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Synthesis, Linear And Nonlinear Photophysical Characterization Of Two Symmetrical Pyrene-Terminated Squaraine Derivatives In Solution, Alfonso Ballestas Barrientos
Synthesis, Linear And Nonlinear Photophysical Characterization Of Two Symmetrical Pyrene-Terminated Squaraine Derivatives In Solution, Alfonso Ballestas Barrientos
Electronic Theses and Dissertations
Two indole-based squaraine dyes bonded to two pyrenyl groups through vinyl- and ethynyl- linkers were synthesized with the aim of enhancing the intramolecular charge transfer interaction in addition to improving their optical properties. The absorption and emission properties of these derivatives were determined in order to gain an insight into the intensity of this type of interaction, their aggregation behavior and compare them with results obtained through quantum chemical calculations. Both compounds presented high photochemical stability in THF, and the linear spectroscopic characterization revealed high extinction coefficients, large fluorescence quantum yields and relatively low tendency of forming excimers in several …
Strategies For Enhanced Genetic Analysis Of Trace Dna From Touch Dna Evidence And Household Dust, Katherine Farash
Strategies For Enhanced Genetic Analysis Of Trace Dna From Touch Dna Evidence And Household Dust, Katherine Farash
Electronic Theses and Dissertations
In forensic casework it is often necessary to obtain genetic profiles from crime scene samples that contain increasingly smaller amounts of genetic material, called Low Template DNA (LTDNA). Two examples of LTDNA sources are touch DNA evidence and dust bunnies. Touch DNA refers to DNA that is left behind through casual contact of a donor with an object or another person. Touch DNA can be used to prove a suspect was present at a crime scene. Dust bunnies, or dust conglomerates, typically contain trapped shed skin cells of anyone in the vicinity along with fibers, dirt, hair, and other trace …
Investigating New Guaiazulenes And Diketopyrropyrroles For Photonic Applications, Ebrahim Ghazvini Zadeh
Investigating New Guaiazulenes And Diketopyrropyrroles For Photonic Applications, Ebrahim Ghazvini Zadeh
Electronic Theses and Dissertations
?-Conjugated systems have been the focus of study in recent years in order to understand their charge transport and optical properties for use in organic electronic devices, fluorescence bioimaging, sensors, and 3D optical data storage (ODS), among others. As a result, several molecular building blocks have been designed, allowing new frontiers to be realized. While various successful building blocks have been fine-tuned at both the electronic and molecular structure level to provide advanced photophysical and optoelectronic characteristics, the azulene framework has been under-appreciated despite its unique electronic and optical properties. Among several attributes, azulenes are vibrant blue naturally occurring hydrocarbons …
Nanoelectronic Devices Using Carbon Nanotubes And Graphene Electrodes: Fabrication And Electronic Transport Investigations, Narae Kang
Electronic Theses and Dissertations
Fabrication of high-performance electronic devices using the novel semiconductors is essential for developing future electronics which can be applicable in large-area, flexible and transparent displays, sensors and solar cells. One of the major bottlenecks in the fabrication of high-performance devices is a large interfacial barrier formation at metal/semiconductor interface originated from Schottky barrier and interfacial dipole barrier which causes inefficient charge injection at the interface. Therefore, having a favorable contact at electrode/semiconductor is highly desirable for high-performance devices fabrication. In this dissertation, the fabrication of nanoelectronic devices and investigation of their transport properties using carbon nanotubes (CNTs) and graphene as …
Photophysics Of Organic Probes And Their Applications In Bioimaging & Photodynamic Therapy, Bosung Kim
Photophysics Of Organic Probes And Their Applications In Bioimaging & Photodynamic Therapy, Bosung Kim
Electronic Theses and Dissertations
Over the past several decades the phenomenon of luminescence (divided into fluorescence and phosphorescence) has received great attention in the field of biological science. This quest has motivated scientists for a variety of applications, including fluorescence imaging. Fluorescence microscopy techniques that provide unique advantages, such as high spatial resolution and superior sensitivity, have been regarded as attractive tools in biophotonics. With the progress of ultrafast laser sources, two-photon absorption (2PA), in which a molecule absorbs two photons simultaneously, has opened possibilities of using it for various applications. Two-photon fluorescence microscopy (2PFM), which affords deeper tissue penetration and excellent three-dimensional (3D) …
