Physics Commons^™

Collisional Redistribution Of Polarized Radiation For Sr-Ar(He) Systems: A Numerical Comparison Of The Semiclassical Decoupiing/Locking Model To Exact Results, Ronald James Bieniek, Paul S. Julienne, Rank Rebentrost

Physics Faculty Research & Creative Works

Abstract Semiclassical formulations of collisional redistribution of polarized radiation are presented at several levels of approximation, from full classical path coupled equations to the backing/decoupling model. These are numerically tested against the results of a quantum mechanical coupled-channels formalism, by the comparison of polarization curves in both spectral wings of the Srf1 So-1 Pi) transition, with Ar and He as collisional perturbers. It is found that the locking/decoupling model can often produce good agreement with exact results if the effects due to trajectories and multiple Condon points are treated properly. Significant discrepancies due to the Condon approximation used ty the …

Change Of Magnetic Properties Of Th₂Fe₁₇ Due To Interstitial Solution Of C And N, T. H. Jacobs, Gary J. Long, Oran Allan Pringle, Fernande Grandjean, K. H. Buschow

Chemistry Faculty Research & Creative Works

The changes in magnetic and crystallographic properties in the series Th₂Fe₁₇C_x and Th₂Fe ₁₇N_x have been studied. The changes in the latter series were also studied by ⁵⁷Fe Mössbauer spectroscopy. The ultimate enhancements of the saturation moments in these series are 13% and 24%, respectively. This is much larger than observed previously in the corresponding rare-earth compounds, although the Curie temperature enhancements are of comparable magnitude. In the Th-Fe-C system a novel compound of the BaCd ₁₁ type was found, having a Curie temperature around 370 K.

Binary Peak Enhancement And Structure In Partially Stripped Ion-Atom Collisions, D. R. Schultz, Ronald E. Olson

Physics Faculty Research & Creative Works

Recent experiments have found both an unexpected enhancement and structure of the binary peak in the spectrum of electrons ejected in partially stripped ion-atom collisions. Utilizing the theoretical approach which has been used to elucidate the origin of this behavior, a survey of their manifestation is presented over a broad range of nuclear and ionic charges (C, F, Fe, I and U ions) and impact energies (0.1 to 100 MeV u-1). For forward binary electron emission it is shown that the greatest enhancement occurs for the lowest projectile ion charge states (highly screened nuclei). The magnitude of the enhancement maximizes …

X-Ray Emission From Slow Highly Charged Ar Ions Interacting With A Ge Surface, Michael Schulz, C. Lewis Cocke, Siegbert Hagmann, Martin P. Stockli, Horst Schmidt-Bocking

Physics Faculty Research & Creative Works

We have measured K x-ray spectra and yields from Ar¹⁷⁺ ions slowly approaching a single-crystal Ge surface. The yields were measured as a function of the projectile velocity component perpendicular to the surface. From the data a characteristic time of approximately 1 psec was extracted for the in-flight filling above the surface of the Ar K vacancy.

Dielectronic Recombination On And Electron-Impact Excitation Of Heliumlike Argon, Rami M. Ali, Chander P. Bhalla, C. Lewis Cocke, Michael Schulz, Martin P. Stockli

Physics Faculty Research & Creative Works

We have measured cross sections for Δn=1 dielectronic recombination (DR) on He-like argon and found good agreement with theoretical calculations based on the Hartree-Fock atomic model. Experimental absolute cross sections were obtained by using the electron-energy dependence of yields of He-like and Li-like argon ions from the Kansas State University electron-beam ion source to measure the ratio of the DR cross section on He-like argon to the electron-impact-ionization cross section of Li-like argon and normalizing to the latter. The K x-ray emission spectra due to Δn=1,2 DR and n=1→2 electron-impact excitation of He-like argon were also observed with a Si(Li) …

Abnormal Behaviour Of Zero Degree Δ-Electron Emission On The Projectile Ionic Charge, O. Jagutzkit, S. Hagtnanni, H. Schmidt-Bockingt, Ronald E. Olson, D. R. Schultz, R. Dornert, R. Kocht, A. Skutlartz, A. González, T. B. Quinterosi, C. Kelbcht, P. Richardt

Physics Faculty Research & Creative Works

The 0° δ-electron emission was investigated by an electron-projectile coincidence technique as a function of incoming and outgoing projectile charge state for 0.53 MeV u^-1Cu^q+ on He. The electron emission spectra vary strongly with initial and final projectile charge state. For pure ionization channels the cross sections follow for low electron energy the q²-scaling law whereas in the binary encounter regime the scaling is reversed. Ctmc calculations are in fair agreement with the experimental data. © 1991 IOP Publishing Ltd.

