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Articles 1 - 30 of 45
Full-Text Articles in Physics
Periodic Nonlinear Refractive Index Of Carbon Disulfide Vapors, Evelyn Strunk
Periodic Nonlinear Refractive Index Of Carbon Disulfide Vapors, Evelyn Strunk
HIM 1990-2015
The purpose of this thesis is to explore the nonlinear refractive index of carbon disulfide vapors as opposed to its liquid form. With CS[sub2] vapors, the vapors are less dense so they will rotate longer than liquid CS[sub2] because there are less intermolecular interactions. The electric field of the beam causes the molecules to align with the electric field and applies a torque to the molecules. After this excitation, the molecules continue rotating. The rotations change the index of refraction of the material. Continuous rotation of the molecules causes the index of refraction to be periodic which means the molecules …
Coarse Grained Monte Carlo Simulation Of The Self-Assembly Of The Hiv-1 Capsid Protein, Jeffrey Weber
Coarse Grained Monte Carlo Simulation Of The Self-Assembly Of The Hiv-1 Capsid Protein, Jeffrey Weber
HIM 1990-2015
In this study, a Monte Carlo simulation was designed to observe the self-assembly of the HIV-1 capsid protein. The simulation allowed a coarse grained model of the capsid protein with defined interaction sites to move freely in three dimensions using the Metropolis criterion. Observations were made as to which parameters affected the assembly the process. The ways in which the assembly were affected were also noted. It was found that proper dimerization of the capsid protein was necessary in order for the lattice to form properly. It was also found that a strong trimeric interface could be responsible for double-layered …
Electronic Properties And Atomic Scale Microscopy Of Two Dimensional Materials: Graphene And Molybdenum Disulfide, Jyoti Katoch
Electronic Properties And Atomic Scale Microscopy Of Two Dimensional Materials: Graphene And Molybdenum Disulfide, Jyoti Katoch
Electronic Theses and Dissertations
Novel two dimensional nanoscale materials like graphene and metal dichalcogenides (MX2) have attracted the attention of the scientific community, due to their rich physics and wide range of potential applications. It has been shown that novel graphene based transparent conductors and radiofrequency transistors are competitive with the existing technologies. Graphene’s properties are influenced sensitively by adsorbates and substrates. As such not surprisingly, physical properties of graphene are found to have a large variability, which cannot be controlled at the synthesis level, reducing the utility of graphene. As a part of my doctorate dissertation, I have developed atomic hydrogen as a …
Frequency Selective Detection Of Infrared Radiation In Uncooled Optical Nano-Antenna Array, Sushrut Modak
Frequency Selective Detection Of Infrared Radiation In Uncooled Optical Nano-Antenna Array, Sushrut Modak
Electronic Theses and Dissertations
Mid-infrared (mid-IR) detection and imaging over atmospheric transparent 3-5 μm and 8-12 μm bands are increasingly becoming important for various space, defense and civilian applications. Various kinds of microbolometers offer uncooled detection of IR radiation. However, broadband absorption of microbolometers makes them less sensitive to spectrally resolved detection of infrared radiation and the fabrication is also very tedious involving multiple complex lithography steps. In this study, we designed an optical nano-antenna array based detector with narrow frequency band of operation. The structure consists of a two-element antenna array comprised of a perforated metallic hole array coupled with an underneath disk …
Self-Heating Control Of Edge Emitting And Vertical Cavity Surface Emitting Lasers, Yu Zhang
Self-Heating Control Of Edge Emitting And Vertical Cavity Surface Emitting Lasers, Yu Zhang
Electronic Theses and Dissertations
Self-heating leads to temperature rise of laser diode and limits the output power, efficiency and modulation bandwidth due to increased loss and decreased differential gain. The main heat sources in laser diode during continuous wave operation are Joule heating and free carrier absorption loss. To control device self-heating, the epi structure needs to be designed with low electrical resistance and low absorption loss, while the heat flux must spread out of the device efficiently. This dissertation presents the control of self-heating of both edge emitting laser diodes and vertical cavity surface emitting lasers (VCSELs). For the 980nm high power edge …
