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Continuous Adsorption And Biotransformation Of Micropollutants By Granular Activated Carbon-Bound Laccase In A Packed-Bed Enzyme Reactor, Ngoc Luong Nguyen, Faisal I. Hai, Anthony Dosseto, Christopher Richardson, William E. Price, Long D. Nghiem
Continuous Adsorption And Biotransformation Of Micropollutants By Granular Activated Carbon-Bound Laccase In A Packed-Bed Enzyme Reactor, Ngoc Luong Nguyen, Faisal I. Hai, Anthony Dosseto, Christopher Richardson, William E. Price, Long D. Nghiem
Faculty of Engineering and Information Sciences - Papers: Part A
Laccase was immobilized on granular activated carbon (GAC) and the resulting GAC-bound laccase was used to degrade four micropollutants in a packed-bed column. Compared to the free enzyme, the immobilized laccase showed high residual activities over a broad range of pH and temperature. The GAC-bound laccase efficiently removed four micropollutants, namely, sulfamethoxazole, carbamazepine, diclofenac and bisphenol A, commonly detected in raw wastewater and wastewater-impacted water sources. Mass balance analysis showed that these micropollutants were enzymatically degraded following adsorption onto GAC. Higher degradation efficiency of micropollutants by the immobilized compared to free laccase was possibly due to better electron transfer between …