Physics Commons^™

Diffractive Imaging Of Laser Induced Molecular Reactions With Kiloelectron-Volt Ultrafast Electron Diffraction, Yanwei Xiong

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

Capturing the structural changes during a molecular reaction with ultrafast electron diffraction (UED) requires a high spatiotemporal resolution and sufficiently high signal-to-noise to record the signals with high fidelity. In this dissertation, I have focused on the development of a tabletop gas phase keV-UED setup with a femtosecond temporal resolution. A DC electron gun was employed to generate electron pulses with a high repetition rate of 5 kHz. The space charge effect in the electron pulse was ameliorated by compressing the 90 keV electron pulse longitudinally with a time varying electric field in an RF cavity. The velocity mismatch between …

Magnetic Skyrmions Unwrapped, Alexey Kovalev

Alexey Kovalev Papers

Experiments with chiral magnets may hold the key to a better understanding of fundamental aspects of transformations between different skyrmionic states, necessary for magnetic memory and logic applications to become a reality.

With the aim of developing computing devices that operate with low power dissipation, scientists have been pursuing the idea of encoding information in magnetic states. Specifically, skyrmions, which can be thought of as whirl-like states of magnetic moments, are promising candidates for this purpose. The advantage of skyrmions lies in their topological protection, a property implying that only a ‘global’ system modification can erase a skyrmion. Realizations of …

Majorana Bound States With Chiral Magnetic Textures, Utkan Güngördü, Alexey Kovalev

Alexey Kovalev Papers

The aim of this Tutorial is to give a pedagogical introduction into realizations of Majorana fermions, usually termed as Majorana bound states (MBSs), in condensed matter systems with magnetic textures. We begin by considering the Kitaev chain model of “spinless” fermions and show how two “half” fermions can appear at chain ends due to interactions. By considering this model and its two-dimensional generalization, we emphasize intricate relation between topological superconductivity and possible realizations of MBS. We further discuss how “spinless” fermions can be realized in more physical systems, e.g., by employing the spin-momentum locking. Next, we demonstrate how magnetic textures …

Majorana Bound States With Chiral Magnetic Textures, Utkan Güngördü, Alexey Kovalev

Department of Physics and Astronomy: Faculty Publications

The aim of this Tutorial is to give a pedagogical introduction into realizations of Majorana fermions, usually termed as Majorana bound states (MBSs), in condensed matter systems with magnetic textures. We begin by considering the Kitaev chain model of “spinless” fermions and show how two “half” fermions can appear at chain ends due to interactions. By considering this model and its two-dimensional generalization, we emphasize intricate relation between topological superconductivity and possible realizations of MBS. We further discuss how “spinless” fermions can be realized in more physical systems, e.g., by employing the spin-momentum locking. Next, we demonstrate how magnetic textures …

Superfluid Spin Transistor, Edward Schwartz, Bo Li, Alexey Kovalev

Alexey Kovalev Papers

We propose to use the Hall response of topological defects, such as merons and antimerons, to spin currents in two-dimensional magnetic insulator with in-plane anisotropy for identification of the Berezinskii-Kosterlitz-Thouless (BKT) transition in a transistorlike geometry. Our numerical results relying on a combination of Monte Carlo and spin dynamics simulations show transition from spin superfluidity to conventional spin transport, accompanied by the universal jump of the spin stiffness and exponential growth of the transverse vorticity current. We propose a superfluid spin transistor in which the spin and vorticity currents are modulated by changes in density of free topological defects, e.g., …

High Sensitivity Multi-Axes Rotation Sensing Using Large Momentum Transfer Point Source Atom Interferometry, Jinyang Li, Gregório R. M. Da Silva, Wayne Cheng-Wei Huang, Mohamed Fouda, Jason Bonacum, Timothy L. Kovachy, Selim M. Shahriar

Department of Physics and Astronomy: Faculty Publications

A point source interferometer (PSI) is a device where atoms are split and recombined by applying a temporal sequence of Raman pulses during the expansion of a cloud of cold atoms behaving approximately as a point source. The PSI can work as a sensitive multi-axes gyroscope that can automatically filter out the signal from accelerations. The phase shift arising from the rotations is proportional to the momentum transferred to each atom from the Raman pulses. Therefore, by increasing the momentum transfer, it should be possible to enhance the sensitivity of the PSI. Here, we investigate the degree of enhancement in …

Kapitza-Dirac Blockade: A Universal Tool For The Deterministic Preparation Of Non-Gaussian Oscillator States, Wayne Cheng-Wei Huang, Herman Batelaan, Markus Arndt