Nonlinear Optical Response Of Simple Molecules And Two-Photon Semiconductor Lasers, Matthew Reichert
Nonlinear Optical Response Of Simple Molecules And Two-Photon Semiconductor Lasers, Matthew Reichert
Electronic Theses and Dissertations
This dissertation investigates two long standing issues in nonlinear optics: complete characterization of the ultrafast dynamics of simple molecules, and the potential of a two-photon laser using a bulk semiconductor gain medium. Within the Born-Oppenheimer approximation, nonlinear refraction in molecular liquids and gases can arise from both bound-electronic and nuclear origins. Knowledge of the magnitudes, temporal dynamics, polarization and spectral dependences of each of these mechanisms is important for many applications including filamentation, white-light continuum generation, all-optical switching, and nonlinear spectroscopy. In this work the nonlinear dynamics of molecules are investigated in both liquid and gas phase with the recently …
Integral Representations Of Positive Linear Functionals, Angela Siple
Integral Representations Of Positive Linear Functionals, Angela Siple
Electronic Theses and Dissertations
In this dissertation we obtain integral representations for positive linear functionals on commutative algebras with involution and semigroups with involution. We prove Bochner and Plancherel type theorems for representations of positive functionals and show that, under some conditions, the Bochner and Plancherel representations are equivalent. We also consider the extension of positive linear functionals on a Banach algebra into a space of pseudoquotients and give under conditions in which the space of pseudoquotients can be identified with all Radon measures on the structure space. In the final chapter we consider a system of integrated Cauchy functional equations on a semigroup, …
Parallel Fabrication And Transport Properties Of Carbon Nanotube Single Electron Transistors, Muhammad Islam
Parallel Fabrication And Transport Properties Of Carbon Nanotube Single Electron Transistors, Muhammad Islam
Electronic Theses and Dissertations
Single electron transistors (SET) have attracted significant attention as a potential building block for post CMOS nanoelectronic devices. However, lack of reproducible and parallel fabrication approach and room temperature operation are the two major bottlenecks for practical realization of SET based devices. In this thesis, I demonstrate large scale single electron transistors fabrication techniques using solution processed single wall carbon nanotubes (SWNTs) and studied their electron transport properties. The approach is based on the assembly of individual SWNTs via dielectrophoresis (DEP) at the selected position of the circuit and formation of tunnel barriers on SWNT. Two different techniques: i) metal-SWNT …
Translocation Of A Semiflexible Polymer Through A Nanopore, Ramesh Adhikari
Translocation Of A Semiflexible Polymer Through A Nanopore, Ramesh Adhikari
Electronic Theses and Dissertations
The transport of a biomolecule through a nanopore occurs in many biological functions such as, DNA or RNA transport across nuclear pores and the translocation of proteins across the eukaryotic endoplasmic reticulum. In addition to the biological processes, it has potential applications in technology such as, drug delivery, gene therapy, and single molecule sensing. The DNA translocation through a synthetic nanopore device is considered as the basis for cheap and fast sequencing technology. Motivated by the experimental advances, many theoretical models have been developed. In this thesis, we explore the dynamics of driven translocation of a semiflexible polymer through a …
On The Theory Of Zeta-Functions And L-Functions, Almuatazbellah Awan
On The Theory Of Zeta-Functions And L-Functions, Almuatazbellah Awan
Electronic Theses and Dissertations
In this thesis we provide a body of knowledge that concerns Riemann zeta-function and its generalizations in a cohesive manner. In particular, we have studied and mentioned some recent results regarding Hurwitz and Lerch functions, as well as Dirichlet's L-function. We have also investigated some fundamental concepts related to these functions and their universality properties. In addition, we also discuss different formulations and approaches to the proof of the Prime Number Theorem and the Riemann Hypothesis. These two topics constitute the main theme of this thesis. For the Prime Number Theorem, we provide a thorough discussion that compares and contrasts …
