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Iowa State University

Series

Materials Science and Engineering

2013

Ames Laboratory Publications

Physics and Astronomy

Articles 1 - 4 of 4

Full-Text Articles in Physics

Two-Dimensional Magnetic Interactions In Lafeaso, Mehmet Ramazanoglu, J. Lamsal, Gregory S. Tucker, J.-Q. Yan, S. Calder, T. Guidi, T. Perring, R. William Mccallum, Thomas A. Lograsso, Andreas Kreyssig, Robert J. Mcqueeney Apr 2013

Two-Dimensional Magnetic Interactions In Lafeaso, Mehmet Ramazanoglu, J. Lamsal, Gregory S. Tucker, J.-Q. Yan, S. Calder, T. Guidi, T. Perring, R. William Mccallum, Thomas A. Lograsso, Andreas Kreyssig, Robert J. Mcqueeney

Ames Laboratory Publications

Inelastic neutron scattering measurements demonstrate that the magnetic interactions in antiferromagnetic LaFeAsO are two dimensional. Spin-wave velocities within the Fe layer and the magnitude of the spin gap are similar to the AFe2As2 based materials. However, the ratio of interlayer and intralayer exchange is found to be less than ∼10−4 in LaFeAsO, very similar to the cuprates, and ∼100 times smaller than that found in AFe2As2 compounds. The results suggest that the effective dimensionality of the magnetic system is highly variable in the parent compounds of the iron arsenides and weak three-dimensional interactions ...


Upper Critical Field Of High-Quality Single Crystals Of Kfe2as2, Yong Liu, Makariy A. Tanatar, Vladimir G. Kogan, Hyunsoo Kim, Thomas A. Lograsso, Ruslan Prozorov Apr 2013

Upper Critical Field Of High-Quality Single Crystals Of Kfe2as2, Yong Liu, Makariy A. Tanatar, Vladimir G. Kogan, Hyunsoo Kim, Thomas A. Lograsso, Ruslan Prozorov

Ames Laboratory Publications

Measurements of temperature-dependent in-plane resistivity ρ(T) were used to determine the upper critical field and its anisotropy in high-quality single crystals of the stoichiometric iron arsenide superconductor KFe2As2. The crystals were characterized by the residual resistivity ratio ρ(300 K)/ρ(0) up to 3000 and the resistive transition midpoint temperature Tc=3.8 K, significantly higher than in previous studies on the same material. We find increased Hc2(T) for both directions of the magnetic field, which scale with the increased Tc. This unusual linear Hc2(Tc) scaling is not ...


Magnetism-Dependent Phonon Anomaly In Lafeaso Observed Via Inelastic X-Ray Scattering, S. E. Hahn, Gregory S. Tucker, J.-Q. Yan, A. H. Said, B. M. Leu, R. William Mccallum, E. E. Alp, Thomas A. Lograsso, Robert J. Mcqueeney, Bruce N. Harmon Mar 2013

Magnetism-Dependent Phonon Anomaly In Lafeaso Observed Via Inelastic X-Ray Scattering, S. E. Hahn, Gregory S. Tucker, J.-Q. Yan, A. H. Said, B. M. Leu, R. William Mccallum, E. E. Alp, Thomas A. Lograsso, Robert J. Mcqueeney, Bruce N. Harmon

Ames Laboratory Publications

The phonon dispersion was measured at room temperature along (0,0,L) in the tetragonal phase of LaFeAsO using inelastic x-ray scattering. Spin-polarized first-principles calculations imposing various types of antiferromagnetic order are in better agreement with the experimental results than nonmagnetic calculations, although the measurements were made well above the magnetic ordering temperature, TN. Splitting observed between two A1g phonon modes at 22 and 26 meV is only reproduced in spin-polarized calculations. Magnetostructural effects similar to those observed in the AFe2As2 (A=Ca,Sr,Ba,Eu) materials are present in LaFeAsO. The inclusion of Fe ...


Native Defects In Tetradymite Bi2(Texse3−X) Topological Insulators, Linlin Wang, Mianliang Huang, Srinivasa Thimmaiah, Aftab Alam, Sergey L. Bud'ko, Adam Kaminski, Thomas A. Lograsso, Paul C. Canfield, Duane D. Johnson Mar 2013

Native Defects In Tetradymite Bi2(Texse3−X) Topological Insulators, Linlin Wang, Mianliang Huang, Srinivasa Thimmaiah, Aftab Alam, Sergey L. Bud'ko, Adam Kaminski, Thomas A. Lograsso, Paul C. Canfield, Duane D. Johnson

Ames Laboratory Publications

Formation energies of native defects in Bi2(TexSe3−x), with comparison to ideal Bi2Te2S, are calculated in density-functional theory to assess transport properties. Bi2Se3 is found to be n type for both Bi- and Se-rich growth conditions, while Bi2Te3 changes fromn to p type going from Te- to Bi-rich conditions, as observed. Bi2Te2Se and Bi2Te2S are generally n type, explaining observed heavily doped n-type behavior in most samples. A (0/−) transition level at 16 meV above valence-band maximum ...