Physics Commons^™

Inductive Measurement Of Optically Hyperpolarized Phosphorous Donor Nuclei In An Isotopically Enriched Silicon-28 Crystal, P. Gumann, O. Patange, C. Ramanathan, H. Haas

Dartmouth Scholarship

We experimentally demonstrate the first inductive readout of optically hyperpolarized phosphorus-31 donor nuclear spins in an isotopically enriched silicon-28 crystal. The concentration of phosphorus donors in the crystal was 1.5×1015  cm−3, 3 orders of magnitude lower than has previously been detected via direct inductive detection. The signal-to-noise ratio measured in a single free induction decay from a 1  cm3 sample (≈1015 spins) was 113. By transferring the sample to an X-band ESR spectrometer, we were able to obtain a lower bound for the nuclear spin polarization at 1.7 K of ∼64%. The 31P-T2 measured with a Hahn echo sequence was …

Sulfur Vacancies In Photorefractive Sn2P2S6 Crystals, Eric M. Golden, Sergey A. Basun, A. A. Grabar, I. M. Stoika, Nancy C. Giles, D. R. Evans, Larry E. Halliburton

Faculty Publications

A photoinduced electron paramagnetic resonance (EPR) spectrum in single crystals of Sn2P2S6 (SPS) is assigned to an electron trapped at a sulfur vacancy. These vacancies are unintentionally present in undoped SPS crystals and are expected to play an important role in the photorefractive behavior of the material. Nonparamagnetic sulfur vacancies are formed during the initial growth of the crystal. Subsequent illumination below 100 K with 442 nm laser light easily converts these vacancies to EPR-active defects. The resulting S = 1/2 spectrum shows well-resolved and nearly isotropic hyperfine interactions with two P ions and two Sn ions. Partially resolved interactions …

Molecular Physics Of Elementary Processes Relevant To Hypersonics: Electron-Molecule Collisions, R Celiberto, V Laporta, A Laricchiuta, J Tennyson, J. M. Wadehra

Physics and Astronomy Faculty Research Publications

Non-resonant, electron-impact, vibro-electronic excitation cross sections, involving vibrationally excited N2 molecules, to the mixed valence-Rydberg b,c,o 1Πu and b′,c′,e′ 1åu+ singlet states are presented. These cross sections are calculated using the so-called similarity approach, accounting for the vibronic coupling among excited states, and compared with the experiments and different theoretical calculations.

New cross sections for the electron-impact resonant vibrational excitation of CO2 molecule are calculated, for the symmetric stretching mode, as a function of the incident electron energy and for the transitions (υ i , 0,0)→(νf , 0,0) with νi = 0,1,2 and for some selected value of νf in …

Effects Of Major Sudden Stratospheric Warmings Identified In Midlatitude Mesospheric Rayleigh-Scatter Lidar Temperatures, Leda Sox, Vincent B. Wickwar, Chad Fish, Josh Herron

Physics Student Research

Mesospheric temperature anomalies associated with Sudden Stratospheric Warmings (SSWs) have been observed extensively in the polar regions. However, observations of these anomalies at midlatitudes are sparse. The very dense 11-year data set, collected between 1993–2004, with the Rayleigh-scatter lidar at the Atmospheric Lidar Observatory (ALO; 41.7°N, 111.8°W) at the Center for Atmospheric and Space Sciences (CASS) on the campus of Utah State University (USU), has been carefully examined for such anomalies. The temperatures derived from these data extend over the mesosphere, from 45 to 90 km. During this period extensive data were acquired during seven major SSW events. In this …

Raman Microspectroscopy For The Early Detection Of Pre-Malignant Changes In Cervical Tissue, Nosheen Rashid, Haq Nawaz, Kelvin W. Poon, Franck Bonnier, Salih Bakhiet, Cara Martin, John O'Leary, Hugh Byrne, Fiona Lyng

