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Continuous Biotransformation Of Bisphenol A And Diclofenac By Laccase In An Enzymatic Membrane Reactor, Ngoc Luong Nguyen, Faisal I. Hai, William Price, Frederic Leusch, Felicity Roddick, Ewan J. Mcadam, Saleh Faraj Magram, Long D. Nghiem
Continuous Biotransformation Of Bisphenol A And Diclofenac By Laccase In An Enzymatic Membrane Reactor, Ngoc Luong Nguyen, Faisal I. Hai, William Price, Frederic Leusch, Felicity Roddick, Ewan J. Mcadam, Saleh Faraj Magram, Long D. Nghiem
Faisal I Hai
A novel enzymatic membrane reactor (EMR) was explored for continuous removal of two trace organic contaminatnts (TrOCs) ubiquitously detected in wastewater - namely bisphenol A (BPA and diclofnac (DCF) - by a commercially available laccase from aspergillus oryzae.
Enhancement Of Removal Of Trace Organic Contaminants By Powdered Activated Carbon Dosing Into Membrane Bioreactors, Ngoc Luong Nguyen, Faisal Ibney Hai, Long Nghiem, Jinguo Kang, William Price, Chul Park, Kazuo Yamamoto
Enhancement Of Removal Of Trace Organic Contaminants By Powdered Activated Carbon Dosing Into Membrane Bioreactors, Ngoc Luong Nguyen, Faisal Ibney Hai, Long Nghiem, Jinguo Kang, William Price, Chul Park, Kazuo Yamamoto
Faisal I Hai
This study compared the removal efficiency of 22 widespread trace organic contaminants by a laboratory-scale membrane bioreactor (MBR) with and without direct addition of powdered activated carbon (PAC) into the activated sludge reactor over a period of 312 days. The removal of hydrophilic and biologically persistent trace organic contaminants was immediately improved to above 95% after the addition of PAC into MBR. However, a compound-specific gradual decrease in removal underscored the requirement for the addition of fresh PAC. Adsorption onto PAC-added sludge appeared to play a significant role in the relatively more effective aqueous phase removal of a few resistant …
Introduction To Membrane Biological Reactors, Faisal Hai, Kazuo Yamamoto, Chung-Hak Lee
Introduction To Membrane Biological Reactors, Faisal Hai, Kazuo Yamamoto, Chung-Hak Lee
Faisal I Hai
This chapter delineats the rationale of combining the membrane and bioreactor technologies and systematically introduces the membrane biological reactors that are the focus of this book. This is followed by a brief account of the history of the various applications of membranes in conjunction with bioreactors and how the initial formats led to the development of the present day commercialized ones. The relative advantages of membrane biological reactors over the conventional biological processes are presented. The current status of the MBR market is described and the drivers propelling its growth along with the constraints are highlighted. The trends in world-wide …
Introduction - A Review Of Membrane Reactors, Fausto Gallucci, Angelo Basile, Faisal Ibney Hai
Introduction - A Review Of Membrane Reactors, Fausto Gallucci, Angelo Basile, Faisal Ibney Hai
Faisal I Hai
In the last decades, membrane catalysis has been studied by several research and the significant progress in this field is summarized in several review articles (Armor 1998, Lin 2001, Lu 2007, Mcleary 2006, Sanchez 2002, Saracco 1994, Shu 1991). Considering a IUPAC definition (Koros 1996), a membrane reactor (MR) is a device for simultaneously performing a reaction (steam reforming, dry reforming, autothermal reforming, etc.) and a membrane-based separation in the same physical device. Therefore, the membrane not only plays the role of a separator, but also takes place in the reaction itself. The term Membrane Bioreactor (MBR), on the other …
Gas-Diffusion, Extractive, Biocatalytic And Electrochemical Membrane Biological Reactors, Oskar Modin, Faisal Hai, Long Nghiem, Angelo Basile, Kensuke Fukushi
Gas-Diffusion, Extractive, Biocatalytic And Electrochemical Membrane Biological Reactors, Oskar Modin, Faisal Hai, Long Nghiem, Angelo Basile, Kensuke Fukushi
Faisal I Hai
Several emerging technologies for treatment or resource recovery from wastewater are based on the combination of membranes and biochemical conversions. In this chapter, we review gas-diffusion, extractive, biocatalytic, and electrochemical membrane bioreactors (MBRs). Gas diffusion MBRs facilitate efficient delivery of a gaseous oxidant or reductant such as oxygen, hydrogen, or methane to microbial biofilms treating wastewater. Extractive MBRs completely separate the wastewater stream from the microbes and make toxic wastewaters amenable to biological treatment. Biocatalytic MBRs utilize enzymes or immobilized microbial cells for degradation of persistent xenobiotics or for synthesis of fine chemicals. Electrochemical MBRs make it possible to utilize …
