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Optimal Battery Operations And Design Considering Capacity Fade Mechanisms, Bharatkumar Suthar

McKelvey School of Engineering Theses & Dissertations

Safely and capacity fade are the key issues that restrict the use of the lithium-ion battery for many applications. These issues are being tackled in a variety of ways. This dissertation focuses on using detailed continuum-level electrochemical models to study transport, kinetics, and mechanical processes in the lithium-ion batteries. These models can be used to quantify the effect of capacity fade mechanisms (side reactions and mechanical degradation) and improve the safety aspects of the lithium ion batteries. Three capacity-fade mechanisms—solid electrolyte interface side reaction, lithium-plating side reaction and mechanical degradation due to intercalation-induced stresses—are considered in the dissertation. Monitoring and …