Physical Sciences and Mathematics Commons^™

The Impacts Of Transported Wildfire Smoke Aerosol On Surface Air Quality In New York State, Wei-Ting Hung

Legacy Theses & Dissertations (2009 - 2024)

In New York State (NYS), summertime long-range transported smoke plumes and high fine mode particulate matter (PM2.5) concentration during the smoke episodes have been reported. Since the frequency, intensity, and burned area of wildfires over Northern America have increased in recent years, the contribution of transported smoke aerosols to local air quality could become more significant. This study aimed to characterize the transport of smoke aerosols and quantify their impacts on the local air quality over NYS. A case study of a transported smoke event in mid-August of 2018 and multi-year analysis of the smoke cases during the summer seasons …

Physical Characteristics And Microphysical Processing Of Atmospheric Aerosol In Rural And Urban New York State, Joseph Marto

Legacy Theses & Dissertations (2009 - 2024)

Atmospheric aerosol has profound impacts on air quality, though particles of differing sizes can have profoundly different characteristics which are understated when measurements are reported as a single parameter (typically number concentration or total mass). To address some of these concerns and to better understand the nature of atmospheric aerosol, continuous particle size distributions have been measured at two sites in New York State. Measurement was performed for particle diameters between 7.6nm - 20µm at Pinnacle State Park (Addison, New York; March 2017-April 2018) and Queens College (May 2018-September 2019) at a 5-minute time resolution. At Pinnacle State Park, aerosol …

Understanding The Effects Of Water Vapor And Temperature On Aerosol Using Novel Measurement Methods, Tyler Jacob Capek

Dissertations, Master's Theses and Master's Reports

Aerosol and water are inexorably linked, and both are ubiquitous within our atmosphere and required components for cloud formation. Relative humidity (RH), a temperature dependent quantity, can have a significant influence on the size, shape, and ultimately, the optical properties of the aerosol. RH can vary substantially on small spatial and short temporal scales in turbulent conditions due to rapid fluctuations in temperature and water vapor mixing ratio. Accurate assessment of optical enhancements due to an increase in RH is key for determining the particles’ impact on the climate and visibility.

A humidity-controlled cavity attenuated phase-shift albedometer (H-CAPS-PM_SSA) …

Improved Estimation Of Pm2.5 Using Lagrangian Satellite-Measured Aerosol Optical Depth, Rolando Olivas Saunders

Theses and Dissertations

Suspended particulate matter (aerosols) with aerodynamic diameters less than 2.5 μm (PM2.5) has negative effects on human health, plays an important role in climate change and also causes the corrosion of structures by acid deposition. Accurate estimates of PM2.5 concentrations are thus relevant in air quality, epidemiology, cloud microphysics and climate forcing studies. Aerosol optical depth (AOD) retrieved by the Moderate Resolution Imaging Spectroradiometer (MODIS) satellite instrument has been used as an empirical predictor to estimate ground-level concentrations of PM2.5. These estimates usually have large uncertainties and errors. The main objective of this work is to assess the value of …

Detailed Modeling Of Soot Size Distribution Evolution And Pollutant Formation Inside Aircraft And Diesel Engines, Chowdhury Golam Moniruzzaman

Legacy Theses & Dissertations (2009 - 2024)

Combustion emission of soot and pollutant gas species contributes to poor regional air quality near emission sources and to climate change. It is important to understand the formation mechanism and time evolution of these pollutants inside the combustion engine, through detailed modeling of combustion chemistry and microphysics as well as comparison with observation. In this thesis, two multi-zone gas parcel combustion engine models, one for aircraft engines and another for diesel engines, have been developed to study soot size distribution evolution and pollutant formation inside the engines as well as emissions. The models take into account size-resolved (sectional) soot aerosol …

Aerosol Characterizaton In El Paso-Juarez Airshed Using Optical Methods, Angel E. Esparza

Open Access Theses & Dissertations

The assessment and characterization of atmospheric aerosols and their optical properties are of great significance for several applications such as air pollution studies, atmospheric visibility, remote sensing of the atmosphere, and impacts on climate change. Decades ago, the interest in atmospheric aerosols was primarily for visibility impairment problems; however, recently interest has intensified with efforts to quantify the optical properties of aerosols, especially because of the uncertainties surrounding the role of aerosols in climate change. The main objective of the optical characterization of aerosols is to understand their properties. These properties are determined by the aerosols' chemical composition, size, shape …

Measurement Of Atmospheric Ammonia Species : Development, Validation, And Field Applications Of An Analytical Method, Jian Hou

Legacy Theses & Dissertations (2009 - 2024)

Ammonia is the primary base in the atmosphere. It reacts readily with atmospheric acids such as sulfuric acid, nitric acid, and hydrochloric acid to form ammonium salts that occur predominantly in the fine aerosol particle (PM2.5) fraction. The ability to measure ammonia species (NHx, the sum of gaseous NH₃ and particulate NH₄+) is essential for the investigation of atmospheric behaviors of NHx. In this dissertation work, a highly sensitive technique has been developed for the measurement of atmospheric NHx species. The method is based on aqueous scrubbing of the atmospheric NH₃ and NH₄+ using …