Enabling Rapid Chemical Analysis Of Plutonium Alloys Via Machine Learning-Enhanced Atomic Spectroscopy Techniques, 2022 Air Force Institute of Technology
Enabling Rapid Chemical Analysis Of Plutonium Alloys Via Machine Learning-Enhanced Atomic Spectroscopy Techniques, Ashwin P. Rao
Theses and Dissertations
Analytical atomic spectroscopy methods have the potential to provide solutions for rapid, high fidelity chemical analysis of plutonium alloys. Implementing these methods with advanced analytical techniques can help reduce the chemical analysis time needed for plutonium pit production, directly enabling the 80 pit-per-year by 2030 manufacturing goal outlined in the 2018 Nuclear Posture Review. Two commercial, handheld elemental analyzers were validated for potential in situ analysis of Pu. A handheld XRF device was able to detect gallium in a Pu surrogate matrix with a detection limit of 0.002 wt% and a mean error of 8%. A handheld LIBS device was …
Developing Optical Devices And Projects For Teaching Engineering, 2022 Bethel University
Developing Optical Devices And Projects For Teaching Engineering, Nathan D. Lemke, John Mccauley, Tristan E. Noble, Grace Riermann, Ellesa St. George, Nathan C. Lindquist, Keith R. Stein, Karen Irene Rogers
Physics and Engineering Faculty Publications
We are creating a suite of tools and techniques based on optics to be used for teaching a variety of engineering topics. Each tool is intended for non-expert use and without the need for high-end equipment such as vibration-free optical tables. Here we report progress on three such tools: image-plane digital holography for measuring mechanical deformation; schlieren imaging of convective flows using a smart phone; and a simple optical communication protocol using LabVIEW. We will present the designs of the tools and preliminary results from teaching engineering labs and projects with these tools. Specific courses impacted to date include Fluid …
Adsorption Of Helium And Hydrogen On Triphenylene And 1,3,5-Triphenylbenzene, 2022 University of Innsbruck
Adsorption Of Helium And Hydrogen On Triphenylene And 1,3,5-Triphenylbenzene, Bergmeister Bergmeister, Kollotzek Kollotzek, Florent Calvo, Elisabeth Gruber, Fabio Zappa, Paul Scheier, Olof E. Echt
Faculty Publications
The adsorption of helium or hydrogen on cationic triphenylene (TPL, C18H12), a planar polycyclic aromatic hydrocarbon (PAH) molecule, and of helium on cationic 1,3,5-triphenylbenzene (TPB, C24H18), a propeller-shaped PAH, is studied by a combination of high-resolution mass spectrometry and classical and quantum computational methods. Mass spectra indicate that HenTPL+ complexes are particularly stable if n = 2 or 6, in good agreement with the quantum calculations which show that for these sizes the helium atoms are strongly localized on either side of the central carbon ring for n = …
Using Optical Tweezersto Probe Dna Polymerase Kappa’S Binding Mechanism To Dna, 2022 Bridgewater State University
Using Optical Tweezersto Probe Dna Polymerase Kappa’S Binding Mechanism To Dna, Joshua Watts
Honors Program Theses and Projects
The integrity of our DNA is constantly under threat from many internal and external factors. If the cell cannot properly protect the integrity of DNA, errors (lesions) in DNA may form which can lead to cancer. Most of these lesions serve as a roadblock to the protein, DNA polymerase (Pol), that replicates the DNA during cell division. The mechanism that is employed to read through these errors is called translesion DNA synthesis (TLS). During this process, a special class of DNA polymerases known as TLS DNA Pols that can tolerate and bypass the lesions in DNA are employed by the …
The 'Quantal Newtonian' First Law: A Complementary Perspective To The Stationary-State Quantum Theory Of Electrons, 2022 CUNY Brooklyn College
The 'Quantal Newtonian' First Law: A Complementary Perspective To The Stationary-State Quantum Theory Of Electrons, Viraht Sahni
Publications and Research
A complementary perspective to the Göttingen-Copenhagen interpretation of stationary-state quantum theory of electrons in an electromagnetic field is described. The perspective, derived from Schrödinger-Pauli theory, is that of the individual electron via its equation of motion or ‘Quantal Newtonian’ First Law. The Law is in terms of ‘classical’ fields experienced by each electron: the sum of the external and internal fields vanishes. The external field is a sum of the electrostatic and Lorentz fields. The internal field is a sum of fields’ representative of Pauli and Coulomb correlations; kinetic effects; electron density; and internal magnetic component. The energy is obtained …
Studying The Synthesis Of 196Hg At Astrophysically Relevant Energies Through The Measurement Of Capture Reaction Cross-Sections Of (P, Γ) (P, N) And (P, Α) Reactions, 2022 Western Michigan University
