Digital Commons Network^™

Uncertainty Quantification Framework For Design Optimization, Austin Ryan Williams

Masters Theses

Difficulty to obtain neutron sources of interest have driven the need for optimization
techniques to tailor a neutron generator as a replacement. A proposed solution uses
off-the-shelf neutron sources coupled with an energy-tuning assembly to mimic the
source of interest (i.e. AmLi, AmBe, thermonuclear fission spectra, etc.). These
energy-tuning assemblies have been designed with complex optimization algorithms
coupled with Monte Carlo simulations. These new system surrogate designs often
do not have an experimental counterpart for validation and comparison, and lack
non-statistical uncertainties. This work aims to improve confidence in the predictions
by providing a tool for fast uncertainty quantification to …

Fabrication, Measurements, And Modeling Of Semiconductor Radiation Detectors For Imaging And Detector Response Functions, Corey David Ahl

Doctoral Dissertations

In the first part of this dissertation, we cover the development of a diamond semiconductor alpha-tagging sensor for associated particle imaging to solve challenges with currently employed scintillators. The alpha-tagging sensor is a double-sided strip detector made from polycrystalline CVD diamond. The performance goals of the alpha-tagging sensor are 700-picosecond timing resolution and 0.5 mm spatial resolution. A literature review summarizes the methodology, goals, and challenges in associated particle imaging. The history and current state of alpha-tagging sensors, followed by the properties of diamond semiconductors are discussed to close the literature review. The materials and methods used to calibrate the …

Total Absorption Spectroscopy Of Mo-106 And Tc-106, Michael Cooper

Doctoral Dissertations

Total absorption spectroscopy is a method of gamma-ray spectroscopy that has gained prominence in the past several decades, as nuclear data revisions are performed on older nuclear data, which is often incomplete. A strong understanding of underlying nuclear data, particularly fission and beta decay data, is essential for nuclear reactors and nuclear fuel decay heat. This PhD work involves the analysis of fission fragments 106Mo [Mo-106] and 106Tc [Tc-106]. These neutron rich isotopes contribute upwards of 6% of the cumulative fission yield of 241Pu [Pu-241] fission, and 4% of 239Pu [Pu-239] fission. Prior data for these two fission fragments only …

Determination Of Near-Sol Carbon Impurity Content Due To Divertor Target Leakage Using Carbon-13 Tracers Via Methane Injection On The Diii-D Tokamak, Jonah David Duran

Doctoral Dissertations

Experiments with outer strike point injection of isotopically enriched methane (¹³CD­₄) in DIII-D L-mode discharges have demonstrated the ability to infer near scrape-off-layer (SOL) impurity density profiles based on: far-SOL collector probe (CP) measurements; a stable isotopic mixing model; and SOL impurity transport modelling. This work enables one of the first in-depth investigations on the source and transport of SOL impurities which could hinder performance of future fusion devices. Modelling by DIVIMP and 3DLIM of ¹³C SOL evolution is consistent with diagnostic observations and indicates that the buildup of injected impurities on plasma-facing surfaces must …

Multi-Objective Optimization Of The Fast Neutron Source By Machine Learning, John L. Pevey

Doctoral Dissertations

The design and optimization of nuclear systems can be a difficult task, often with prohibitively large design spaces, as well as both competing and complex objectives and constraints. When faced with such an optimization, the task of designing an algorithm for this optimization falls to engineers who must apply engineering knowledge and experience to reduce the scope of the optimization to a manageable size. When sufficient computational resources are available, unsupervised optimization can be used.

