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Full-Text Articles in Physics

Theoretical Framework Of Exchange Coupled Tripartite Spin Systems With Magnetic Anisotropy And Predictions Of Spin And Electronic Transport Properties For Their Use In Quantum Architectures, Eric Switzer Aug 2023

Theoretical Framework Of Exchange Coupled Tripartite Spin Systems With Magnetic Anisotropy And Predictions Of Spin And Electronic Transport Properties For Their Use In Quantum Architectures, Eric Switzer

Electronic Theses and Dissertations, 2020-

There has been significant interest in spin systems involving two or more coupled spins as a single logical qubit, particularly for scalable quantum computing architectures. Recent realizations include the so-called singlet-triplet qubits and coupled magnetic molecules. An important class of coupled-spin systems, the three-spin paradigm for spin greater than 1/2, has not yet been fully realized in scalable qubit architectures. In this thesis, I develop the theoretical framework to investigate a class of tripartite spin models for realistic systems. First, I model a spin 1/2 particle (e.g., an electron) and two spin 1 particles (in a dimer arrangement) coupled with …


Theoretical Analysis Of Charge Conduction And Rectification In Self-Assembled-Monolayers In Molecular Junctions, Francis Adoah Aug 2023

Theoretical Analysis Of Charge Conduction And Rectification In Self-Assembled-Monolayers In Molecular Junctions, Francis Adoah

Electronic Theses and Dissertations, 2020-

As electrical devices shrink to the atomic scale, it is expected that Moore's law will soon be obsolete for semiconductor devices. In 1974, Avriam and Ratner predicted that organic devices could replace semiconductor technology, leading to extensive research on molecular-based organic devices. This dissertation delves into the theoretical frameworks used to examine the transport in molecular junctions and aims to enhance our comprehension of charge transport and conduction properties. The studies presented in this thesis illustrates that a molecule's alteration by just a single atom can change it from an insulator to a conductor, and also that, by fine-tuning the …


Due Tomorrow, Do Tomorrow: Measuring And Reducing Procrastination Behavior Among Introductory Physics Students In An Online Environment, Zachary Felker Aug 2023

Due Tomorrow, Do Tomorrow: Measuring And Reducing Procrastination Behavior Among Introductory Physics Students In An Online Environment, Zachary Felker

Electronic Theses and Dissertations, 2020-

This work is focused on the measurement and prevention of procrastination behavior among college level introductory physics students completing online assignments in the form of mastery-based online learning modules. The research is conducted in two studies. The first study evaluates the effectiveness of offering students the opportunity to earn a small amount of extra credit for completing portions of their homework early. Unsupervised machine learning is used to identify an optimum cutoff duration which differentiates taking a short break during a continuous study session from a long break between two different study sessions. Using this cutoff, the study shows that …


Reflective Planar Optics With Cholesteric Liquid Crystal For Near-Eye Displays, Yannanqi Li Jan 2023

Reflective Planar Optics With Cholesteric Liquid Crystal For Near-Eye Displays, Yannanqi Li

Electronic Theses and Dissertations, 2020-

Display market has undergone dramatic changes as the near eye displays (NED) are gaining increasing attention because they offer a deeper level of human-computer interaction with the advancement of electronic devices and computer sciences. The NEDs can be presented in two ways: virtual reality (VR) and augmented reality (AR). The former is completely immersive while the latter combines the digital information with the surrounding scenes. Although several VR headsets have been commercialized for consumers and AR products for prosumers because of their high cost, but there is still a long way to go to satisfy the strict requirements of human …


Integrated Frequency Combs For Applications In Optical Communications & Microwave Photonics, Chinmay Shirpurkar Jan 2023

Integrated Frequency Combs For Applications In Optical Communications & Microwave Photonics, Chinmay Shirpurkar

Electronic Theses and Dissertations, 2020-

This dissertation reviews the advancements made in chip-scale optical frequency combs and their applications towards optical communications and optical to RF links. We review different chip-scale comb sources and in particular, chip-scale Kerr microresonator frequency combs. Then, we establish the theoretical background in nonlinear optics which allows the formation and stabilization of Kerr solitons in nonlinear cavities. We also discuss the concept of optical injection locking and in particular, multi-tone injection locking which precedes the idea of regenerative harmonic injection locking. We then go on to show the experimental work involved in soliton generation and characterization. We show efforts towards …


