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 Transport (3)
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 Fourier transform infrared spectroscopy (2)

 Superfluorescence (2)
 Molecular dynamics (2)
 Dissociation energies (2)
 Electronphonon interactions. (2)
 Electronelectron interactions (2)
 Bond formation (2)
 Rotation constants (2)
 SF (2)
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 Energy transfer (1)
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 Decaying states (1)
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 Calcium (1)
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Articles 1  21 of 21
FullText Articles in Physics
Universal Electric Current Of Interacting ResonantLevel Models With Asymmetric Interactions: An Extension Of The Landauer Formula, Akinori Nishino, Naomichi Hatano, Gonzalo Ordonez
Universal Electric Current Of Interacting ResonantLevel Models With Asymmetric Interactions: An Extension Of The Landauer Formula, Akinori Nishino, Naomichi Hatano, Gonzalo Ordonez
Scholarship and Professional Work  LAS
We study the electron transport in open quantumdot systems described by the interacting resonantlevel models with Coulomb interactions. We consider the situation in which the quantum dot is connected to the left and right leads asymmetrically. We exactly construct manyelectron scattering eigenstates for the twolead system, where twobody bound states appear as a consequence of onebody resonances and the Coulomb interactions. By using an extension of the Landauer formula, we calculate the average electric current for the system under bias voltages in the first order of the interaction parameters. Through a renormalizationgroup technique, we arrive at the universal electric current ...
TimeReversal Symmetric Resolution Of Unity Without Background Integrals In Open Quantum Systems, Naomichi Hatano, Gonzalo Ordonez
TimeReversal Symmetric Resolution Of Unity Without Background Integrals In Open Quantum Systems, Naomichi Hatano, Gonzalo Ordonez
Scholarship and Professional Work  LAS
We present a new complete set of states for a class of open quantum systems, to be used in expansion of the Green’s function and the timeevolution operator. A remarkable feature of the complete set is that it observes timereversal symmetry in the sense that it contains decaying states (resonant states) and growing states (antiresonant states) parallelly. We can thereby pinpoint the occurrence of the breaking of timereversal symmetry at the choice of whether we solve Schrödinger equation as an initialcondition problem or a terminalcondition problem. Another feature of the complete set is that in the subspace of the ...
Optically Tunable Bound States In The Continuum, Yingyue Boretz, Gonzalo Ordonez, Satoshi Tanaka, Tomio Petrosky
Optically Tunable Bound States In The Continuum, Yingyue Boretz, Gonzalo Ordonez, Satoshi Tanaka, Tomio Petrosky
Scholarship and Professional Work  LAS
We demonstrate the existence of tunable bound states in the continuum (BICs) in a onedimensional quantum wire with two impurities induced by an intense monochromatic radiation field. We find that there is an interesting type of BIC due to the Fano interference between two optical transition channels, in addition to the ordinary BIC due to geometrical interference between electron wave functions emitted by impurities. In both cases the BIC can be achieved by tuning the frequency of the radiation field. Evidence of the BIC can be obtained by observing the absorption rate of a probe photon.
Phase Diagram Of The OneDimensional HubbardHolstein Model At Half And Quarter Filling, Rahul Hardikar, R. T. Clay
Phase Diagram Of The OneDimensional HubbardHolstein Model At Half And Quarter Filling, Rahul Hardikar, R. T. Clay
Scholarship and Professional Work  LAS
The HubbardHolstein model is one of the simplest to incorporate both electronelectron and electronphonon interactions. In one dimension at half filling, the Holstein electronphonon coupling promotes onsite pairs of electrons and a Peierls chargedensity wave, while the Hubbard onsite Coulomb repulsion U promotes antiferromagnetic correlations and a Mott insulating state. Recent numerical studies have found a possible third intermediate phase between Peierls and Mott states. From direct calculations of charge and spin susceptibilities, we show that (i) as the electronphonon coupling is increased, first a spin gap opens, followed by the Peierls transition. Between these two transitions, the metallic intermediate ...