The optimization of the Fast Neutron Source (FNS) at the University of Tennessee is presented as an example for the methodologies developed in this work. …

A Bulk Driven Transimpedance Cmos Amplifier For Sipm Based Detection, Shahram Hatefi Hesari

Masters Theses

The contribution of this work lies in the development of a bulk driven operational
transconducctance amplifier which can be integrated with other analog circuits and
photodetectors in the same chip for compactness, miniaturization and reducing the
power. Silicon photomultipliers, also known as SiPMs, when coupled with scintillator materials are used in many imaging applications including nuclear detection. This thesis discuss the design of a bulk-driven transimpedance amplifier suitable for detectors where the front end is a SiPM. The amplifier was design and fabricated in a standard standard CMOS process and is suitable for integration with CMOS based SiPMs and commercially …

Enigma - Ongoing Development Towards Novel Beta-Decay Spectroscopy Station At Isolde, Philipp Wagenknecht

Masters Theses

Beta decay and collinear laser spectroscopy are proven efficient tools to study nuclear structure far from stability. Two areas of significance are investigations into nuclear deformation and shape coexistence, as well as delayed neutron emissions used in nuclear energy applications. This contribution presents the ongoing development towards a novel beta-decay spectroscopy station for the VITO experiment at CERN’s radioactive ion beam facility ISOLDE. The setup will utilize both collinear laser spectroscopy and beta-decay spectroscopy to measure the energy and spin-parities of the ground and excited states of radioactive beams. Initial designs of the support structure, magnetic field, and detector array …

Design And Evaluation Of A Unique Weighted-Sum-Based Anger Camera, Matthew W. Seals

Masters Theses

Anger camera imaging technology has become widely popular for neutron diffraction imaging due to recent shortages in Helium-3 (He-3). Research into neutron diffraction optimized Anger camera by the Oak Ridge National Laboratory (ORNL) detectors group has provided an alternative to He-3 Tube-based detectors with a high-resolution Anger camera. However, the cost of these high-resolution Anger camera technology can make it less attractive than He-3 tubes when a large Field of View (FOV) is desired. Currently, there is a need for a lower-cost alternative to this high-resolution anger camera. Further applications for Anger camera have become of interest with the advent …

Purification Of I-129 From Spent Pwr Fuel, Sydney B. Whitaker, Kaitlyn Pierson, Kaylie Richard, Samantha Cahill

Chancellor’s Honors Program Projects

No abstract provided.

Exploring The Viability Of Investment In Small Modular Nuclear Reactors (Smrs): Mitigating Climate Change Through Advancements In Energy Generation, Alec V. Apostoaei

Chancellor’s Honors Program Projects

No abstract provided.

Uncertainty Estimates In Few-Body Physics, Daniel Odell Jr

Doctoral Dissertations

Uncertainty estimates in theoretical physics are just as important as they are in experimental physics. As a theorist, one must qualify a given calculation with the assumptions on which the calculation is performed. Such a practice equips the scientific community with the context necessary to evaluate the validity of a theory. It also provides some basis upon which the theory can develop improvements. The work presented here concerns itself with two sources of uncertainty in theoretical physics. First, we discuss numerical uncertainties. Particularly, we quantify the uncertainties introduced by basis truncations and the exploit it to extrapolate infinite-basis results. Second, …

Analysis Of Adjoint Flux Calculation For Detector Response Estimation In Typical Pwr Conditions, Shane Henderson

Masters Theses

Reactor power is sensed by ex-core instrumentation by measuring the core neutron leakage. The measured magnitude of this leakage is sensitive to the conditions in which the reactor is operating. By being able to accurately estimate the neutron flux which will reach the detector position we can accurately estimate the power level and power distribution for a variety of operating conditions. The analysis presented here seeks to establish a minimum parameter set for solving an adjoint reactor problem at given conditions which can then be used to estimate the response using the forward solution at a different set of conditions. …

Nestle To Origami Coupling: A Nuclear Non-Proliferation Tool For Lwr Fuel Assembly Isotope Analysis, Margaret Alva Kurtts

