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University Of Nevada, Las Vegas Advanced Accelerator Applications University Participation Program: Quarterly Report, Third Quarter (September To November 2001), Anthony Hechanova

Transmutation Research Program Reports (TRP)

This Quarterly Report is a primary deliverable from the University of Nevada, Las Vegas (UNLV) Advanced Accelerator Applications (AAA) University Participation Program (UPP) Director to the U.S. Department of Energy (DOE) as described in the UNLV AAA proposal and Statement of Work for the Third Quarter.

The UNLV AAA UPP Director implements the program’s administration using staff from the Harry Reid Center for Environmental Studies (HRC) to ensure that work conducted under the UNLV AAA UPP meets program objectives. The UNLV AAA UPP consists of three components: Program Support, Research Infrastructure Augmentation, and Student Research.

Nuclear Criticality Analyses Of Separations Processes For The Transmutation Fuel Cycle: Quaterly Report, William Culbreth, Pang Tao

Separations Campaign (TRP)

During the first quarter of the work, the tasks included training students in the use of Monte Carlo codes used in radiation transport studies and the assessment of neutron multiplication factors for specific problems outlined by ANL-East through Drs. Laidler and Vandegrift.

The proposal also included objectives for the first year of work on this project, as listed below. The work conducted in the first quarter of the project was in partial completion of these objectives.

• Train UNLV students in the use of SCALE and/or MCNP for the assessment of nuclear criticality.

• Assess neutron multiplication factor, k_{eff …}

Radiation Transport Modeling Of Beam-Target Experiments For The Aaa Project: Quaterly Report, William Culbreth

Reactor Campaign (TRP)

The national development of technology to transmute nuclear waste depends upon the generation of high energy neutrons produced by proton spallation. Proton accelerators, such as LANSCE at the Los Alamos National Laboratory, are capable of producing 800 MeV protons. By bombarding a lead/bismuth target, each proton may generate 500 or more neutrons that can activate fission products or induce the fission of transuranic isotopes.

The Monte Carlo radiation transport code MCNPX developed at LANL is an important tool in the design of transmuter technology. It must be validated, however, for the neutron energy that will be employed. Experiments are being …

Design And Evaluation Of Processes For Fuel Fabrication: Quarterly Progress Report #1, Georg F. Mauer

Fuels Campaign (TRP)

The first three months of the project covered the following:

• Literature review: A comprehensive study of the pertinent publications pertaining to transmuter fuels composition and manufacturing processes was conducted.

• Visit at ANL West in Idaho Falls, ID: Dr. Mauer visited the ANL West facility and met with his National Laboratory Collaborator, Dr. Mitchell K. Meyer, Group Leader, Fabrication Development on October 14 and 15, 2001.

• Student Paper Presentation at the ANS Annual Meeting by Ph.D. student Mr. Jae-Kyu Lee. Title: Transmuter Fuel Fabrication Processes.

Analysis Of Corrosion Of Steel By Lead Bismuth Eutectic, John Farley, Dale L. Perry

Transmutation Sciences Materials (TRP)

We examined stainless samples that were exposed to LBE in experiments conducted by the Russians, under contract to Los Alamos. We examined both corroded and uncorroded samples using the Scanning Electron Microscope (SEM), the Energy Dispersive X-Ray (EDAX) Spectroscopy, and the X-ray Photoelectron Spectrometer (XPS). We found that the surface of the corroded sample is covered by oxygen-containing compounds, presumably mostly iron oxide. In samples exposed for shorter times or lower temperatures, we found that some areas were covered by an oxide layer, and some areas was uncovered. We found that the level of Cr in the uncovered area is …

Design And Analysis For Melt Casting Metallic Fuel Pins Incorporating Volatile Actinides: Quarterly Progress Report 8/16/01- 11/15/01, Yitung Chen, Randy Clarksean, Darrell Pepper

Fuels Campaign (TRP)

An important aspect of the Advanced Accelerator Applications (AAA) program is the development of a casting process by which volatile actinide element (i.e., americium) can be incorporated into metallic alloy fuel pins. The traditional metal fuel casting process uses an inductively heated crucible. The process involves evacuation of the furnace. The evacuation of the furnace also evacuates quartz rods used as fuel pin molds. Once evacuated the open ends of the molds are lowered into the melt; the casting furnace is then rapidly pressurized, forcing the molten metal up into the evacuated molds where solidification occurs.

This process works well …

Assessment Of Criticality Safety For Cylindrical Containers To Be Used In The Processing Of Spent Fuel, William Culbreth, Daniel R. Lowe, Jason Viggato

Separations Campaign (TRP)

The UREX process separates uranium from transuranic wastes (TRU) and fission products (FP). Nuclear reactors require fissile isotopes that will absorb neutrons and break apart into smaller nuclei while releasing a large amount of energy as well as multiple neutrons. Fissile isotopes in spent fuel include not only ²³⁵U, but also ²³⁹Pu, ²⁴¹Pu, and several isotopes of americium (Am) and curium (Cm).

TRU contains the actinides with atomic numbers greater than that of uranium. This includes Pu, Np, Am, and Cm. When TRU is separated from uranium, the TRU still poses a significant risk of sustaining a …

University Of Nevada, Las Vegas Advanced Accelerator Applications University Participation Program: Quarterly Report, Second Quarter (June To August 2001), Anthony Hechanova

Transmutation Research Program Reports (TRP)

This Quarterly Report is a primary deliverable from the University of Nevada, Las Vegas (UNLV) Advanced Accelerator Applications (AAA) University Participation Program (UPP) Director to the U.S. Department of Energy (DOE) as described in the UNLV AAA proposal.