Distribution Of Laser Induced Heating In Multi-Component Chalcogenide Glass And Its Associated Effects, Laura Sisken
Distribution Of Laser Induced Heating In Multi-Component Chalcogenide Glass And Its Associated Effects, Laura Sisken
Electronic Theses and Dissertations
Chalcogenide glasses are well known to have good transparency into the infrared spectrum. These glasses though tend to have low thresholds as compared to oxide glasses for photo-induced changes and thermally-induced changes. Material modification such as photo-induced darkening, bleaching, refractive index change, densification or expansion, ablation of crystallization have been demonstrated, and are typically induced by a thermal furnace-based heat treatment, an optical source such as a laser, or a combination of photo-thermal interactions. Solely employing laser-based heating has an advantage over a furnace, since one has the potential to be able to spatially modify the materials properties with much …
Highly-Sensitive Stoichiometric Analysis Of Yag Ceramics Using Laser-Induced Breakdown Spectroscopy (Libs), Jahromi, Ali Kazemi
Highly-Sensitive Stoichiometric Analysis Of Yag Ceramics Using Laser-Induced Breakdown Spectroscopy (Libs), Jahromi, Ali Kazemi
Electronic Theses and Dissertations
Transparent ceramics are an important class of optical materials with applications in high-strength windows, radiation detectors and high-power lasers. Despite the many successful developments of the past decades, their challenging fabrication still needs to be perfected to achieve a better consistency in optical quality. In particular, ternary phase materials such as Yttrium Aluminum Garnet (YAG, Y3Al5O12), a long standing high-power laser host, require a precise control of stoichiometry, often beyond the precision of current analytical techniques, in order to reduce scattering losses and the presence of deleterious point defects. This work explores the potential of Laser-Induced Breakdown Spectroscopy (LIBS) for …
High Resolution Time-Resolved Imaging System In The Vacuum Ultraviolet Region, Yuseong Jang
High Resolution Time-Resolved Imaging System In The Vacuum Ultraviolet Region, Yuseong Jang
Electronic Theses and Dissertations
High-power debris-free vacuum ultraviolet (VUV) light sources have applications in several scientific and engineering areas, such as high volume manufacturing lithography and inspection tools in the semiconductor industry, as well as other applications in material processing and photochemistry. For the past decades, the semiconductor industry has been driven by what is called "Moore's Law". The entire semiconductor industry relies on this rule, which requires chip makers to pack transistors more tightly with every new generation of chips, shrinking the size of transistors. The ability to solve roadmap challenges is, at least partly, proportional to our ability to measure them. The …
High Performance Three-Dimensional Display Based On Polymer-Stabilized Blue Phase Liquid Crystal, Yifan Liu
High Performance Three-Dimensional Display Based On Polymer-Stabilized Blue Phase Liquid Crystal, Yifan Liu
Electronic Theses and Dissertations
Autostereoscopic 2D/3D (two-dimension/three-dimension) switchable display has been attracting great interest in research and practical applications for several years. Among different autostereoscopic solutions, direction-multiplexed 3D displays based on microlens array or parallax barrier are viewed as the most promising candidates, due to their compatibility with conventional 2D display technologies. These 2D/3D switchable display system designs rely on fast switching display panels and photonics devices, including adaptive focus microlens array and switchable slit array. Polymer-stabilized blue phase liquid crystal (PS-BPLC) material provides a possible solution to meet the aforementioned fast response time requirement. However, present display and photonic devices based on blue …
Holographic Recording And Applications Of Multiplexed Volume Bragg Gratings In Photo-Thermo-Refractive Glass, Daniel Ott
Holographic Recording And Applications Of Multiplexed Volume Bragg Gratings In Photo-Thermo-Refractive Glass, Daniel Ott
Electronic Theses and Dissertations
Recent developments in holographic recording of volume Bragg gratings (VBGs) in photo-thermo-refractive (PTR) glass have demonstrated their utility as components in high power laser systems for spectral narrowing, transverse mode control, beam combining, and pulse stretching/compression. VBG structures are capable of diffracting incident light into a single diffraction order with high efficiency given the Bragg condition is met. The Bragg condition depends on both the wavelength and angle of the incident light making VBGs useful for filtering and manipulating both the wavelength and angular spectrum of a source. This dissertation expands upon previous research in PTR VBGs by investigating multiplexed …