High-Dynamic-Range And High-Efficiency Near-Eye Display Systems, En-Lin Hsiang Jan 2023

High-Dynamic-Range And High-Efficiency Near-Eye Display Systems, En-Lin Hsiang

Electronic Theses and Dissertations, 2020-

Near-eye display systems, which project digital information directly into the human visual system, are expected to revolutionize the interface between digital information and physical world. However, the image quality of most near-eye displays is still far inferior to that of direct-view displays. Both light engine and imaging optics of near-eye display systems play important roles to the degraded image quality. In addition, near-eye displays also suffer from a relatively low optical efficiency, which severely limits the device operation time. Such an efficiency loss originates from both light engines and projection processes. This dissertation is devoted to addressing these two critical …


Compact And High Optical Efficiency Near-Eye Displays With Liquid Crystal Flat Optics, Junyu Zou Jan 2023

Compact And High Optical Efficiency Near-Eye Displays With Liquid Crystal Flat Optics, Junyu Zou

Electronic Theses and Dissertations, 2020-

Since the concepts of augmented reality (AR) and virtual reality (VR) were introduced, they have attracted people's attention worldwide, both in the industry and research areas. As the most promising hardware architecture that can bring AR/VR into daily life, near eye displays (NEDs) have been studied and investigated heavily over the past half-century, especially the concept of "Metaverse" introduced by some top companies in recent years. However, the form factor and optical efficiency are two major bottlenecks for the current NEDs before they can become the major platform. Liquid crystal (LC) flat optics have several advantages, including compact, high diffraction …


Observation Of Novel Phases Of Quantum Matter Beyond Topological Insulator, Sabin Regmi Dec 2022

Observation Of Novel Phases Of Quantum Matter Beyond Topological Insulator, Sabin Regmi

Electronic Theses and Dissertations, 2020-

Because of the unique electronic properties, intriguing novel phenomena, and potentiality in quantum device applications, the quantum materials with non-trivial band structures have enticed a bulk of research works over the last two decades. The experimental discovery of the three-dimensional topological insulators (TIs) - bulk insulators with surface conduction via spin-polarized electrons - kicked off the flurry of research interests towards such materials, which resulted in the experimental discovery of new topological phases of matter beyond TIs. The topological semimetallic phase in Dirac, Weyl, and nodal-line semimetals is an example, where the classification depends on the dimensionality, degeneracy, and symmetry …


Imaging Based Beam Steering For Optical Communication And Lidar Applications, Sajad Saghaye Polkoo Jan 2022

Imaging Based Beam Steering For Optical Communication And Lidar Applications, Sajad Saghaye Polkoo

Electronic Theses and Dissertations, 2020-

Optical beam steering is a key component in any application that requires dynamic (i.e. realtime control) of beam propagation through free-space. Example applications include remote sensing, spectroscopy, laser machining, targeting, Lidar, optical wireless communications (OWC) and more. The pointing control requirements for many of these applications can be met by traditional mechanical steering techniques; however, these solutions tend to be bulky, slow, expensive, power hungry and prone to mechanical failures leading to short component lifetimes. Two emerging applications, Lidar imaging and OWC, truly need improved beam-steering capabilities to flourish and support the advancement of self-driving cars or relieve the congestion …


Raman Excitation Laser Effects On Peak Parameters And Peak Metamorphic Temperatures Of Primitive Carbonaceous Chondrites, Amy Lebleu-Debartola Jan 2022

Raman Excitation Laser Effects On Peak Parameters And Peak Metamorphic Temperatures Of Primitive Carbonaceous Chondrites, Amy Lebleu-Debartola