Department of Physics and Astronomy: Faculty Publications

Harmonic oscillators count among the most fundamental quantum systems with important applications in molecular physics, nanoparticle trapping, and quantum information processing. Their equidistant energy level spacing is often a desired feature, but at the same time a challenge if the goal is to deterministically populate specific eigenstates. Here, we show how interference in the transition amplitudes in a bichromatic laser field can suppress the sequential climbing of harmonic oscillator states (Kapitza-Dirac blockade) and achieve selective excitation of energy eigenstates, cat states, and other non-Gaussian states. This technique can transform the harmonic oscillator into a coherent two-level system or be used …

Plasmonic Waveguides To Enhance Quantum Electrodynamic Phenomena At The Nanoscale, Ying Li, Christos Argyropoulos

Department of Electrical and Computer Engineering: Faculty Publications

The emerging field of plasmonics can lead to enhanced light-matter interactions at extremely nanoscale regions. Plasmonic (metallic) devices promise to efficiently control both classical and quantum properties of light. Plasmonic waveguides are usually used to excite confined electromagnetic modes at the nanoscale that can strongly interact with matter. The analysis of these nanowaveguides exhibits similarities with their low frequency microwave counterparts. In this article, we review ways to study plasmonic nanostructures coupled to quantum optical emitters from a classical electromagnetic perspective. These quantum emitters are mainly used to generate single-photon quantum light that can be employed as a quantum bit …

Spin Superfluidity In Noncollinear Antiferromagnets, Bo Li, Alexey Kovalev

Alexey Kovalev Papers

We explore the spin superfluid transport in exchange interaction-dominated three-sublattice antiferromagnets. The system in the long-wavelength regime is described by an SO(3) invariant field theory. Additional corrections from Dzyaloshinskii-Moriya interactions or anisotropies can break the symmetry; however, the system still approximately holds a U(1)-rotation symmetry. Thus, the power-law spatial decay signature of spin superfluidity is identified in a nonlocal-measurement setup where the spin injection is described by the generalized spin-mixing conductance. We suggest iron jarosites as promising material candidates for realizing our proposal.

Spirals And Skyrmions In Antiferromagnetic Triangular Lattices, Wuzhang Fang, Aldo Raeliarijaona, Po-Hao Chang, Alexey Kovalev, K. D. Belashchenko

Alexey Kovalev Papers

We study realizations of spirals and skyrmions in two-dimensional antiferromagnets with a triangular lattice on an inversion-symmetry-breaking substrate. As a possible material realization, we investigate the adsorption of transition-metal atoms (Cr, Mn, Fe, or Co) on a monolayer of MoS2, WS2, or WSe2 and obtain the exchange, anisotropy, and Dzyaloshinskii-Moriya interaction parameters using first-principles calculations. Using energy minimization and parallel-tempering Monte Carlo simulations, we determine the magnetic phase diagrams for a wide range of interaction parameters. We find that skyrmion lattices can appear even with weak Dzyaloshinskii-Moriya interactions, but their stability is hindered by magnetic anisotropy. However, a weak easy …

Unbounded Derivations Of C*-Algebras And The Heisenberg Commutation Relation, Lara M. Ismert

Department of Mathematics: Dissertations, Theses, and Student Research

This dissertation investigates the properties of unbounded derivations on C*-algebras, namely the density of their analytic vectors and a property we refer to as "kernel stabilization." We focus on a weakly-defined derivation δ_D which formalizes commutators involving unbounded self-adjoint operators on a Hilbert space. These commutators naturally arise in quantum mechanics, as we briefly describe in the introduction.

A first application of kernel stabilization for δ_D shows that a large class of abstract derivations on unbounded C*-algebras, defined by O. Bratteli and D. Robinson, also have kernel stabilization. A second application of kernel stabilization provides a sufficient condition …

Free Electron Sources And Diffraction In Time, Eric R. Jones

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

The quantum revolution of the last century advanced synergistically with technology, for example, with control of the temporal and spatial coherence, and the polarization state of light. Indeed, experimental confirmation of the quirks of quantum theory, as originally highlighted by Einstein, Podolsky, and Rosen, through Bohm, and then Bell, have been performed with photons, i.e., electromagnetic wave packets prepared in the same quantum states. Experimental tests of quantum mechanics with matter wave packets have been limited due to challenges in preparing all of the packets with similar quantum states. While great strides have been made for trapped atoms and Bose-Einstein …

