Open Access. Powered by Scholars. Published by Universities.®
Articles 1 - 4 of 4
Full-Text Articles in Engineering
Femtosecond Pulse Compression Via Self-Phase Modulation In 1-Decanol, Jacob A. Stephen
Femtosecond Pulse Compression Via Self-Phase Modulation In 1-Decanol, Jacob A. Stephen
Electronic Theses and Dissertations
Ultrafast science is a branch of photonics with far reaching applications in and outside the realm of physics. Ultrashort laser pulses on the order of femtoseconds (1 fs = 1 × 10−15 s) are widely used for ultrafast science. Many lasers can produce pulses on the order of 100 fs, with state of the art, high end lasers being capable of producing pulses around 30 fs. However, many experiments require pulses around 10 fs or shorter. Femtosecond pulses are typically generated using spectral broadening via self-phase modulation, followed by dispersion compensation. The most common spectral broadening technique exploits the nonlinear …
White Light Continuum For Broadband Nonlinear Spectroscopy, Trenton Ensley
White Light Continuum For Broadband Nonlinear Spectroscopy, Trenton Ensley
Electronic Theses and Dissertations
Supercontinuum (SC) generation, oftentimes referred to as white-light continuum (WLC), has been a subject of interest for more than 40 years. From the first observation of WLC in condensed media in the early 1970s to the first observation of WLC in gases in the mid-1980s, much work has been devoted to developing a framework for understanding the complex nature of this phenomenon as well as discovering its utility in various applications. The main effort of this dissertation is to develop a WLC for the purpose of broadband nonlinear spectroscopy and use it in spectroscopic measurements. The ability to generate a …
Techniques For Characterization Of Third Order Optical Nonlinearities, Manuel Ferdinandus
Techniques For Characterization Of Third Order Optical Nonlinearities, Manuel Ferdinandus
Electronic Theses and Dissertations
This dissertation describes the development of novel techniques for characterization of nonlinear properties of materials. The dissertation is divided into two parts, a background and theory section and a technique development section. In the background and theory section we explain the origins of the nonlinear optical response of materials across many different spatial and temporal scales. The mechanisms that we are most interested in are the electronic nuclear and reorientational responses, which occur on the range of sub-femtosecond to several picoseconds. The electronic mechanism is due to the electrons of a material experiencing a non-parabolic potential well due a strong …
Characterization Of The Nonlinear Refractive Index Of Carbon Disulfide Over An Extended Spectral And Temporal Range, Marcus Seidel
Characterization Of The Nonlinear Refractive Index Of Carbon Disulfide Over An Extended Spectral And Temporal Range, Marcus Seidel
Electronic Theses and Dissertations
The intensity dependent refractive index change of a medium is frequently described in terms of the product n₂ · I where n₂ is the nonlinear refractive index and I the light intensity. The nonlinear refractive index is often treated as constant which is a reasonable assumption if the light interacts only with bound electrons. In the case of carbon disulfide (CS₂) however, nuclear motions contribute to n₂. These motions occur on the sub picosecond time scale and thus become especially relevant for ultrashort laser pulses. The neat liquid CS₂ is studied because it exhibits a large nonlinear refractive index in …