Open Access. Powered by Scholars. Published by Universities.®
Articles 1 - 2 of 2
Full-Text Articles in Engineering
Probe-Pulse Optimization For Nonresonant Suppression In Hybrid Fs/Ps Coherent Anti-Stokes Raman Scattering At High Temperature, Joseph D. Miller, Mikhail N. Slipchenko, Terrence R. Meyer
Probe-Pulse Optimization For Nonresonant Suppression In Hybrid Fs/Ps Coherent Anti-Stokes Raman Scattering At High Temperature, Joseph D. Miller, Mikhail N. Slipchenko, Terrence R. Meyer
Terrence R Meyer
Hybrid femtosecond/picosecond coherent anti-Stokes Raman scattering (fs/ps CARS) offers accurate thermometry at kHz rates for combustion diagnostics. In high-temperature flames, selection of probe-pulse characteristics is key to simultaneously optimizing signal-to-nonresonant-background ratio, signal strength, and spectral resolution. We demonstrate a simple method for enhancing signal-to-nonresonant-background ratio by using a narrowband Lorentzian filter to generate a time-asymmetric probe pulse with full-width-half-maximum (FWHM) pulse width of only 240 fs. This allows detection within just 310 fs after the Raman excitation for eliminating nonresonant background while retaining 45% of the resonant signal at 2000 K. The narrow linewidth is comparable to that of a …
Single-Shot Gas-Phase Thermometry Using Purerotational Hybrid Femtosecond/Picosecond Coherent Anti-Stokes Raman Scattering, Joseph D. Miller, Sukesh Roy, Mikhail N. Slipchenko, James R. Gord, Terrence R. Meyer
Single-Shot Gas-Phase Thermometry Using Purerotational Hybrid Femtosecond/Picosecond Coherent Anti-Stokes Raman Scattering, Joseph D. Miller, Sukesh Roy, Mikhail N. Slipchenko, James R. Gord, Terrence R. Meyer
Terrence R Meyer
High-repetition-rate, single-laser-shot measurements are important for the investigation of unsteady flows where temperature and species concentrations can vary significantly. Here, we demonstrate singleshot, pure-rotational, hybrid femtosecond/picosecond coherent anti-Stokes Raman scattering (fs/ps RCARS) thermometry based on a kHz-rate fs laser source. Interferences that can affect nanosecond (ns) and ps CARS, such as nonresonant background and collisional dephasing, are eliminated by selecting an appropriate time delay between the 100-fs pump/Stokes pulses and the pulse-shaped 8.4-ps probe. A time- and frequency-domain theoretical model is introduced to account for rotational-level dependent collisional dephasing and indicates that the optimal probe-pulse time delay is 13.5 ps …