Membrane Biological Reactors: Theory, Modeling, Design, Management And Applications To Wastewater Reuse, Faisal Hai, Kazou Yamamoto, Chung-Hak Lee
Membrane Biological Reactors: Theory, Modeling, Design, Management And Applications To Wastewater Reuse, Faisal Hai, Kazou Yamamoto, Chung-Hak Lee
Faisal I Hai
Membrane Biological Reactors: Theory, Modeling, Design, Management and Applications to Wastewater Reuse comprehensively covers the salient features and emerging issues associated with the MBR technology. The book provides thorough coverage starting from biological aspects and fundamentals of membranes, via modeling and design concepts, to practitioners’ perspective and good application examples. Membrane Biological Reactors focuses on all the relevant emerging issues raised by including the latest research from renowned experts in the field. It is a valuable reference to the academic and professional community and suitable for undergraduate and postgraduate teaching in Environmental Engineering, Chemical Engineering and Biotechnology.
Comparison Between Sequential And Simultaneous Application Of Activated Carbon With Membrane Bioreactor For Trace Organic Contaminant Removal, Luong N. Nguyen, Faisal I. Hai, Jinguo Kang, Long D. Nghiem, William E. Price, Wenshan Guo, Huu H. Ngo, Kuo-Lun Tung
Comparison Between Sequential And Simultaneous Application Of Activated Carbon With Membrane Bioreactor For Trace Organic Contaminant Removal, Luong N. Nguyen, Faisal I. Hai, Jinguo Kang, Long D. Nghiem, William E. Price, Wenshan Guo, Huu H. Ngo, Kuo-Lun Tung
Faisal I Hai
The removal efficiency of 22 selected trace organic contaminants by sequential application of granular activated carbon (GAC) and simultaneous application of powdered activated carbon (PAC) with membrane bioreactor (MBR) was compared in this study. Both sequential application of GAC following MBR treatment (MBR–GAC) and simultaneous application of PAC within MBR (PAC–MBR) achieved improved removal (over 95%) of seven hydrophilic and biologically persistent compounds, which were less efficiently removed by MBR-only treatment (negligible to 70%). However, gradual breakthrough of these compounds occurred over an extended operation period. Charged compounds, particularly, fenoprop and diclofenac, demonstrated the fastest breakthrough (complete and 50–70%, in …
Coupling Granular Activated Carbon Adsorption With Membrane Bioreactor Treatment For Trace Organic Contaminant Removal: Breakthrough Behaviour Of Persistent And Hydrophilic Compounds, Luong N. Nguyen, Faisal I. Hai, William E. Price, Jinguo Kang, Long D. Nghiem
Coupling Granular Activated Carbon Adsorption With Membrane Bioreactor Treatment For Trace Organic Contaminant Removal: Breakthrough Behaviour Of Persistent And Hydrophilic Compounds, Luong N. Nguyen, Faisal I. Hai, William E. Price, Jinguo Kang, Long D. Nghiem
Faisal I Hai
This study investigated the removal of trace organic contaminants by a combined membrane bioreactor - granular activated carbon (MBR-GAC) system over a period of 196 days. Of the 22 compounds investigated here, all six hydrophilic compounds with electron-withdrawing functional groups (i.e., metronidazole, carbamazepine, ketoprofen, naproxen, fenoprop and diclofenac) exhibited very low removal efficiency by MBR-only treatment. GAC post-treatment initially complemented MBR treatment very well; however, a compound-specific gradual deterioration of the removal of the above-mentioned problematic compounds was noted. While a 20% breakthrough of all four negatively charged compounds namely ketoprofen, naproxen, fenoprop and diclofenac occurred within 1000-3000 bed volumes …
Application Of Membrane Technology For The Development Of Sustainable Biotechnology Processes, Faisal Hai, Oskar Modin
Application Of Membrane Technology For The Development Of Sustainable Biotechnology Processes, Faisal Hai, Oskar Modin
Faisal I Hai
The scope of application of membranes in biotechnology has widened significantly in the recent years. Although many of the membrane options are yet to achieve wide industrial applications, they show tremendous potential for the transformation and synthesis of valueadded products, energy production, therapeutic applications and environmental remediation. This chapter provides an overview of membrane applications in selected established and emerging biotechnology processes. Approaches to overcoming the technology bottlenecks that impede the scale-up of such systems have been discussed in this chapter.