Testing Quantum Coherence In Stochastic Electrodynamics With Squeezed Schrödinger Cat States, Wayne Cheng-Wei Huang, Herman Batelaan

Department of Physics and Astronomy: Faculty Publications

The interference pattern in electron double-slit diffraction is a hallmark of quantum mechanics. A long-standing question for stochastic electrodynamics (SED) is whether or not it is capable of reproducing such effects, as interference is a manifestation of quantum coherence. In this study, we used excited harmonic oscillators to directly test this quantum feature in SED. We used two counter-propagating dichromatic laser pulses to promote a ground-state harmonic oscillator to a squeezed Schrödinger cat state. Upon recombination of the two well-separated wavepackets, an interference pattern emerges in the quantum probability distribution but is absent in the SED probability distribution. We thus …

Duality And Free Energy Analyticity Bounds For Few-Body Ising Models With Extensive Homology Rank, Yi Jiang, Ilya Dumer, Alexey Kovalev, Leonid Pryadko

Department of Physics and Astronomy: Faculty Publications

We consider pairs of few-body Ising models where each spin enters a bounded number of interaction terms (bonds) such that each model can be obtained from the dual of the other after freezing k spins on large-degree sites. Such a pair of Ising models can be interpreted as a two-chain complex with k being the rank of the first homology group. Our focus is on the case where k is extensive, that is, scales linearly with the number of bonds n. Flipping any of these additional spins introduces a homologically nontrivial defect (generalized domain wall). In the presence of …

Numerical And Analytical Bounds On Threshold Error Rates For Hypergraph-Product Codes, Alexey Kovalev, Sanjay Prabhakar, Ilya Dumer, Leonid P. Pryadko

Department of Physics and Astronomy: Faculty Publications

We study analytically and numerically decoding properties of finite-rate hypergraph-product quantum low density parity-check codes obtained from random (3,4)-regular Gallager codes, with a simple model of independent X and Z errors. Several nontrivial lower and upper bounds for the decodable region are constructed analytically by analyzing the properties of the homological difference, equal minus the logarithm of the maximum-likelihood decoding probability for a given syndrome. Numerical results include an upper bound for the decodable region from specific heat calculations in associated Ising models and a minimum-weight decoding threshold of approximately 7%.

Distance Verification For Classical And Quantum Ldpc Codes, Ilya Dumer, Alexey Kovalev, Leonid P. Pryadko

Department of Physics and Astronomy: Faculty Publications

The techniques of distance verification known for general linear codes are first applied to the quantum stabilizer codes. Then, these techniques are considered for classical and quantum (stabilizer) low-density-parity-check (LDPC) codes. New complexity bounds for distance verification with provable performance are derived using the average weight spectra of the ensembles of LDPC codes. These bounds are expressed in terms of the erasure-correcting capacity of the corresponding ensemble. We also present a new irreducible-cluster technique that can be applied to any LDPC code and takes advantage of parity-checks’ sparsity for both the classical and quantum LDPC codes. This technique reduces complexity …

Two-Color Multiphoton Emission From Nanotips, Wayne Cheng-Wei Huang, Maria Becker, Joshua Beck, Herman Batelaan

Department of Physics and Astronomy: Faculty Publications

Two-color multiphoton emission from polycrystalline tungsten nanotips has been demonstrated using two-color laser fields. The two-color photoemission is assisted by a three-photon multicolor quantum channel, which leads to a twofold increase in quantum efficiency. Weak-field control of two- color multiphoton emission was achieved by changing the efficiency of the quantum channel with pulse delay. The result of this study complements two-color tunneling photoemission in strong fields, and has potential applications for nanowire-based photonic devices. Moreover, the demonstrated two-color multiphoton emission may be important for realizing ultrafast spin-polarized electron sources via optically injected spin current.

On The Ising Character Of The Quantum-Phase Transition In Lihof4, Ralph Skomski

Ralph Skomski Publications

It is investigated how a transverse magnetic field affects the quantum-mechanical character of LiHoF₄, a system generally considered as a textbook example for an Ising-like quantum-phase transition. In small magnetic fields, the low-temperature behavior of the ions is Ising-like, involving the nearly degenerate low-lying J_z = ± 8 doublet. However, as the transverse field increases, there is a substantial admixture of states having | J_z | < 8. Near the quantum-phase-transition field, the system is distinctively non-Ising like, and all J_z eigenstates yield ground-state contributions of comparable magnitude. A classical analog to this mechanism is the micromagnetic single point in magnets with uniaxial anisotropy. Since Ho³⁺ has …

