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Multicenter Distorted-Wave Approach For Electron-Impact Ionization Of Molecules, Esam Ali, Don H. Madison
Multicenter Distorted-Wave Approach For Electron-Impact Ionization Of Molecules, Esam Ali, Don H. Madison
Physics Faculty Research & Creative Works
We have previously used the molecular three-body distorted-wave model to examine electron-impact single ionization of molecules. One of the possible weaknesses of this approach lies in the fact that the continuum electron wave functions do not depend on the orientation of the molecule. Here we introduce a model called the multicenter molecular three-body distorted-wave (MCM3DW) approach, for which the continuum electron wave functions depend on the orientation of the molecule at the time of ionization. The MCM3DW results are compared with experimental data taken from work by Dorn and colleagues [Ren, Phys. Rev. A 91, 032707 (2015)10.1103/PhysRevA.91.032707; Phys. Rev. A …
Electron-Impact Ionization Of H₂O At Low Projectile Energy: Internormalized Triple-Differential Cross Sections In Three-Dimensional Kinematics, Xueguang Ren, Sadek Amami, Khokon Hossen, Esam Ali, Chuangang Ning, James Colgan, Don H. Madison, Andrew Dorn
Electron-Impact Ionization Of H₂O At Low Projectile Energy: Internormalized Triple-Differential Cross Sections In Three-Dimensional Kinematics, Xueguang Ren, Sadek Amami, Khokon Hossen, Esam Ali, Chuangang Ning, James Colgan, Don H. Madison, Andrew Dorn
Physics Faculty Research & Creative Works
We report a combined experimental and theoretical study of the electron-impact ionization of water (H2O) at the relatively low incident energy of E0=81eV in which either the 1b1 or 3a1 orbitals are ionized leading to the stable H2O cation. The experimental data were measured by using a reaction microscope, which can cover nearly the entire 4π solid angle for the secondary electron emission over a range of ejection energies. We present experimental data for the scattering angles of 6⁰ and 10⁰ for the faster of the two outgoing electrons as a function …
Kinematically Complete Study Of Low-Energy Electron-Impact Ionization Of Argon: Internormalized Cross Sections In Three-Dimensional Kinematics, Xueguang Ren, Sadek Amami, Oleg Zatsarinny, Thomas Pflüger, Marvin Weyland, Alexander Dorn, Don H. Madison, Klaus Bartschat
Kinematically Complete Study Of Low-Energy Electron-Impact Ionization Of Argon: Internormalized Cross Sections In Three-Dimensional Kinematics, Xueguang Ren, Sadek Amami, Oleg Zatsarinny, Thomas Pflüger, Marvin Weyland, Alexander Dorn, Don H. Madison, Klaus Bartschat
Physics Faculty Research & Creative Works
As a further test of advanced theoretical methods to describe electron-impact single-ionization processes in complex atomic targets, we extended our recent work on Ne(2p) ionization [X. Ren, S. Amami, O. Zatsarinny, T. Pflüger, M. Weyland, W. Y. Baek, H. Rabus, K. Bartschat, D. Madison, and A. Dorn, Phys. Rev. A 91, 032707 (2015)PLRAAN1050-294710.1103/PhysRevA.91.032707] to Ar(3p) ionization at the relatively low incident energy of E0 = 66 eV. The experimental data were obtained with a reaction microscope, which can cover nearly the entire 4π solid angle for the secondary electron emission. We present experimental data for detection angles of 10, …
Experimental And Theoretical Triple-Differential Cross Sections For Tetrahydrofuran Ionized By Low-Energy 26-Ev-Electron Impact, Esam Ali, Xueguang Ren, Alexander Dorn, Chuangang Ning, James Colgan, Don H. Madison
Experimental And Theoretical Triple-Differential Cross Sections For Tetrahydrofuran Ionized By Low-Energy 26-Ev-Electron Impact, Esam Ali, Xueguang Ren, Alexander Dorn, Chuangang Ning, James Colgan, Don H. Madison
Physics Faculty Research & Creative Works
We report an experimental and theoretical study of low-energy electron-impact ionization of tetrahydrofuran, which is a molecule of biological interest. The experiments were performed using an advanced reaction microscope specially built for electron-impact ionization studies. The theoretical calculations were performed within the molecular three-body distorted-wave model. Reasonably good agreement is found between experiment and theory.
