Physics Commons^™

Atomic-Level Mechanisms Of Fast Relaxation In Metallic Glasses, Leo W. Zella

Doctoral Dissertations

Glasses are ubiquitous in daily life and have unique properties which are a consequence of the underlying disordered structure. By understanding the fundamental processes that govern these properties, we can modify glasses for desired applications. Key to understanding the structure-dynamics relationship in glasses is the variety of relaxation processes that exist below the glass transition temperature. Though these relaxations are well characterized with macroscopic experimental techniques, the microscopic nature of these relaxations is difficult to elucidate with experimental tools due to the requirements of timescale and spatial resolution. There remain many questions regarding the microscopic nature of relaxation in glass …

A Measurement Of Neutron Polarization And Transmission For The Nedm@Sns Experiment, Kavish Imam

Doctoral Dissertations

The D.O.E Nuclear Science Advisory Committee Long Range Plan has called for experimental programs to explore fundamental symmetry violations and their implications in nuclear, particle and cosmological physics. The neutron electric dipole moment experiment at the Spallation Neutron Source (nEDM@SNS) aims to search for new physics in the Time-reversal (T) and Charge-Parity (CP) symmetry violating sector by setting a new limit on the nEDM down to a few x 10^-28 e·cm using a novel cryogenic technique, which combines the unique properties of polarized Ultracold Neutrons (UCN), polarized ³He, and superfluid ⁴He. The experiment will employ a cryogenic …

Short Range Correlation Measurements In The Quasielastic Region With An 11 Gev Beam, Casey Morean

Doctoral Dissertations

Electron scattering is a significant means of studying internal high momentum
nucleon and quark distributions in nuclei. Thomas Jefferson National Accelerator
Facility (JLab) with its 11GeV beam is capable of studying high momentum nucleons
with unmatched precision. The role of short range nucleon configurations and
quark distributions is significant for understanding the dynamics of nuclei and their
underlying components. Scattering cross section measurements in the kinematic
regime x > 1, where the free nucleon is forbidden, are sensitive to high momentum
nucleons, which are believed to come from short range correlations (SRCs). SRCs are
strongly interacting, high momentum nucleons with a …

Generative Adversarial Game With Tailored Quantum Feature Maps For Enhanced Classification, Anais Sandra Nguemto Guiawa

Doctoral Dissertations

In the burgeoning field of quantum machine learning, the fusion of quantum computing and machine learning methodologies has sparked immense interest, particularly with the emergence of noisy intermediate-scale quantum (NISQ) devices. These devices hold the promise of achieving quantum advantage, but they grapple with limitations like constrained qubit counts, limited connectivity, operational noise, and a restricted set of operations. These challenges necessitate a strategic and deliberate approach to crafting effective quantum machine learning algorithms.

This dissertation revolves around an exploration of these challenges, presenting innovative strategies that tailor quantum algorithms and processes to seamlessly integrate with commercial quantum platforms. A …

Dinitrogen Functionalization Using A Molybdenum Atom: Bridging The Gap Between Small And Coordination Complexes Via Quantum Mechanical Methods, Maria Virginia White

Doctoral Dissertations

Chemistry devotes a significant amount of its research to understanding small molecule activation from an electronic structure perspective to help with the investigation of the reaction pathways of catalytically active substances that can promote biomimetic catalysis. A large portion of the energy used annually in our planet is used for the artificial nitrogen fixation (Haber-Bosch process), which renders dinitrogen activation a subject of study. Molybdenum, a fourth row transitional metal, has demonstrated its effectiveness as an essential component of the dinitrogen reduction catalytic process. To better understand the multiple dinitrogen molybdenum binding modes, the work described herein combines wave function …

Chirality, Symmetry-Breaking, And Chemical Substitution In Multiferroics, Kiman Park

Doctoral Dissertations

Multiferroic materials attract significant attention due to their potential utility in a broad range of device applications. The inclusion of heavy metal centers in these materials enhances their magnetoelectric properties, yielding fascinating physical phenomena such as the Dzyaloshinskii–Moriya interaction, nonreciprocal directional dichroism, enhancement of spin-phonon coupling, and spin-orbit-entangled ground states. This dissertation provides a comprehensive survey of magnetoelectric multiferroics containing heavy metal centers and explores spectroscopic techniques under extreme conditions. A microscopic examination of phase transitions, symmetry-breaking, and structure-property relationships enhances the fundamental understanding of coupling mechanisms.