Articles

Cervical cancer is the third most common cancer affecting women worldwide. The mortality associated with cervical cancer can, however, be significantly reduced if the disease is detected at the pre-malignant stage. The aim of this study was to evaluate the potential of Raman microspectroscopy for elucidation of the biochemical changes associated with the pre-malignant stages of cervical cancer. Formalin fixed paraffin preserved tissue sections from cervical biopsies classified as negative for intraepithelial lesion and malignancy (NILM), low grade squamous intraepithelial lesion (LSIL) or high grade squamous intraepithelial lesion (HSIL) were analysed by Raman spectral mapping. Raman mapping, with K-Means Cluster …

Light Transport In Pt-Invariant Photonic Structures With Hidden Symmetries, M. H. Teimourpour, Ramy El-Ganainy, A. Eisfeld, A. Szameit, Demetrios N. Christodoulides

Department of Physics Publications

We introduce a recursive bosonic quantization technique for generating classical PT photonic structures that possess hidden symmetries and higher order exceptional points. We study light transport in these geometries and we demonstrate that perfect state transfer is possible only for certain initial conditions. Moreover, we show that for the same propagation direction, left and right coherent transports are not symmetric with field amplitudes following two different trajectories. A general scheme for identifying the conservation laws in such PT-symmetric photonic networks is also presented.

Nonlinear Dichroism In Back-To-Back Double Ionization Of He By An Intense Elliptically Polarized Few-Cycle Extreme Ultraviolet Pulse, Jean Marcel Ngoko Djiokap, N. L. Manakov, A. V. Meremianin, S. X. Hu, L. B. Madsen, Anthony F. Starace

Anthony F. Starace Publications

Control of double ionization of He by means of the polarization and carrier-envelope phase (CEP) of an intense, few-cycle extreme ultraviolet (XUV) pulse is demonstrated numerically by solving the six-dimensional two-electron, time-dependent Schrödinger equation for He interacting with an elliptically polarized XUV pulse. Guided by perturbation theory (PT), we predict the existence of a nonlinear dichroic effect (∝ I^3/2) that is sensitive to the CEP, ellipticity, peak intensity I, and temporal duration of the pulse. This dichroic effect (i.e., the difference of the two-electron angular distributions for opposite helicities of the ionizing XUV pulse) originates from interference of …

Molecular Interactions With Ice: Molecular Embedding, Adsorption, Detection, And Release, K D. Gibson, Grant G. Langlois, Wenxin Li, Daniel Killelea, S J. Sibener

Chemistry: Faculty Publications and Other Works

The interaction of atomic and molecular species with water and ice is of fundamental importance for chemistry. In a previous series of publications, we demonstrated that translational energy activates the embedding of Xe and Kr atoms in the near surface region of ice surfaces. In this paper, we show that inert molecular species may be absorbed in a similar fashion.We also revisit Xe embedding, and further probe the nature of the absorption into the selvedge. CF4 molecules with high translational energies (≥3 eV) were observed to embed in amorphous solid water. Just as with Xe, the initial adsorption rate is …

Conservation Of The Spin And Orbital Angular Momenta In Electromagnetism, Konstantin Y. Bliokh, Justin Dressel, Franco Nori

Mathematics, Physics, and Computer Science Faculty Articles and Research

We review and re-examine the description and separation of the spin and orbital angular momenta (AM) of an electromagnetic field in free space. While the spin and orbital AM of light are not separately meaningful physical quantities in orthodox quantum mechanics or classical field theory, these quantities are routinely measured and used for applications in optics. A meaningful quantum description of the spin and orbital AM of light was recently provided by several authors, which describes separately conserved and measurable integral values of these quantities. However, the electromagnetic field theory still lacks corresponding locally conserved spin and orbital AM currents. …

Magnetic Correlations And Pairing In The 1/5-Depleted Square Lattice Hubbard Model, Ehsan Khatami, Rajiv R.P. Singh, Warren E. Pickett, Richard T. Scalettar