Low-Energy (E₀ = 65 Ev) Electron-Impact Ionization Of Neon: Internormalized Triple-Differentical Cross Sections In 3d Kinematics, Xueguang Ren, Sadek M. Amami, Oleg I. Zatsarinny, Thomas Pfluger, Marvin Weyland, Woon Yong Baek, Hans Rabus, Klaus Bartschat, Don H. Madison, Alexander Dorn
Low-Energy (E₀ = 65 Ev) Electron-Impact Ionization Of Neon: Internormalized Triple-Differentical Cross Sections In 3d Kinematics, Xueguang Ren, Sadek M. Amami, Oleg I. Zatsarinny, Thomas Pfluger, Marvin Weyland, Woon Yong Baek, Hans Rabus, Klaus Bartschat, Don H. Madison, Alexander Dorn
Physics Faculty Research & Creative Works
We present a combined experimental and theoretical study on the low-energy (E0 = 65 eV) electron- impact ionization of neon. The experimental data are compared to predictions from a hybrid second-order distorted-wave Born plus R-matrix approach (DWB2-RM), the distorted-wave Born approximation with inclusion of post-collision interaction (DWBA-PCI), a three-body distorted-wave approach (3DW), and a B-spline R-matrix (BSR) with pseudostates approach. Excellent agreement is found between experiment and the 3DW and BSR theories. The importance of PCI effects is clearly visible in this low-energy electron-impact ionization process.
Interference Effects For Intermediate Energy Electron-Impact Ionization Of H₂ And N₂ Molecules, Zehra Nur Ozer, Hari Chaluvadi, Don H. Madison, Mevlut Dogan
Interference Effects For Intermediate Energy Electron-Impact Ionization Of H₂ And N₂ Molecules, Zehra Nur Ozer, Hari Chaluvadi, Don H. Madison, Mevlut Dogan
Physics Faculty Research & Creative Works
We have studied electron impact ionization of H2 and N2 molecules at intermediate energies to look for possible two center interference effects experimentally and theoretically. Here we report a study of the interference factor I for 250 eV electron-impact ionization. The experimental measurements are performed using a crossed-beam-type electron-electron coincidence spectrometer and theoretical calculations are obtained using the Molecular Three Body Distorted Wave Approximation (M3DW). We found that the I-factor demonstrated strong evidence for two-center interference effects for both H2 and N2. We also found that the I-factor is more sensitive to projectile angular scans …
Target Electron Ionization In Li²⁺-L-Li Collisions: A Multi-Electron Perspective, Maciej Dominik Piewanowski, Laszlo Gulyas, Marko W. Horbatsch, Johannes Goullon, Natalia Ferreira, Renate Hubele, Vitor L B D De Jesus, H. Lindenblatt, Katharina R. Schneider, Michael Schulz, Michael Schuricke, Z. Song, Shaofeng Zhang, Daniel Fischer, Tom Kirchner
Target Electron Ionization In Li²⁺-L-Li Collisions: A Multi-Electron Perspective, Maciej Dominik Piewanowski, Laszlo Gulyas, Marko W. Horbatsch, Johannes Goullon, Natalia Ferreira, Renate Hubele, Vitor L B D De Jesus, H. Lindenblatt, Katharina R. Schneider, Michael Schulz, Michael Schuricke, Z. Song, Shaofeng Zhang, Daniel Fischer, Tom Kirchner
Physics Faculty Research & Creative Works
Target electron removal in Li2+-Li collisions at 2290 keV/amu is studied experimentally and theoretically for ground and excited lithium target configurations. It is shown that in outer-shell ionization a single-electron process plays the dominant part. However, the K-shell ionization results are more difficult to interpret. According to our calculations, the process is shown to be strongly single-particle like. On one hand, a high resemblance between theoretical single-particle ionization and exclusive inner-shell ionization is demonstrated, and contributions from multi-electron processes are found to be weak. On the other hand, it is indicated by the discrepancy between experimental and single-particle …
