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Full-Text Articles in Physics

Exploring Laser Induced Breakdown Spectroscopy (Libs) For Post-Detonation Nuclear Forensics Debris Analysis, Justin Knoll, Chad Schools, David Fobar Mar 2019

Exploring Laser Induced Breakdown Spectroscopy (Libs) For Post-Detonation Nuclear Forensics Debris Analysis, Justin Knoll, Chad Schools, David Fobar

Purdue Workshop on Nonproliferation: Technology and Approaches

In the unlikely but catastrophic event of a nuclear terrorist attack our government leadership will need reliable information to rapidly inform critical decisions. This research explores the use of Laser Induced Breakdown Spectroscopy (LIBS) as a potential analysis tool in the National Technical Nuclear Forensics process. The current state of post detonation nuclear forensics requires ground and air samples be collected and shipped to state-of-the-art laboratories for radiochemical analysis. The samples undergo many measurements and useable data is produced as these measurements are completed. This data flows back into the process to guide additional measurements and inform the process of …


Thermal Neutron Analysis For Improvised Explosive Device Detection, Matthew David Marziale Mar 2016

Thermal Neutron Analysis For Improvised Explosive Device Detection, Matthew David Marziale

Open Access Dissertations

In this dissertation, the design of a system to detect improvised explosive devices is considered. The technique utilized is thermal neutron analysis. In this method, thermal neutrons are used to interrogate a volume for the presence of nitrogen, which is used as an indicator of explosive, given its unusual high energy line in the gamma ray spectrum generated by thermal capture reactions on explosive material. The performance of the system is then considered for a number of devices used to represent an improvised explosive device, including a 155 mm shell, an antitank mine, and a air to surface bomb. The …


Effect Of Helium Ions Energy On Molybdenum Surfaces Under Extreme Conditions, Joseph Fiala, Jitendra K. Tripathi, Sean Gonderman, Ahmed Hassanein Aug 2015

Effect Of Helium Ions Energy On Molybdenum Surfaces Under Extreme Conditions, Joseph Fiala, Jitendra K. Tripathi, Sean Gonderman, Ahmed Hassanein

The Summer Undergraduate Research Fellowship (SURF) Symposium

Plasma facing components (PFCs) in fusion devices must be able to withstand high temperatures and erosion due to incident energetic ion radiations. Tungsten has become the material of choice for PFCs due to its high strength, thermal conductivity, and low erosion rate. However, its surface deteriorates significantly under helium ion irradiation in fusion-like conditions and forms nanoscopic fiber-like structures, or fuzz. Fuzz is brittle in nature and has relatively lower thermal conductivity than that of the bulk material. Small amounts of fuzz may lead to excessive contamination of the plasma, preventing the fusion reaction from taking place. Despite recent efforts, …


An Investigation Into The Phenomenological Relation Between Solar Activity And Nuclear Beta-Decay Rates, Tasneem M. Mohsinally Apr 2015

An Investigation Into The Phenomenological Relation Between Solar Activity And Nuclear Beta-Decay Rates, Tasneem M. Mohsinally

Open Access Dissertations

We investigate experimental evidence for time-varying nuclear decay rates, in contrast to the widely-accepted view that nuclear decaying isotopes disintegrate at a constant rate unaffected by external conditions. We study several past cases of radioactive isotopes exhibiting annual periodicities in their decay rates, presumably related to the annual variation in Earth-Sun distance. Following recent indications of shorter-lived anomalies in 54Mn decay rates concomitant with an X-class flare in 2006, we attempt to design and develop a series of unique signal detection algorithms to identify regions of anomalous activity in a nuclear decay signal. With stringent threshold cut-offs and filtering …


Hydrogen Loading System Development And Evaluation Of Tritiated Substrates To Optimize Performance In Tritium Based Betavoltaics, Thomas E. Adams Oct 2014

Hydrogen Loading System Development And Evaluation Of Tritiated Substrates To Optimize Performance In Tritium Based Betavoltaics, Thomas E. Adams

Open Access Dissertations

State-of-the-art hydrogen loading system onto thin metallic films based on differential pressure in calibrated chambers has been developed for conditions pressures and temperatures up to 69 bar and 500°C, respectively. Experiments on hydrogen loading on to palladium films of thickness 50 and 250 nm were conducted at pressure ranging from 0.2 bar to 10 bar at temperature 310°C. For first time film hydrogen loading was carried out at 1 bar and at room temperature which temperature. Beta flux exiting surface of metal tritide films has been modeled with MC-SET (Monte Carlo Simulation of Electron Trajectories in solids). Surface beta flux …