TemperatureDriven Transition From The Wigner Crystal To The BondChargeDensity Wave In The QuasiOneDimensional QuarterFilled Band, R. T. Clay, Rahul Hardikar, S. Mazumdar
TemperatureDriven Transition From The Wigner Crystal To The BondChargeDensity Wave In The QuasiOneDimensional QuarterFilled Band, R. T. Clay, Rahul Hardikar, S. Mazumdar
Scholarship and Professional Work  LAS
It is known that within the interacting electron model Hamiltonian for the onedimensional 1/4filled band, the singlet ground state is a Wigner crystal only if the nearestneighbor electronelectron repulsion is larger than a critical value. We show that this critical nearestneighbor Coulomb interaction is different for each spin subspace, with the critical value decreasing with increasing spin. As a consequence, with the lowering of temperature, there can occur a transition from a Wigner crystal chargeordered state to a spinPeierls state that is a bondchargedensity wave with charge occupancies different from the Wigner crystal. This transition is possible because spin ...
Electron Trapping In A OneDimensional Semiconductor Quantum Wire With Multiple Impurities, S. Tanaka, S. Garmon, Gonzalo Ordonez, T. Petrosky
Electron Trapping In A OneDimensional Semiconductor Quantum Wire With Multiple Impurities, S. Tanaka, S. Garmon, Gonzalo Ordonez, T. Petrosky
Scholarship and Professional Work  LAS
We demonstrate the trapping of a conduction electron between two identical adatom impurities in a onedimensional semiconductor quantumdot array system (quantum wire). Bound steady states arise even when the energy of the adatom impurity is located in the continuous onedimensional energy miniband. The steady state is a realization of the bound state in continuum (BIC) phenomenon first proposed by von Neuman and Wigner [Phys. Z. 30, 465 (1929)]. We analytically solve the dispersion equation for this localized state, which enables us to reveal the mechanism of the BIC. The appearance of the BIC state is attributed to the quantum interference ...
Bound States In The Continuum In QuantumDot Pairs, Gonzalo Ordonez, Kyungsun Na, Sungyun Kim
Bound States In The Continuum In QuantumDot Pairs, Gonzalo Ordonez, Kyungsun Na, Sungyun Kim
Scholarship and Professional Work  LAS
It is shown that for two open quantum dots connected by a wire, “bound states in the continuum” of a single electron are formed at nearly periodic distances between the dots. This is due to FabryPérot interference between quasibound states in each dot. The bound states are nonlocal, describing the electron trapped in both dots at the same time. Theoretical and numerical results show that trapped states exist even if the wire connecting the dots is relatively long.
Monte Carlo LeastSquares Fitting Of Experimental Signal Waveforms, Xianming Han, Vladimir Pozdina, C. Haridas, Prabhakar Misra
Monte Carlo LeastSquares Fitting Of Experimental Signal Waveforms, Xianming Han, Vladimir Pozdina, C. Haridas, Prabhakar Misra
Scholarship and Professional Work  LAS
This paper focuses on why the regular least{squares ¯tting technique is unstable when used to ¯t exponential functions to signal waveforms, since such functions are highly correlated. It talks about alternative approaches, such as the search method, which has a slow convergence rate of 1=N1=M, for M parameters, where N is the number of computations performed. We have used the Monte Carlo method, utilizing both search and random walk, to devise a stable least{squares ¯tting algorithm that converges rapidly at a rate 1=N1=2, regardless of the number of parameters used in ¯tting the waveforms ...