Modeling Social Norms In Real-World Agent-Based Simulations, Rahmatollah Beheshti
Modeling Social Norms In Real-World Agent-Based Simulations, Rahmatollah Beheshti
Electronic Theses and Dissertations
Studying and simulating social systems including human groups and societies can be a complex problem. In order to build a model that simulates humans' actions, it is necessary to consider the major factors that affect human behavior. Norms are one of these factors: social norms are the customary rules that govern behavior in groups and societies. Norms are everywhere around us, from the way people handshake or bow to the clothes they wear. They play a large role in determining our behaviors. Studies on norms are much older than the age of computer science, since normative studies have been a …
Mahalanobis Kernel-Based Support Vector Data Description For Detection Of Large Shifts In Mean Vector, Vu Nguyen
Electronic Theses and Dissertations
Statistical process control (SPC) applies the science of statistics to various process control in order to provide higher-quality products and better services. The K chart is one among the many important tools that SPC offers. Creation of the K chart is based on Support Vector Data Description (SVDD), a popular data classifier method inspired by Support Vector Machine (SVM). As any methods associated with SVM, SVDD benefits from a wide variety of choices of kernel, which determines the effectiveness of the whole model. Among the most popular choices is the Euclidean distance-based Gaussian kernel, which enables SVDD to obtain a …
Folate Conjugated Hyperbranched Polyester Nanoparticles For Prostate Tumor-Targeted Delivery Of A Cytotoxic Peptide Via Prostate Specific Membrane Antigen, Orielyz Flores-Fernandez
Folate Conjugated Hyperbranched Polyester Nanoparticles For Prostate Tumor-Targeted Delivery Of A Cytotoxic Peptide Via Prostate Specific Membrane Antigen, Orielyz Flores-Fernandez
Electronic Theses and Dissertations
Prostate Cancer is the second most deadly cancer in men, after lung cancer. The need for new and effective therapeutics that can constrain prostate cancer progression are challenged by the lack of suitable delivery strategies that target prostate cancer tissue. To study CT20p as potential chemotherapeutic agent in the treatment of prostate cancer we proposed the use of targetable hyperbranched polyester (HBPE) based nanoparticles as delivery system. Folic acid was conjugated to the nanocarrier to improve the selectivity of the nanoparticle towards specific cell surface targets in prostate cancer cell lines. Specifically we evaluated LNCaP that up-regulated the PSMA receptor. …
Research On Improving Reliability, Energy Efficiency And Scalability In Distributed And Parallel File Systems, Junyao Zhang
Research On Improving Reliability, Energy Efficiency And Scalability In Distributed And Parallel File Systems, Junyao Zhang
Electronic Theses and Dissertations
With the increasing popularity of cloud computing and "Big data" applications, current data centers are often required to manage petabytes or exabytes of data. To store this huge amount of data, thousands or tens of thousands storage nodes are required at a single site. This imposes three major challenges for storage system designers: (1) Reliability---node failure in these datacenters is a normal occurrence rather than a rare situation. This makes data reliability a great concern. (2) Energy efficiency---a data center can consume up to 100 times more energy than a standard office building. More than 10% of this energy consumption …
Mid-Infrared Plasmonics, Farnood Khalilzadeh Rezaie
Mid-Infrared Plasmonics, Farnood Khalilzadeh Rezaie
Electronic Theses and Dissertations
This dissertation reports investigations into materials for, and applications of, infrared surface plasmon polaritons (SPP). SPPs are inhomogeneous electromagnetic waves that are bound to the surface of a conductor. Tight confinement of electromagnetic energy, the primary virtue of SPPs for so-called "plasmonic" applications, requires plasma frequencies for the conductor near the intended infrared operational frequencies. This requires carrier concentrations that are much less than those of usual metals such as gold and silver. I have investigated the optical properties and SPP excitation resonances of two materials having infrared plasma frequencies, namely the semimetal bismuth and the transparent conducting fluorine-doped tin-oxide …