Studying The Synthesis Of 196Hg At Astrophysically Relevant Energies Through The Measurement Of Capture Reaction Cross-Sections Of (P, Γ) (P, N) And (P, Α) Reactions, Khushi Bhatt
Dissertations
Understanding the origin of all the chemical elements is an important question for the nuclear-astrophysics community. There are many unanswered questions like: What astrophysical events are responsible for the synthesis of what particular chemical elements? How many different elements were made in total? What is the abundance of each synthesized element? etc. Currently, scientists are largely depending upon theory and simulations to define nuclear and astrophysical reaction. This makes it critical to have accurate experimental nuclear physics data to input in astrophysical theoretical models. However, out of more than 20000 reactions involved in these calculations, only a very few are …
Using Coherence And Interference To Study The Few Body Dynamics In Simple Atomic Collisions Systems, 2022 Missouri University of Science and Technology
Using Coherence And Interference To Study The Few Body Dynamics In Simple Atomic Collisions Systems, Sujan Bastola
Doctoral Dissertations
"Atomic Collision experiments are best suited to sensitively test the few-body dynamics of simple systems. The few-body dynamics, in turn, can be sensitively affected by interference effects. However, an important requirement to observe interference effects in atomic scattering experiments is that the incoming projectile beam must be coherent. The coherence properties of the incoming projectile can be controlled by the geometry of the collimating slit placed before the target. We performed a kinematically complete experiment where a 75 keV proton beam is crossed with a molecular hydrogen beam to study the dissociative capture process. The motivation for this project was …
Quantum Dots In Two-Dimensional Tungsten Diselenide, 2022 University of Arkansas, Fayetteville
Quantum Dots In Two-Dimensional Tungsten Diselenide, Jeb Allen Michael Stacy
Graduate Theses and Dissertations
This work focuses on the investigation of single and double quantum dots in two-dimensional transition metal dichalcogenide tungsten diselenide (WSe_2) as a means to evaluate the valley degree of freedom as a potential qubit and ambipolar tungsten diselenide monolayers as single photon sources. Gate-defined quantum dots in monolayer and bilayer WSe_2 were fabricated and characterized. Single dot devices are gated from above and below the WSe_2 to accumulate a hole gas. Temperature dependence of Coulomb-blockade peak height is consistent with single-level transport. Excited-state transport in the quantum dot is shown for both monolayer and bilayer devices. Magnetic field dependence of …
Probing The Equation Of State Of Neutron Stars With Heavy Ion Collisions, 2022 Western Michigan University
Probing The Equation Of State Of Neutron Stars With Heavy Ion Collisions, Om Bhadra Khanal
Dissertations
The equation of state (EOS) is a fundamental property of nuclear matter, important for studying the structure of systems as diverse as the atomic nucleus and the neutron star. Nuclear reactions, especially heavy-ion collisions in the laboratories, can produce the nuclear matter similar to those contained in neutron stars. The density and the momentum dependence of the EOS of asymmetric nuclear matter, especially the symmetry energy term, is widely unconstrained. Finding appropriate constrains, especially at higher densities of the nuclear matter, requires the development of new devices, new experimental measurements as well as advances in theoretical understanding of nuclear collisions …
Hierarchically Structured Photoelectrodes Via Atomic Layer Deposition, 2022 University of Arkansas, Fayetteville
Hierarchically Structured Photoelectrodes Via Atomic Layer Deposition, Justin Rowan Reed Demoulpied
Graduate Theses and Dissertations
In the search for a sustainable method to meet increasing energy needs, solar energy emerges as an underutilized, plentiful resource. Solar intermittency and requirements for transportation necessitate storing solar energy in the form of chemical bonds via artificial photosynthesis. Photoelectrochemical (PEC) water splitting generates hydrogen fuel from solar energy and water. A semiconducting material that successfully meets the complex requirements for building an industrially scalable PEC device has yet to emerge. This is leading to a reevaluation of materials previously overlooked within PEC research, mainly materials with limitations such as minimal charge carrier mobility and propensity to corrosion under illumination …
Study Of Single-Photon Wave-Packets With Atomically Thin Nonlinear Mirrors, 2022 University of Arkansas, Fayetteville