In A2Mo3O8 (A = Fe, Zn, Ni, and Mn), we use optical spectroscopy …

Exploring Skyrmions Dynamics And Structure Using Neutron Scattering, W-L-Namila Chandula Liyanage

Doctoral Dissertations

Magnetic skyrmions are topologically protected chiral spin textures with great potential for next-generation consumer technologies. These magnetic structures can be described as spins continuously wrapping into a closed coplanar loop, featuring a core and fencing perimeter with opposite out-of-plane orientations. While conventional depictions of magnetic skyrmions use a two-dimensional projection, recent research underscores the importance of their three-dimensional structure in determining their topology and stability. Magnetic skyrmions typically emerge just below the curie temperature of a magnetic material, creating what is known as a skyrmion pocket. In most materials the stability pocket is at low temperatures and finite fields, however …

Sub-Chandrasekhar Type Ia Supernovae Scenarios With Increased Pathways For Neutronization, Fernando Hernan Rivas

Doctoral Dissertations

Type Ia supernovae are thermonuclear explosions of white dwarfs (WD), electron-degenerate cores of old intermediate mass stars(under 8$M_{\odot}$). Reaching energies of $10^{51}$\si{\erg}, they outshine whole galaxies as they synthesize and distribute most of the iron group elements (IGE; V, Cr, Mn, Fe, Co, Ni) into the interstellar medium, thus being one of the main agents in cosmic chemical evolution. Also, given their notably homogeneous lightcurves, they form the last step in the cosmic distance ladder outdistancing Cepheid variables by orders of magnitude. Though calibration of said lightcurves is dependent on a high number of confirmed events, the limits of statistical …

Fabrication, Measurements, And Modeling Of Semiconductor Radiation Detectors For Imaging And Detector Response Functions, Corey David Ahl

Doctoral Dissertations

In the first part of this dissertation, we cover the development of a diamond semiconductor alpha-tagging sensor for associated particle imaging to solve challenges with currently employed scintillators. The alpha-tagging sensor is a double-sided strip detector made from polycrystalline CVD diamond. The performance goals of the alpha-tagging sensor are 700-picosecond timing resolution and 0.5 mm spatial resolution. A literature review summarizes the methodology, goals, and challenges in associated particle imaging. The history and current state of alpha-tagging sensors, followed by the properties of diamond semiconductors are discussed to close the literature review. The materials and methods used to calibrate the …

Path Integral Monte Carlo For Entanglement In Bosonic Lattices At T = 0, Emanuel Casiano-Diaz

Doctoral Dissertations

Path-Integral Monte Carlo Worm Algorithm is one of many Quantum Monte Carlo (QMC) methods that serve as powerful tools for the simulation of quantum many-body systems. Developed in the late 90’s, this algorithm has been used with great success to study a wide array of physical models where exact calculation of observables is not possible due to the exponential size of the Hilbert space. One type of systems that have eluded PIMC-WA implementation are lattice models at zero temperature, which are of relevance in experimental settings, such as in optical lattices of ultra-cold atoms. In this thesis, we develop a …

Pointing Control And Stabilization Of The High-Energy Uv Laser For Laser-Assisted Charge Exchange, Martin Joseph Kay

Doctoral Dissertations

Laser-Assisted Charge Exchange (LACE) is an experimental method of charge exchange injection into a proton accumulator ring that is being developed at the Spallation Neutron Source (SNS) in Oak Ridge National Laboratory (ORNL) as an alternative to hazardous injection foils. The current scheme of LACE requires a high-energy, low-repetition-rate UV (355 nm) laser beam (140 mJ pulses at 10 Hz) to be transported over 65 meters to the laser-particle interaction point (IP) in a high-radiation area of the accelerator. Thermal effects and other disturbances along the free-space laser transport line cause the beam to slowly drift away from the IP …

Total Absorption Spectroscopy Of Mo-106 And Tc-106, Michael Cooper

Doctoral Dissertations

Total absorption spectroscopy is a method of gamma-ray spectroscopy that has gained prominence in the past several decades, as nuclear data revisions are performed on older nuclear data, which is often incomplete. A strong understanding of underlying nuclear data, particularly fission and beta decay data, is essential for nuclear reactors and nuclear fuel decay heat. This PhD work involves the analysis of fission fragments 106Mo [Mo-106] and 106Tc [Tc-106]. These neutron rich isotopes contribute upwards of 6% of the cumulative fission yield of 241Pu [Pu-241] fission, and 4% of 239Pu [Pu-239] fission. Prior data for these two fission fragments only …

