Open Access. Powered by Scholars. Published by Universities.®
Articles 1 - 11 of 11
Full-Text Articles in Physics
Pressure - Temperature Phase Diagram Of Crsite3, J L. Musfeldt, David Mandrus, Zhenxian Liu
Pressure - Temperature Phase Diagram Of Crsite3, J L. Musfeldt, David Mandrus, Zhenxian Liu
Chemistry Publications and Other Works
van der Waals solids are well known to host remarkable phase diagrams with competing phases, unusual energy transfer processes, and elusive states of matter. Among this class of materials, chalcogenides have emerged as the most flexible and relevant platforms for unraveling charge-structure-function relationships. In order to explore the properties of complex chalcogenides under external stimuli, we measured the far infrared spectroscopic response of CrSiTe3 under extreme pressure-temperature conditions. Analysis of the 368 cm−1 Si-Te stretching mode and the manner in which it is screened by the closure of the indirect gap reveals that the insulator-metal transition takes place immediately after …
Magnetism Of Novel Rare-Earth-Free Intermetallic Compounds, Haohan Wang
Magnetism Of Novel Rare-Earth-Free Intermetallic Compounds, Haohan Wang
Department of Physics and Astronomy: Dissertations, Theses, and Student Research
Rare-earth-free magnets have drawn lots of interest because of their low cost, and the production is not limited by the shortage of rare-earth elements. This dissertation focuses on three rare-earth-free materials, Fe-Co-Ti alloys, Fe-Ni-B alloys, and Co-Si. All of them are synthesized by arc melting followed by melt-spinning. Fe3+xCo3−xTi2 (x = 0, 2, 3) alloys exhibit hexagonal crystal structures and show non-collinear spin structures according to neutron diffraction. The magnetic moments have projections on both the c-axis and basal plane, and the corresponding misalignment angle exhibits a nonlinear decrease with …
Magnetism In Curved Geometries, R. Streubel, E. Y. Tsymbal, P. Fischer
Magnetism In Curved Geometries, R. Streubel, E. Y. Tsymbal, P. Fischer
Evgeny Tsymbal Publications
No abstract provided.
Observation Of A Pressure-Induced Transition From Interlayer Ferromagnetism To Intralayer Antiferromagnetism In Sr4Ru3O10, H. Zheng, W. H. Song, J. Terzic, H. D. Zhao, Y. F. Ni, Lance E. Delong, P. Schlottmann, G. Cao
Observation Of A Pressure-Induced Transition From Interlayer Ferromagnetism To Intralayer Antiferromagnetism In Sr4Ru3O10, H. Zheng, W. H. Song, J. Terzic, H. D. Zhao, Y. F. Ni, Lance E. Delong, P. Schlottmann, G. Cao
Physics and Astronomy Faculty Publications
Sr4Ru3O10 is a Ruddlesden-Popper compound with triple Ru-O perovskite layers separated by Sr-O rock-salt layers. This compound presents a rare coexistence of interlayer (c-axis) ferromagnetism and intralayer (basal-plane) metamagnetism at ambient pressure. Here we report the observation of pressure-induced, intralayer itinerant antiferromagnetism arising from the interlayer ferromagnetism. The application of modest hydrostatic pressure generates an anisotropy that may cause a flattening and a tilting of RuO6 octahedra. All magnetic and transport results from this study indicate these lattice distortions diminish the c-axis ferromagnetism and basal-plane metamagnetism, and induce a basal-plane antiferromagnetic state. …
Ambipolar Ferromagnetism By Electrostatic Doping Of A Manganite, L. M. Zheng, X. Renshaw Wang, W. M. Lü, C. J. Li, Tula R. Paudel, Z. Q. Liu, Z. Huang, S. W. Zeng, Kun Han, Z. H. Chen, X. P. Qiu, M. S. Li, Shize Yang, B. Yang, Matthew F. Chisholm, L. W. Martin, S. J. Pennycook, Evgeny Y. Tsymbal, J. M. D. Coey, W. W. Cao
Ambipolar Ferromagnetism By Electrostatic Doping Of A Manganite, L. M. Zheng, X. Renshaw Wang, W. M. Lü, C. J. Li, Tula R. Paudel, Z. Q. Liu, Z. Huang, S. W. Zeng, Kun Han, Z. H. Chen, X. P. Qiu, M. S. Li, Shize Yang, B. Yang, Matthew F. Chisholm, L. W. Martin, S. J. Pennycook, Evgeny Y. Tsymbal, J. M. D. Coey, W. W. Cao
Evgeny Tsymbal Publications
Complex-oxide materials exhibit physical properties that involve the interplay of charge and spin degrees of freedom. However, an ambipolar oxide that is able to exhibit both electron-doped and hole-doped ferromagnetism in the same material has proved elusive. Here we report ambipolar ferromagnetism in LaMnO3, with electron–hole asymmetry of the ferromagnetic order. Starting from an undoped atomically thin LaMnO3 film, we electrostatically dope the material with electrons or holes according to the polarity of a voltage applied across an ionic liquid gate. Magnetotransport characterization reveals that an increase of either electron-doping or hole-doping induced ferromagnetic order in this …
Suppression Of Magnetism In Ba5Alir2O11: Interplay Of Hund's Coupling, Molecular Orbitals, And Spin-Orbit Interaction, Sergey V. Streltsov, Gang Cao, Daniel I. Khomskii
Suppression Of Magnetism In Ba5Alir2O11: Interplay Of Hund's Coupling, Molecular Orbitals, And Spin-Orbit Interaction, Sergey V. Streltsov, Gang Cao, Daniel I. Khomskii
Center for Advanced Materials Faculty Publications
The electronic and magnetic properties of Ba5AlIr2O11 containing Ir-Ir dimers are investigated using the generalized gradient approximation (GGA) and GGA + spin-orbit coupling (SOC) calculations. We found that the strong suppression of the magnetic moment in this compound recently found by Terzic et al. [Phys. Rev. B 91, 235147 (2015)] is not due to charge ordering but is related to the joint effect of the spin-orbit interaction and strong covalency, resulting in the formation of metal-metal bonds. They conspire and act against the intraatomic Hund's rule exchange interaction to reduce total magnetic moment of the …
Fabrication And Study Of The Structure And Magnetism Of Rare-Earth Free Nanoclusters, Bhaskar Das
Fabrication And Study Of The Structure And Magnetism Of Rare-Earth Free Nanoclusters, Bhaskar Das
Department of Physics and Astronomy: Dissertations, Theses, and Student Research
No abstract provided.