Electronic Theses and Dissertations, 2020-

MicroRaman (µRaman) spectroscopy is often regarded as a non-destructive technique, utilized to analyze limited materials, both terrestrial and extraterrestrial. Carbonaceous chondrite meteorites are of particular interest but they are dark (low albedo) materials, and thus absorb the majority of incident visible light. Raman excitation lasers can induce considerable localized heating, even when low laser powers are used. It has been previously suggested to utilize low power lasers of =0.4 mW to minimize damaging carbonaceous samples in several fields, including Meteoritics, Geology, Chemistry, and Paleontology. Peak Metamorphic Temperatures (PMT) experienced by the meteorite can be estimated from Raman fitting parameters related …


Light Trapping Transparent Electrodes, Mengdi Sun Jan 2022

Light Trapping Transparent Electrodes, Mengdi Sun

Electronic Theses and Dissertations, 2020-

Transparent electrodes represent a critical component in a wide range of optoelectronic devices such as high-speed photodetectors and solar cells. Fundamentally, the presence of any conductive structures in the optical path leads to dissipation and reflection, which adversely affects device performance. Many different approaches have been attempted to minimize such shadowing losses, including the use of transparent conductive oxides (TCOs), metallic nanowire mesh grids, graphene-based contacts, and high-aspect ratio metallic wire arrays. In this dissertation I discuss a conceptually different approach to achieve transparent electrodes, which involves recapturing photons initially reflected by highly conductive electrode lines. To achieve this, light-redirecting …


Electronic And Optoelectronic Properties Of Two-Dimensional Heterostructures For Next-Generation Device Technologies, Jesse Thompson Jan 2022

Electronic And Optoelectronic Properties Of Two-Dimensional Heterostructures For Next-Generation Device Technologies, Jesse Thompson

Electronic Theses and Dissertations, 2020-

Since monolayer graphene was isolated in 2004, there has been significant interest in integrating layered materials into innovative device designs and hybrid materials to help solve pressing technological challenges. This is partially because they can typically be thinned to a two-dimensional (2D) form without suffering from roughness-induced scattering and can exhibit thickness-dependent variations in properties such as their energy band gap. This dissertation reports on investigations of electronic and optoelectronic device physics in 2D material heterostructures. The investigation of electronic device physics focuses on the interface between 2D molybdenum disulfide (MoS2) and gold (Au), which behaves as a resistive switching …


Machine Learning In Fiber Optics, Xiaowen Hu Jan 2022

Machine Learning In Fiber Optics, Xiaowen Hu

Electronic Theses and Dissertations, 2020-

Recent burgeoning machine learning has revolutionized our ways of looking at the world. Being extraordinarily good at pattern recognition, machine learning has been widely applied to many fields to solve challenging problems. This dissertation demonstrates the applications of machine learning on scanning-free fiber-optic imaging systems (FOISs), and on the design of anti-resonant fibers. In the first part, we propose a semi-supervised learning framework called the adaptive inverse mapping (AIP) to stabilize the imaging performance through multimode fibers (MMFs). We show that if the state of the MMF is traced closely, the output images can be used as probes to correct …


Uncooled Microbolometer Imaging Systems For Machine Vision, Robert Grimming Jan 2022

Uncooled Microbolometer Imaging Systems For Machine Vision, Robert Grimming

Electronic Theses and Dissertations, 2020-

Over the last 20 years, the cost of uncooled microbolometer-based imaging systems has drastically decreased while performance has increased. In the simplest terms, the figure of merit for these types of thermal detectors is given in terms of the τ-NETD product, the combination of the thermal time constant and the noise equivalent temperature difference. Considering these factors, optimal system design parameters are investigated to maximize visual information content. This dissertation focuses on improving scene information in the longwave infrared (LWIR) spectrum that has had its validity and quality degraded by noise, blur, and reflected radiance. Taken together, noise and blur …


Observation Of Anisotropic Properties In Topological Quantum Materials, Gyanendra Dhakal Jan 2022

Observation Of Anisotropic Properties In Topological Quantum Materials, Gyanendra Dhakal

Electronic Theses and Dissertations, 2020-

The discovery of the three-dimensional topological insulator (TI) has enormously impacted our understanding of quantum materials. These novel materials are characterized by the topology rather than some order parameters. The TIs are the materials that exhibit insulating properties in the bulk while possessing the metallic state on the surface. These surface states are protected by time-reversal symmetry; as a result, the electrons featuring surface states are spin-polarized. After the discovery of TIs, other topological semimetallic (TSM) states were discovered, which enhanced the understanding and widened the reach of topological materials. Discoveries of various topological phases such as Dirac, Weyl, nodal …