Unlocking The Potential Of Machine Learning In The Derivation Of Low-Energy Models For Metallic Magnets, Vikram Sharma

Doctoral Dissertations

Condensed matter physics often grapples with complex many-particle problems lacking definitive closed-form solutions, necessitating approximation strategies to investigate low-energy sectors of the Hilbert space. Perturbation theory, though widely used for this purpose, is limited when expansion terms diverge. This work introduces a machine learning (ML) assisted protocol to extract effective low-energy models for lattice models of fermions interacting with classical fields, specifically focusing on the Kondo Lattice Model (KLM).

Skyrmions, featuring whirling spin texture and topological protection, are promising candidates for future spintronic devices. Materials featuring conduction electrons coupled to localized $f$-electrons' net moment are ideal for realizing skyrmions and …

Neutrino Physics At A Research Reactor: Backgrounds And Analysis, Blaine Alexander Heffron

Doctoral Dissertations

The field of neutrino physics has a rich history and is currently the subject of much active research. The discovery of neutrino oscillations led to the conclusion that neutrinos have mass which was in contradiction to the Standard Model. Now researchers are investigating a number of open questions regarding neutrino properties such as their mass values or the existence of CP violation in the weak interaction. In order to answer these questions experimental and analytical techniques of neutrino detection are becoming more advanced, entering into an era of precision neutrino detection.

Nuclear reactors as a source of antineutrinos have played …

Core-Collapse Supernova Simulations With Spectral Two-Moment Neutrino Transport, Ran Chu

Doctoral Dissertations

The primary focus of this dissertation is to develop a next-generation, state-of-the-art neutrino kinetics capability that will be used in the context of the next-generation, state-of-the-art core-collapse supernova (CCSN) simulation frameworks \thornado\ and \FLASH.\index{CCSN} \thornado\ is a \textbf{t}oolkit for \textbf{h}igh-\textbf{or}der \textbf{n}eutrino-r\textbf{ad}iation hydr\textbf{o}dynamics, which is a collection of modules that can be incorporated into a simulation code/framework, such as \FLASH, together with a nuclear equation of state (EOS)\index{EOS} library, such as the \WeakLib\ EOS tables. The first part of this work extends the \WeakLib\ code to compute neutrino interaction rates from~\cite{Bruenn_1985} and produce corresponding opacity tables.\index{Bruenn 1985} The processes of emission, …

Development Of A New High-Resolution Neutron Detector And Beta-Delayed Neutron Spectroscopy Of 24o., Shree K. Neupane

Doctoral Dissertations

An efficient neutron detection system with good energy resolution is needed to correctly characterize the decays of neutron-rich nuclei where beta-delayed neutron emission is a dominant decay mode. Precision neutron spectroscopy probes nuclear structure effects in neutron-rich nuclei and is essential to exploit the opportunities in new-generation radioactive beam facilities. A new high-resolution neutron detector, Neutron dEtector with Xn Tracking (NEXT), has been constructed, characterized, and tested in decay and reaction experiments. Its essential capability is the neutron interaction position localization, which enables improvement in energy resolution without compromising detection efficiency in the time-of-flight measurements. Neutron-gamma discrimination capability of NEXT …

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Constraining The 30p(P,Γ)31s Reaction Using 30p(D,Pγ)31p With Goddess, Rajesh Ghimire

Doctoral Dissertations

The ³⁰P(p,γ)³¹S reaction acts as a bottleneck for classical nova nucleosynthesis beyond A=30 in ONe novae, due in part to the long lifetime of ³⁰P (∼2.5 minutes) with respect to the timescale of a nova outburst. Also, the ³⁰P(p,γ)³¹S reaction rate directly affects the isotopic ratio of ³⁰Si/²⁸Si, which is an important nova identifier in the analysis of pre-solar grains. O/S, S/Al, O/P, and P/Al elemental abundance ratios can be used as nuclear thermometers for classical novae by constraining the ³⁰P(p,γ)³¹S reaction rate.