The UNLV AAA UPP Director implements the program’s administration using staff from the Harry Reid Center for Environmental Studies (HRC) to ensure that work conducted under the UNLV AAA UPP meets program objectives. The UNLV AAA UPP consists of three components: Program Administration, Research Infrastructure Augmentation, and Student Research.

Design And Analysis For Melt Casting Metallic Fuel Pins Incorporating Volatile Actinides: Quarterly Report 5/15/01-8/15/01, Yitung Chen, Darrell Pepper, Randy Clarksean

Fuels Campaign (TRP)

No abstract provided.

Analysis Of Corrosion Of Steel By Lead Bismuth Eutectic, John Farley, Dale L. Perry

Transmutation Sciences Materials (TRP)

The goal is to achieve a basic understanding of the corrosion of stainless steel by Lead Bismuth Eutectic (LBE), which has been proposed for use in the transmuter as both a coolant and as a sputtering target.

Nuclear Criticality Analyses Of Separations Processes For The Transmutation Fuel Cycle, William Culbreth, Pang Tao

Separations Campaign (TRP)

To mitigate the waste created by conventional fission reactors, spent nuclear fuel must be mechanically separated from its cladding. For the development of fuel processing technology to support the Advanced Accelerator Applications (AAA) Program, aqueous and pyrochemical processes will be used to further separate technetium and iodine, uranium and the higher actinides (see Figure 1 for an example of the process layout)1. The higher actinides, including plutonium, americium, curium, and neptunium will be separated from the waste to facilitate their fabrication into new fuel for placement in a transmuter. High-energy neutrons generated by spallation in the transmuter break down these …

Radiation Transport Modeling Of Beam-Target Experiments For The Aaa Project, William Culbreth

Reactor Campaign (TRP)

The AAA program will rely on the use of an accelerator-based transmuter to expose spent nuclear fuel to high-energy neutrons. The neutron flux will be sufficient to activate or fission the long-lived isotopes of Tc, I, Pu, Am, Cm, and Np that present a significant safety hazard in commercial spent fuel. Transmuter fuel will be subcritical and a high-energy proton accelerator is needed to maintain the necessary neutron flux through the use of a neutron spallation target. The maximum neutron energy produced by spallation (~ 600 MeV) is significantly higher than that produced by a commercial light water reactor (~ …

Design And Evaluation Of Processes For Fuel Fabrication, Georg F. Mauer

Fuels Campaign (TRP)

The objective of this project is the design and evaluation of manufacturing processes for transmuter fuel fabrication. A detailed design description for the manufacturing of each candidate fuel type would support the informed selection of fuel for a transmutation system. We will collect pertinent manufacturing and process-related information and create an information database that will document the design, operations, and cost implications of various fuel choices. Fabrication processes for different fuel types will likely differ in terms of equipment types, throughput, and cost.

Year 1 of the project will be devoted to the analysis and assessment of the multiple steps …

University Of Nevada, Las Vegas Advanced Accelerator Applications University Participation Program: Quarterly Report First Quarter (March-May 2001), Anthony Hechanova

Transmutation Research Program Reports (TRP)

This Quarterly Report is a primary deliverable from the University of Nevada, Las Vegas (UNLV) Advanced Accelerator Applications (AAA) University Participation Program (UPP) director to the U.S. Department of Energy Office of Nuclear Energy, Science and Technology (DOE-NE) as defined in the UNLV AAA Proposal.

The foundation of the UNLV AAA University Participation Program started as a grassroots effort in the late 1990s among community members and local, state, and federal representatives to encourage research and development of technical alternatives to direct disposal of used nuclear fuel which had been targeted since the early 1980s for Yucca Mountain, Nevada. A …

Design And Analysis For Melt Casting Metallic Fuel Pins Incorporating Volatile Actinides, Yitung Chen, Darrell Pepper, Randy Clarksean

Fuels Campaign (TRP)

UNLV investigators will evaluate and select a process for the melt casting of metallic fuel pins that contain volatile actinides. This work will be performed with the guidance of Argonne National Laboratory (ANL) engineers to insure that their knowledge and experience benefits the project. The research to be conducted during year one will center on selecting, evaluating, and modeling potential alternatives to the traditional injection casting process used at ANL. Processing conditions will be analyzed, basic models utilized, and detailed heat and mass transfer models will be developed to analyze the most promising processes. The goal of the first year …

Experimental Investigation Of Steel Corrosion In Lead Bismuth Eutectic (Lbe): Characterization, Species Identification, And Chemical Reactions, John Farley, Dale L. Perry

Transmutation Sciences Materials (TRP)

The goal of the present research is to achieve a basic understanding of corrosion of steels by Lead Bismuth Eutectic (LBE). Liquid LBE is under consideration in the transmuter as both a coolant and a target material. There have been studies of LBE, especially by the Russians, but a fundamental understanding and verification of its role in the corrosion of steels is still very 2 incomplete. Post-experiment testing and analysis will be performed on steel samples that have been in intimate contact with LBE. Chemical alterations and resulting chemical species will be measured at the steel surface. Techniques to be …