Study Of Single-Photon Wave-Packets With Atomically Thin Nonlinear Mirrors, Christopher Klenke
Graduate Theses and Dissertations
A novel controlled phase gate for photonic quantum computing is proposed by exploiting the powerful nonlinear optical responses of atomically thin transition metal dichalcogenides (TMDs) and it is shown that such a gate could elicit a π-rad phase shift in the outgoing electric field only in the case of two incident photons and no other cases. Firstly, the motivation for such a gate is developed and then the implementation of monolayer TMDs is presented as a solution to previous realization challenges. The single-mode case of incident photons upon a TMD is derived and is then used to constrain the more …
Development Of High Quantum Efficiency Strained Superlattice Spin Polarized Photocathodes Via Metal Organic Chemical Vapor Deposition, 2022 Old Dominion University
Development Of High Quantum Efficiency Strained Superlattice Spin Polarized Photocathodes Via Metal Organic Chemical Vapor Deposition, Benjamin Belfore
Electrical & Computer Engineering Theses & Dissertations
Spin polarized photocathodes are necessary to examine parity violations and other fundamental phenomena in the field of high energy physics. To create these devices, expensive and complicated growth processes are necessary. While integral to accelerator physics, spin polarized electrons could have other exciting applications in materials science and other fields of physics. In order to explore these other applications feasibly, the relative supply of spin polarized photocathodes with a high rate of both polarization and photoemission needs to be increased. One such way to increase this supply is to develop the means to grow them faster and at a larger …
Resonant Energy Exchange In Ultracold Rydberg Atoms, 2022 Ursinus College
Resonant Energy Exchange In Ultracold Rydberg Atoms, Samantha Grubb, Alan Okinaka
Physics and Astronomy Summer Fellows
Ultracold Rydberg atoms serve as good systems in which resonant dipole-dipole interactions can be observed. The goal of our work is to design a simulation in which energy exchange among many nearly evenly spaced energy levels is observed. These observations are useful for understanding the time evolution of complicated quantum systems, and have applications in quantum computing and simulating. We are utilizing a supercomputer to run our simulation as well as studying the system experimentally. Once we obtain simulated results, we plan to compare them with the results obtained in a lab.
Weakness Of Weak Values: Incompatibility Of Anomalous Pulse-Spectrum Amplification And Optical Frequency Combs, 2022 Chapman University
Weakness Of Weak Values: Incompatibility Of Anomalous Pulse-Spectrum Amplification And Optical Frequency Combs, John C. Howell
Mathematics, Physics, and Computer Science Faculty Articles and Research
We probe the use of optical frequency combs to place lower bounds on anomalous amplification of a weak-value-measured pulse delay, potentially reaching a theoretical temporal resolution of better than 10−34 s. Owing to the interferometric behavior of weak values, we show that anomalous weak value amplification of a time delay is not equivalent to a temporal linear phase ramp. We show that the anomalous weak value is a rearrangement of amplitudes that generates an apparent shift that can be measured in direct detection, but does not change the actual frequency offset of a spectral distribution measurable in coherent detection. …
Atomic Gradiometry Based On The Interference Of Microwave Optical Sidebands, 2022 University of New Mexico - Main Campus
Atomic Gradiometry Based On The Interference Of Microwave Optical Sidebands, Kaleb L. Campbell
Optical Science and Engineering ETDs
We describe a novel pulsed magnetic gradiometer based on the optical interference of sidebands generated using two spatially separated alkali vapor cells. The sidebands are produced with high efficiency using parametric frequency conversion of a probe beam interacting with Rubiduim 87 atoms in a coherent superposition of magnetically sensitive hyperfine ground states. First, experimental evidence of the sideband process is described for both steady-state and pulsed operation. Then, a theoretical framework is developed that accurately models sideband generation based on density matrix formalism. The gradiometer is then constructed using two spatially separated vapor cells, and a beat-note is generated. The …
Neutron Interferometry Using A Single Modulated Phase Grating, 2022 Louisiana State University and Agricultural and Mechanical College
Neutron Interferometry Using A Single Modulated Phase Grating, Ivan J. Hidrovo Giler
LSU Master's Theses