Doctoral Dissertations

NESTLE to ORIGAMI coupling is a versatile nuclear modeling tool that allows researchers to directly observe the impact of operator induced changes on LWR assembly isotope production. The paper presents an experimental method by which to test the ability of an operator to manipulate the core neutron spectrum in order to produce higher quality plutonium for weapons use. The paper presents two plutonium production scenarios and evaluates their feasibility based on potential for detection and production capacity. Reactor modeling of a VVER-1000 uses NESTLE core simulation software. NESTLE outputs burnup and relative power information for all nodes in the core. …

Jet-Hadron Correlations Relative To The Event Plane Pb--Pb Collisions At The Lhc In Alice, Joel Anthony Mazer

Doctoral Dissertations

In relativistic heavy ion collisions at the Large Hadron Collider (LHC), a hot, dense and strongly interacting medium known as the Quark Gluon Plasma (QGP) is produced. Quarks and gluons from incoming nuclei collide to produce partons at high momenta early in the collisions. By fragmenting into collimated sprays of hadrons, these partons form 'jets'. Within the framework of perturbative Quantum Chromodynamics (pQCD), jet production is well understood in pp collisions. We can use jets measured in pp interactions as a baseline reference for comparing to heavy ion collision systems to detect and study jet quenching. The jet quenching mechanism …

Subcritical Facility Design, Kacie Breeding

Chancellor’s Honors Program Projects

No abstract provided.

Neutron Generator Driven Subcritical Fast Neutron Source Facility, Zachary Bingham, Duncan Brocklehurst, Will Cureton, Daniel Peffley, Colton Oldham, James Ghawaly

Chancellor’s Honors Program Projects

No abstract provided.

Development, Synthesis, And Analysis Of Surrogate Post-Detonation Nuclear Melt Glass, Andrew Vincent Giminaro

Doctoral Dissertations

With the threats facing the world today, there is an ever-increasing need for training the the fields of radiochemistry and nuclear forensics. Training and research in these fields requires reference materials that accurately represent materials that could potentially be encountered. Unfortunately, many of the historical samples of debris from nuclear weapons tests remains classified. Because of this, there is a need for realistic surrogates. This research focuses on the development of surrogates for the bulk and particulate nuclear melt glass that is expected to be found in an urban setting after a nuclear event.

A mathematical model for the creation …

Assessment Of Reactivity Equivalence For Enhanced Accident Tolerant Fuels In Light Water Reactors, Nathan Michael George

Doctoral Dissertations

The neutronic behavior of accident tolerant fuel (ATF) concepts was simulated in light water reactors (LWRs) to establish design parameters to match reactivity lifetime requirements of standard UO₂ [uranium dioxide]/Zircaloy fuel. The two concepts discussed in this dissertation are fully ceramic micro-encapsulated (FCM) fuel and alternate cladding concepts. To compare the required fuel alterations against standard UO₂/Zircaloy fuel, a 2D lattice-physics based reactivity equivalence method was established to estimate excess reactivity at the completion of each weighted batch cycle.

In the case of FCM fuel, the uranium-based tristructural isotropic (TRISO) kernel and the surrounding particle layers/matrix material …

Development Of A Method For Incorporating Fault Codes In Prognostic Analysis, Eric Allen Strong

Doctoral Dissertations

Information from fault codes associated with a component may be used as an indicator of its health. A fault code is defined as a timestamp at which a component is not operating according to recommended guidelines. The type of fault codes which are relevant for this analysis represent mild or moderate deviations from normal behavior, rather than those requiring immediate repair. Potentially, fault codes may be used to determine the Remaining Useful Life (RUL) of a component by predicting its failure time, which will improve safety and reduce maintenance costs associated with the component. In this dissertation, methods have been …

Cd Dipping To Reduce Reactivity Of Fuel Assemblies In Spent Fuel Pools, John Clark Stooksbury

Chancellor’s Honors Program Projects

No abstract provided.