Intermediate Phase Of The One Dimensional HalfFilled HubbardHolstein Model, R. T. Clay, Rahul Hardikar
Intermediate Phase Of The One Dimensional HalfFilled HubbardHolstein Model, R. T. Clay, Rahul Hardikar
Scholarship and Professional Work  LAS
We present a numerical study of the HubbardHolstein model in one dimension at half filling, including finitefrequency quantum phonons. At half filling, the effects of the electronphonon and electronelectron interactions compete with the Holstein phonon coupling acting as an effective negative Hubbard onsite interaction U that promotes onsite electron pairs and a Peierls chargedensity wave state. Most previous work on this model has assumed that only Peierls or Mott phases are possible at half filling. However, there has been speculation that a third metallic phase exists between the Peierls and Mott phases. We confirm the intermediate phase, and show that ...
Superfluorescence Polarization: Signature Of Collisional Redistribution, A. Kumarakrishnan, S. Chudasama, Xianming Han
Superfluorescence Polarization: Signature Of Collisional Redistribution, A. Kumarakrishnan, S. Chudasama, Xianming Han
Scholarship and Professional Work  LAS
We have studied effects of magnetic sublevel degeneracy on the polarization of superfluorescent pulses generated on the Ca 4s4p1P1–3d4s1D2 transition at 5.5μm. These pulses were generated from a cell of length 50 cm by optically pumping calcium vapor on the 4s21S0–4s4p1P1 transition in the presence of Ar gas. The axis of ellipticity of superfluorescence (SF) polarization is oriented parallel to the axis of the pumplaser polarization at large detunings, and undergoes an abrupt rotation through 90° for detunings close to resonance. The distribution of populations in the magnetic sublevels of the 1P1 state can be estimated using ...
Superfluorescence From Optically Trapped Calcium Atoms, Xianming Han
Superfluorescence From Optically Trapped Calcium Atoms, Xianming Han
Scholarship and Professional Work  LAS
We have studied superfluorescence (SF) under highly unfavorable conditions of rapid collisional and radiative distribution in a Dopplerbroadened medium. Nanosecond SF pulses at 5.5 μm were generated on the Ca 4s4p1P1–3d4s1D2 transition from a column of calcium vapor buffered with Ar by optically pumping the 4s21S0–4s4p1P1 transition. The Rabi frequency associated with the intense pump pulse prevents the occurrence of SF while the pump laser is on. As a result, the predicted scaling laws that describe the properties of SF in a transversely excited system, such as peak heights, pulse widths, and delay times, are shown to ...
MagneticFieldInduced AlignmentToOrientation Conversion In Sodium, G. W. Schinn, Xianming Han
MagneticFieldInduced AlignmentToOrientation Conversion In Sodium, G. W. Schinn, Xianming Han
Scholarship and Professional Work  LAS
We report a detailed investigation of excitedstate alignmenttoorientation conversion in the presence of an external magnetic field. This counterintuitive phenomenon occurs under intermediatecoupling conditions. A weak, linearly polarized, cw laser beam was used to excite and align the Na 3P3/2 state in an atomic beam along the z direction. The degree of circular polarization of the resulting fluorescence was detected along the z direction as a function of magneticfield strength. The spectrally integrated transitions originating from individual F levels of the 3S1/2 state yield a maximum circularpolarization fraction of ∼40%; integrating the circular polarization over all the allowed ...
Fine‐Structure Mixing Within The Zn(43pj) Multiplet By Collisions With The Noble Gases, Xianming Han, J. F. Kelly
Fine‐Structure Mixing Within The Zn(43pj) Multiplet By Collisions With The Noble Gases, Xianming Han, J. F. Kelly
Scholarship and Professional Work  LAS
Measurements of rate coefficients for intramultiplet state transfer of Zn(4 ^{3} P _{1}→4 ^{3} P _{ J’}) by collisions with the rare gases are presented. The state‐to‐state binary rate coefficients are derived from least‐squares fittings of the time‐resolved triexponential behavior of the 4 ^{3} P _{1}fluorescence. These rate coefficients were studied systematically over a temperature range of 690–1100 K in order to characterize the velocity dependence of the collisional coupling. The systematic behavior of the rate coefficients with varying temperature and noble gas species is qualitatively consistent with a nearly adiabatic coupling limit ...
