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Atmospheric Chemistry Of A 33–34 Hour Old Volcanic Cloud From Hekla Volcano (Iceland): Insights From Direct Sampling And The Application Of Chemical Box Modeling, William I. Rose, Genevieve A. Millard, Tamsin A. Mather, Donald E. Hunton, Bruce Anderson, Clive Oppenheimer, Brett F. Thornton, Terrence M. Gerlach, Albert A. Viggiano, Yutaka Kondo, Thomas M. Miller, John O. Ballenthin
Atmospheric Chemistry Of A 33–34 Hour Old Volcanic Cloud From Hekla Volcano (Iceland): Insights From Direct Sampling And The Application Of Chemical Box Modeling, William I. Rose, Genevieve A. Millard, Tamsin A. Mather, Donald E. Hunton, Bruce Anderson, Clive Oppenheimer, Brett F. Thornton, Terrence M. Gerlach, Albert A. Viggiano, Yutaka Kondo, Thomas M. Miller, John O. Ballenthin
Department of Geological and Mining Engineering and Sciences Publications
On 28 February 2000, a volcanic cloud from Hekla volcano, Iceland, was serendipitously sampled by a DC-8 research aircraft during the SAGE III Ozone Loss and Validation Experiment (SOLVE I). It was encountered at night at 10.4 km above sea level (in the lower stratosphere) and 33–34 hours after emission. The cloud is readily identified by abundant SO2 (≤1 ppmv), HCl (≤70 ppbv), HF (≤60 ppbv), and particles (which may have included fine silicate ash). We compare observed and modeled cloud compositions to understand its chemical evolution. Abundances of sulfur and halogen species indicate some oxidation of sulfur gases but …
Halogen Emissions From A Small Volcanic Eruption: Modeling The Peak Concentrations, Dispersion, And Volcanically Induced Ozone Loss In The Stratosphere, G. A. Millard, T. A. Mather, D. M. Pyle, William I. Rose, B. Thornton
Halogen Emissions From A Small Volcanic Eruption: Modeling The Peak Concentrations, Dispersion, And Volcanically Induced Ozone Loss In The Stratosphere, G. A. Millard, T. A. Mather, D. M. Pyle, William I. Rose, B. Thornton
Department of Geological and Mining Engineering and Sciences Publications
Aircraft measurements in the Hekla, Iceland volcanic plume in February 2000 revealed large quantities of hydrogen halides within the stratosphere correlated to volcanic SO2. Investigation of the longer-term stratospheric impact of these emissions, using the 3D chemical transport model, SLIMCAT suggests that volcanic enhancements of H2O and HNO3 increased HNO3·3H2O particle availability within the plume. These particles activated volcanic HCl and HBr, enhancing model plume concentrations of ClOx (20 ppb) and BrOx (50 ppt). Model O3 concentrations decreased to near-zero in places, and plume average O3 remained 30% lower after two weeks. Reductions in the model O3column reduced UV shielding …