Thorium Research In The Manhattan Project Era, Kirk Frederick Sorensen

Masters Theses

Research on thorium as an energy source began in 1940 under the direction of Glenn Seaborg at the University of California, Berkeley. Following the discovery of plutonium-239 and its fissile qualities, similar experiments demonstrated that uranium-233 bred from thorium was also fissile. Seaborg viewed uranium-233 as a potential backup to plutonium-239, whose production was one of the Manhattan Project's primary efforts. The central appeal of U-233 was that the chemistry of uranium was well understood, unlike plutonium, but plutonium-239 had the potential to be produced from natural uranium in a critical nuclear reactor. Natural thorium lacked fissile isotopes and so …

Beta-Delayed Neutron Spectroscopy Of Fission Fragments Using The Versatile Array Of Neutron Detectors At Low Energy, Stanley Vincent Paulauskas

Doctoral Dissertations

This work details the study of nuclear decay in the region of doubly magic 78Ni using the Versatile Array of Neutron Detectors at Low Energy (VANDLE). This detector system uses the time-of-flight technique to measure the energy of beta-delayed neutrons. VANDLE uses a fully digital data acquisition system equipped with timing algorithms developed as part of the experimental work. The experiment examined nearly 30 beta-delayed neutron precursors produced at the Hollifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory. This work discusses three of these nuclei: 77,78Cu and 84Ga. Results from the experiment provide details of the Gamow-Teller decay …

Sensitivity And Uncertainty Analysis Of A Fixed Source Criticality Accident Alarm System Benchmark Experiment, Kevin Howard Reynolds

Doctoral Dissertations

The Department of Energy (DOE) Nuclear Criticality Safety Program (NCSP) funded the development of a criticality accident alarm system (CAAS) benchmark to be published by the International Criticality Safety Benchmark Evaluation Project (ICSBEP) in the International Handbook of Evaluated Criticality Safety Benchmark Experiments (handbook). While there are shielding related benchmark evaluations published in the handbook, the effort in this dissertation concerns a first of its kind experiment that has been conceived from the ground up as a pulsed critical fixed source benchmark.

The experiment was designed in conjunction with the French government and conducted at their SILENE reactor facility at …

Coalescing Memory, Michael Christopher Housley

Chancellor’s Honors Program Projects

No abstract provided.

Simulations Of Ti-Y-O Nanoclusters In Ferritic Alloys, Natalie Browning Camilli

Masters Theses

Nanostructured ferritic alloys possess high strength and resistance to radiation effects due to the presence of nanoprecipitates. Though nanostructured ferritic alloys have desirable mechanical properties, the exact composition and structure of the nanoprecipitates is unknown; thus, atomistic simulations involving the formation of nanoclusters give insight as to their structure. This thesis focuses on the structure, formation and radiation stability of Ti-Y-O [titanium-yttrium-oxygen] nanoclusters in iron. The activation energies for diffusion and the diffusion coefficients of oxygen interstitial atoms in iron are determined. The binding energies of various combinations of oxygen interstitial atoms and iron vacancies are also tabulated. Thermodynamic formation …

The Use Of A Fluidized Bed In A Spent Fuel Pool, Charles R. Menke, Natalie B. Camilli, Nathan A. Capps, Claire Fage, Timothy R. Hillard, Matthew B. Nash, Matthew L. Thornbury

Chancellor’s Honors Program Projects

No abstract provided.

Energy Functional For Nuclear Masses, Michael Giovanni Bertolli

Doctoral Dissertations

An energy functional is formulated for mass calculations of nuclei across the nuclear chart with major-shell occupations as the relevant degrees of freedom. The functional is based on Hohenberg-Kohn theory. Motivation for its form comes from both phenomenology and relevant microscopic systems, such as the three-level Lipkin Model. A global fit of the 17-parameter functional to nuclear masses yields a root- mean-square deviation of χ[chi] = 1.31 MeV, on the order of other mass models. The construction of the energy functional includes the development of a systematic method for selecting and testing possible functional terms. Nuclear radii are computed within …