Atomic, Molecular and Optical Physics Commons^™

Computational Study Of The Hydration Of Sulfuric Acid Dimers: Implications For Acid Dissociation And Aerosol Formation, Berhane Temelso, Thuong Ngoc Phan, George C. Shields

Faculty Journal Articles

We have investigated the thermodynamics of sulfuric acid dimer hydration using ab initio quantum mechanical methods. For (H₂SO₄)₂(H₂O)_n where n = 0−6, we employed high-level ab initio calculations to locate the most stable minima for each cluster size. The results presented herein yield a detailed understanding of the first deprotonation of sulfuric acid as a function of temperature for a system consisting of two sulfuric acid molecules and up to six waters. At 0 K, a cluster of two sulfuric acid molecules and one water remains undissociated. Addition of a second …

Development And Implementation Of Acoustic Feedback Control For Scanning Probe Microscopy, Rodolfo Fernandez Rodriguez

Dissertations and Theses

A remote-sensing acoustic method for implementing position control feedback in Scanning Probe Microscopy (SPM) is presented. The capabilities of this feedback control using the new Whispering Gallery Acoustic Sensing (WGAS) method is demonstrated in a Shear-force Scanning Probe Microscope that uses a sharp probe attached to a piezoelectric Quartz Tuning Fork (QTF) firmly mounted on the microscope's frame. As the QTF is electrically driven its mechanical response reaches the SPM frame which then acts as a resonant cavity producing acoustic modes measured with an acoustic sensor strategically placed on the SPM head. The novelty of the WGAS resides in using …

Using Frequency-Narrowed, Tunable Laser Diode Arrays With Integrated Volume Holographic Gratings For Spin-Exchange Optical Pumping At High Resonant Fluxes And Xenon Densities, Nicholas Whiting, Panayiotis Nikolaou, Neil A. Eschmann, Michael J. Barlow, R Lammert, J Ungar, W Hu, Laurent Vaissie, Boyd M. Goodson

Nicholas Whiting

Measurement Of The Neutron -Asymmetry Parameter A0 With Ultracold Neutrons, Bradley Plaster, R. Rios, Thomas J. Bowles, Leah J. Broussard, Richard Carr, Steven Clayton, Scott Currie, Bradley W. Filippone, Peter Geltenbort, Kevin P. Hickerson, J. Todd Hoagland, Gary E. Hogan, B. Hona, Anthoney T. Holley, Takeyasu M. Ito, Chenyu Liu, Jingyang Liu, Mark Makela, J. W. Martin, Daniel Melconian, Michael P. Mendenhall, Charles L. Morris, R. Mortensen, Robert W. Pattie, Margaret L. Pitt, John C. Ramsey, R. Russell, Andy Saunders, R. Schmid, Susan J. Seestrom, Sky Sjue, Walter E. Sondheim, E. Tatar, B. Tipton, Robert B. Vogelaar, Brittany Vorndick, Christopher Wrede, Y. P. Xu, H. Yan, Andrew R. Young, J. Yuan

Robert W. Pattie Jr.

Picosecond Rotationally Resolved Stimulated Emission Pumping Spectroscopy Of No, Chakree Tanjaroon, Scott Reeve, Alan Ford Ford, W. Dean Murray, Kevin Lyon, Bret Yount, Dan Britton, William Burns, Susan D. Allen, J. Bruce Johnson

Scott Reeve

No abstract provided.

Cavity Ringdown Spectroscopy Of 13c2h2 In The 12900-13400 Region.Pdf, Christopher J. Lue, Michael Sullivan, Mark Draganjac, Scott Reeve

Scott Reeve

No abstract provided.

Superhalogen Properties Of Cumcln Clusters: Theory And Experiment, Y. J. Ko, H. Wang, K. Pradhan, P. Koirala, Anil K. Kandalam, K. H. Bowen, P. Jena

Physics & Engineering Faculty Publications

No abstract provided.

Achieving Laser Wavelength Stability For Use In Neutral Atom Quantum Computing, Jennifer H. Rushing

Physics

Quantum computing may still be decades away from realization but the pieces necessary for the construction of the first quantum chip are beginning to come together. One piece still eluding researchers is the ability to address individual atoms within a scalable quantum chip structure. The resolution to this issue may be found in any one of several promising implementations, including the use of neutral atoms trapped in 2D optical lattices. One method of constructing such lattices, which has been shown to be computationally viable, employs the diffraction pattern just behind a circular aperture. Laser wavelength stability plays a crucial role …

Water Ice Films In Cryogenic Vacuum Chambers, Jesse Michael Labello

Doctoral Dissertations

The space simulation chambers at Arnold Engineering Development Complex (AEDC) allow for the testing and calibration of seeker sensors in cryogenic, high vacuum environments. During operation of these chambers, contaminant films can form on the components in the chamber and disrupt operation. Although these contaminant films can be composed of many molecular species, depending on the species outgassed by warm chamber components and any leaks or virtual leaks (pockets of gas trapped within a vacuum chamber) that may be present, water vapor is most common, and it will be the focus of this dissertation. In this dissertation, some properties of …

Dipole-Dipole Interaction Between Rubidium Rydberg Atoms, Emily Altiere, Donald P. Fahey, Michael W. Noel, Rachel J. Smith, Thomas J. Carroll