Kinematically Complete Study Of Low-Energy Electron-Impact Ionization Of Neon: Internormalized Cross Sections In Three-Dimensional Kinematics, Xueguang Ren, Sadek Amami, Oleg Zatsarinny, Thomas Pflüger, Marvin Weyland, Woon Yong Baek, Hans Rabus, Klaus Bartschat, Don H. Madison, Alexander Dorn
Kinematically Complete Study Of Low-Energy Electron-Impact Ionization Of Neon: Internormalized Cross Sections In Three-Dimensional Kinematics, Xueguang Ren, Sadek Amami, Oleg Zatsarinny, Thomas Pflüger, Marvin Weyland, Woon Yong Baek, Hans Rabus, Klaus Bartschat, Don H. Madison, Alexander Dorn
Physics Faculty Research & Creative Works
Low-energy (E0 0=65eV) electron-impact single ionization of Ne (2p) has been investigated to thoroughly test state-of-the-art theoretical approaches. The experimental data were measured using a reaction microscope, which can cover nearly the entire 4π solid angle for the secondary electron emission energies ranging from 2 to 8 eV, and projectile scattering angles ranging from 8.5⁰ to 20.0⁰. The experimental triple-differential cross sections are internormalized across all measured scattering angles and ejected energies. The experimental data are compared to predictions from a hybrid second-order distorted-wave Born plus R-matrix approach, the distorted-wave Born approximation with the inclusion of postcollision interaction (PCI), …
X-Ray Emission Produced In Charge-Exchange Collisions Between Highly Charged Ions And Argon: Role Of The Multiple Electron Capture, Sebastian Otranto, N. D. Cariatore, Ronald E. Olson
X-Ray Emission Produced In Charge-Exchange Collisions Between Highly Charged Ions And Argon: Role Of The Multiple Electron Capture, Sebastian Otranto, N. D. Cariatore, Ronald E. Olson
Physics Faculty Research & Creative Works
In this work we use the classical trajectory Monte Carlo method within an eight-electron scheme to theoretically study photonic spectra that follow charge-exchange processes between highly charged ions of charge states 10+, 17+, 18+, and 36+ with neutral argon. The energy range considered is 18 eV/amu to 4 keV/amu, covering typical electron beam ion traps and solar wind energies. The role played by multiple electron capture processes for the different collision systems under consideration is explicitly analyzed and its contribution separated as arising from radiative decay and autoionizing multiple capture. For the present collision systems we find that multiple electron …
Universality Of Returning Electron Wave Packet In High-Order Harmonic Generation With Midinfrared Laser Pulses, Anh-Thu Le, Hui Wei, Cheng Jin, Vu Ngoc Tuoc, Toru Morishita, C. D. Lin
Universality Of Returning Electron Wave Packet In High-Order Harmonic Generation With Midinfrared Laser Pulses, Anh-Thu Le, Hui Wei, Cheng Jin, Vu Ngoc Tuoc, Toru Morishita, C. D. Lin
Physics Faculty Research & Creative Works
We show that a returning electron wave packet in high-order harmonic generation (HHG) with midinfrared laser pulses converges to a universal limit for a laser wavelength above about 3µm. The results are consistent among the different methods: a numerical solution of the time-dependent Schrödinger equation, the strong-field approximation, and the quantum orbits theory. We further analyze how the contribution from different electron "trajectories" survives the macroscopic propagation in the medium. Our result thus provides a new framework for investigating the wavelength scaling law for the HHG yields.
