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Full-Text Articles in Physics
Rhodizonic Acid On Noble Metals: Surface Reactivity And Coordination Chemistry, Donna A. Kunkel, James Hooper, Scott Simpson, Sumit Beniwal, Katie L. Morrow, Douglas C. Smith, Kimberly Cousins, Stephen Ducharme, Eva Zurek, Axel Enders
Rhodizonic Acid On Noble Metals: Surface Reactivity And Coordination Chemistry, Donna A. Kunkel, James Hooper, Scott Simpson, Sumit Beniwal, Katie L. Morrow, Douglas C. Smith, Kimberly Cousins, Stephen Ducharme, Eva Zurek, Axel Enders
Axel Enders
A study of the two-dimensional crystallization of rhodizonic acid on the crystalline surfaces of gold and copper is presented. Rhodizonic acid, a cyclic oxocarbon related to the ferroelectric croconic acid and the antiferroelectric squaric acid, has not been synthesized in bulk crystalline form yet. Capitalizing on surface-assisted molecular self-assembly, a two-dimensional analogue to the well-known solution-based coordination chemistry, two-dimensional structures of rhodizonic acid were stabilized under ultrahigh vacuum on Au(111) and Cu(111) surfaces. Scanning tunneling microscopy, coupled with first-principles calculations, reveals that on the less reactive Au surface, extended two-dimensional islands of rhodizonic acid are formed, in which the molecules …
Reconstructing The Bulk Fermi Surface And Superconducting Gap Properties From Neutron Scattering Experiments, Tanmoy Das, R. S. Markiewicz, A. Bansil
Reconstructing The Bulk Fermi Surface And Superconducting Gap Properties From Neutron Scattering Experiments, Tanmoy Das, R. S. Markiewicz, A. Bansil
Robert Markiewicz
We develop an analytical tool to extract bulk electronic properties of unconventional superconductors from inelastic neutron scattering spectra. We show that the upward and downward branches of the spin excitation spectra have distinct origins, with the upper branch representing a gapped spin-wave dispersion and the lower branch associated with Bogoliubov quasiparticle scattering on the Fermi surface. Combined, they produce an "hourglass" dispersion with 45 degrees rotation of the spectrum, as found experimentally. The downward dispersion can be inverted to reveal the Fermi momentum dispersion of the single-particle spectrum as well as the corresponding superconducting (SC) gap function, analogously to the …
Effect Of Orbital Symmetry Of The Tip On Scanning Tunneling Spectra Of Bi₂Sr₂Cacu₂O₈+Δ, Ilpo Suominen, Jouko Nieminen, R. S. Markiewicz, A. Bansil
Effect Of Orbital Symmetry Of The Tip On Scanning Tunneling Spectra Of Bi₂Sr₂Cacu₂O₈+Δ, Ilpo Suominen, Jouko Nieminen, R. S. Markiewicz, A. Bansil
Robert Markiewicz
We discuss how variations in the scanning tunneling microscope (STM) tip, whether unintentional or intentional, can lead to changes in topographic images and dI/dV spectra. We consider the possibility of utilizing functionalized tips in order to improve the sensitivity of STM experiments to local irregularities at the surface or hidden below the surface layers. The change in the tip symmetry can radically alter the contrast of the topographic image due to changes in tip-surface overlap. The dI/dV curves change their shape according to which sample bands the tip orbital tends to overlap. In addition, relative phases between competing tunneling channels …
Effect Of Orbital Symmetry Of The Tip On Scanning Tunneling Spectra Of Bi₂Sr₂Cacu₂O₈+Δ, Ilpo Suominen, Jouko Nieminen, R. S. Markiewicz, A. Bansil
Effect Of Orbital Symmetry Of The Tip On Scanning Tunneling Spectra Of Bi₂Sr₂Cacu₂O₈+Δ, Ilpo Suominen, Jouko Nieminen, R. S. Markiewicz, A. Bansil
Arun Bansil
We discuss how variations in the scanning tunneling microscope (STM) tip, whether unintentional or intentional, can lead to changes in topographic images and dI/dV spectra. We consider the possibility of utilizing functionalized tips in order to improve the sensitivity of STM experiments to local irregularities at the surface or hidden below the surface layers. The change in the tip symmetry can radically alter the contrast of the topographic image due to changes in tip-surface overlap. The dI/dV curves change their shape according to which sample bands the tip orbital tends to overlap. In addition, relative phases between competing tunneling channels …
Reconstructing The Bulk Fermi Surface And Superconducting Gap Properties From Neutron Scattering Experiments, Tanmoy Das, R. Markiewicz, A. Bansil
Reconstructing The Bulk Fermi Surface And Superconducting Gap Properties From Neutron Scattering Experiments, Tanmoy Das, R. Markiewicz, A. Bansil
Arun Bansil
We develop an analytical tool to extract bulk electronic properties of unconventional superconductors from inelastic neutron scattering spectra. We show that the upward and downward branches of the spin excitation spectra have distinct origins, with the upper branch representing a gapped spin-wave dispersion and the lower branch associated with Bogoliubov quasiparticle scattering on the Fermi surface. Combined, they produce an "hourglass" dispersion with 45 degrees rotation of the spectrum, as found experimentally. The downward dispersion can be inverted to reveal the Fermi momentum dispersion of the single-particle spectrum as well as the corresponding superconducting (SC) gap function, analogously to the …
Competing Order Scenario Of Two-Gap Behavior In Hole-Doped Cuprates, Tanmoy Das, R. Markiewicz, A. Bansil
Competing Order Scenario Of Two-Gap Behavior In Hole-Doped Cuprates, Tanmoy Das, R. Markiewicz, A. Bansil
Arun Bansil
Angle-dependent studies of the gap function provide evidence for the coexistence of two distinct gaps in hole doped cuprates, where the gap near the nodal direction scales with the superconducting transition temperature Tc, while that in the antinodal direction scales with the pseudogap temperature. We present model calculations which show that most of the characteristic features observed in the recent angle-resolved photoemission spectroscopy (ARPES) as well as scanning tunneling microscopy (STM) two-gap studies are consistent with a scenario in which the pseudogap has a non-superconducting origin in a competing phase. Our analysis indicates that, near optimal doping, superconductivity can quench …
Competing Order Scenario Of Two-Gap Behavior In Hole-Doped Cuprates, Tanmoy Das, R. S. Markiewicz, A. Bansil
Competing Order Scenario Of Two-Gap Behavior In Hole-Doped Cuprates, Tanmoy Das, R. S. Markiewicz, A. Bansil
Robert Markiewicz
Angle-dependent studies of the gap function provide evidence for the coexistence of two distinct gaps in hole doped cuprates, where the gap near the nodal direction scales with the superconducting transition temperature Tc, while that in the antinodal direction scales with the pseudogap temperature. We present model calculations which show that most of the characteristic features observed in the recent angle-resolved photoemission spectroscopy (ARPES) as well as scanning tunneling microscopy (STM) two-gap studies are consistent with a scenario in which the pseudogap has a non-superconducting origin in a competing phase. Our analysis indicates that, near optimal doping, superconductivity can quench …