Characterization Of Gold Black And Its Application In Un-Cooled Infrared Detectors, Deep Panjwani
Characterization Of Gold Black And Its Application In Un-Cooled Infrared Detectors, Deep Panjwani
Electronic Theses and Dissertations
Gold black porous coatings were thermally evaporated in the chamber backfilled with inert gas pressure and their optical properties were studied in near-far-IR wavelengths. The porosities of coatings were found to be extremely high around ~ 99%. Different approaches of effective medium theories such as Maxwell-Garnett, Bruggeman, Landau-Lifshitz-Looyenga and Bergman Formalism were utilized to calculate refractive index (n) and extinction coefficient (k). The aging induced changes on electrical and optical properties were studied in regular laboratory conditions using transmission electron microscopy, Fourier transform infrared spectroscopy, and fore-probe electrical measurements. A significant decrease in electrical resistance in as deposited coating was …
Structure-Property Relationship Of The Two-Photon Circular Dichroism Of Compounds With Axial And Helical Chirality, Carlos Diaz
Structure-Property Relationship Of The Two-Photon Circular Dichroism Of Compounds With Axial And Helical Chirality, Carlos Diaz
Electronic Theses and Dissertations
Back in 1894 Lord Kelvin coined the term "chiral" in order to refer to molecules whose mirror images were not superimposable with themselves. Over the years, research has demonstrated the important role that chiral molecules play in life, chemistry, and biology as well as their importance in the development of new drugs and technologies. The efforts to understand chiral systems have been mainly driven by spectroscopic methods that leverage on the opposite responses that enantiomers have to linear or circularly polarized light of both handedness. More specifically, Electronic Circular Dichroism (ECD) which measures the differences in linear absorption of left …
Optical Propagation Of Self-Sustaining Wavefronts And Nonlinear Dynamics In Parabolic Multimode Fibers, Matthew Mills
Optical Propagation Of Self-Sustaining Wavefronts And Nonlinear Dynamics In Parabolic Multimode Fibers, Matthew Mills
Electronic Theses and Dissertations
The aim of this thesis is to introduce my work which has generally been focused on optical wavefronts that have the unusual property of resisting commonplace phenomena such as diffraction and dispersion. Interestingly, these special beams are found both in linear and nonlinear situations. For example, in the linear regime, localized spatio-temporal waves which resemble the spherical harmonic symmetries of the hydrogen quantum orbitals can simultaneously negotiate both diffractive and dispersive effects. In the nonlinear regime, dressed optical filaments can be arranged to propagate multi-photon produced plasma channels orders of magnitude longer than expected. The first portion of this dissertation …
Convective Heat Transfer In Quasi-One-Dimensional Magnetic Fluid In Horizontal Field And Temperature Gradients, Jun Huang
Electronic Theses and Dissertations
In this work we studied the convective heat transfer in a magnetic fluid in both zero and applied magnetic fields. The natural convection is observed in a quasi-one dimensional magnetic fluid in a horizontal temperature gradient. The horizontal non-homogeneous magnetic fields were applied across the sample cell either parallel or anti-parallel to the temperature gradient. The temperature profile was measured by eight thermocouples and temperature sensitive paint. The flow velocity field and streamlines were obtained by optical flow method. Calculated Nusselt numbers, Rayleigh number, and Grashof number show that the convective flow is the main heat transfer mechanism in applied …
Quantum Chemical Studies For The Engineering Of Metal Organic Materials, Hector Javier Rivera Jacquez
Quantum Chemical Studies For The Engineering Of Metal Organic Materials, Hector Javier Rivera Jacquez
Electronic Theses and Dissertations
Metal Organic Materials (MOM) are composed of transition metal ions as connectors and organic ligands as linkers. MOMs have been found to have high porosity, catalytic, and optical properties. Here we study the gas adsorption, color change, and non-linear optical properties of MOMs. These properties can be predicted using theoretical methods, and the results may provide experimentalists with guidance for rational design and engineering of novel MOMs. The theory levels used include semi-empirical quantum mechanical calculations with the PM7 Hamiltonian and, Density Functional Theory (DFT) to predict the geometry and electronic structure of the ground state, and Time Dependent DFT …