Entangled Photon Pairs In Disordered Photonic Lattices, Lane Martin
Entangled Photon Pairs In Disordered Photonic Lattices, Lane Martin
Electronic Theses and Dissertations
Photonic lattices consisting of arrays of evanescently coupled waveguides fabricated with precisely controlled parameters have enabled the study of discrete optical phenomena, both classical and quantum, and the simulation of other physical phenomena governed by the same dynamics. In this dissertation, I have experimentally demonstrated transverse Anderson localization of classical light in arrays with off-diagonal coupling disorder and investigated theoretically and experimentally the propagation of entangled photon pairs through such disordered systems. I discovered a new phenomenon, Anderson co-localization, in which a spatially entangled photon pair in a correlated transversally extended state localizes in the correlation space, though neither photon …
Injection-Locked Vertical Cavity Surface Emitting Lasers (Vcsels) For Optical Arbitrary Waveform Generation, Sharad Bhooplapur
Injection-Locked Vertical Cavity Surface Emitting Lasers (Vcsels) For Optical Arbitrary Waveform Generation, Sharad Bhooplapur
Electronic Theses and Dissertations
Complex optical pulse shapes are typically generated from ultrashort laser pulses by manipulating the optical spectrum of the input pulses. This generates complex but periodic time-domain waveforms. Optical Arbitrary Waveform Generation (OAWG) builds on the techniques of ultrashort pulse-shaping, with the goal of making non-periodic, truly arbitrary optical waveforms. Some applications of OAWG are coherently controlling chemical reactions on a femtosecond time scale, improving the performance of LADAR systems, high-capacity optical telecommunications and ultra wideband signals processing. In this work, an array of Vertical Cavity Surface Emitting Lasers (VCSELs) are used as modulators, by injection-locking each VCSEL to an individual …
Dynamical Spin Injection In Graphene, Simranjeet Singh
Dynamical Spin Injection In Graphene, Simranjeet Singh
Electronic Theses and Dissertations
Within the exciting current trend to explore novel low-dimensional systems, the possibility to inject pure spin currents in graphene and other two-dimensional crystals has attracted considerable attention in the past few years. The theoretical prediction of large spin relaxation times and experimentally observed mesoscopic-scale spin diffusion lengths places graphene as a promising base system for future spintronics devices. This is due to the unique characteristics intrinsic to the two-dimensional lattice of carbon atoms forming graphene, such as the lack of nuclear spins and weak spin-orbit coupling of the charge carriers. Interestingly for some spintronic applications, the latter can be chemically …
The Effect Of Electron-Hole Pairs In Semiconductor And Topological Insulator Nanostructures On Plasmon Resonances And Photon Polarizations., Hari Paudel
Electronic Theses and Dissertations
The generation of electron-hole pairs in materials has great importance. In direct bandgap semiconductor materials, the mechanism of radiative recombination of electron-hole pairs leads to the emission of photons, which is the basis of Light Emitting Diodes (LEDs). The excitation of electron-hole pairs by absorption of photons is the active process in photodiodes, solar cells, and other semiconductor photodetector devices. In optoelectronic devices such as optical switches which are based on transmission and reflection of the photons, electron-hole pairs excitation is a key for the device performance. Diodes and transistors are also great discoveries in electronics which rely on the …
Nonlinear Integrated Photonics On Silicon And Gallium Arsenide Substrates, Jichi Ma
Nonlinear Integrated Photonics On Silicon And Gallium Arsenide Substrates, Jichi Ma
Electronic Theses and Dissertations
Silicon photonics is nowadays a mature technology and is on the verge of becoming a blossoming industry. Silicon photonics has also been pursued as a platform for integrated nonlinear optics based on Raman and Kerr effects. In recent years, more futuristic directions have been pursued by various groups. For instance, the realm of silicon photonics has been expanded beyond the well-established near-infrared wavelengths and into the mid-infrared (3 - 5 µm). In this wavelength range, the omnipresent hurdle of nonlinear silicon photonics in the telecommunication band, i.e., nonlinear losses due to two-photon absorption, is inherently nonexistent. With the lack of …