However, direct measurement of …

The Impact Of A Nuclear Disturbance On A Space-Based Quantum Network, Alexander Miloshevsky

Doctoral Dissertations

Quantum communications tap into the potential of quantum mechanics to go beyond the limitations of classical communications. Currently, the greatest challenge facing quantum networks is the limited transmission range of encoded quantum information. Space-based quantum networks offer a means to overcome this limitation, however the performance of such a network operating in harsh conditions is unknown. This dissertation analyzes the capabilities of a space-based quantum network operating in a nuclear disturbed environment. First, performance during normal operating conditions is presented using Gaussian beam modeling and atmospheric modeling to establish a baseline to compare against a perturbed environment. Then, the DEfense …

Imaging Normal Fluid Flow In He Ii With Neutrons And Lasers — A New Application Of Neutron Beams For Studies Of Turbulence, Xin Wen

Doctoral Dissertations

Turbulence is ubiquitous in life —from biology to astrophysics. The best direct numeric simulations (DNS) have only been benchmarked against low resolution, time-averaged experimental configurations—partly because of limitations in computing power. With time, computing power has greatly increased, so there is need for higher quality data of turbulent flow. In this dissertation, we explore a solution that enables quantitative visualization measurement of the velocity field in liquid helium, which has the potential of breaking new ground for high Reynolds number turbulence research and model testing.

Our technique involves creation of clouds of molecular tracers using 3He-neutron absorption reaction in liquid …

The Structure Of 71ni Via Beta-Delayed Neutron Spectroscopy Of 71co, Andrew Keeler

Doctoral Dissertations

Studies of beta decays can give insights into the underlying structure of the nucleus. In particular, decays of closed-shell and near-closed-shell nuclei can provide important benchmarks for structure models, which are used in simulations of r-process nucleosynthesis. This work reports on a study of beta decays of ⁷¹Co produced in an experiment that was carried out in October 2016 at MSU’s National Superconducting Cyclotron Laboratory (NSCL) using the Versatile Array of Neutron Detectors at Low Energy (VANDLE). In order to carry out this experiment, a novel position-sensitive scintillating detector was developed to enable the sub-nanosecond timing response that VANDLE …

Understanding Liquid Dynamics Using The Van Hove Function From Inelastic Neutron Scattering Measurements, Yadu Krishnan Sarathchandran

Doctoral Dissertations

Liquid state physics remains relatively unexplored compared to solid-state physics, which achieved massive progress over the last century. The theoretical and experimental methodologies used in solid-state physics are not suitable to study the liquid state due to the latter's strong time dependence and the lack of periodicity in structure. The approaches based on phonon dynamics break down when phonons are over-damped and localized in liquids. The microscopic nature of atomic dynamics and many-body interactions leading to liquid state properties such as viscosity and dielectric loss in liquids remain unclear. Inelastic neutron scattering measurements were done to study the microscopic origins …

Studying Electron Dynamics For Quantum Materials With Real Space Resolution: A Wannier Orbital Approach To Spectroscopy Using High-Performance Supercomputers, Casey J. Eichstaedt

Doctoral Dissertations

Quantum materials have a promising future for energy and security applications which will lay the bedrock for material science research for decades to follow. Partic- ularly, ‘one-dimensional’ Mott-insulating cuprates such as SrCuO 2 and (Ca)Sr 2 CuO 3 have been deemed to fall under a ‘fractionalization’ paradigm in which the electrons disintegrate into bosonic collective excitations of their fundamental constituents— spin, charge, and ‘orbital’ degrees of freedom— due to the anisotropic crystalline structure, deeming them outside the band theory of solids. Here, I provide ab initio theory for the ‘one-dimensional’ cuprates SrCuO 2 and (Ca)Sr 2 CuO 3 using no …

Topological States In Matter, Hasitha W. Suriya Arachchige

Doctoral Dissertations

Topologically nontrivial spin textures, mesoscopic spin configurations that cannot be continuously transformed to an elementary magnetic configuration such as a ferromagnet or antiferromagnet, are of interest due to their ability to exhibit magnetic solitons, with topological protection. Such properties have the potential for applications in future data storage and communication devices. For example, spin textures found in materials such as MnSi, Cu2OSe3, Co-Zn-Mn alloys, and GaV4S8, commonly known as skyrmions, are driven by the interplay of atomic-scale exchange interactions, single-ion anisotropy, and an applied magnetic field. Of particular importance to this class of materials is the presence of a Dyaloshinski …