Synthesis And Characterization Of New Probes For Use In Fluorescence And X-Ray Ct Bioimaging, Simon Tang
Synthesis And Characterization Of New Probes For Use In Fluorescence And X-Ray Ct Bioimaging, Simon Tang
Electronic Theses and Dissertations
The pursuit of more suitable drugs intended for possible biological applications are a continuously growing topic of research within the scientific community. One of these suitable qualities includes the need for hydrophilicity and or some appropriate delivery system for the drug to enter into biological systems. A system of analyzing and following these compounds would then, however, be necessary to conduct any kind of mechanistic or interaction studies for he said drug within the biological system. Just to name a few, fluorescence and X-ray computed tomography (CT) methods allow for imaging of biological systems but require the need of compounds …
Observations, Thermochemical Calculations, And Modeling Of Exoplanetary Atmospheres, Jasmina Blecic
Observations, Thermochemical Calculations, And Modeling Of Exoplanetary Atmospheres, Jasmina Blecic
Electronic Theses and Dissertations
This dissertation as a whole aims to provide the means to better understand hot-Jupiter planets through observing, performing thermochemical calculations, and modeling their atmospheres. We used Spitzer multi-wavelength secondary-eclipse observations to characterize planetary atmospheres. We chose targets with high signal-to-noise ratios, as their deep eclipses allow us to detect signatures of spectral features and assess planetary atmospheric structure and composition with greater certainty. Chapter 1 gives a short introduction. Chapter 2 presents the Spitzer secondary-eclipse analysis and atmospheric characterization of WASP-14b. The decrease in flux when a planet passes behind its host star reveals the planet dayside thermal emission, which, …
Reasoning Tradeoffs In Implicit Invocation And Aspect Oriented Languages, Jose Sanchez Salazar
Reasoning Tradeoffs In Implicit Invocation And Aspect Oriented Languages, Jose Sanchez Salazar
Electronic Theses and Dissertations
To reason about a program means to state or conclude, by logical means, some properties the program exhibits; like its correctness according to certain expected behavior. The continuous need for more ambitious, more complex, and more dependable software systems demands for better mechanisms to modularize them and reason about their correctness. The reasoning process is affected by the design decisions made by the developer of the program and by the features supported by the programming language used. Beyond Object Orientation, Implicit Invocation and Aspect Oriented languages pose very hard reasoning challenges. Important tradeoffs must be considered while reasoning about a …
Vanadium Oxide Microbolometers With Patterned Gold Black Or Plasmonic Resonant Absorbers, Evan Smith
Vanadium Oxide Microbolometers With Patterned Gold Black Or Plasmonic Resonant Absorbers, Evan Smith
Electronic Theses and Dissertations
High sensitivity uncooled microbolometers are necessary to meet the needs of the next generation of infrared detectors, which seek low power consumption and production cost without sacrificing performance. Presented here is the design, fabrication, and characterization of a microbolometer with responsivity enhanced by novel highly absorptive coatings. The device utilizes a gold-doped vanadium oxide film in a standard air bridge design. Performance estimations are calculated from current theory, and efforts to maximize signal to noise ratio are shown and evaluated. Most notably, presented are the experimental results and analysis from the integration of two different absorptive coatings: a patterned gold …
Tiling With Polyominoes, Polycubes, And Rectangles, Michael Saxton
Tiling With Polyominoes, Polycubes, And Rectangles, Michael Saxton
Electronic Theses and Dissertations
In this paper we study the hierarchical structure of the 2-d polyominoes. We introduce a new infinite family of polyominoes which we prove tiles a strip. We discuss applications of algebra to tiling. We discuss the algorithmic decidability of tiling the infinite plane Z x Z given a finite set of polyominoes. We will then discuss tiling with rectangles. We will then get some new, and some analogous results concerning the possible hierarchical structure for the 3-d polycubes.