Dynamical (E,2e) Studies Of Tetrahydropyran And 1,4-Dioxane, J. D. Builth-Williams, G. Da Silva, L. Chiari, D. B. Jones, Hari Chaluvadi, Don H. Madison, M. J. Brunger
Dynamical (E,2e) Studies Of Tetrahydropyran And 1,4-Dioxane, J. D. Builth-Williams, G. Da Silva, L. Chiari, D. B. Jones, Hari Chaluvadi, Don H. Madison, M. J. Brunger
Physics Faculty Research & Creative Works
We present experimental and theoretical results for the electron-impact ionization of the highest occupied molecular orbitals of tetrahydropyran and 1,4-dioxane. Using an (e,2e) technique in asymmetric coplanar kinematics, angular distributions of the slow ejected electron, with an energy of 20 eV, are measured when incident electrons at 250 eV ionize the target and scatter through an angle of either -10° or -15°. The data are compared with calculations performed at the molecular 3-body distorted wave level. Fair agreement between the theoretical model and the experimental measurements was observed. The similar structures for these targets provide key insights for assessing the …
Triply Differential (E,2e) Studies Of Phenol, Silva G. Da, R. F. Neves, L. Chiari, D. B. Jones, E. Ali, Don H. Madison, C. G. Ning, K. L. Nixon, M. C. Lopes, M. J. Brunger
Triply Differential (E,2e) Studies Of Phenol, Silva G. Da, R. F. Neves, L. Chiari, D. B. Jones, E. Ali, Don H. Madison, C. G. Ning, K. L. Nixon, M. C. Lopes, M. J. Brunger
Physics Faculty Research & Creative Works
We have measured (e,2e) triple differential cross sections (TDCS) for the electron-impact ionisation of phenol with coplanar asymmetrical kinematics for an incident electron energy of 250 eV. Experimental measurements of the angular distribution of the slow outgoing electrons at 20 eV are obtained when the incident electron scatters through angles of -5°, -10°, and -15°, respectively. The TDCS data are compared with calculations performed within the molecular 3-body distorted wave model. In this case, a mixed level of agreement, that was dependent on the kinematical condition being probed, was observed between the theoretical and experimental results in the binary peak …
Light Sea Fermions In Electron-Proton And Muon-Proton Interactions, Ulrich D. Jentschura
Light Sea Fermions In Electron-Proton And Muon-Proton Interactions, Ulrich D. Jentschura
Physics Faculty Research & Creative Works
The proton radius conundrum [Pohl, Nature 466, 213 (2010)NATUAS0028-083610. 1038/nature09250 and Antognini, Science 339, 417 (2013)SCIEAS0036-807510.1126/ science.1230016] highlights the need to revisit any conceivable sources of electron-muon nonuniversality in lepton-proton interactions within the standard model. Superficially, a number of perturbative processes could appear to lead to such a nonuniversality. One of these is a coupling of the scattered electron into an electronic vacuum-polarization loop as opposed to a muonic one in the photon exchange of two valence quarks, which is present only for electron projectiles as opposed to muon projectiles. However, we show that this effect actually is part of …
Tracing Multiple Scattering Patterns In Absolute (E, 2e) Cross Sections For H₂ And He Over A 4Π Solid Angle, Xueguang Ren, Arne Senftleben, Thomas Pflüger, Alexander Dorn, James Colgan, Michael S. Pindzola, Ola A. Al-Hagan, Don H. Madison, Igor Bray, Dmitry V. Fursa, Joachim Hermann Ullrich
Tracing Multiple Scattering Patterns In Absolute (E, 2e) Cross Sections For H₂ And He Over A 4Π Solid Angle, Xueguang Ren, Arne Senftleben, Thomas Pflüger, Alexander Dorn, James Colgan, Michael S. Pindzola, Ola A. Al-Hagan, Don H. Madison, Igor Bray, Dmitry V. Fursa, Joachim Hermann Ullrich
Physics Faculty Research & Creative Works
Absolutely normalized (e,2e) measurements for H2 and He covering the full solid angle of one ejected electron are presented for 16 eV sum energy of both final state continuum electrons. For both targets rich cross-section structures in addition to the binary and recoil lobes are identified and studied as a function of the fixed electron's emission angle and the energy sharing among both electrons. For H2 their behavior is consistent with multiple scattering of the projectile as discussed before. For He the binary and recoil lobes are significantly larger than for H2 and partly cover the multiple …
Dynamical (E, 2e) Studies Using Tetrahydrofuran As A Dna Analog, Christopher J. Colyer, Susan M. Bellm, B. Lohmann, G. Friedrich Hanne, Ola A. Al-Hagan, Don H. Madison, Chuangang Ning
Dynamical (E, 2e) Studies Using Tetrahydrofuran As A Dna Analog, Christopher J. Colyer, Susan M. Bellm, B. Lohmann, G. Friedrich Hanne, Ola A. Al-Hagan, Don H. Madison, Chuangang Ning
Physics Faculty Research & Creative Works
Triple differential cross sections for the electron-impact ionization of the outer valence orbital of tetrahydrofuran have been measured using the (e, 2e) technique. The measurements have been performed with coplanar asymmetric kinematics, at an incident electron energy of 250 eV and at an ejected electron energy of 10 eV, over a range of momentum transfers. The experimental results are compared with theoretical calculations carried out using the molecular three-body distorted wave model. The results obtained are important for gaining an understanding of electron driven processes at a molecular level and for modeling energy deposition in living tissue.