Event Generator Tunes Obtained From Underlying Event And Multiparton Scattering Measurements, Cms Collaboration, Ekaterina Cms Avdeeva, Kenneth A. Bloom, S. Bose, Daniel Claes, Aaron Dominguez, Caleb Fangmeier, Rebeca Gonzalez Suarez, Rami Kamalieddin, J. Keller, D. Knowlton, Ilya Kravchenko, F. Meier, Jose Monroy, F. Ratnikov, J. E. Siado, Gregory Snow

Kenneth Bloom Publications

New sets of parameters (“tunes”) for the underlying-event (UE) modelling of the PYTHIA8, PYTHIA6 and HERWIG++ MonteCarlo event generators are constructed using different parton distribution functions. Combined fits to CMS UE proton–proton (pp) data at √s = 7 TeV and to UE proton–antiproton (pp) data from the CDF experiment at lower √s, are used to study the UE models and constrain their parameters, providing thereby improved predictions for proton–proton collisions at 13 TeV. In addition, it is investigated whether the values of the parameters obtained from fits to UE observables are consistent with the values determined from fitting observables sensitive …

Measurement Of The Differential Cross Section And Charge Asymmetry For Inclusive Pp → W± + X Production At √S = 8 Tev, Ekaterina Avdeeva, Rachel Bartek, Kenneth A. Bloom, Suvadeep Bose, Daniel R. Claes, Aaron Dominguez, Caleb Fangmeier, Rebeca Gonzalez Suarez, Rami Kamalieddin, Daniel Knowlton, Ilya Kravchenko, Jose Monroy, F. Meier, F. Ratnikov, J. E. Siado, Gregory Snow, B. Stieger, Cms Collaboration

Department of Physics and Astronomy: Faculty Publications

The differential cross section and charge asymmetry for inclusive pp → W^± + X → μ^±ν + X production at √s = 8 TeV are measured as a function of muon pseudorapidity. The data sample corresponds to an integrated luminosity of 18.8 fb⁻¹ recorded with the CMS detector at the LHC. These results provide important constraints on the parton distribution functions of the proton in the range of the Bjorken scaling variable x from 10⁻³ to 10⁻¹.

Momentum Exchange In The Electron Double-Slit Experiment, Herman Batelaan, Eric Jones, Wayne Cheng-Wei Huang, Roger Bach

Department of Physics and Astronomy: Faculty Publications

We provide support for the claim that momentum is conserved for individual events in the electron double slit experiment. The natural consequence is that a physical mechanism is responsible for this momentum exchange, but that even if the fundamental mechanism is known for electron crystal diffraction and the Kapitza–Dirac effect, it is unknown for electron diffraction from nano-fabricated double slits. Work towards a proposed explanation in terms of particle trajectories affected by a vacuum field is discussed. The contentious use of trajectories is discussed within the context of oil droplet analogues of double slit diffraction.

Spin-Dependent Two-Color Kapitza-Dirac Effects, Scot Mcgregor, Wayne Cheng-Wei Huang, Herman Batelaan, Bradley Allan Shadwick

Department of Physics and Astronomy: Faculty Publications

In this paper we present an analysis of the spin behavior of electrons propagating through a laser field. We present an experimentally realizable scenario in which spin-dependent effects of the interaction between the laser and the electrons are dominant. The laser interaction strength and incident electron velocity are in the nonrelativistic domain. This analysis may thus lead to novel methods of creating and characterizing spin-polarized nonrelativistic femtosecond electron pulses.

Discrete Excitation Spectrum Of A Classical Harmonic Oscillator In Zero-Point Radiation, Wayne Cheng-Wei Huang, Herman Batelaan

Department of Physics and Astronomy: Faculty Publications

We report that upon excitation by a single pulse, a classical harmonic oscillator immersed in the classical electromagnetic zero-point radiation exhibits a discrete harmonic spectrum in agreement with that of its quantum counterpart. This result is interesting in view of the fact that the vacuum field is needed in the classical calculation to obtain the agreement.

Thresholds For Correcting Errors, Erasures, And Faulty Syndrome Measurements In Degenerate Quantum Codes, Ilya Dumer, Alexey Kovalev, Leonid P. Pryadko

Department of Physics and Astronomy: Faculty Publications

We suggest a technique for constructing lower (existence) bounds for the fault-tolerant threshold to scalable quantum computation applicable to degenerate quantum codes with sublinear distance scaling. We give explicit analytic expressions combining probabilities of erasures, depolarizing errors, and phenomenological syndrome measurement errors for quantum low-density parity-check codes with logarithmic or larger distances. These threshold estimates are parametrically better than the existing analytical bound based on percolation.