Towards High-Flux Isolated Attosecond Pulses With A 200 Tw Cpa, Eric Cunningham
Towards High-Flux Isolated Attosecond Pulses With A 200 Tw Cpa, Eric Cunningham
Electronic Theses and Dissertations
Attosecond pulses have been developed as a means for investigating phenomena that proceed on the order of the atomic unit of time (24 as). Unfortunately, these extreme ultraviolet (XUV) pulses by themselves contain too few photons to initiate nonlinear dynamics or dress states in an attosecond pump--attosecond probe scheme. As a result, most attosecond experiments thus far have featured complementary near infrared (NIR) femtosecond lasers for instigating electron dynamics. In order to access the benefits of all-attosecond measurements and open attosecond physics to new fields of exploration, the photon flux of these pulses must be increased. One way to boost …
Quantitative Assessment Of The Effects Of Microbial Degradation Of A Simple Hydrocarbon Mixture, Jessica Kindell
Quantitative Assessment Of The Effects Of Microbial Degradation Of A Simple Hydrocarbon Mixture, Jessica Kindell
Electronic Theses and Dissertations
Ignitable liquids consist of either a single organic compound or a complex organic mixture. In regards to fire debris analysis, the analyst is responsible for determining if an ignitable liquid residue is present. However, when extracted from soil-containing fire debris evidence, chemical degradation from microorganisms is observed to result in the loss of compounds based on chemical structure. It can also happen when the evidence container is stored at room temperature before analysis. This can present a challenge to the fire debris analyst when identifying and classifying the ignitable liquid residue based on the criteria established by standard test methods. …
Investigation Of Optical And Electronic Properties Of Au Decorated Mos2, Udai Bhanu
Investigation Of Optical And Electronic Properties Of Au Decorated Mos2, Udai Bhanu
Electronic Theses and Dissertations
Achieving tunability of two dimensional (2D) transition metal dichalcogenides (TMDs) functions calls for the introduction of hybrid 2D materials by means of localized interactions with zero dimensional (0D) materials. A metal-semiconductor interface, as in gold (Au) - molybdenum disulfide (MoS2), is of great interest from the standpoint of fundamental science as it constitutes an outstanding platform to investigate optical and electronic properties due to charge transfer. The applied aspects of such systems introduce new options for electronics, photovoltaics, detectors, catalysis, and biosensing. Here in this dissertation, we study the charge transfer interaction between Au nanoparticals and MoS2 flakes and its …
Nano And Nanostructured Materials For Optical Applications, Panit Chantharasupawong
Nano And Nanostructured Materials For Optical Applications, Panit Chantharasupawong
Electronic Theses and Dissertations
Nano and nanostructured materials offer unique physical and chemical properties that differ considerably from their bulk counterparts. For decades, due to their fascinating properties, they have been extensively explored and found to be beneficial in numerous applications. These materials are key components in many cutting-edge optic and photonic technologies, including photovoltaics, waveguides and sensors. In this dissertation, the uses of nano and nanostructured materials for optical applications are investigated in the context of optical limiting, three dimensional displays, and optical sensing. Nanomaterials with nonlinear optical responses are promising candidates for self-activating optical limiters. In the first part of this study, …
Two-Photon Absorption In Bulk Semiconductors And Quantum Well Structures And Its Applications, Himansu Pattanaik
Two-Photon Absorption In Bulk Semiconductors And Quantum Well Structures And Its Applications, Himansu Pattanaik
Electronic Theses and Dissertations
The purpose of this dissertation is to provide a study and possible applications of two-photon absorption (2PA), in direct-gap semiconductors and quantum-well (QW) semiconductor structures. One application uses extremely nondegenerate (END) 2PA, for mid-infrared (mid-IR) detection in uncooled semiconductors. The use of END, where the two photons have very different energies gives strong enhancement comapared to degenerate 2PA. This END-2PA enhanced detection is also applied to mid-IR imaging and light detection and ranging (LIDAR) in uncooled direct-gap photodiodes. A theoretical study of degenerate 2PA (D-2PA) in quantum wells, QWs, is presented, along with a new theory of ND 2PA in …