Self-Imaging Of Molecules From Diffraction Spectra By Laser-Induced Rescattering Electrons, Junliang Xu, Zhangjin Chen, Anh-Thu Le, C. D. Lin
Self-Imaging Of Molecules From Diffraction Spectra By Laser-Induced Rescattering Electrons, Junliang Xu, Zhangjin Chen, Anh-Thu Le, C. D. Lin
Physics Faculty Research & Creative Works
We study high-energy angle-resolved photoelectron spectra of molecules in strong fields. In an oscillating laser electric field, electrons released earlier in the pulse may return to recollide with the target ion, in a process similar to scattering by laboratory prepared electrons. If midinfrared lasers are used, we show that the images generated by the returning electrons are similar to images observed in typical gas-phase electron diffraction (GED). These spectra can be used to retrieve the positions of atoms in a molecule as in GED. Since infrared laser pulses of durations of a few femtoseconds are already available today, the study …
Correlated Two-Photon Emission By Transitions Of Dirac-Volkov States In Intense Laser Fields: Qed Predictions, Erik Lotstedt, Ulrich D. Jentschura
Correlated Two-Photon Emission By Transitions Of Dirac-Volkov States In Intense Laser Fields: Qed Predictions, Erik Lotstedt, Ulrich D. Jentschura
Physics Faculty Research & Creative Works
In an intense laser field, an electron may decay by emitting a pair of photons. The two photons emitted during the process, which can be interpreted as a laser-dressed double Compton scattering, remain entangled in a quantifiable way: namely, the so-called concurrence of the photon polarizations gives a gauge-invariant measure of the correlation of the hard gamma rays. We calculate the differential rate and concurrence for a backscattering setup of the electron and photon beam, employing Volkov states and propagators for the electron lines, thus accounting nonperturbatively for the electron-laser interaction. The nonperturbative results are shown to differ significantly compared …
Accurate Retrieval Of Target Structures And Laser Parameters Of Few-Cycle Pulses From Photoelectron Momentum Spectra, Samuel Micheau, Zhangjin Chen, Anh-Thu Le, J. Rauschenberger, M. F. Kling, C. D. Lin
Accurate Retrieval Of Target Structures And Laser Parameters Of Few-Cycle Pulses From Photoelectron Momentum Spectra, Samuel Micheau, Zhangjin Chen, Anh-Thu Le, J. Rauschenberger, M. F. Kling, C. D. Lin
Physics Faculty Research & Creative Works
We illustrate a new method of analyzing three-dimensional momentum images of high-energy photoelectrons generated by intense phase-stabilized few-cycle laser pulses. Using photoelectron momentum spectra that were obtained by velocity-map imaging of above-threshold ionization of xenon and argon targets, we show that the absolute carrier-envelope phase, the laser peak intensity, and pulse duration can be accurately determined simultaneously (with an error of a few percent). We also show that the target structure, in the form of electron-target ion elastic differential cross sections, can be retrieved over a range of energies. The latter offers the promise of using laser-generated electron spectra for …
Quantitative Rescattering Theory For Nonsequential Double Ionization Of Atoms By Intense Laser Pulses, Samuel Micheau, Zhangjin Chen, Anh-Thu Le, C. D. Lin
Quantitative Rescattering Theory For Nonsequential Double Ionization Of Atoms By Intense Laser Pulses, Samuel Micheau, Zhangjin Chen, Anh-Thu Le, C. D. Lin
Physics Faculty Research & Creative Works
Laser-induced electron recollisions are fundamental to many strong field phenomena in atoms and molecules. Using the recently developed quantitative rescattering theory, we demonstrate that the nonsequential double ionization (NSDI) of atoms by lasers can be obtained quantitatively in terms of inelastic collisions of the target ions with the free returning electrons where the latter are explicitly given by a spectrum-characterized wave packet. Using argon atoms as target, we calculated the NSDI yield including contributions from direct (e,2e) electron-impact ionization and electron-impact excitation accompanied by subsequent field ionization. We further investigate the dependence of total NSDI on the carrier-envelope phase of …