Faculty Publications

We study the single-orbital Hubbard model on the 1/5-depleted square-lattice geometry, which arises in such diverse systems as the spin-gap magnetic insulator CaV4O9 and ordered-vacancy iron selenides, presenting new issues regarding the origin of both magnetic ordering and superconductivity in these materials. We find a rich phase diagram that includes a plaquette singlet phase, a dimer singlet phase, a Néel and a block-spin antiferromagnetic phase, and stripe phases. Quantum Monte Carlo simulations show that the dominant pairing correlations at half filling change character from d wave in the plaquette phase to extended s wave upon transition to the Néel phase. …

Observation Of Heavy- And Light-Hole Split Direct Bandgap Photoluminescence From Tensile-Strained Gesn (0.03% Sn), Thomas R. Harris, Yung Kee Yeo, Mee-Yi Ryu, Richard T. Beeler, John Kouvetakis

Faculty Publications

Temperature- (T-) and laser power-dependent photoluminescence (PL) measurements have been made for the tensile-strained, undoped GeSn (0.03% Sn) film grown on Si substrate. The PL results show not only clear strain-split direct bandgap transitions to the light-hole (LH) and heavy-hole (HH) bands at energies of 0.827 and 0.851 eV at 10 K, respectively, but also clearly show both strong direct and indirect bandgap related PL emissions at almost all temperatures, which are rarely observed. This split of PL emissions can be directly observed only at low T and moderate laser power, and the two PL peaks merge into one broad …

Wigner High-Electron-Correlation Regime Of Nonuniform Density Systems: A Quantal-Density-Functional-Theory Study, Douglas Achan, Lou Massa, Viraht Sahni

Publications and Research

The Wigner regime of a system of electrons in an external field is characterized by a low electron density and a high electron-interaction energy relative to the kinetic energy. The low-correlation regime is in turn described by a high electron density and an electron-interaction energy smaller than the kinetic energy. The Wigner regime of a nonuniform-electron-density system is investigated via quantal density functional theory (QDFT). Within QDFT, the contributions of electron correlations due to the Pauli exclusion principle, Coulomb repulsion, and correlation-kinetic effects are separately delineated and explicitly defined. The nonuniform-electron-density system studied is that of the Hooke's atom in …

Environmental Testing Of Lasers For Jpl's Cold Atom Laboratory, Carey L. Baxter

STAR Program Research Presentations

NASA’s Cold Atom Lab (CAL) is a multi-user facility designed to study ultra-cold quantum gases in the microgravity environment of the International Space Station (ISS). One of the main goals of CAL is to explore the unknown territory of extremely low temperatures—possibly as low as the picokelvin range!—where new and fascinating quantum phenomena can be observed. At such temperatures matter stops behaving as particles and instead becomes macroscopic matter waves. CAL will be remotely controlled to perform a multitude of experiments and is scheduled to launch in 2016. In order to anticipate problems that might occur during and post-launch, including …

A Prototype Microwave Cavity Control Circuit For Use In Next Generation Free Electron Laser, Josh Thompson, Peter Neal Barrina, Jiayi Jiang, Joe Frisch, Steve Smith, Daniel Van Winkle

STAR Program Research Presentations

One of the current programs at SLAC National Accelerator Laboratory is the Linac Coherent Light Source, or LCLS. Using the existing hardware of the last third of their linear accelerator (or “linac”), SLAC has created one of the most energetic X-ray free electron lasers (or “FEL”). Since 2009, LCLS has used this FEL to perform a wide range of experiments across all sciences, most notably ultrafast filming at the molecular scale. As requests for beam-time with this laser increases, SLAC is purposing a linac upgrade to better match this demand. This upgrade, named LCLS-II, will replace existing copper radio frequency …

Does A Plastron Improve Heat Transfer?, Madani A. Khan, Jeffrey Alston, Andrew Guenthner