Population Of Highly Excited Intermediate Resonance States By Electron Transfer And Excitation, Reinhold S. Schuch, Edson L B Justiniano, Michael Schulz, Sheldon Datz, Peter F. Dittner, J. P. Giese, Herbert F. Krause, Harald Schone, Charles Randy Vane, Stephen M. Shafroth

Physics Faculty Research & Creative Works

Coincidences between two sulfur K x rays were detected from collisions of hydrogenlike S ions with H₂ gas in the projectile energy range between 150 and 225 MeV. These K x rays are emitted in the decay of doubly excited states formed in the collisions via transfer and excitation. The excitation function for two coincident Kβ transitions peaks at about 175 MeV, slightly above the expected KMM resonance energy for resonant transfer and excitation (RTE). This demonstrates the occurrence of ΔN≥2 transitions (i.e., KMM and higher resonances) in the RTE process. The cross sections for the population of the …

Extrapolation Of The Experimental Data Of Electron Scattering, Hansen Chen

Opportunities for Undergraduate Research Experience Program (OURE)

Our problem of interest is electron-atom scattering. One type of experiment is to measure the number of electrons exciting an atom from a initial s-state to a final p-state. These measurements are proportional to the differential cross section (DCS)….

The plane wave Bom approximation is known not to be accurate enough. However Lassetre claims that even if PWBA (plane wave Bom approximation) is not reliable, a more accurate theory should still extrapolate to the optical oscillator strength.

The theory we are using is significantly better than the PWBA. According to Lassetre’s theorem, our theory should extrapolate to the optical oscillator …

Nonlinear Dynamics And The Lorenz Water Wheel, Richard Margis

Opportunities for Undergraduate Research Experience Program (OURE)

Undoubtedly one of the most exciting frontiers in physics today is the study of nonlinear systems, more popularly called chaos. Chaos is the key to many time-dependent processes in as varied fields as meteorology (such as weather modeling), mechanics (the three-body problem in gravitational fields), and economics (prediction of trends in the stock market).

Transport Anomalies In The High-Temperature Hopping Conductivity And Thermopower Of Sr-Doped La(Cr,Mn)O,₃, Ryne P. Raffaelle, Harlan U. Anderson, Don M. Sparlin, Paul Ernest Parris

Materials Science and Engineering Faculty Research & Creative Works

A minimum exists in the electrical conductivity of the perovskite-type ceramic LaCr_1-xMn_xO₃ as a function of Mn content near x=0.05. This minimum has been explained in terms of a crossover from multiple trapping to percolation among energetically lower Mn sites. In this paper electrical conductivity and Seebeck measurements are presented on a similar series in which 10 mol % Sr was substituted for La in order to increase the small polaron concentration through the compensation of Sr ions according to the Verway mechanism. The data suggests that there is an apparent suppression of the Verway …

Combustion Aerosol Morphology, Ronald P. Holland

Opportunities for Undergraduate Research Experience Program (OURE)

The following report entitled Carbon Aerosol Morphology is the result of research done through the University of Missouri--Rolla Graduate School program entitled Opportunities for Undergraduate Research Experience (OURE). My appointment was for the Summer - 1990 with the Cloud and Aerosol Sciences Laboratory, Department of Physics, located in Norwood Hall. The goal of this appointment was to study the size and morphology of combustion aerosols whose characteristics are dependent on the history of the particle, e.g. exposure to chemicals, scavenging effects, and other time dependent factors. Computer image processing software is available in the department for this purpose.

Aerosol Particle Bounding In Cascade Impactors, Bisma Husen

Opportunities for Undergraduate Research Experience Program (OURE)

Particle deposition characteristics were observed from the aerosol sampling results of a UNICO cascade impactor. A simple model of particle motion combined with Hiemenz flow of stagnation flow on a flat plate were developed and discussed.

