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Full-Text Articles in Physics
Real-Time Observation Of Molecular Spinning With Angular High-Harmonic Spectroscopy, Lixin He, Pengfei Lan, Anh-Thu Le, Baoning Wang, Bincheng Wang, Xiaosong Zhu, Peixiang Lu, C. D. Lin
Real-Time Observation Of Molecular Spinning With Angular High-Harmonic Spectroscopy, Lixin He, Pengfei Lan, Anh-Thu Le, Baoning Wang, Bincheng Wang, Xiaosong Zhu, Peixiang Lu, C. D. Lin
Physics Faculty Research & Creative Works
We demonstrate an angular high-harmonic spectroscopy method to probe the spinning dynamics of a molecular rotation wave packet in real time. With the excitation of two time-delayed, polarization-skewed pump pulses, the molecular ensemble is impulsively kicked to rotate unidirectionally, which is subsequently irradiated by another delayed probe pulse for high-order harmonic generation (HHG). The spatiotemporal evolution of the molecular rotation wave packet is visualized from the time-dependent angular distributions of the HHG yields and frequency shift measured at various polarization directions and time delays of the probe pulse. The observed frequency shift in HHG is demonstrated to arise from the …
Young-Type Interference In (E, 2e) Ionization Of H₂, D. S. Milne-Brownlie, Matthew S. Foster, Junfang Gao, B. Lohmann, Don H. Madison
Young-Type Interference In (E, 2e) Ionization Of H₂, D. S. Milne-Brownlie, Matthew S. Foster, Junfang Gao, B. Lohmann, Don H. Madison
Physics Faculty Research & Creative Works
We have investigated the electron impact single ionization of the hydrogen molecule, with fully determined kinematics. The experimental and theoretical results are compared with He ionization under the same conditions. The results indicate that the ejected electron angular distribution for H2 is modified due to Young-type interference between ionization amplitudes for scattering from the two centers in the hydrogen molecule. The observable result is a suppression of the backward scattering (recoil) peak compared with the binary peak.
Temperature Dependence Of Droplet Nucleation In A Yukawa Fluid, Jinsong Li, Gerald Wilemski
Temperature Dependence Of Droplet Nucleation In A Yukawa Fluid, Jinsong Li, Gerald Wilemski
Physics Faculty Research & Creative Works
We have studied the temperature dependence of gas-to-liquid nucleation in Yukawa fluids with gradient theory and density functional theory. Each of these nonclassical theories exhibits a weaker (i.e., better) temperature dependence than classical nucleation theory. At fixed temperature, the reversible work to form a critical nucleus found from gradient theory approaches the value given by density functional theory as the supersaturation increases. At high temperatures, the two theories remain quite close over a wide range of vapor densities. As the temperature is reduced, the difference between the two theories increases with decreasing vapor density. Compared to the classical theory we …
Local Versus Nonlocal Order-Parameter Field Theories For Quantum Phase Transitions, Dietrich Belitz, Theodore R. Kirkpatrick, Thomas Vojta
Local Versus Nonlocal Order-Parameter Field Theories For Quantum Phase Transitions, Dietrich Belitz, Theodore R. Kirkpatrick, Thomas Vojta
Physics Faculty Research & Creative Works
General conditions are formulated that allow us to determine which quantum phase transitions in itinerant electron systems can be described by a local Landau-Ginzburg-Wilson (LGW) theory solely in terms of the order parameter. A crucial question is the degree to which the order parameter fluctuations couple to other soft modes. Three general classes of zero-wave-number order parameters, in the particle-hole spin-singlet and spin-triplet channels and in the particle-particle channel, respectively, are considered. It is shown that the particle-hole spin-singlet class does allow for a local LGW theory, while the other two classes do not. The implications of this result for …
Short-Pulse Laser-Induced Stabilization Of Autoionizing States, Heider N. Ereifej, J. Greg Story
Short-Pulse Laser-Induced Stabilization Of Autoionizing States, Heider N. Ereifej, J. Greg Story
Physics Faculty Research & Creative Works
Atoms in doubly excited states above the first ionization limit can decay via autoionization in which an electron is emitted leaving an ion, or by photoemission which leaves the atom in a singly excited state. In this paper, it is demonstrated that interaction between the atoms and a laser pulse that is short compared to the autoionization lifetime can lead to large enhancement of the photoemission process by stimulating the atoms to emit a photon. Since the resultant singly excited atoms do not autoionize, this process can be viewed as an enhancement of the stabilization of the doubly excited atoms …