Control Of Coherence In Attosecond Atomic Ionization, Saad Mehmood Jan 2022

Control Of Coherence In Attosecond Atomic Ionization, Saad Mehmood

Electronic Theses and Dissertations, 2020-

The motion of electrons in atoms, molecules, and in condensed matter unfolds on a time scale from the attosecond (1 as = 10-18 s) to several femtoseconds (1 fs= 10-15 s). The advent of attosecond light pulses has opened the way to the time-resolved study of electronic motion and of ionization processes using pump-probe spectroscopy. In this thesis, we examine three aspects of the ionization dynamics in poly-electronic atoms: i) the coherence of the emerging charged fragments, ii) two-photon ionization pathways, and iii) the reconstruction of photoionization amplitudes from experimental observable. We focus on the role of autoionizing states and …


Computational And Experimental Studies Of Adsorption And Reactions On Molybdenum Nitride And Silica Covered Ruthenium Surfaces, Muhammad Sajid Jan 2022

Computational And Experimental Studies Of Adsorption And Reactions On Molybdenum Nitride And Silica Covered Ruthenium Surfaces, Muhammad Sajid

Electronic Theses and Dissertations, 2020-

Fundamental studies of material surfaces are of continued interest to the development and improvement of many modern technologies, e.g. catalysis, energy efficient electronics, and high-capacity batteries etc. This dissertation targets two distinct sets of molecule-surface interactions relevant to the continued development of structure-property correlations using tools from Density Functional Theory with added verification from ultrahigh vacuum surface-science experiments. These include Haber-Bosch interactions at molybdenum-nitride surfaces and separation-dependent interactions between simple aromatics and Ru(0001) used to model a metal contact of Organic Electronic Devices (OEDs). In the first study, we focus on computational modelling of nitrogen fixation reactions on Mo- and …


Methods And Characterization Of Topological And Disordered-Induced Protection Of Coherence In Quantum Systems, Sayandip Dhara Jan 2022

Methods And Characterization Of Topological And Disordered-Induced Protection Of Coherence In Quantum Systems, Sayandip Dhara

Electronic Theses and Dissertations, 2020-

Quantum computers can efficiently simulate natural processes and solve certain types of mathematical problems. Two of the key issues preventing the development of platforms to realize a scalable quantum machine are the decoherence of the qubits due to the interaction with the environment and the existence of a large overhead to correct errors. Although there already exist noisy intermediate-scale quantum machines, we still need to improve much to be able to solve problems faster than the already existing classical computers. In this dissertation, we explore two approaches to tackle both issues. We propose a scheme where, using quasi-Majorana zero modes …


Development Of Holographic Phase Masks For Wavefront Shaping, Nafiseh Mohammadian Jan 2022

Development Of Holographic Phase Masks For Wavefront Shaping, Nafiseh Mohammadian

Electronic Theses and Dissertations, 2020-

This dissertation explores a new method for creating holographic phase masks (HPMs), which are phase transforming optical elements holographically recorded in photosensitive glass. This novel hologram recording method allows for the fast production of HPMs of any complexity, as opposed to the traditional multistep process, which includes the design and fabrication of a master phase mask operating in the UV region before the holographic recording step. We holographically recorded transmissive HPMs that are physically robust (they are recorded in a silicate glass volume), can handle tens of kilowatts of continuous wave (CW) laser power, are un-erasable, user defined, require no …


Physics And Applications Of Space-Time Wave Packets, Murat Yessenov Jan 2022

Physics And Applications Of Space-Time Wave Packets, Murat Yessenov

Electronic Theses and Dissertations, 2020-

Space-time wave packets (STWP) constitute a broad class of pulsed optical fields that are rigidly transported in linear media without diffraction or dispersion, and are therefore propagation-invariant in absence of optical nonlinearities or waveguiding structures. Such wave packets exhibit unique characteristics, such as controllable group velocities in free space and exotic refractive phenomena. At the root of these behaviors is a fundamental feature underpinning STWP: their spectra are not separable with respect to the spatial and temporal degrees of freedom. Indeed, the spatio-temporal structure is endowed with angular dispersion, in which each spatial frequency is associated with a single prescribed …


