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Full-Text Articles in Physics

Chiral Light Intrinsically Couples To Extrinsic/Pseudo-Chiral Metasurfaces Made Of Tilted Gold Nanowires, Alessandro Belardini, Marco Centini, Grigore Leahu, David C. Hooper, Roberto Li Voti, Eugenio Fazio, Joseph W. Haus, Andrew Sarangan, Ventsislav K. Valev, Concita Sibilia Feb 2017

Chiral Light Intrinsically Couples To Extrinsic/Pseudo-Chiral Metasurfaces Made Of Tilted Gold Nanowires, Alessandro Belardini, Marco Centini, Grigore Leahu, David C. Hooper, Roberto Li Voti, Eugenio Fazio, Joseph W. Haus, Andrew Sarangan, Ventsislav K. Valev, Concita Sibilia

Andrew Sarangan

Extrinsic or pseudo-chiral (meta)surfaces have an achiral structure, yet they can give rise to circular dichroism when the experiment itself becomes chiral. Although these surfaces are known to yield differences in reflected and transmitted circularly polarized light, the exact mechanism of the interaction has never been directly demonstrated. Here we present a comprehensive linear and nonlinear optical investigation of a metasurface composed of tilted gold nanowires. In the linear regime, we directly demonstrate the selective absorption of circularly polarised light depending on the orientation of the metasurface. In the nonlinear regime, we demonstrate for the first time how second harmonic …


Monoclinic Optical Constants, Birefringence, And Dichroism Of Slanted Titanium Nanocolumns Determined By Generalized Ellipsometry, Daniel Schmidt, Benjamin Booso, Tino Hofmann, Eva Schubert, Andrew Sarangan, Mathias Schubert Sep 2015

Monoclinic Optical Constants, Birefringence, And Dichroism Of Slanted Titanium Nanocolumns Determined By Generalized Ellipsometry, Daniel Schmidt, Benjamin Booso, Tino Hofmann, Eva Schubert, Andrew Sarangan, Mathias Schubert

Andrew Sarangan

Generalized spectroscopic ellipsometry determines the principal monoclinic optical constants of thin films consisting of slanted titanium nanocolumns deposited by glancing angle deposition under 85° incidence and tilted from the surface normal by 47°. Form birefringence measured for wavelengths from 500 to 1000 nm renders the Ti nanocolumns monoclinic absorbing crystals with c-axis along the nanocolumns, b-axis parallel to the film interface, and 67.5° monoclinic angle between the aand c-axes. The columnar thin film reveals anomalous optical dispersion, extreme birefringence, strong dichroism, and differs completely from bulk titanium. Characteristic bulk interband transitions are absent in the spectral range investigated.