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Full-Text Articles in Physics
Combining Atomic Force Microscopy And Shear-Force Acoustic Near-Field Microscopy To Characterize Confined Mesoscopic Fluids, Monte Allen Kozell, Theodore Brockman, Andres H. La Rosa
Combining Atomic Force Microscopy And Shear-Force Acoustic Near-Field Microscopy To Characterize Confined Mesoscopic Fluids, Monte Allen Kozell, Theodore Brockman, Andres H. La Rosa
Physics Faculty Publications and Presentations
An atomic force microscopy (AFM) cantilever is integrated into to a quartz tuning fork (QTF) to probe the viscoelastic properties of mesoscopic fluid layers confined between two solid surfaces under shear. Two procedures to fabricate the AFM/QTF probe are described herein. In the first, a nano-manipulator is used to transport a commercially available afm cantilever from its chip holder to the edge of a QTF tine. In the second, an afm cantilever is fabricated at the edge of the QTF tine itself. In both cases we exploit the capabilities of a dual-beam system (focused ion beam/scanning electron microscope), equipped with …
Confined Fluid Analyzed With Near-Field Acoustic Detection, Rodolfo Fernandez Rodriguez, Theodore Brockman, J. Bai, Andres H. La Rosa
Confined Fluid Analyzed With Near-Field Acoustic Detection, Rodolfo Fernandez Rodriguez, Theodore Brockman, J. Bai, Andres H. La Rosa
Physics Faculty Publications and Presentations
Measurement of the damping and elastic interactions between two solids interfaces (one being the apex of a tapered probe that is attached to one tine of a quartz tuning fork while the other is a flat substrate) under relative lateral oscillatory motion are reported. The solid boundaries are separated by a nanometer sized gap, and emphasis is placed on the role played by the mesoscopic fluid trapped in between. The measurements were implemented using two new acoustic techniques that have been integrated into a tuning fork based scanning probe microscope; the whole metrology system offers sub-nanometer precision for controlling the …
Finite Element Method Analysis Of Whispering Gallery Acoustic Sensing, T. Le, H. Tran, Rodolfo Fernandez Rodriguez, C.J. Solano Salinas, Nima Laal, R. Bringas, J. Quispe, F. Segundo, Andres H. La Rosa
Finite Element Method Analysis Of Whispering Gallery Acoustic Sensing, T. Le, H. Tran, Rodolfo Fernandez Rodriguez, C.J. Solano Salinas, Nima Laal, R. Bringas, J. Quispe, F. Segundo, Andres H. La Rosa
Physics Faculty Publications and Presentations
Whispering Gallery Acoustic Sensing (WGAS) has recently been introduced as a sensing feedback mechanism to control the probe-sample separation distance in scanning probe microscopy that uses a quartz tuning fork as a sensor (QTF-SPM). WGAS exploits the SPM supporting frame as a resonant acoustic cavity to monitor the nanometer-sized amplitude of the QTF oscillations. Optimal WGAS sensitivity depends on attaining an exact match between the cavity's frequency peak response and the TF resonance frequency. However, two aspects play against this objective: i) the unpredictable variability of the TF resonance frequency (upon attaching a SPM-probe to one of its tines), …
Probe Damage Evaluation In Frequency-Modulation Shear-Force Acoustic Near-Field Microscopy, Theodore Brockman, Rodolfo Fernandez Rodriguez, J. Bai, Monte Allen Kozell, Andres H. La Rosa
Probe Damage Evaluation In Frequency-Modulation Shear-Force Acoustic Near-Field Microscopy, Theodore Brockman, Rodolfo Fernandez Rodriguez, J. Bai, Monte Allen Kozell, Andres H. La Rosa
Physics Faculty Publications and Presentations
Shear-force acoustic near-field microscopy (SANM) and Whispering Gallery Acoustic Sensing have recently been introduced as a tandem system to characterize the viscoelastic response of fluids confined between two solid-boundaries in relative oscillatory lateral motion. SANM uses a) a laterally oscillating tapered probe (attached to a quartz tuning fork QTF) as one of the trapping boundaries, and b) an acoustic sensor (attached to the other flat-substrate boundary) that independently monitors the fluid’s acoustic emission. On the other and, WGAS is another technique that uses an acoustic transducer (attached to the frame holding the probe) to monitor the probe’s lateral motion amplitude. …
Acousto Characterization Of Fluid-Like Mesoscopic Films Under Shear, Rodolfo Fernandez, Xiaohua Wang, Andres H. La Rosa
Acousto Characterization Of Fluid-Like Mesoscopic Films Under Shear, Rodolfo Fernandez, Xiaohua Wang, Andres H. La Rosa
Physics Faculty Publications and Presentations
Full understanding of the physics underlying the striking changes-in viscoelasticity, relaxation time, and phase transitions-that mesoscopic fluid-like systems undergo when placed under confinement or when adsorbed at solid surfaces constitutes a long standing scientific challenge. One of the methods used to characterize these films consists of bringing a solid boundary closer to another solid boundary (while in relative lateral periodic motion) with a liquid trapped in between. In addition, using a tapered probe (~ 50 nm apex diameter) as one of the boundaries improves the lateral resolution of the measurement. In this scenario, the dynamics of the fluid is inferred …
Nonlocal Effects On Optical And Molecular Interactions With Metallic Nanoshells, P.T. Leung, Railing Chang
Nonlocal Effects On Optical And Molecular Interactions With Metallic Nanoshells, P.T. Leung, Railing Chang
Physics Faculty Publications and Presentations
Theoretical studies of the optical response of metallic nanoshells have been carried out, where quantum effects are partially accounted for through the application of a nonlocal response model for shells of mesoscopic dimensions. Both far field and near field interactions are considered, with the incident source being a plane wave and an emitting molecular dipole, respectively. It is found that these nonlocal effects can lead to significant deviations from macroscopic electrodynamic theory, for shells of ultrasmall dimensions (nm) or ultrathin thickness (~1 nm), and are particularly significant for processes involving higher multipolar responses of the nanoshells. It is further concluded …
Nonlocal Electrodynamic Modeling Of Fluorescence Characteristics For Molecules In A Spherical Cavity, Pui T. Leung, M. H. Hider
Nonlocal Electrodynamic Modeling Of Fluorescence Characteristics For Molecules In A Spherical Cavity, Pui T. Leung, M. H. Hider
Physics Faculty Publications and Presentations
The emission characteristics for molecules in a spherical metallic microcavity are computed using a nonlocal electrodynamic model, based on a theory previously published by Fuchs and Claro [Phys. Rev. B 35, 3722 (1987)] for the multipole polarizability of a sphere. Both radially and tangentially oriented molecules at arbitrary locations inside the cavity are considered, and the results are compared with those from both the local response theory and those for molecules outside a spherical particle. The issue of reciprocity of the solutions for each of the sphere and cavity cases, respectively, is examined in the light of the nonlocal effects. …