-Text Articles in Physical Sciences and Mathematics
Collisional Transfer Of Population And Orientation In Nak, Seth T. Ashman, C. M. Wolfe, J. Huennekens, B. Beser, J. Bai, A. M. Lyyra
Collisional Transfer Of Population And Orientation In Nak, Seth T. Ashman, C. M. Wolfe, J. Huennekens, B. Beser, J. Bai, A. M. Lyyra
Engineering & Physics Faculty Publications
We report current work to study transfer of population and orientation in collisions of NaK molecules with argon and potassium atoms using polarization labeling (PL) and laser- induced fluorescence (LIF) spectroscopy. In the PL experiment, a circularly polarized pump laser excites a specific NaK A1Σ +(v 0=16, J 0 ) ← X1Σ +(v 00=0, J 0 ± 1) transition, creating an orientation (non-uniform MJ0 level distribution) in both levels. The linearly polarized probe laser is scanned over various 31Π(v, J 0±1) ← A1Σ +(v 0=16, J 0 ) transitions. The probe laser passes through a crossed linear polarizer before detection, …
Experimental Studies Of The Nacs 53Π0 And 1(A)3Σ+ States, Seth T. Ashman, Brett Mcgeehan, Christopher Wolfe, Carl Faust, John Huennekens
Experimental Studies Of The Nacs 53Π0 And 1(A)3Σ+ States, Seth T. Ashman, Brett Mcgeehan, Christopher Wolfe, Carl Faust, John Huennekens
Engineering & Physics Faculty Publications
We present experimental studies of the NaCs molecule that are currently underway in our laboratory. The opticaloptical double resonance method is used to obtain Doppler-free excitation spectra for several excited states. Selected data from the 53Π0 electronic state are used to obtain Rydberg-Klein-Rees (RKR) and Inverse Perturbation Approach (IPA) potential curves. We are also mapping the repulsive wall of the 1(a) 3Σ +potential using many resolved bound-free fluorescence spectra from individual ro-vibrational levels of the 53Π0 electronic state to the 1(a) 3Σ + state. Using the determined 53Π0 state potential we fit the repulsive wall of the 1(a) 3Σ + …