Differential, Partial Cross Sections For Electron Excitation Of The Sodium 3p State, Xianming Han, G. W. Schwinn, A. Gallagher
Differential, Partial Cross Sections For Electron Excitation Of The Sodium 3p State, Xianming Han, G. W. Schwinn, A. Gallagher
Scholarship and Professional Work  LAS
Using a powerful laserbased experimental method, the cross section for electron excitation of Na(3S) atoms to the Na(3P) state has been decomposed into partial components with respect to changes in the spin and angular momentum of the atomic electron, and these partial cross sections are further reduced to their differential character with respect to the electron scattering angle. Partial, differential cross sections are reported for electron collision energies from threshold 2.1 to 3.6 eV, and compared to available calculations.
The Spectroscopy And Molecular Dynamics Of The High Frequency Ν1 6 Intermolecular Vibrations In Hcn‐‐‐Hf And Dcn‐‐‐Df, B. A. Wofford, M. W. Jackson, Shannon Lieb, J. W. Bevan
The Spectroscopy And Molecular Dynamics Of The High Frequency Ν1 6 Intermolecular Vibrations In Hcn‐‐‐Hf And Dcn‐‐‐Df, B. A. Wofford, M. W. Jackson, Shannon Lieb, J. W. Bevan
Scholarship and Professional Work  LAS
Gas phase rovibrational analysis of the high frequency intermolecular hydrogen bonded bending overtone 2ν^{0} _{6} [ν_{0}=1132.4783(2) cm^{−} ^{1}] in HCN‐‐‐HF and its corresponding perdeuterated fundamental ν^{1} _{6} [ν_{0}=409.1660(2) cm^{−} ^{1}] are reported. Evaluated rovibrational parameters provide the basis for quantitative modeling of the molecular dynamics associated with this vibration. A quantum mechanical calculation permits determination of the quadratic and quartic force constants K _{6} _{6}=537(17) and K _{6} _{6} _{6} _{6}=4.98(12) cm^{−} ^{1} which in turn are used to estimate the pertinent cubic band ...
Erratum: Determination Of Dissociation Energies And Thermal Functions Of Hydrogen Bond Formation Using High Resolution Ftir Spectroscopy [J. Chem. Phys. 8 7, 5674 (1987)], B. A. Wofford, M. E. Eliades, Shannon Lieb, J. W. Bevan
Erratum: Determination Of Dissociation Energies And Thermal Functions Of Hydrogen Bond Formation Using High Resolution Ftir Spectroscopy [J. Chem. Phys. 8 7, 5674 (1987)], B. A. Wofford, M. E. Eliades, Shannon Lieb, J. W. Bevan
Scholarship and Professional Work  LAS
Erratum
SpinExchange Cross Section For Electron Excitation Of Na 3s 3p Determined By A Novel Spectroscopic Technique, Xianming Han, G. W. Schwinn, A. Gallagher
SpinExchange Cross Section For Electron Excitation Of Na 3s 3p Determined By A Novel Spectroscopic Technique, Xianming Han, G. W. Schwinn, A. Gallagher
Scholarship and Professional Work  LAS
An experimental technique is described which enables determination of the partial cross sections for electron excitation of atoms as a function of changes in spin and orbital angular momentum. This method provides a good signaltonoise ratio in the energy region near threshold, and could be used to study long or shortlived excited states of many atomic systems. Measurements for Na 3S−3P, nearthreshold excitation are reported here. The results are generally in good agreement with the closecoupling calculations of D. L. Moores and D. W. Norcross [J. Phys. B 5, 1482 (1972)] for the largest ΔmS and ΔmL components of ...
