Physics Commons^™

Dislocations And Vacancies In Two-Dimensional Mixed Crystals Of Spheres And Dimers, Sharon J. Gerbode, Desmond C. Ong, Chekesha M. Liddell, Itai Cohen

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In colloidal crystals of spheres, dislocation motion is unrestricted. On the other hand, recent studies of relaxation in crystals of colloidal dimer particles have demonstrated that the dislocation dynamics in such crystals are reminiscent of glassy systems. The observed glassy dynamics arise as a result of dislocation cages formed by certain dimer orientations. In the current study, we use experiments and simulations to investigate the transition that arises when a pure sphere crystal is doped with an increasing concentration of dimers. Specifically, we focus on both dislocation caging and vacancy motion. Interestingly, we find that any nonzero fraction of dimers …

Glassy Dislocation Dynamics In 2d Colloidal Dimer Crystals, Sharon J. Gerbode, Ugmang Agarwal, Desmond C. Ong, Chekesha M. Liddell, Fernando Escobedo, Itai Cohen

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Although glassy relaxation is typically associated with disorder, here we report on a new type of glassy dynamics relating to dislocations within 2D crystals of colloidal dimers. Previous studies have demonstrated that dislocation motion in dimer crystals is restricted by certain particle orientations. Here, we drag an optically trapped particle through such dimer crystals, creating dislocations. We find a two-stage relaxation response where initially dislocations glide until encountering particles that cage their motion. Subsequent relaxation occurs logarithmically slowly through a second process where dislocations hop between caged configurations. Finally, in simulations of sheared dimer crystals, the dislocation mean squared displacement …

Restricted Dislocation Motion In Crystals Of Colloidal Dimer Particles, Sharon J. Gerbode, Stephanie H. Lee, Chekesha M. Liddell, Itai Cohen

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Received 2 April 2008; published 1 August 2008; corrected 1 October 2008

At high area fractions, monolayers of colloidal dimer particles form a degenerate crystal (DC) structure in which the particle lobes occupy triangular lattice sites while the particles are oriented randomly along any of the three lattice directions. We report that dislocation glide in DCs is blocked by certain particle orientations. The mean number of lattice constants between such obstacles is Z̅ _exp=4.6±0.2 in experimentally observed DC grains and Z̅ _sim=6.18±0.01 in simulated monocrystalline DCs. Dislocation propagation beyond these obstacles is observed to proceed through dislocation reactions. …

Quadrupole Couplings Of N12 And B12 Implanted In Metal Single-Crystals, Richard C. Haskell, Francis David Corell, Leon Madansky

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Measurements have been made of the quadrupole couplings of 12N implanted in single crystals of Be and Mg and of 12B implanted in a single crystal of Zn. A comparison of the 12N couplings in Be and Mg suggests that (i) the final stopping sites of the implanted 12N ions are substitutional sites, i.e., the 12N ions occupy metal-ion lattice positions, and (ii) the 12N ions implanted in Be and Mg have the same charge state and quadrupole shielding factor. A procedure is outlined for deducing Q(12N). The 12B couplings in Zn imply the existence of two inequivalent stopping sites. …

Study Of Stopping Sites Of B12 Nuclei Implanted In Hexagonal Single-Crystals, Francis David Correll, Richard C. Haskell, Leon Madansky

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A series of experiments to study the stopping sites of 12B nuclei implanted in single crystals of Be and Mg will be discussed. Previous measurements of the quadrupole couplings of 12B in these metals indicated that two different stopping sites existed, one of which produced a negligible quadrupole coupling.

Nuclear Quadrupole Coupling Of B-12 In A Single Be Crystal, R. L. Williams Jr., Richard C. Haskell, Leon Madansky

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Quadrupole resonance lines of β-unstable 12B have been distinctly resolved in a single crystal of Be, and have behaved properly under field reversal and variation of the angle θ between crystal c axis and external magnetic field.

Observation Of Quadrupole Splitting Of B-12 In A Single Crystal, R. L. Williams Jr., Richard C. Haskell, Leon Madansky

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The quadrupole coupling of B-12 implanted in Be-9 has been observed using a single crystal of Be. One sees a narrow resonance line, the location of which depends in the normal way on the orientation of the crystalline c-axis with respect to the external magnetic field direction. The coupling constant is given by e2qQ/h = 54.9(6) kHz. This is consistent with our previous measurement using a Be foil. Using the field gradient at Be-9 lattice sites, calculated by Pomerantz and Das, one finds Q(B-12) = about 34.6 mb.