STAR Program Research Presentations

Superamphiphobic surfaces strongly repel both water and oils. In this work, aluminum coupons are processed by sanding with various grit of sand paper to impart microscale roughness. Subsequent submersion of the aluminum substrate in boiling water grows nanoscale grass-like structures. The oxide layer of Al is slightly soluble in water. During a fast diffusion/equilibrium, Al₂O₃ nanograss grows on the surface. A low energy coating is then deposited on the surface. The micro and nanoscale features create re-entrant structures that trap air enabling contact liquid to be in a Cassie-Baxter state. Superamphiphobicity of the samples were confirmed by …

Low-Lying Neutron Unbound States In 12be, J. K. Smith, T. Baumann, D. Bazin, J. Brown, S. Casarotto, P. A. Deyoung, N. Frank, J. Hinnefeld, M. Hoffman, M. D. Jones, Z. Kohley, B. Luther, B. Marks, N. Smith, J. Snyder, A. Spyrou, Sharon L. Stephenson, M. Thoennessen, N. Viscariello, S. J. Williams

Physics and Astronomy Faculty Publications

The neutron decay of an unbound resonance in 12Be has been measured at 1243 ± 21 keV decay energy with a width of 634 ± 60 keV. This state was populated with a one-proton removal reaction from a 71 MeV/u 13B beam incident upon a beryllium target. The invariant mass reconstruction of the resonance was achieved by measuring the daughter fragment in coincidence with neutrons. Despite being above the 2n separation energy, the state decays predominantly by the emission of one neutron to 11Be, setting an upper limit on the branching ratio for the two-neutron decay channel to 10Be of …

Exceptional Points And Lasing Self-Termination In Photonic Molecules, Ramy El-Ganainy, M. Khajavikhan, Li Ge

Department of Physics Publications

We investigate the rich physics of photonic molecule lasers using a non-Hermitian dimer model.We show that several interesting features, predicted recently using a rigorous steady-state ab initio laser theory (SALT), can be captured by this toy model. In particular, we demonstrate the central role played by exceptional points (EPs) in both pump-selective lasing and laser self-termination phenomena. Due to its transparent mathematical structure, our model provides a lucid understanding for how different physical parameters (optical loss, modal coupling between microcavities, and pump profiles) affect the lasing action. Interestingly, our analysis also confirms that, for frequency mismatched cavities, operation in the …

Copper Doping Of Zno Crystals By Transmutation Of 64Zn To 65Cu: An Electron Paramagnetic Resonance And Gamma Spectroscopy Study, Matthew C. Recker, John W. Mcclory, Maurio S. Holston, Eric M. Golden, Nancy C. Giles, Larry E. Halliburton

Faculty Publications

Transmutation of ⁶⁴Zn to ⁶⁵Cu has been observed in a ZnO crystal irradiated with neutrons. The crystal was characterized with electron paramagnetic resonance (EPR) before and after the irradiation and with gamma spectroscopy after the irradiation. Major features in the gamma spectrum of the neutron-irradiated crystal included the primary 1115.5 keV gamma ray from the ⁶⁵Zn decay and the positron annihilation peak at 511 keV. Their presence confirmed the successful transmutation of ⁶⁴Zn nuclei to ⁶⁵Cu. Additional direct evidence for transmutation was obtained from the EPR of Cu²⁺ ions (where ⁶³Cu and ^{65 …}

Monte Carlo Simulations Of Atmospheric Loss By Stellar Winds From Exoplanets, Daniel P. Violette

University Scholar Projects

Hot Jupiters are a class of extra-solar planets. Massive gas giants on the same size scale as Jupiter, they orbit their host stars closely. This proximity results in large stellar winds capable of stripping away a planet’s atmosphere. Developing a more complete understanding of atmospheric mass loss and evolution in planetary bodies is critical, and Hot Jupiter systems are accessible analogues.