Determination Of Dissociation Energies And Thermal Functions Of Hydrogen‐Bond Formation Using High Resolution Ftir Spectroscopy, B. A. Wofford, M. E. Eliades, Shannon Lieb, J. W. Bevan
Determination Of Dissociation Energies And Thermal Functions Of Hydrogen‐Bond Formation Using High Resolution Ftir Spectroscopy, B. A. Wofford, M. E. Eliades, Shannon Lieb, J. W. Bevan
Scholarship and Professional Work  LAS
A technique which employs high resolution Fourier transform infrared spectroscopy is demonstrated for evaluation of hydrogen bonddissociation energiesD _{0} and D _{ e }. Results for HCN‐‐HF give a D _{0}=20.77(22) and D _{ e } =28.77(45) kJ/mol which are compared with previously determined values obtained from microwave absolute intensity measurements and a b i n i t i o molecular orbital calculations. Rovibrational band information available for HCN‐‐HF also permits evaluation of thermal functions of dimer formation in kJ/mol: ΔU ^{○} _{298.2} =20.1(2), ΔH ^{○} _{298.2} =22.6(2 ...
Molecular Dynamics In Hydrogen‐Bonded Interactions: A Preliminary Experimentally Determined Harmonic Stretching Force Field For Hcn‐‐‐Hf, B. A. Wofford, Shannon Lieb, J. W. Bevan
Molecular Dynamics In Hydrogen‐Bonded Interactions: A Preliminary Experimentally Determined Harmonic Stretching Force Field For Hcn‐‐‐Hf, B. A. Wofford, Shannon Lieb, J. W. Bevan
Scholarship and Professional Work  LAS
Observation of the 2ν_{1} overtone band in the hydrogen‐bonded complex HCN‐‐‐HF permits evaluation of the anharmonicity constant X _{1} _{1}=−116.9(1) cm^{−} ^{1} and determination of the anharmonicity corrected fundamental frequency ω_{1}. This information, and available data from previous rovibrational analyses in the common and perdeuterated isotopic species of HCN‐‐‐HF, offer an opportunity for calculation of an approximate stretching harmonic force field. With the assumptions f _{1} _{2}=f _{2} _{4}=0.0, the remaining force constants (in mdyn/Å) are evaluated as: f _{1} _{1}=8.600(20), f _{2} _{2}=6 ...
Preliminary Rovibrational Analysis Of The Nν6+Ν1−Nν6 Vibration In Hcn⋅⋅⋅Hf, E. Kyrö, K. Mcmillan, M. Eliades, D. Danzeiser, P. ShojaChaghervand, Shannon Lieb, J. W. Bevan
Preliminary Rovibrational Analysis Of The Nν6+Ν1−Nν6 Vibration In Hcn⋅⋅⋅Hf, E. Kyrö, K. Mcmillan, M. Eliades, D. Danzeiser, P. ShojaChaghervand, Shannon Lieb, J. W. Bevan
Scholarship and Professional Work  LAS
A preliminary rotation‐vibration analysis of the n=0 and n=1 subbands associated with the nν_{6}+ν_{1}−nν_{6} hydrogen‐bonded vibration in HCN⋅⋅⋅HF has been completed. The following excited staterotational constantsB′ and band origin frequencies ν_{0} have been determined for the complex. The results are consistent with a rotation‐vibration interaction constant α_{1}=−68.3±1 MHz which correlates with an excited stater(N⋅⋅⋅F) internuclear distance of 2.762 Å, a decrease of 0.034 Å relative to the ground state.Excited state lifetimes associated with assigned transitions ...
TravellingWave SubDoppler Excited Molecule Energy Transfer Spectroscopy, Khalid Iqbal, Shannon G. Lieb, J. W. Bevan
TravellingWave SubDoppler Excited Molecule Energy Transfer Spectroscopy, Khalid Iqbal, Shannon G. Lieb, J. W. Bevan
Scholarship and Professional Work  LAS
A general formulation of traveling‐wave sub‐Doppler excited molecule energy transferspectroscopy is presented. The line profile analysis is applied to that determined experimentally for the R(22) ν3 HCN transition. Pn the noise equivalent power of the detector is demonstrated to be ⩽10−12 W. Finally, the technique is applied to resolve the KsR(7) ν1 transition head in NH3.