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Physics

North Carolina Agricultural and Technical State University

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Sources And Atmospheric Oxidation Of Sulfur Dioxide And Formaldehyde Based On Wintertime Aircraft Observations Over The Eastern United States, Jaime R. Green Jan 2019

Sources And Atmospheric Oxidation Of Sulfur Dioxide And Formaldehyde Based On Wintertime Aircraft Observations Over The Eastern United States, Jaime R. Green

Dissertations

Plume intercepts from flights on the NSF-C-130 during the Wintertime Investigation of Transport, Emission and Reactivity (WINTER) campaign were used to estimate (1) the oxidation rates of Sulfur Dioxide (SO2) under wintertime conditions and the factors that determine SO2 removal; and (2) to examine the oxidation, lifetime and source apportionment of formaldehyde (HCHO). Observations suggest that OH governs the rate SO2 oxidation in the eastern United States during winter. The range of mean oxidation rates during the day from power plants were 0.22–0.71%/hr, producing SO2 lifetimes of 13–43 days, if SO2 consumption is assumed to occur during 10.5 hr of …