Both results and analysis were compared to recent models on particle bouncing errors or secondary deposition which included vortices formation around the edge of the slot, back spin (Magnus effect), and hydrodynamic conditions of the particles. The analysis was limited to a laminar inviscid and incompressible case. The main obstacle in the observation was the fact that impactor nozzles were unsymmetrical to a considerable …

Fourier Transform Infrared (Ftir) Spectroscopy Analysis Of Combustion Aerosol, Gary Jacquin

Opportunities for Undergraduate Research Experience Program (OURE)

In conjunction with my co-op program at McDonnell-Douglas, my current OURE project is the analysis of combustion aerosols using Fourier Transform Infrared (FTIR) Spectroscopy. Aerosol science is a very important field as it is concerned with atmospheric chemistry, atmospheric physics, climate, public health, and environmental issues.

In the Cloud and Aerosol Sciences Laboratory (CASL) at UMR, combustion aerosols are generated by an in-house designed torch or burner. The fuels, JP4 and JP5, are provided by McDonnell-Douglas. Some other commercial fuels are also used. The primary objective of my OURE project was to generate and collect combustion aerosols for chemical analysis. …

Process For Scanning Photographic Slides Of Laser Light Scattering With A Transmission Densitometer, Don Newburry

Opportunities for Undergraduate Research Experience Program (OURE)

Non-symmetric variations in photographic slides of polarized laser light scattering experimental results are difficult to see. This paper explains a process developed for measuring the light density at points throughout the slide area using a transmission densitometer, so an accurate description of the laser light scattering may be obtained. A slide was tested using the described process and the results are presented. The results turned out well, but there were some errors introduced by the instability of the densitometer and by human error in reading the chart recorder output.

A Measurement Of The Relative Efficiency Of A Channeltron, Steve Scott

Opportunities for Undergraduate Research Experience Program (OURE)

The original goal of this project was to determine the characteristics of a channeltron, a device used to detect electrons. While most channeltrons have entrance cones which are quite small, the channeltron we were to study had a significantly larger one. Due to its large size, the possibility existed that the channeltron would be more efficient at detecting electrons which hit near the center of the channeltron entrance than at detecting the electrons which hit near the edge. The main purpose of the experiment was to determine the relative detection efficiency of the channeltron as a function of the position …

A Mössbauer-Effect Study Of A Series Of R₂Fe₁₄C Hard Magnetic Materials, Gary J. Long, Oran Allan Pringle, Gaya Kanishka Marasinghe, Fernande Grandjean, K. H. Buschow

Chemistry Faculty Research & Creative Works

The ⁵⁷Fe Mössbauer-effect spectra of the series of hard magnetic materials, R₂Fe₁₄C, where R is Nd, Gd, Tb, Dy, Ho, and Lu, have been measured at 295 K. All of these carbides exhibit uniaxial magnetic anisotropy. The spectra resemble those obtained for the related R ₂Fe₁₄B compounds and have been fit with the model used earlier for Nd₂Fe₁₄B. The magnitude of the hyperfine field on each site, as a function of rare earth, parallels the Curie temperature; the maximum hyperfine fields and the maximum Curie temperature are observed …

Intraconfiguration Interactions In Barium 6p1/2Nf Autoionizing States, Xiao Wang, J. Greg Story, William E. Cooke

Physics Faculty Research & Creative Works

Measurements are reported of the energies and linewidths of the J=2, 3, and 4 components of the 6p_1/214f and 6p_1/219f states of barium. These states are anomalously broad, having autoionization lifetimes of approximately 1/2 of a classical Rydberg orbit period, and previously measurements have discerned no differences among the various J components. This work shows that the differences can be observed, and are consistent with calculations. The variations between states would be large if the states were LS coupled, but the large 6p ionic fine-structure forces recoupling into jj configurations. The spherical symmetry of the 6p …

Realization Of A Measurement Of A Weak Value, N. W M Ritchie, J. Greg Story, Randall G. Hulet

Physics Faculty Research & Creative Works

We present the first realization of a measurement of a weak value, a concept recently introduced by Aharonov, Albert, and Vaidman (AAV). Our experiment uses a birefringent crystal to separate the two linear-polarization components of a laser beam by a distance small compared to the laser-beam waist. This weak measurement is followed by a strong measurement which translates the centroid of the beam by a distance far larger than the birefringence-induced separation. In addition, we present data corresponding to orthogonal initial and final states, for which the weak value is not defined. This interference effect may have application in the …

Recent Advances In The Comparison Of Matter— And Antimatter—Atom Collisions, D. R. Schultz, Ronald E. Olson, C. O. Reinhold

Physics Faculty Research & Creative Works

The relatively recent advent of low energy antimatter projectiles has spurred a rapid advance in the comparison of matter- and antimatter-atom collisions. These experimental studies have in turn stimulated a great deal of theoretical effort to explain their results, and together both theory and experiment have shed new light on the dynamics of ion-atom collisions. Here we review these developments with particular emphasis on the processes of ionization and charge transfer. © 1991 IOP Publishing Ltd.