Neutron grating interferometry provides information on phase and small-angle scatter in addition to attenuation. Previously, phase grating moiré interferometers (PGMI) with two or three phase gratings have been developed. These phase-grating systems use the moiré far-field technique to avoid the need for high-aspect absorption gratings used in Talbot-Lau interferometers (TLI) which reduce the neutron flux reaching the detector. We demonstrate through simulations a novel phase grating interferometer system for cold neutrons that requires a single modulated phase grating (MPG) for phase-contrast imaging, as opposed to the two or three phase gratings in previously employed PGMI systems. We compare the MPG …
Characterization Of Electrophoretic Deposited Zinc Oxide Nanopartices For The Fabrication Of Next-Generation Nanoscale Electronic Applications, 2022 Louisiana State University and Agricultural and Mechanical College
Characterization Of Electrophoretic Deposited Zinc Oxide Nanopartices For The Fabrication Of Next-Generation Nanoscale Electronic Applications, Fawwaz Abduh A. Hazzazi
LSU Doctoral Dissertations
Several reports state that it is crucial to analyze nanoscale semiconductor materials and devices with potential benefits to meet the need for next-generation nanoelectronics, bio, and nanosensors. The progress in the electronics field is as significant now, with modern technology constantly evolving and a greater focus on more efficient robust optoelectronic applications. This dissertation focuses on the study and examination of the practicality of Electrophoretic Deposition (EPD) of zinc oxide (ZnO) nanoparticles (NPs) for use in semiconductor applications.
The feasibility of several synthesized electrolytes, with and without surfactants and APTES surface functionalization, is discussed. The primary objective of this study …
Surpassing The Standard Quantum Limit Using An Optical Spring, 2022 Louisiana State University and Agricultural and Mechanical College
Surpassing The Standard Quantum Limit Using An Optical Spring, Torrey Cullen
LSU Doctoral Dissertations
In 1916, Albert Einstein predicted the existence of gravitational waves based on his new theory of general relativity. He predicted an accelerating mass with a non-zero quadrupole moment would emit energy in the form of gravitational waves. Often referred to as ripples in space-time, gravitational waves are extremely small by the time reach Earth, potentially having traveled hundreds of megaparsecs. It is common for these ripples in space-time to stretch and squeeze matter 1000 times smaller than the width of a proton.
Laser interferometer observatories were first built in the 1990s in the US and Europe, and as sensitivity improvements …
Localized Surface Plasmon Resonance Of Copper Nanoparticles Using Finite Element Method, 2022 PhD Student, Faculty of Science, Beirut Arab University
Localized Surface Plasmon Resonance Of Copper Nanoparticles Using Finite Element Method, Samaya El Samad, Salem Marhaba
BAU Journal - Science and Technology
The aim of this paper is to study the interaction of the electromagnetic wave with plasmonic nanoparticles. Localized Surface Plasmon resonance (LSPR) characteristics are governed by the intrinsic properties of the nanoparticle (size, shape and dielectric environment). The extinction cross-section spectra of Cu nanoparticles are calculated using finite element method (FEM). By increasing both the size of the nanoparticle and the dielectric environment, the simulations show a red-shifting and broadening on the LSPR spectrum with enhancement of the spectral amplitude. The extinction cross section spectra are calculated using polarized light for non-spherical or assembled nanoparticles. We investigated the LSPR of …
Ultrafast Electron Diffraction: Visualizing Dynamic States Of Matter, 2022 Lawrence Berkeley National Laboratory
Ultrafast Electron Diffraction: Visualizing Dynamic States Of Matter, D. Filipetto, P. Musumed, R. K. Li, B. J. Siwick, M. R. Otto, Martin Centurion, J. P.F. Nunes
Martin Centurion Publications
Since the discovery of electron-wave duality, electron scattering instrumentation has developed into a powerful array of techniques for revealing the atomic structure of matter. Beyond detecting local lattice variations in equilibrium structures with the highest possible spatial resolution, recent research efforts have been directed towards the long sought-after dream of visualizing the dynamic evolution of matter in real-time. The atomic behavior at ultrafast timescales carries critical information on phase transition and chemical reaction dynamics, the coupling of electronic and nuclear degrees of freedom in materials and molecules, the correlation between structure, function and previously hidden metastable or nonequilibrium states of …