Physics and Astronomy Faculty Publications

Ultracold Rydberg atoms in a static electric field can exchange energy via the dipole-dipole interaction. The Stark effect shifts the energy levels of the atoms which tunes the energy exchange into resonance at specific values of the electric field (F¨orster resonances). We excite rubidium atoms to Rydberg states by focusing either a 480 nm beam from a tunable dye laser or a pair of diode lasers into a magneto-optical trap. The trap lies at the center of a configuration of electrodes. We scan the electric field by controlling the voltage on the electrodes while measuring the fraction of atoms that …

Equation Of State From The Potts-Percolation Model Of A Solid, Miron Kaufman

Physics Faculty Publications

We expand the Potts-percolation model of a solid to include stress and strain. Neighboring atoms are connected by bonds. We set the energy of a bond to be given by the Lennard-Jones potential. If the energy is larger than a threshold the bond is more likely to fail, whereas if the energy is lower than the threshold, the bond is more likely to be alive. In two dimensions we compute the equation of state: stress as a function of interatomic distance and temperature by using renormalization-group and Monte Carlo simulations. The phase diagram, the equation of state, and the isothermal …

Peeling Adhesive Tape Emits Electromagnetic Radiation At Terahertz Frequencies, J. Horvat, R. A. Lewis

Roger A. Lewis

An unusual concept for a simple and inexpensive terahertz source is presented: unpeeling adhesive tape. The observed spectrum of this terahertz radiation exhibits a peak at 2 THz and a broader peak at 18 THz. The radiation is not polarized. The mechanism of terahertz radiation is tribocharging of the adhesive tape and subsequent discharge, possibly bremsstrahlung with absorption or energy density focusing during the dielectric breakdown of a gas. The accompanying optical emission is also a consequence of tribocharging.

Peeling Adhesive Tape Emits Electromagnetic Radiation At Terahertz Frequencies, J. Horvat, R. A. Lewis

Josip Horvat

An unusual concept for a simple and inexpensive terahertz source is presented: unpeeling adhesive tape. The observed spectrum of this terahertz radiation exhibits a peak at 2 THz and a broader peak at 18 THz. The radiation is not polarized. The mechanism of terahertz radiation is tribocharging of the adhesive tape and subsequent discharge, possibly bremsstrahlung with absorption or energy density focusing during the dielectric breakdown of a gas. The accompanying optical emission is also a consequence of tribocharging.

Dc Pulsed Atmospheric Pressure Plasma Jet Image Information, Denis P. Dowling, F T. O'Neill, Vladimir Milosavljevic, Victor J. Law

Articles

This paper presents optical imaging and optical emission spectroscopy (OES) data of an atmospheric-pressure plasma jet. It is shown how the visual information and OES information of the air discharge are related as the blown arc extends from the nozzle (2-4 mm) with a molecular nitrogen rotational temperature on the order of 1700 K and the flowing afterglow beyond this region is dominated by the cooler (300-K) NO-O chemiluminescent reaction that produces NO₂ species.

Wave-Function Functionals For The Density, Marlina Slamet, Xiao-Yin Pan, Viraht Sahni

Publications and Research

We extend the idea of the constrained-search variational method for the construction of wave-function functionals psi[chi] of functions chi. The search is constrained to those functions chi such that psi[chi] reproduces the density rho(r) while simultaneously leading to an upper bound to the energy. The functionals are thereby normalized and automatically satisfy the electron-nucleus coalescence condition. The functionals psi[chi] are also constructed to satisfy the electron-electron coalescence condition. The method is applied to the ground state of the helium atom to construct functionals psi[chi] that reproduce the density as given by the Kinoshita correlated wave function. The expectation of single-particle …

Photoelectron Spectroscopic Study Of Iron-Pyrene Cluster Anions, Xiang Li, Kit H. Bowen Jr., Puru Jena, Anil K. Kandalam

Physics & Engineering Faculty Publications

No abstract provided.

Wavelength Dependence Of Transverse Mode Coupling With/Without E-Block Of Gan Laser Cavity, Krishneel Lal

Electrical Engineering

No abstract provided.

Selection Of Dd Branch In Fusion Reactions To Minimize Neutron Output, Courtney Matzkind

Von Braun Symposium Student Posters

No abstract provided.

Structural Evolution And Stabilities Of Neutral And Anionic Clusters Of Lead Sulfide: Joint Anion Photoelectron And Computational Studies, Pratik Koirala, Boggavarapu Kiran, Anil K. Kandalam, Charles A. Fancher, Helen L. De Clercq, Xiang Li, Kit H. Bowen

Physics & Engineering Faculty Publications

No abstract provided.

Distributed Spacing Stochastic Feature Selection And Its Application To Textile Classification, Jeffrey D. Clark

Theses and Dissertations

Many situations require the need to quickly and accurately locate dismounted individuals in a variety of environments. In conjunction with other dismount detection techniques, being able to detect and classify clothing (textiles) provides a more comprehensive and complete dismount characterization capability. Because textile classification depends on distinguishing between different material types, hyperspectral data, which consists of several hundred spectral channels sampled from a continuous electromagnetic spectrum, is used as a data source. However, a hyperspectral image generates vast amounts of information and can be computationally intractable to analyze. A primary means to reduce the computational complexity is to use feature …