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Faculty Publications

Series

2014

CO2 gasification

Articles 1 - 2 of 2

Full-Text Articles in Engineering

Co2 Gasification Rates Of Petroleum Coke In A Pressurized Flat-Flame Burner Entrained-Flow Reactor, Aaron D. Lewis, Emmett G. Fletcher, Thomas H. Fletcher Jan 2014

Co2 Gasification Rates Of Petroleum Coke In A Pressurized Flat-Flame Burner Entrained-Flow Reactor, Aaron D. Lewis, Emmett G. Fletcher, Thomas H. Fletcher

Faculty Publications

Two petcoke samples were gasified by CO2 at total pressures of 10 and 15 atm in a high-pressure flat-flame burner reactor at conditions where the bulk phase consisted of either 40 or 90 mol % CO2 with gas temperatures up to 1909 K. Particle diameters of 45−75 μm were used in the experiments. The morphology of the two petroleum coke chars was drastically different and evaluated using scanning electron microscopy images of the chars. The mass release data caused by CO2 gasification of the petcoke chars were fit to a global first-order model, and the optimal kinetic parameters are reported. …


Co2 Char Gasification Rates Of Sawdust, Switchgrass, And Corn Stover In A Pressurized Entrained-Flow Reactor, Thomas H. Fletcher, Aaron D. Lewis, Emmett G. Fletcher Jan 2014

Co2 Char Gasification Rates Of Sawdust, Switchgrass, And Corn Stover In A Pressurized Entrained-Flow Reactor, Thomas H. Fletcher, Aaron D. Lewis, Emmett G. Fletcher

Faculty Publications

An entrained-flow flat-flame burner reactor was used to measure apparent CO2 gasification rates of near-spherical biomass chars of poplar sawdust, switchgrass, and corn stover using particle residence times1258−1891 K and 6.1− 13.5 atm, respectively. A new method was developed to produce near-spherical particles from nonspherical biomass chars. The apparent CO2 gasification rates for the three biomass chars with mean diameters near 100 μm were fit to a global first-order model, and the optimal kinetic parameters are reported. The measured gasification rate of poplar sawdust was about 3.9 times faster than that of switchgrass char, but only about 20% faster than …