Gapless Symmetry-Protected Topological Order, Thomas Scaffidi, Daniel E. Parker, Romain Vasseur
Gapless Symmetry-Protected Topological Order, Thomas Scaffidi, Daniel E. Parker, Romain Vasseur
Physics Department Faculty Publication Series
We introduce exactly solvable gapless quantum systems in d dimensions that support symmetry-protected topological (SPT) edge modes. Our construction leads to long-range entangled, critical points or phases that can be interpreted as critical condensates of domain walls “decorated” with dimension (d−1) SPT systems. Using a combination of field theory and exact lattice results, we argue that such gapless SPT systems have symmetry-protected topological edge modes that can be either gapless or symmetry broken, leading to unusual surface critical properties. Despite the absence of a bulk gap, these edge modes are robust against arbitrary symmetry-preserving local perturbations near the …
Ground-State Tuning Of Metal-Insulator Transition By Compositional Variations In Bair1−XRuXO3 (0 ≤ X ≤ 1), Shujuan Yuan, Kamal H. Butrouna, Jsaminka Terzic, Hao Zheng, Saicharan Aswartham, Lance E. Delong, Feng Ye, P. Schlottmann, Gang Cao
Ground-State Tuning Of Metal-Insulator Transition By Compositional Variations In Bair1−XRuXO3 (0 ≤ X ≤ 1), Shujuan Yuan, Kamal H. Butrouna, Jsaminka Terzic, Hao Zheng, Saicharan Aswartham, Lance E. Delong, Feng Ye, P. Schlottmann, Gang Cao
Physics and Astronomy Faculty Publications
Hexagonal BaIrO3 is a magnetic insulator driven by the spin-orbit interaction (SOI), whereas BaRuO3 is an enhanced paramagnetic metal. Our investigation of structural, magnetic, transport, and thermal properties reveals that substitution of Ru4+ (4d4) ions for Ir4+ (5d5) ions in BaIrO3 reduces the magnitudes of the SOI and a monoclinic structural distortion and rebalances the competition between the SOI and the lattice degrees of freedom to render an evolution from a magnetic insulting state to a robust metallic state. The central findings of this paper are as follows: (1) light …
Evolution Of Magnetism In The Single-Crystal Honeycomb Iridates (Na1−XLiX)2Iro3, Gang Cao, Tongfei Qi, L. Li, Jsaminka Terzic, Vincent Shian Cao, Shujuan Yuan, M. Tovar, Ganpathy Murthy, Ribhu K. Kaul
Evolution Of Magnetism In The Single-Crystal Honeycomb Iridates (Na1−XLiX)2Iro3, Gang Cao, Tongfei Qi, L. Li, Jsaminka Terzic, Vincent Shian Cao, Shujuan Yuan, M. Tovar, Ganpathy Murthy, Ribhu K. Kaul
Physics and Astronomy Faculty Publications
We report the successful synthesis of single crystals of the layered iridate (Na1−xLix)2IrO3, 0 ≤ x ≤ 0.9, and a thorough study of its structural, magnetic, thermal, and transport properties. This compound allows a controlled interpolation between Na2IrO3 and Li2IrO3, while maintaining the quantum magnetism of the honeycomb Ir4+ planes. The measured phase diagram demonstrates a suppression of the Néel temperature TN at an intermediate x, indicating that the magnetic orders in Na2IrO3 and Li2IrO3 …
Thermodynamics Of Magnetic Multilayers, Tathagata Mukherjee
Thermodynamics Of Magnetic Multilayers, Tathagata Mukherjee
Department of Physics and Astronomy: Dissertations, Theses, and Student Research
Our interest in thermodynamics of magnetic thin film heterostructure began by exploring the possibility to use magnetic nanostructures in the search for optimized magnetocaloric materials for potential room temperature refrigeration. In the present thesis magnetic thin film heterostructures are experimentally realized by Molecular Beam Epitaxy (MBE) and Pulsed Laser Deposition (PLD). Co/Cr and Fe/Cr superlattices were fabricated using mean-field theoretical concepts as guiding principles. The potential of artificial antiferromagnets for near room-temperature refrigeration is explored. Magnetocaloric properties are deduced from measurements of the temperature and field dependence of the magnetization of our samples. The effects of intra-plane and inter-plane exchange …