Coupling Powdered Activated Carbon (Pac) Adsorption With Membrane Bioreactor (Mbr) Treatment For Enhanced Removal Of Trace Organics, Luong Nguyen, Faisal Ibney Hai, Long Nghiem, Jinguo Kang, William Price
Coupling Powdered Activated Carbon (Pac) Adsorption With Membrane Bioreactor (Mbr) Treatment For Enhanced Removal Of Trace Organics, Luong Nguyen, Faisal Ibney Hai, Long Nghiem, Jinguo Kang, William Price
Faisal I Hai
the occurrence of trace organics such as pesticides, pharmaceutically active compounds, natural and synthetic hormones as well as varous industrial compounds in the aquatic environment is of great concern due to their potential adverse effects on human health and those of other biota. Therefore, the removal of these compounds from wastewater is an important consideration to ensure safe drinking water and better protection of the environment. In the literature, several techniques have been explored for trace organics removal, namely, conventional activated sludge, membrane bioreactors (MBRs), and absorptioin. However it has been found that neither MBR nor activated carbon on its …
Rejection And Fate Of Trace Organic Compounds (Trocs) During Membrane Distillation, Kaushalya Wijekoon, Faisal Ibney Hai, Jinguo Kang, William E. Price, Tzahi Cath, Long D. Nghiem
Rejection And Fate Of Trace Organic Compounds (Trocs) During Membrane Distillation, Kaushalya Wijekoon, Faisal Ibney Hai, Jinguo Kang, William E. Price, Tzahi Cath, Long D. Nghiem
Faisal I Hai
In this study, we examined the feasibility of membrane distillation (MD) for removing trace organic compounds (TrOCs) during water and wastewater treatment. A set of 29 compounds was selected to represent major TrOC groups, including pharmaceuticals, steroid hormones, phytoestrogens, UV-filters, industrial chemicals, and pesticides that occur ubiquitously in municipal wastewater. Results reported here suggest that rejection and fate and transport of TrOC during MD are governed by their volatility and, to a lesser extent, hydrophobicity. All TrOCs with pKH > 9 (which can be classified as non-volatile) were well removed by MD. Among the 29 TrOCs investigated in this study, three …
High Retention Membrane Bioreactors: Challenges And Opportunities, Wenhai Luo, Faisal Ibney Hai, William Price, Wenshan Guo, Hao H. Ngo, Kazuo Yamamoto, Long Nghiem
High Retention Membrane Bioreactors: Challenges And Opportunities, Wenhai Luo, Faisal Ibney Hai, William Price, Wenshan Guo, Hao H. Ngo, Kazuo Yamamoto, Long Nghiem
Faisal I Hai
Extensive research has focussed on the development of novel high retention membrane bioreactor (HR-MBR) systems for wastewater reclamation in recent years. HR-MBR integrates high rejection membrane separation with conventional biological treatment in a single step. High rejection membrane separation processes currently used in HR-MBR applications include nanofiltration, forward osmosis, and membrane distillation. In these HR-MBR systems, organic contaminants can be effectively retained, prolonging their retention time in the bioreactor and thus enhancing their biodegradation. Therefore, HR-MBR can offer a reliable and elegant solution to produce high quality effluent. However, there are several technological challenges associated with the development of HR-MBR, …
A Novel Membrane Distillation-Thermophilic Bioreactor System: Biological Stability And Trace Organic Compound Removal, Kaushalya Wijekoon, Faisal Hai, Jinguo Kang, William Price, Wenshan Guo, Hao Ngo, Tzahi Cath, Long Nghiem
A Novel Membrane Distillation-Thermophilic Bioreactor System: Biological Stability And Trace Organic Compound Removal, Kaushalya Wijekoon, Faisal Hai, Jinguo Kang, William Price, Wenshan Guo, Hao Ngo, Tzahi Cath, Long Nghiem