Effects Of Sample Orientation On The Corrosion Of Zinc In Ammonium Sulfate And Sodium Hydroxide Solutions, D. Abayarathna, Edward Boyd Hale, Thomas J. O'Keefe, Y. M. Wang, D. Radovic

Physics Faculty Research & Creative Works

The corrosion and electrochemical properties of three zinc single crystal surfaces with different orientations have been investigated. In near-neutral 1 M (NH₄)₂SO₄, the corrosion rates on all three surfaces were found to be similar. However, the SEM morphologies of the corresponding corroded surfaces were markedly different from each other, but consistent with preferential attack of {1120} surfaces. In alkaline 0.5 N NaOH solution, the three sample orientations showed significantly different reactivities, with the (1120) surface exhibiting the highest reactivity and corrosion rate. Here, passivation ultimately occurred and the difference in the corrosion performance of …

Electrical Conductivity, Seebeck Coefficient And Defect Chemistry Of Ca-Doped Ycro3, G. F. Carini, Harlan U. Anderson, Don M. Sparlin, M. M. Nasrallah

Materials Science and Engineering Faculty Research & Creative Works

The electrical transport behavior and defect structure of Ca-doped YCrO₃ were studied using electrical conductivity and Seebeck coefficient measurements as a function of oxygen activity and temperature. Defect models derived from the electrical conductivity data were found to adequately relate the concentration of charge carriers to the acceptor dopant and oxygen vacancy concentrations. Thermodynamic properties were calculated and found to be consistent with the model. Activation energy and carrier mobility data were also obtained. The analysis of the electrical conductivity, Seebeck and mobility data suggest that the conduction process in Ca-doped YCrO₃ occurs via the small polaron hopping …

Defect Structure, Nonstoichiometry, And Phase Stability Of Ca-Doped Ycro3, G. F. Carini, Harlan U. Anderson, M. M. Nasrallah, Don M. Sparlin

Materials Science and Engineering Faculty Research & Creative Works

The dependence of the defect structure of Ca-doped YCrO₃ on oxygen activity and temperature was investigated by high temperature thermogravimetric measurements. Defect models developed from electrical conductivity data obtained in a previous study were used to interpret the thermogravimetric data. A correlation was found between the electrical conductivity and the thermogravimetric data which suggested that these data were concomitantly dependent on the acceptor dopant and oxygen vacancy dependance of the thermodynamic parameters. Kröger-Vink type diagrams showing the regions of stability with respect to oxygen activity and temperature were constructed. The TGA data show that Ca-doped YCrO₃ is even …

Feq⁺+ H, H2and He Electron Loss And He2++ H(N = 1, 2) Electron Capture Cross Sections: Processes Of Interest In Fusion Plasmas, D. R. Schultz, L. Meng, C. O. Reinhold, Ronald E. Olson

Physics Faculty Research & Creative Works

Cross sections have been calculated utilizing the classical trajectory Monte Carlo method for collisional processes of special interest to plasma fusion research. Specifically, H₁H₂and He total electron loss cross sections for the impact by Fe^q+(1 < q < 26) impurity ions, in the energy range of 50 to 500keV/u, are presented. These results illustrate a clear departure for low charge states (q < 10) from scaling of the cross section with projectile charge (q). Further, cross sections for electron capture from both the ground and n = 2 states of H by 30 to lOOkeV/u He²⁺impact are tabulated as function of final n-level, yielding information for neutral beam heating models. © 1991 IOP Publishing Ltd.

Quantum Interference In Clothed-Ion-Atom Binary Peak Structures, C. O. Reinhold, D. R. Schultz, Ronald E. Olson, C. Kelbch, R. Koch, H. Schmidt-Böcking

Physics Faculty Research & Creative Works

An impulse approximation for ionizing collisions of clothed ions with atoms is used to explain the origin of an anomalous oscillation in the ejected electron spectrum in the region of the binary peak. In addition, measurements which evidence this feature for 1-MeV/u U²¹⁺ ions colliding with helium are presented. It is shown that this behavior arises from interference structures in the elastic differential cross section for the scattering of target electrons from the impinging ion and that it is associated with the well-known phenomenon of rainbow scattering. © 1991 The American Physical Society.