Differential Cross Sections For The Ionization Of Oriented H₂ Molecules By Electron Impact, James Colgan, Michael S. Pindzola, Francis J. Robicheaux, Christian V. Kaiser, Andrew James Murray, Don H. Madison
Differential Cross Sections For The Ionization Of Oriented H₂ Molecules By Electron Impact, James Colgan, Michael S. Pindzola, Francis J. Robicheaux, Christian V. Kaiser, Andrew James Murray, Don H. Madison
Physics Faculty Research & Creative Works
A nonperturbative close-coupling technique is used to calculate differential cross sections for the electron-impact ionization of H2 at an energy of 35.4 eV. Our approach allows cross sections for any orientation of the molecule with respect to the incident electron beam to be analyzed. New features in the resulting cross sections are found compared with the case where the molecular orientation is averaged, and also with cross sections for He at equivalent electron kinematics. When averaged over all possible molecular orientations, good agreement is found with recent experimental results.
Laser Channeling Of Bethe-Heitler Pairs, Erik Lotstedt, Ulrich D. Jentschura, Christoph H. Keitel
Laser Channeling Of Bethe-Heitler Pairs, Erik Lotstedt, Ulrich D. Jentschura, Christoph H. Keitel
Physics Faculty Research & Creative Works
Electron-positron pair creation is analyzed for an arrangement involving three external fields: a high-frequency gamma photon, the Coulomb field of a nucleus, and a strong laser wave. The frequency of the incoming gamma photon is assumed to be larger than the threshold for pair production in the absence of a laser, and the peak electric field of the laser is assumed to be much weaker than Schwinger's critical field. The total number of pairs produced is found to be essentially unchanged by the laser field, while the differential cross section is drastically modified. We show that the laser can channel …
Double Ionization Of Helium By Ion Impact Analyzed Using Four-Body Dalitz Plots, M. F. Ciappina, Michael Schulz, T. Kirchner, Daniel Fischer, R. Moshammer, J. D. Ullrich
Double Ionization Of Helium By Ion Impact Analyzed Using Four-Body Dalitz Plots, M. F. Ciappina, Michael Schulz, T. Kirchner, Daniel Fischer, R. Moshammer, J. D. Ullrich
Physics Faculty Research & Creative Works
We have performed experimental and theoretical studies of double ionization of helium by 6 MeV proton impact using a recently developed tool, four-particle Dalitz plots [Schulz et al., J. Phys. B 22, 3091 (2007)] which enable the representation of multiple differential cross sections as a function of all four fragments in a single spectrum without loss of any part of the total cross section. As a result, the relative importance of the various interactions between the fragments can be studied in great detail. Comparisons of experimental data with theoretical first-order calculations and simulations for the higher-order (TS-2) process show that …
Alignment Of Heavy Few-Electron Ions Following Excitation By Relativistic Coulomb Collisions, Andrey S. Surzhykov, Ulrich D. Jentschura, Th H. Stohlker, Alexandre Gumberidze, Stephan Fritzsche
Alignment Of Heavy Few-Electron Ions Following Excitation By Relativistic Coulomb Collisions, Andrey S. Surzhykov, Ulrich D. Jentschura, Th H. Stohlker, Alexandre Gumberidze, Stephan Fritzsche
Physics Faculty Research & Creative Works
The Coulomb excitation of highly charged few-electron ions in relativistic collisions with protons and low- Z atoms is studied within the framework of first-order perturbation theory and the multiconfiguration Dirac-Fock method. Apart from the computation of the total excitation cross sections, a detailed theoretical analysis has been performed for the magnetic sublevel population of the residual ions. To describe this population, general expressions are derived for the alignment parameters of the excited states of the ions, taking into account the relativistic and many-electron effects. Calculations are performed for the K→L and K→M excitation of helium- and lithiumlike uranium ions and …