Compact Lens Technologies: Curved Image Sensor And Volumetric Imaging Efficiency, Zhao Ma Jan 2022

Compact Lens Technologies: Curved Image Sensor And Volumetric Imaging Efficiency, Zhao Ma

Electronic Theses and Dissertations, 2020-

Compact image systems bring up people's attention in the field of target recognition, surveillance, situation awareness or even photography. Conventional metrics assess image system based on image quality without considering systems' volume. More comprehensive metrics, such as General Image-Quality Equation and the Targeting Task Performance metric, incorporates all image system components from object, lenses to detector and even imaging processing algorithm. All these key factors prohibit these metrics from being applied to image system in a convenient manner. Here, we propose a simple metric, volumetric imaging efficiency, considering both image quality and volume. Only concentrate on optical lenses enables the …


Volume Bragg Gratings With Complex Phase Structures: A Three-Dimensional Foundation For Laser-Beam Engineering, Lam Mach Jan 2022

Volume Bragg Gratings With Complex Phase Structures: A Three-Dimensional Foundation For Laser-Beam Engineering, Lam Mach

Electronic Theses and Dissertations, 2020-

Bragg diffraction is a natural phenomenon that arises from the coherent interference of scattered waves in multilayer structures with a well-defined periodicity. In practice, the physical size of these multilayer structures varies depending on the intended application, from micrometer-thick dielectric mirrors with tens of layers to centimeter-long Bragg gratings with ten-thousands of layers. The scope of this work centers around a unique class of multilayer elements developed in bulk photo-thermo-refractive (PTR) glass – the volume Bragg grating (VBG). The content of this thesis places an emphasis on the volume nature of these Bragg devices, implying a three-dimensional structure whereupon arbitrary …


Design Of A High-Power Terahertz Emitter Array Using A High-Temperature Superconductor, Ruqayyah Shouk Jan 2022

Design Of A High-Power Terahertz Emitter Array Using A High-Temperature Superconductor, Ruqayyah Shouk

Electronic Theses and Dissertations, 2020-

By applying a dc voltage V across the stack of intrinsic Josephson junctions naturally present in the high-temperature superconductor consisting of two parts bismuth, two parts strontium, one part calcium, two parts copper, and a bit more than eight parts oxygen, several groups have been able to obtain coherent THz emission at output powers in the µW range. In order to enhance the output power well into the mW range suitable for many applications, we have studied a compact design of a stand-alone mesa array with gold layers on the top and bottom of the superconductor. In this design, an …


Terahertz Spintronics With Antiferromagnetic Insulators, Gyan Khatri Jan 2022

Terahertz Spintronics With Antiferromagnetic Insulators, Gyan Khatri

Electronic Theses and Dissertations, 2020-

The existence of the THz gap in the electromagnetic spectrum is not only preventing the advancement of several technologies but also hindering research and developmental activities due to a lack of research facilities operating in the gap region. There is a plethora of materials with dynamics lying in the THz gap region whose study could potentially lead to the development of new technologies for the generation, detection, and processing of THz signals. Antiferromagnets are gaining recent interest due to their high frequency dynamics lying in the THz region, and their potential uses as active elements in THz spintronics devices have …


Characterizing The Particle Size Distribution In Saturn's Rings Using Cassini Uvis Stellar Occultation Data, Stephanie Eckert Jan 2022

Characterizing The Particle Size Distribution In Saturn's Rings Using Cassini Uvis Stellar Occultation Data, Stephanie Eckert

Electronic Theses and Dissertations, 2020-

NASA's Cassini mission to Saturn revolutionized modern understanding of the planet's vast and intricate ring system. We use stellar occultation data from Cassini's UVIS High Speed Photometer (HSP) to characterize the particle size distribution in the rings with two methods. First, we discern the sizes of the smallest particles at ring edges by forward-modeling observed diffraction signatures which appear as spikes in the signal, the shape and amplitude of which depends on the size and abundance of the smallest particles. We then probe the upper end of the size distribution using occultation statistics. Although the distribution of photon counts in …