Optical And Magnetic Properties Of Nanostructures, Neha Nayyar
Optical And Magnetic Properties Of Nanostructures, Neha Nayyar
Electronic Theses and Dissertations
In this thesis, Density Functional Theory and Time-Dependent Density-Functional Theory approaches are applied to study the optical and magnetic properties of several types of nanostructures. In studies of the optical properties we mainly focused on the plasmonic and excitonic effects in pure and transition metal-doped noble metal nanochains and their conglomerates. In the case of pure noble metal chains, it was found that the (collective) plasmon mode is pronounceable when the number of atoms in the chain is larger than 5. The plasmon energy decreases with further with increasing number of atoms (N) and is almost N-independent when N is …
On-Chip Optical Stabilization Of High-Speed Mode-Locked Quantum Dot Lasers For Next Generation Optical Networks, Abhijeet Ardey
On-Chip Optical Stabilization Of High-Speed Mode-Locked Quantum Dot Lasers For Next Generation Optical Networks, Abhijeet Ardey
Electronic Theses and Dissertations
Monolithic passively mode-locked colliding pulse semiconductor lasers generating pico- to sub-picosecond terahertz optical pulse trains are promising sources for future applications in ultra-high speed data transmission systems and optical measurements. However, in the absence of external synchronization, these passively mode-locked lasers suffer from large amplitude and timing jitter instabilities resulting in broad comb linewidths, which precludes many applications in the field of coherent communications and signal processing where a much narrower frequency line set is needed. In this dissertation, a novel quantum dot based coupled cavity laser is presented, where for the first time, four-wave mixing (FWM) in the monolithically …
Terahertz And Sub-Terahertz Tunable Resonant Detectors Based On Excitation Of Two Dimensional Plasmons In Ingaas/Inp Hemts, Esfahani, Nima Nader
Terahertz And Sub-Terahertz Tunable Resonant Detectors Based On Excitation Of Two Dimensional Plasmons In Ingaas/Inp Hemts, Esfahani, Nima Nader
Electronic Theses and Dissertations
Plasmons can be generated in the two dimensional electron gas (2DEG) of grating-gated high electron mobility transistors (HEMTs). The grating-gate serves dual purposes, namely to provide the required wavevector to compensate for the momentum mismatch between the free-space radiation and 2D-plasmons, and to tune the 2DEG sheet charge density. Since the plasmon frequency at a given wavevector depends on the sheet charge density, a gate bias can shift the plasmon resonance. In some cases, plasmon generation results in a resonant change in channel conductance which allows a properly designed grating-gated HEMT to be used as a voltage-tunable resonant detector or …
Photonic Filtering For Applications In Microwave Generation And Metrology, Marcus Bagnell
Photonic Filtering For Applications In Microwave Generation And Metrology, Marcus Bagnell
Electronic Theses and Dissertations
This work uses the photonic filtering properties of Fabry-Perot etalons to show improvements in the electrical signals created upon photodetection of the optical signal. First, a method of delay measurement is described which uses multi-heterodyne detection to find correlations in white light signals at 20 km of delay to sub millimeter resolution. By filtering incoming white light with a Fabry-Perot etalon, the pseudo periodic signal is suitable for measurement by combining and photodetecting it with an optical frequency comb. In this way, optical data from a large bandwidth can be downconverted and sampled on low frequency electronics. Second, a high …
Multifunctional, Multimaterial Particle Fabrication Via An In-Fiber Fluid Instability, Joshua Kaufman
Multifunctional, Multimaterial Particle Fabrication Via An In-Fiber Fluid Instability, Joshua Kaufman
Electronic Theses and Dissertations
Spherical micro- and nano-particles have found widespread use in many various applications from paint to cosmetics to medicine. Due to the multiplicity of desired particle material(s), structure, size range, and functionality, many approaches exist for generating such particles. Bottom-up methods such as chemical synthesis have a high yield and work with a wide range of materials; however, these processes typically lead to large polydispersity and cannot produce structured particles. Top-down approaches such as microfluidics overcome the polydispersity issue and may produce a few different structures in particles, but at lower rates and only at the micro-scale. A method that can …