Overcoming Atmospheric Effects In Quantum Cryptography, Brian Joseph Rollick

Doctoral Dissertations

Quantum Computers will have the potential to greatly assist us in problems such as searching, optimization and even drug discovery. Unfortunately, among these newfound capabilities is one which allows one to break RSA encryption in orders of magnitude less time. One promising countermeasure to secure our communication today and in the future is the one time pad, although it is very difficult to generate and distribute. Quantum Key Distribution offers a practical method for two authenticated parties to generate a key. Whereby the parties, Alice and Bob, share quantum states and use physical laws to place an upper bound on …

Semi-Classical Theories Of Quantum Magnets, Hao Zhang

Doctoral Dissertations

Recent progress in magnetism has been driven by embracing the complexity associated with entangled spin, orbital, and lattice degrees of freedom and by understanding the emergent quantum behaviors of magnetic systems. Over the past decades, intense efforts have been devoted to “extreme quantum materials” comprising low-dimensional lattices of spin S = 1/2 degrees of freedom, that are candidates to host quantum spin liquid phases with no classical counterpart. Finite-spin (S ≥ 1) systems that exhibit ground states with short-ranged entanglement have not been the center of much attention because they are expected to behave semi-classically. However, as we will demonstrate …

How Dynamic Bond Results In The Unique Viscoelastic Behavior Of The Associating Polymers, Sirui Ge

Doctoral Dissertations

Associating polymer is a special kind of polymer possessing transient reversible bonds in addition to the conventional covalent bonds. The reversible bonds provide unique dynamics and fascinating viscoelastic properties, resulting in attractive applications for these polymers, such as self-healing and shape memory materials. Despite many years of studies, the understanding of dynamics of polymers with reversible bonds, especially on molecular level, is still in the rudimentary stage, preventing the rational design of the potential novel functional materials based on associating polymers. In this dissertation, we provide a detailed and quantitative understanding of the dynamics and viscoelastic properties of associating polymers. …

Quantum Computational Simulations For Condensed Matter Systems, Trevor Alan Keen

Doctoral Dissertations

In condensed matter physics, and especially in the study of strongly correlated electron systems, numerical simulation techniques are crucial to determine the properties of the system including interesting phases of matter that arise from electron-electron interactions. Many of these interesting phases of matter, including but not limited to Mott-insulating materials and possibly high-temperature superconducting systems, can be modeled by the Hubbard model. Although it is one of the simplest models to include electron-electron interactions, it cannot be solved analytically in more than one dimension and thus numerical techniques must be employed. Although there have been great strides in classical numerical …

Numerical Studies Of Correlated Topological Systems, Rahul Soni

Doctoral Dissertations

In this thesis, we study the interplay of Hubbard U correlation and topological effects in two different bipartite lattices: the dice and the Lieb lattices. Both these lattices are unique as they contain a flat energy band at E = 0, even in the absence of Coulombic interaction. When interactions are introduced both these lattices display an unexpected multitude of topological phases in our U -λ phase diagram, where λ is the spin-orbit coupling strength. We also study ribbons of the dice lattice and observed that they qualitative display all properties of their two-dimensional counterpart. This includes flat bands near …

Improving Sensitivities In 0𝒗ββ Decay Searches By Utilizing Pen As A Structural Scintillating Material, Brennan Theresa Hackett

Doctoral Dissertations

Neutrinoless double beta decay, 0nbb is currently the only experimental test to unambiguously determine the majorana nature of the neutrino. There is a large international effort to measure 0nbb decay, with several detector technologies being pursued. This dissertation will consider the LEGEND experiment (Large Enriched Germanium Experiment for Neutrinoless bb Decay), an international effort to measure 0nbb decay with ⁷⁶Ge as both the target isotope and the detecting material.

LEGEND has a 200 kg stage and a 1000 kg stage, each requiring extremely low levels of background radiation at Q_bb (E = 2.039 MeV). These ultra-low background levels …

Measurement Of Jet Constituent Yields In Pb-Pb Collisions At √Snn = 5.02 Tev Using The Alice Detector, Charles P. Hughes

Doctoral Dissertations

Hard partonic scatterings serve as an important probe of quark-gluon-plasma (QGP) properties. The properties of jets and their constituents can provide a tool for understanding the partonic energy loss mechanisms. Low momentum jets offer a unique window into partonic energy loss because they reconstruct the partons which have lost a significant amount of energy to the QGP medium. The main difficulty in studying low momentum jets in heavy ion collisions is the presence of a significant uncorrelated background of low momentum hadrons from soft processes. One way to deal with this background is to use jet- hadron correlations to fit …