Spin Glass Reflection Of The Decoding Transition For Quantum Error Correcting Codes, Alexey Kovalev, Leonid P. Pryadko

Department of Physics and Astronomy: Faculty Publications

We study the decoding transition for quantum error correcting codes with the help of a mapping to random-bond Wegner spin models. Families of quantum low density parity-check (LDPC) codes with a finite decoding threshold lead to both known models (e.g., random bond Ising and random plaquette Z₂ gauge models) as well as unexplored earlier generally non-local disordered spin models with non-trivial phase diagrams. The decoding transition corresponds to a transition from the ordered phase by proliferation of "post-topological" extended defects which generalize the notion of domain walls to non-local spin models. In recently discovered quantum LDPC code families with …

Demonstrating Entanglement By Testing Bell's Theorem In Majorana Wires, David E. Drummond, Alexey Kovalev, Chang-Yu Hou, Kirill Shtengel, Leonid P. Pryadko

Department of Physics and Astronomy: Faculty Publications

We propose an experiment that would establish the entanglement of Majorana zero modes in semiconductor nanowires by testing the Bell and Clauser-Horne-Shimony-Holt inequalities. Our proposal is viable with realistic system parameters, simple “keyboard” gating, and projective measurement. Theoretical models and simulation results indicate entanglement can be demonstrated with moderately accurate gate operations. In addition to providing further evidence for the existence of the Majorana bound states, our proposal could be used as an experimental stepping stone to more complicated braiding experiments.

Parafermion Stabilizer Codes, Utkan Güngördü, Rabindra Nepal, Alexey Kovalev

Department of Physics and Astronomy: Faculty Publications

We define and study parafermion stabilizer codes, which can be viewed as generalizations of Kitaev’s onedimensional (1D) model of unpaired Majorana fermions. Parafermion stabilizer codes can protect against lowweight errors acting on a small subset of parafermion modes in analogy to qudit stabilizer codes. Examples of several smallest parafermion stabilizer codes are given. A locality-preserving embedding of qudit operators into parafermion operators is established that allows one to map known qudit stabilizer codes to parafermion codes. We also present a local 2D parafermion construction that combines topological protection of Kitaev’s toric code with additional protection relying on parity conservation.

Numerical Techniques For Finding The Distances Of Quantum Codes, Ilya Dumer, Alexey Kovalev, Leonid P. Pryadko

Department of Physics and Astronomy: Faculty Publications

We survey the existing techniques for calculating code distances of classical codes and apply these techniques to generic quantum codes. For classical and quantum LDPC codes, we also present a new linked-cluster technique. It reduces complexity exponent of all existing deterministic techniques designed for codes with small relative distances (which include all known families of quantum LDPC codes), and also surpasses the probabilistic technique for sufficiently high code rates.

Dynamics Underlying The Gaussian Distribution Of The Classical Harmonic Oscillator In Zero-Point Radiation, Wayne Cheng-Wei Huang, Herman Batelaan

Department of Physics and Astronomy: Faculty Publications

Stochastic electrodynamics (SED) predicts a Gaussian probability distribution for a classical harmonic oscillator in the vacuum field. This probability distribution is identical to that of the ground state quantum harmonic oscillator. Thus, the Heisenberg minimum uncertainty relation is recovered in SED. To understand the dynamics that give rise to the uncertainty relation and the Gaussian probability distribution, we perform a numerical simulation and follow the motion of the oscillator. The dynamical information obtained through the simulation provides insight to the connection between the classic double-peak probability distribution and the Gaussian probability distribution. A main objective for SED research is to …

Electron-Phonon Coupling And Structural Phase Transitions On Au/Mo(112), Keisuke Fukutani

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

The electronic structures, many-body interactions and Fermi surface topologies of Au/Mo(112) were investigated in detail and were found to play important roles in the newly discovered order-disorder structural phase transition of the system. First, the high-resolution angle-resolved photoemission spectroscopy was utilized to characterize the electronic band structure of Mo(112) in far greater details than before. This elucidated the existence of several surface-derived states and their dispersion relations in high precisions near the Fermi level, as well as the symmetries of the bulk and surface electronic states, which are in good quantitative agreement with the ab-initio calculations. Such thorough understanding of …