Large Area Conformal Infrared Frequency Selective Surfaces, Jeffrey D'Archangel
Large Area Conformal Infrared Frequency Selective Surfaces, Jeffrey D'Archangel
Electronic Theses and Dissertations
Frequency selective surfaces (FSS) were originally developed for electromagnetic filtering applications at microwave frequencies. Electron-beam lithography has enabled the extension of FSS to infrared frequencies; however, these techniques create sample sizes that are seldom appropriate for real world applications due to the size and rigidity of the substrate. A new method of fabricating large area conformal infrared FSS is introduced, which involves releasing miniature FSS arrays from a substrate for implementation in a coating. A selective etching process is proposed and executed to create FSS particles from crossed-dipole and square-loop FSS arrays. When the fill-factor of the particles in the …
Theoretical And Numerical Studies Of Phase Transitions And Error Thresholds In Topological Quantum Memories, Pejman Jouzdani
Theoretical And Numerical Studies Of Phase Transitions And Error Thresholds In Topological Quantum Memories, Pejman Jouzdani
Electronic Theses and Dissertations
This dissertation is the collection of a progressive research on the topic of topological quantum computation and information with the focus on the error threshold of the well-known models such as the unpaired Majorana, the toric code, and the planar code. We study the basics of quantum computation and quantum information, and in particular quantum error correction. Quantum error correction provides a tool for enhancing the quantum computation fidelity in the noisy environment of a real world. We begin with a brief introduction to stabilizer codes. The stabilizer formalism of the theory of quantum error correction gives a well-defined description …
Quantitative Scanning Transmission Electron Microscopy Of Thick Samples And Of Gold And Silver Nanoparticles On Polymeric Surfaces, Aniruddha Dutta
Quantitative Scanning Transmission Electron Microscopy Of Thick Samples And Of Gold And Silver Nanoparticles On Polymeric Surfaces, Aniruddha Dutta
Electronic Theses and Dissertations
Transmission Electron Microscopy (TEM) is a reliable tool for chemical and structural studies of nanostructured systems. The shape, size and volumes of nanoparticles on surfaces play an important role in surface chemistry. As nanostructured surfaces become increasingly important for catalysis, protective coatings, optical properties, detection of specific molecules, and many other applications, different techniques of TEM can be used to characterize the properties of nanoparticles on surfaces to provide a path for predictability and control of these systems. This dissertation aims to provide fundamental understanding of the surface chemistry of Electroless Metallization onto Polymeric Surfaces (EMPS) through characterization with TEM. …
Broad Bandwidth, All-Fiber, Thulium-Doped Photonic Crystal Fiber Amplifier For Potential Use In Scaling Ultrashort Pulse Peak Powers, Alex Sincore
Electronic Theses and Dissertations
Fiber based ultrashort pulse laser sources are desirable for many applications; however generating high peak powers in fiber lasers is primarily limited by the onset of nonlinear effects such as self-phase modulation, stimulated Raman scattering, and self-focusing. Increasing the fiber core diameter mitigates the onset of these nonlinear effects, but also allows unwanted higher-order transverse spatial modes to propagate. Both large core diameters and single-mode propagation can be simultaneously attained using photonic crystal fibers. Thulium-doped fiber lasers are attractive for high peak power ultrashort pulse systems. They offer a broad gain bandwidth, capable of amplifying sub-100 femtosecond pulses. The longer …
Laser Filamentation - Beyond Self-Focusing And Plasma Defocusing, Khan Lim
Laser Filamentation - Beyond Self-Focusing And Plasma Defocusing, Khan Lim
Electronic Theses and Dissertations
Laser filamentation is a highly complex and dynamic nonlinear process that is sensitive to many physical parameters. The basic properties that define a filament consist of (i) a narrow, high intensity core that persists for distances much greater than the Rayleigh distance, (ii) a low density plasma channel existing within the filament core, and (iii) a supercontinuum generated over the course of filamentation. However, there remain many questions pertaining to how these basic properties are affected by changes in the conditions in which the filaments are formed; that is the premise of the work presented in this dissertation. To examine …