Optimization-Based Approaches To Low-Coherence Optical Diffraction Tomography, Seth Smith-Dryden Jan 2022

Optimization-Based Approaches To Low-Coherence Optical Diffraction Tomography, Seth Smith-Dryden

Electronic Theses and Dissertations, 2020-

Quantitative optical phase imaging techniques, such as optical diffraction tomography (ODT), are useful tools for refractive-index profiling. Many of them, however, rely on the weak-scattering assumptions, thus cannot be applied to multiple-scattering objects, or turbid media. In this thesis, I report several approaches for expanding the efficacy of ODT techniques and adapting them to new applications by use of low-coherence broadband illumination. First, I developed a method for ODT reconstruction using regularized convex optimization with a new phase-based fidelity criterion. The new criterion is necessary because objects with very different refractive-index distributions may produce similar diffracted fields (magnitude and principal-phase) …


Third Order Nonlinear Optics In Solids, Nicholas Cox Jan 2022

Third Order Nonlinear Optics In Solids, Nicholas Cox

Electronic Theses and Dissertations, 2020-

Nonlinear optical effects occur when strong electromagnetic waves induce changes in a medium that affect its own propagation or that of another wave. Third order optical nonlinearities scale linearly with irradiance and lead to effects like two-photon absorption and nonlinear refraction. This work focuses on the experimental and theoretical study of two-photon absorption in crystalline solids. We begin by detailing the quantum mechanical states of electrons in solids along with the computational approaches to calculate their band structure. Next, a theoretical model for the linear and nonlinear optical interaction of light with matter is presented in a many-body formalism. This …


Diffractive Liquid Crystal Optical Elements For Near-Eye Displays, Jianghao Xiong Jan 2022

Diffractive Liquid Crystal Optical Elements For Near-Eye Displays, Jianghao Xiong

Electronic Theses and Dissertations, 2020-

Liquid crystal planar optics (LCPO) with versatile functionalities is emerging as a promising candidate for overcoming various challenges in near-eye displays, like augmented reality (AR) and virtual reality (VR), while maintaining a small form factor. This type of novel optical element exhibits unique properties, such as high efficiency, large angular/spectral bandwidths, polarization selectivity, and dynamic modulation. The basic molecular configuration of these novel reflective LCPO is analyzed, based on the simulation of molecular dynamics. In contrast to previously assumed planar-twist structure, our analysis predicts a slanted helix structure, which agrees with the measured results. The optical simulation model is established …


Patterned Liquid Crystal Devices For Near-Eye Displays, Kun Yin Jan 2022

Patterned Liquid Crystal Devices For Near-Eye Displays, Kun Yin

Electronic Theses and Dissertations, 2020-

As a promising next-generation display, augmented reality (AR) and virtual reality (VR) have shown attractive features and attracted broad interests from both academia and industry. Currently, these near-eye displays (NEDs) have enabled numerous applications, ranging from education, medical, entertainment, to engineering, with the help of compact and functional patterned liquid crystal (LC) devices. The interplay between LC patterns and NEDs stimulates the development of novel LC devices with unique surface alignments and volume structures, which in turn feedback to achieve more compact and versatile NEDs. This dissertation will focus on the patterned LC with applications in NEDs. Firstly, we propose …


First And Third Order Susceptibility Of Organic Molecules, Hao-Jung Chang Jan 2022

First And Third Order Susceptibility Of Organic Molecules, Hao-Jung Chang

Electronic Theses and Dissertations, 2020-

Illuminating a material with intense laser excitation may change its properties and result in nonlinear absorption (NLA) and nonlinear refraction (NLR). In this dissertation we study the nonlinear absorption of organic compounds, the effect of extremely nondegenerate NLR in semiconductors, and the linear refractive index of organic solvents. In liquids, the refractive index has been studied for decades and different kinds of refractometers have been proposed. However, most of the reported values are in the visible region and only for commonly used solvents. We proposed a new interferometer-based refractometer that allows us to measure the refractive index from the visible …