Potential For Ultrafast Dynamic Chemical Imaging With Few-Cycle Infrared Lasers, Toru Morishita, Anh-Thu Le, Zhangjin Chen, C. D. Lin
Potential For Ultrafast Dynamic Chemical Imaging With Few-Cycle Infrared Lasers, Toru Morishita, Anh-Thu Le, Zhangjin Chen, C. D. Lin
Physics Faculty Research & Creative Works
We studied the photoelectron spectra generated by an intense few cycle infrared laser pulse. By focusing on the angular distributions of the back rescattered high energy photoelectrons, we show that accurate differential elastic scattering cross-sections of the target ion by free electrons can be extracted. Since the incident direction and the energy of the free electrons can be easily changed by manipulating the laser's polarization, intensity and wavelength, these extracted elastic scattering cross-sections, in combination with more advanced inversion algorithms, may be used to reconstruct the effective single-scattering potential of the molecule, thus opening up the possibility of using few-cycle …
Isotope Shift In The Dielectronic Recombination Of Three-Electron ANd⁵⁷⁺, Carsten Brandau, Ch Kozhuharov, Zoltan Harman, Alfred K. Muller, Stefan Schippers, S. Kozhedub, Dietrich Bernhardt, Stefan Bohm, J. Jacobi, Eric W. Schmidt, Paul H. Mokler, Fritz J. Bosch, Heinz Jurgen Kluge, Th H. Stohlker, Klaus Beckert, P. Beller, Fritz Nolden, Markus Steck, Alexandre Gumberidze, Regina Reuschl, Uwe Spillmann, Fred John Currell, I. I. Tupitsyn, Vladimir M. Shabaev, Ulrich D. Jentschura
Isotope Shift In The Dielectronic Recombination Of Three-Electron ANd⁵⁷⁺, Carsten Brandau, Ch Kozhuharov, Zoltan Harman, Alfred K. Muller, Stefan Schippers, S. Kozhedub, Dietrich Bernhardt, Stefan Bohm, J. Jacobi, Eric W. Schmidt, Paul H. Mokler, Fritz J. Bosch, Heinz Jurgen Kluge, Th H. Stohlker, Klaus Beckert, P. Beller, Fritz Nolden, Markus Steck, Alexandre Gumberidze, Regina Reuschl, Uwe Spillmann, Fred John Currell, I. I. Tupitsyn, Vladimir M. Shabaev, Ulrich D. Jentschura
Physics Faculty Research & Creative Works
Isotope shifts in dielectronic recombination spectra were studied for Li-like ANd57+ ions with A = 142 and A = 150. From the displacement of resonance positions energy shifts δE142 150(2s-2p1/2) = 40.2(3)(6) meV [(stat)(sys)] and δE142 150(2s - 2p3/2) = 42.3(12)(20)meV of 2s - 2pj transitions were deduced. An evaluation of these values within a full QED treatment yields a change in the mean-square charge radius of 142 150δ⟨ r2⟩ = -1.36(1)(3) fm2. The approach is conceptually new and combines the advantage of a …
Triple-Differential Cross Sections For Target Ionization With Simultaneous Projectile Detachment In 200-Kev H⁻ + He Collisions, T. Ferger, Michael Schulz, Daniel Fischer, B. Najjari, R. Moshammer, J. D. Ullrich
Triple-Differential Cross Sections For Target Ionization With Simultaneous Projectile Detachment In 200-Kev H⁻ + He Collisions, T. Ferger, Michael Schulz, Daniel Fischer, B. Najjari, R. Moshammer, J. D. Ullrich
Physics Faculty Research & Creative Works
We have performed a kinematically complete experiment for target ionization with simultaneous projectile detachment (TIPD) in 200-keV H− + He collisions. From the data we extracted triple-differential cross sections (TDCSs) for each electron separately. These TDCSs closely resemble corresponding data for single ionization by charged-particle impact. Surprisingly, the contributions from higher-order processes to TIPD, proceeding through two independent interactions of each electron with the core of the respective other collision partner, are found to be somewhat larger than the first-order process proceeding through the electron-electron interaction.