Multimaterial Fibers In Photonics And Nanotechnology, Guangming Tao
Multimaterial Fibers In Photonics And Nanotechnology, Guangming Tao
Electronic Theses and Dissertations
Recent progress in combing multiple materials with distinct optical, electronic, and thermomechanical properties monolithically in a kilometer-long fiber drawn from a preform offers unique multifunctionality at a low cost. A wide range of unique in-fiber devices have been developed in fiber form-factor using this strategy. Here, I summary my recent results in this nascent field of 'multimaterial fibers'. I will focus on my achievements in producing robust infrared optical fibers and in appropriating optical fiber production technology for applications in nanofabrication. The development of optical components suitable for the infrared (IR) is crucial for applications in this spectral range to …
Pressure And Temperature Response Of A Stimuli-Responsive Polymer Probed With Raman Microscopy, Coleman Cariker
Pressure And Temperature Response Of A Stimuli-Responsive Polymer Probed With Raman Microscopy, Coleman Cariker
HIM 1990-2015
Poly(N-isopropylacrylamide) (PNIPAM) is a thermo-responsive hydrogel; that is, it is a macromolecule which exists in a hydrated state beneath its lower critical solution temperature (LCST). Polymers such as PNIPAM undergo a phase transition in response to changes in temperature, pressure, pH, salt concentration, and the addition of co-solvents. Previously, visible-light microscopic measurements of the pressure-induced phase transition have been hindered by the lack of a pressurization apparatus with the short working distance and optical transmission properties necessary for high resolution microscopy. We employ a high pressure setup which uses a fused silica micro-capillary to contain the sample. Our experiment reveals …
Micro-Raman Spectroscopy Of Carbonaceous Chondrite Meteorites, Asmail Habach
Micro-Raman Spectroscopy Of Carbonaceous Chondrite Meteorites, Asmail Habach
HIM 1990-2015
Analyzing the constituents of meteorites has played an important role in forming the contemporary theories of solar system evolution, planets formation, and stellar evolution. Meteorites are often a complex mixture of common rock forming silicates, such as olivines and pyroxenes, with a range of exotic species including hydrated silicates, and in some cases organic compounds. We used Micro-Raman spectroscopy to analyze the compositions of three carbonaceous chondrites: NWA852, Murchison and Allende. Raman spectra were measured using laser sources with different excitation wavelengths: HeNe 633 nm and Nd:YAG 532 nm. We were able to detect 9 minerals in NWA852, 3 minerals …
Electronic Transport And Correlations In Single Magnetic Molecule Devices, Javier Romero
Electronic Transport And Correlations In Single Magnetic Molecule Devices, Javier Romero
Electronic Theses and Dissertations
In this dissertation, we study the most important microscopic aspects that grant molecules such as Single Molecule Magnets (SMMs) their preferential spin direction. We do so by proposing and solving a model that includes correlations between electrons occupying atomic orbitals. In addition, we study the relation between the non-equilibrium electronic transport signatures in a SMM model weakly coupled to a three-terminal single electron transistor device, and the interference features of the SMM model in the presence of a magnetic field. Finally, we investigate the equilibrium transport features in a giant-spin model of a SMM in the Kondo regime. We study …
Techniques For Characterization Of Third Order Optical Nonlinearities, Manuel Ferdinandus
Techniques For Characterization Of Third Order Optical Nonlinearities, Manuel Ferdinandus
Electronic Theses and Dissertations
This dissertation describes the development of novel techniques for characterization of nonlinear properties of materials. The dissertation is divided into two parts, a background and theory section and a technique development section. In the background and theory section we explain the origins of the nonlinear optical response of materials across many different spatial and temporal scales. The mechanisms that we are most interested in are the electronic nuclear and reorientational responses, which occur on the range of sub-femtosecond to several picoseconds. The electronic mechanism is due to the electrons of a material experiencing a non-parabolic potential well due a strong …