Physics Commons^™

Particle Moment Canting In Cofe2o4 Nanoparticles, K. Hasz, Yumi Ijiri, Kathryn L. Krycka, Julie A. Borchers, R.A. Booth, S. Oberdick, S.A. Majetich

Faculty & Staff Scholarship

Polarization-analyzed small-angle neutron scattering methods are used to determine the spin morphology in high crystalline anisotropy, 11 nm diameter CoFe2O4 nanoparticle assemblies with randomly oriented easy axes. In moderate to high magnetic fields, the nanoparticles adopt a uniformly canted structure, rather than forming domains, shells, or other arrangements. The observed canting angles agree quantitatively with those predicted from an energy model dominated by Zeeman and anisotropy competition, with implications for the technological use of such nanoparticles.

Lattice-Tuned Magnetism Of Ru4+(4D4) Ions In Single Crystals Of The Layered Honeycomb Ruthenates Li2Ruo3 And Na2Ruo3, J. C. Wang, Jsaminka Terzic, T. F. Qi, Feng Ye, Shujuan Yuan, Saicharan Aswartham, S. V. Streltsov, D. I. Khomskii, Ribku K. Kaul, Gang Cao

Physics and Astronomy Faculty Publications

We synthesize and study single crystals of the layered honeycomb lattice Mott insulators Na₂RuO₃ and Li₂RuO₃ with magnetic Ru⁴⁺(4d⁴) ions. The newly found Na₂RuO₃ features a nearly ideal honeycomb lattice and orders antiferromagnetically at 30 K. Single crystals of Li₂RuO₃ adopt a honeycomb lattice with either C2/m or more distorted P2₁/m below 300 K, depending on detailed synthesis conditions. We find that Li₂RuO₃ in both structures hosts a well-defined magnetic state, in contrast to …

Boron Nitride Nanotubes For Spintronics, Kamal B. Dhungana, Ranjit Pati

Department of Physics Publications

With the end of Moore's law in sight, researchers are in search of an alternative approach to manipulate information. Spintronics or spin-based electronics, which uses the spin state of electrons to store, process and communicate information, offers exciting opportunities to sustain the current growth in the information industry. For example, the discovery of the giant magneto resistance (GMR) effect, which provides the foundation behind modern high density data storage devices, is an important success story of spintronics; GMR-based sensors have wide applications, ranging from automotive industry to biology. In recent years, with the tremendous progress in nanotechnology, spintronics has crossed …

Evidence For Magnetic Clusters In Ni₁₋ₓvₓ Close To The Quantum Critical Concentration, R. Wang, S. Ubaid-Kassis, A. Schroeder, P. J. Baker, F. L. Pratt, S. J. Blundell, T. Lancaster, I. Franke, J. S. Möller, Thomas Vojta

Physics Faculty Research & Creative Works

The d-metal alloy Ni_1-xV_x undergoes a quantum phase transition from a ferromagnetic ground state to a paramagnetic ground state as the vanadium concentration x is increased. We present magnetization, ac-susceptibility and muon-spin relaxation data at several vanadium concentrations near the critical concentration x_c ~ 11.6 % at which the onset of ferromagnetic order is suppressed to zero temperature. Below x_c, the muon data reveal a broad magnetic field distribution indicative of a long-range ordered ferromagnetic state with spatial disorder. We show evidence of magnetic clusters in the ferromagnetic phase and close to the phase …

Analysis Of Critical Behavior In Magnetic Materials, Dustin David Belyea

USF Tampa Graduate Theses and Dissertations

This work contains a broad study of a variety of magnetic materials undergoing second order phase transitions. In general this leads to an overall increase in information and analytical methods to further the field of magnetocalorics. Specifically, critical aspects of magnetocaloric materials were compared within systems in relation to structure, stoichiometry, magnetic minority phases and magnetic contaminants. Detailed analyses were developed to quantify techniques which were in the past used mainly in a qualitative way, leading to a more complete understanding of how critical phenomena impacts the magnetocaloric response.

Neutron Scattering Studies Of Cuprates And Iron Pnictides, Mengshu Liu

Doctoral Dissertations

Presented within are neutron scattering studies of several different high temperature superconducting materials: BaFe_1.9Ni_0.1As₂ [Barium Iron Nickel Arsenic], BaFe_1.85Ni_0.15As₂ [Barium Iron Nickel Arsenic], Ba_0.67K_0.33Fe₂As₂ [Barium Potassium Iron Arsenic], and Pr_0.88LaCe_0.12CuO_4-y [Praseodymium Lanthanum Cerium Copper Oxide]. The main focus is on the magnetic excitations within the systems.

For BaFe_1.9Ni_0.1As₂ [Barium Iron Nickel Arsenic], we measured the intensity of its magnetic excitations and compared the results with excitations in antiferromagnetic non-superconducting BaFe₂As_{2 …}

Novel Magnetism Of Ir5+(5D4) Ions In The Double Perovskite Sr2Yiro6, Gang Cao, Tongfei Qi, Li Li, Jsaminka Terzic, Shujuan Yuan, Lance E. De Long, Ganpathy Murthy, Ribhu K. Kaul

Physics and Astronomy Faculty Publications

We synthesize and study single crystals of a new double-perovskite Sr₂YIrO₆. Despite two strongly unfavorable conditions for magnetic order, namely, pentavalent Ir⁵⁺(5d⁴) ions which are anticipated to have J_eff=0 singlet ground states in the strong spin-orbit coupling (SOC) limit and geometric frustration in a face-centered cubic structure formed by the Ir⁵⁺ ions, we observe this iridate to undergo a novel magnetic transition at temperatures below 1.3 K. We provide compelling experimental and theoretical evidence that the origin of magnetism is in an unusual interplay between strong noncubic crystal …

Metal Oxide Growth, Spin Precession Measurements And Raman Spectroscopy Of Cvd Graphene, Akitomo Matsubayashi

Legacy Theses & Dissertations (2009 - 2024)

The focus of this dissertation is to explore the possibility of wafer scale graphene-based spintronics. Graphene is a single atomic layer of sp2 bonded carbon atoms that has attracted much attention as a new type of electronic material due to its high carrier mobilities, superior mechanical properties and extremely high thermal conductivity. In addition, it has become an attractive material for use in spintronic devices owing to its long electron spin relaxation time at room temperature. This arises in part from its low spin-orbit coupling and negligible nuclear hyperfine interaction. In order to realize wafer scale graphene spintronics, utilization of …