Two-Loop Bethe Logarithms For Non- S Levels, Ulrich D. Jentschura
Two-Loop Bethe Logarithms For Non- S Levels, Ulrich D. Jentschura
Physics Faculty Research & Creative Works
Two-loop Bethe logarithms are calculated for excited P and D states in hydrogenlike systems, and estimates are presented for all states with higher angular momenta. These results complete our knowledge of the P and D energy levels in hydrogen at the order of α8 mec2, where me is the electron mass and c is the speed of light, and scale as Z6, where Z is the nuclear charge number. Our analytic and numerical calculations are consistent with the complete absence of logarithmic terms of order (απ)2 (Zα)6 ln [(Zα)-2] …
K Α₁ Radiation From Heavy, Heliumlike Ions Produced In Relativistic Collisions, Andrey S. Surzhykov, Ulrich D. Jentschura, Th H. Stohlker, Stephan Fritzsche
K Α₁ Radiation From Heavy, Heliumlike Ions Produced In Relativistic Collisions, Andrey S. Surzhykov, Ulrich D. Jentschura, Th H. Stohlker, Stephan Fritzsche
Physics Faculty Research & Creative Works
Bound-state transitions in few-electron, heavy ions following radiative electron capture are studied within the framework of the density matrix theory and the multiconfiguration Dirac-Fock approach. Special attention is paid to the K α1 (1 s1/2 2 p3/2 1.3PJ=1,2→1s21/2 1SJ=0) radiative decay of heliumlike uranium U90+ projectiles. This decay has recently been observed at the GSI facility in Darmstadt, giving rise to a surprisingly isotropic angular distribution, which is inconsistent with previous experiments and calculations based on a "one-particle" model. We show that the unexpected isotropy essentially results from …
Multiple Scattering Mechanisms In Simultaneous Projectile-Electron And Target-Electron Ejection In H⁻ + He Collisions, Michael Schulz, T. Ferger, Daniel Fischer, R. Moshammer, J. D. Ullrich
Multiple Scattering Mechanisms In Simultaneous Projectile-Electron And Target-Electron Ejection In H⁻ + He Collisions, Michael Schulz, T. Ferger, Daniel Fischer, R. Moshammer, J. D. Ullrich
Physics Faculty Research & Creative Works
We studied simultaneous electron ejection from both collision partners in 200-keV H-+He collisions in a kinematically complete experiment by measuring the fully momentum-analyzed recoil ions and both active electrons in coincidence. The data were analyzed in terms of Dalitz spectra, in which the momentum exchange between three particles is plotted simultaneously in a single spectrum. We found that the energy transfer occurs predominantly between the active electrons, but most of the momentum is exchanged in elastic scattering between the cores of the collision partners.
Hyperspherical Close-Coupling Calculations For Electron-Capture Cross Sections In Low-Energy Ne¹⁰⁺ +H (1s) Collisions, P. Barragan, Anh-Thu Le, C. D. Lin
Hyperspherical Close-Coupling Calculations For Electron-Capture Cross Sections In Low-Energy Ne¹⁰⁺ +H (1s) Collisions, P. Barragan, Anh-Thu Le, C. D. Lin
Physics Faculty Research & Creative Works
We present total and partial electron-capture cross sections for Ne¹⁰⁺ +H (1s) collisions at energies from 0.01 eV to 1 keV using the hyperspherical close-coupling method. Good agreements with the previous calculations by the classical-trajectory Monte-Carlo method are found for total capture cross section, but not for partial cross sections, especially below about 200 eV/amu. We found that the total cross section is mainly due to the population of n=7 channels and only at energies above 50 eV/amu n = 5,6 channels begin to contribute to the total cross section.