Faisal I Hai
The removal of trace organic compounds (TrOCs) by a novel membrane distillation-thermophilic bioreactor (MDBR) system was examined. Salinity build-up and the thermophilic conditions to some extent adversely impacted the performance of the bioreactor, particularly the removal of total nitrogen and recalcitrant TrOCs. While most TrOCs were well removed by the thermophilic bioreactor, compounds containing electron withdrawing functional groups in their molecular structure were recalcitrant to biological treatment and their removal efficiency by the thermophilic bioreactor was low (0-53%). However, the overall performance of the novel MDBR system with respect to the removal of total organic carbon, total nitrogen, and TrOCs …
Biocatalytic Membrane Reactors For The Removal Of Recalcitrant And Emerging Pollutants From Wastewater, F Hai, L Nghiem, O Modin
Biocatalytic Membrane Reactors For The Removal Of Recalcitrant And Emerging Pollutants From Wastewater, F Hai, L Nghiem, O Modin
Faisal I Hai
The potential fields of application of biocatalytic membrane reactors have widened considerably in recent years. Although biocatalytic membrane reactors, in general, are yet to achieve broad industrial application, in the not too far future they are expected to play a major role, not only for the production, transformation and valorization of raw materials but also for environmental remediations. This chapter comprehensively reviews the laboratory scale studies which demonstrate the potential of biocatalytic membrane reactors in wastewater treatment applications. Studies reponed in the literature, however, serve as proof of concept only. Issues that need to be addressed in order to achieve …
Removal Of Bisphenol A And Diclofenac By A Novel Fungal Membrane Bioreactor Operated Under Non-Sterile Conditions, Shufan Yang, Faisal I. Hai, Long D. Nghiem, Luong N. Nguyen, Felicity Roddick, William E. Price
Removal Of Bisphenol A And Diclofenac By A Novel Fungal Membrane Bioreactor Operated Under Non-Sterile Conditions, Shufan Yang, Faisal I. Hai, Long D. Nghiem, Luong N. Nguyen, Felicity Roddick, William E. Price
Faisal I Hai
Previous studies have confirmed significant removal of various trace organic contaminants (TrOCs) by white-rot fungal cultures under sterile batch test conditions. However, little is known about TrOC removal in continuous flow fungal reactors in a non-sterile environment. This study reports the removal of two TrOCs, namely, bisphenol A and diclofenac, by a fungal membrane bioreactor (MBR).
Degradation Of Azo Dye Acid Orange 7 In A Membrane Bioreactor By Pellets And Attached Growth Of Coriolus Versicolour, Faisal I. Hai, Kazuo Yamamoto, Fumiyuki Nakajima, Kensuke Fukushi, Long D. Nghiem, William E. Price, Bo Jin
Degradation Of Azo Dye Acid Orange 7 In A Membrane Bioreactor By Pellets And Attached Growth Of Coriolus Versicolour, Faisal I. Hai, Kazuo Yamamoto, Fumiyuki Nakajima, Kensuke Fukushi, Long D. Nghiem, William E. Price, Bo Jin
Faisal I Hai
The aim of this study was to systematically compare the degradation of azo dye acid orange 7 by spongy pellets and attached biofilm of Coriolus versicolour (NBRC 9791) in a membrane bioreactor (MBR) under non-sterile conditions. Mild stirring (35 rpm) resulted in spherical (φ = 0.5 cm), spongy pellets and concomitantly triggered high enzymatic activity of the fungus, allowing for excellent decolouration (>99%) of a synthetic wastewater containing the dye. However, bacterial contamination eventually damaged the fungus pellets, leading to decreased decolouration efficiency. Promotion of attached growth on a plastic support along with formation of spherical spongy pellets allowed …