This project will seek to create a computational model capable of estimating mass loss rates due to stellar winds. A Monte Carlo method is utilized to take an ensemble of single, high-energy energetic neutral particles, produced by kilo-electronvolt stellar …

Monte Carlo Simulations Of Atmospheric Loss By Stellar Winds From Exoplanets, Daniel Violette

Honors Scholar Theses

Hot Jupiters are a class of extra-solar planets. Massive gas giants on the same size scale as Jupiter, they orbit their host stars closely. This proximity results in large stellar winds capable of stripping away a planet’s atmosphere. Developing a more complete understanding of atmospheric mass loss and evolution in planetary bodies is critical, and Hot Jupiter systems are accessible analogues.

This project will seek to create a computational model capable of estimating mass loss rates due to stellar winds. A Monte Carlo method is utilized to take an ensemble of single, high-energy energetic neutral particles, produced by kilo-electronvolt stellar …

Photoelectron Spectroscopy Of Boron Aluminum Hydride Cluster Anions, Haopeng Wang, Xinxing Zhang, Yeon Je Ko, Gerd Gantefoer, Kit H. Bowen, Xiang Li, Boggavarapu Kiran, Anil K. Kandalam

Physics & Engineering Faculty Publications

No abstract provided.

Electron Matter Interferometry And The Electron Double-Slit Experiment, Roger Bach

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

Quantum mechanics has fundamentally changed the way scientists think about the world. Quantum mechanical theory has found it's way into our everyday lives through advances in technology. In this dissertation a fundamental quantum mechanical demonstration and the technological development of a new quantum mechanical device are presented.

Double-slit diffraction is a corner stone of quantum mechanics. It illustrates key features of quantum mechanics: interference and the particle-wave duality of matter. Here we demonstrate the full realization of Richard Feynman's famous thought experiment. By placing a movable mask in front of a double-slit to control the transmission through the individuals slits. …

X-Ray Second Harmonic Generation, S. Shwartz, Matthias Fuchs, J. B. Hastings, Y. Inubushi, T. Ishikawa, T. Katayama, D. A. Reis, T. Sato, K. Tono, M. Yabashi, S. Yudovich, S. E. Harris

Matthias Fuchs Publications

We report clear experimental evidence for second harmonic generation at hard x-ray wavelengths. Using a 1.7 Å pumping beam generated by a free electron laser, we observe second harmonic generation in diamond. The generated second harmonic is of order 10 times the background radiation, scales quadratically with pump pulse energy, and is generated over a narrow phase-matching condition. Of importance for future experiments, our results indicate that it is possible to observe nonlinear x-ray processes in crystals at pump intensities exceeding 10¹⁶ W/cm².

Supersymmetric Mode Converters, Matthias Heinrich, Mohammad-Ali Miri, Simon Stützer, Ramy El-Ganainy, Stefan Nolte, Alexander Szameit, Demetrios N. Christodoulides

Department of Physics Publications

Originally developed in the context of quantum field theory, the concept of supersymmetry can be used to systematically design a new class of optical structures. In this work, we demonstrate how key features arising from optical supersymmetry can be exploited to control the flow of light for mode division multiplexing applications. Superpartner configurations are experimentally realized in coupled optical networks, and the corresponding light dynamics in such systems are directly observed. We show that supersymmetry can be judiciously utilized to remove the fundamental mode of a multimode optical structure, while establishing global phase matching conditions for the remaining set of …

Hydration Of The Sulfuric Acid−Methylamine Complex And Implications For Aerosol Formation, Danielle J. Bustos, Berhane Temelso, George C. Shields

Faculty Journal Articles

The binary H₂SO₄−H₂O nucleation is one of the most important pathways by which aerosols form in the atmosphere, and the presence of ternary species like amines increases aerosol formation rates. In this study, we focus on the hydration of a ternary system of sulfuric acid (H₂SO₄), methylamine (NH₂CH₃), and up to six waters to evaluate its implications for aerosol formation. By combining molecular dynamics (MD) sampling with high-level ab initio calculations, we determine the thermodynamics of forming H₂SO₄(NH₂CH₃)(H …

The Viability Of Aluminum Zintl Anion Moieties Within Magnesium-Aluminum Clusters, Haopeng Wang, Yeon Jae Ko, Xinxing Zhang, Gerd Gantefoer, Hansgeorg Schnoeckel, Bryan W. Eichhorn, Puru Jena, Boggavarapu Kiran, Anil K. Kandalam, Kit H. Bowen Jr.