Double-Pulse Nd:Yag-Co2 Libs Excitation For Bulk And Trace Analytes, Jason R. Becker, Patrick Skrodzki, Prasoon Diwakar, Sivanandan Harilal, Ahmed Hassanein Aug 2014

Double-Pulse Nd:Yag-Co2 Libs Excitation For Bulk And Trace Analytes, Jason R. Becker, Patrick Skrodzki, Prasoon Diwakar, Sivanandan Harilal, Ahmed Hassanein

The Summer Undergraduate Research Fellowship (SURF) Symposium

Laser-induced breakdown spectroscopy [LIBS] is a commonly used technique for multi-element analyses for various applications such as space exploration, nuclear forensics, environmental analysis, process monitoring. The advantages of the LIBS technique include robustness, ease of use, field portability, and real-time, non-invasive multi-element analyses. However, in comparison to other lab based analytical techniques, it suffers from low precision and low sensitivity. In order to overcome these drawbacks, various approaches have been used, including double-pulse LIBS [DPLIBS]. Typically, various wavelength combinations of two Nd: yttrium aluminum garnet [YAG] lasers have been used for DPLIBS. However, the use of long wavelength (CO2 …


Doube-Pulse Laser-Induced Breakdown Spectroscopy Of Multi-Element Sample Containing Low- And High-Z Analytes, Patrick J. Skrodzki, Jason R. Becker, Prasoon K. Diwakar Ph. D., Sivanandan S. Harilal Ph. D., Ahmed Hassanein Ph. D. Aug 2014

Doube-Pulse Laser-Induced Breakdown Spectroscopy Of Multi-Element Sample Containing Low- And High-Z Analytes, Patrick J. Skrodzki, Jason R. Becker, Prasoon K. Diwakar Ph. D., Sivanandan S. Harilal Ph. D., Ahmed Hassanein Ph. D.

The Summer Undergraduate Research Fellowship (SURF) Symposium

Laser-induced breakdown spectroscopy (LIBS) is a portable, remote, non-invasive analytical technique which effectively distinguishes neutral and ionic species for a range of low- to high-Z elements in a multi-element target. Subsequently, LIBS holds potential in special nuclear material (SNM) sensing and nuclear forensics requiring minimal sample preparation and detecting isotopic shifts which allows for differentiation in SNM (namely U) enrichment levels. Feasible applications include not only nonproliferation and homeland security but also nuclear fuel prospecting and industrial safeguard endorsement. Elements of higher mass with complex atomic structures, such as U, however, result in crowded emission spectra with LIBS, and characteristic …


Characterizing New Calibration Sources In Liquid Xenon Dark Matter Searches, Evan P. Bray, Rafael Lang, Sean Macmullin Aug 2014

Characterizing New Calibration Sources In Liquid Xenon Dark Matter Searches, Evan P. Bray, Rafael Lang, Sean Macmullin

The Summer Undergraduate Research Fellowship (SURF) Symposium

In order to use the XENON1T liquid xenon detector as a means for detecting dark matter, the response to nuclear and electronic recoils must be well calibrated. Electronic-recoil calibration of XENON1T will be done by using the noble gas radon-220 that emanates from a custom thorium-228 source to observe the electron recoils that its daughter elements induce in liquid xenon. A silicon PIN diode was constructed to ensure that the Th228 source does not contaminate the system with the long-lived isotopes Th228 (T1/2 of 1.9 y) or Radium-224 (T1/2 of 3.6 d). The PIN diode was fixed in a custom …


Investigation Of Time Varying Nuclear Decay Rates, Peter G. Barton, Rafael F. Lang Oct 2013

Investigation Of Time Varying Nuclear Decay Rates, Peter G. Barton, Rafael F. Lang

The Summer Undergraduate Research Fellowship (SURF) Symposium

Since the discovery of radioactive decay, radioactive decay rates have consistently shown to be constant. Recently, groups of researchers around the world have noticed variation in the decay rates of different radioactive isotopes, while other groups have noticed no such effect. If the variation is truly varying decay rates, this would imply groundbreaking new physics and would have implications for practices such as carbon dating. More sophisticated experiments are required to determine if the variations are truly new physics or systematic effects inherent to nuclear decay experiments. We are building an experiment where activity data from various radioactive sources will …