Physics & Engineering Faculty Publications

No abstract provided.

In-Package Atmospheric Pressure Cold Plasma Treatment Of Cherry Tomatoes, N. Misra, Kevin Keener, Paula Bourke, J Mosnier, Patrick Cullen

Articles

Cold plasma is increasingly under research for decontamination of foods, especially fresh fruits and vegetables. The effect of cold plasma on food quality, however, remains under researched. This study investigates the effects of cold plasma generated within a sealed package from a dielectric barrier discharge on the physical quality parameters and respiration rates of cherry tomatoes. Respiration rates and weight loss were monitored continuously, while other parameters are reported at the end of storage period. Differences among weight loss, pH and firmness for control and treated cherry tomatoes were insignificant towards the end of storage life. Changes in respiration rates …

Triplet Ground State Of The Neutral Oxygen-Vacancy Donor In Rutile Tio2, A. T. Brant, Eric M. Golden, Nancy C. Giles, Shan Yang, M. A. R. Sarker, S. Watauchi, M. Nagao, I. Tanaka, D. A. Tryk, A. Manivannan, Larry E. Halliburton

Faculty Publications

Electron paramagnetic resonance (EPR) is used to investigate the triplet (S = 1) ground state of the neutral oxygen vacancy in bulk rutile TiO₂ crystals. This shallow donor consists of an oxygen vacancy with two nearest-neighbor, exchange-coupled ³⁺ ions located along the [001] direction and equidistant from the vacancy. The spins of the two trapped electrons, one at each ³⁺ ion, align parallel to give the S = 1 state. These neutral oxygen vacancies are formed near 25 K in as-grown oxidized TiO₂ crystals by illuminating with sub-band-gap 442 nm laser light. The angular dependence of the EPR …

Neutral Nitrogen Acceptors In Zno: The 67Zn Hyperfine Interactions, Eric M. Golden, S. M. Evans, Larry E. Halliburton, Nancy C. Giles

Faculty Publications

Electron paramagnetic resonance (EPR) is used to characterize the ⁶⁷Zn hyperfine interactions associated with neutral nitrogen acceptors in zinc oxide. Data are obtained from an n-type bulk crystal grown by the seeded chemical vapor transport method. Singly ionized nitrogen acceptors (N⁻) initially present in the crystal are converted to their paramagnetic neutral charge state (N⁰) during exposure at low temperature to 442 or 633 nm laser light. The EPR signals from these N⁰ acceptors are best observed near 5 K. Nitrogen substitutes for oxygen ions and has four nearest-neighbor cations. The zinc ion …

Development Of High-Purity Optical Grade Single-Crystal Cvd Diamond For Intracavity Cooling, Andrew M. Bennett, Benjamin J. Wickham, Harpreet K. Dhillon, Ying Chen, Scott Webster, Giorgio Turri, Michael Bass

Publications

Microwave assisted chemical vapour deposited bulk diamond products have been used in a range of high power laser systems, due to low absorption across a range of wavelengths and exceptional thermal properties. However the application of polycrystalline products has frequently been limited to applications at longer wavelengths or thermal uses outside of the optical path due to the birefringence and scatter that are intrinsic properties of the polycrystalline materials. However, there are some solid state structures, including thin disc gain modules and amplifiers, that will gain significantly in terms of potential output powers if diamond could be used as a …