Physics Commons^™

Fragmentation Processes Following Core Excitation In Acetylene And Ethylene By Partial Ion Yield Spectroscopy, Maria Novella Piancastelli, Wayne C. Stolte, Gunnar Ohrwall, S-W Yu, D. Bull, K. Lantz, Alfred S. Schlachter, Dennis W. Lindle

Chemistry and Biochemistry Faculty Research

Partial ion yield spectroscopy provides a very detailed picture of fragmentation processes following core excitation in isolated molecules. We exploit this potential in the analysis of decay processes following C1s→π and C1s→Rydberg excitations in ethylene and acetylene. We show that the relative intensity of spectral features related to the excitation to empty molecular orbitals or to Rydberg states is a function of the time variation of the fragmentation process. Namely, we see an intensity increase in the Rydberg states compared to the molecular orbitals as the fragmentation process becomes more extensive, a result attributable to the diffuse nature of the …

Simultaneous Trapping Of Rubidium And Metastable Argon In A Magneto-Optical Trap, C. I. Sukenik, H. C. Busch

Physics Faculty Publications

We have simultaneously confined rubidium and metastable argon in a dual-species magneto-optical trap (MOT). Here a binary mixture of atomic species from different groups of the periodic table have been optically confined at ultracold temperatures. We describe the apparatus and characterize the individual, single species MOTs and the dual-species MOT. Both fluorescence and ion production are monitored. With both species trapped, we observe ~5106 85Rb atoms and ~2106 40Ar* atoms. Realization of the dual-species trap opens the way for detailed studies of Penning and associative ionization, photoassociative spectroscopy, and eventually for the production of bound, ultracold RbAr molecules.

Ion Contribution To The Astrophysical Important 447.15, 587.56 And 667.82 Nm He I Spectral Lines Broadening, Vladimir Milosavljevic, Stevan Djenize

Articles

Characteristics of the astrophysical important Stark broadened 447.15 nm, 587.56 nm and 667.82 nm spectral line profiles have been measured at electron densities between 0.3 10 and 8.2 10 m and electron temperatures between 8000 and 33 000 K in plasmas created in five various discharge conditions using a linear, low-pressure, pulsed arc as an optically thin plasma source operated in a helium-nitrogen-oxygen gas mixture. On the basis of the observed asymmetry of the line profiles we have obtained their ion broadening parameters ( A) caused by influence of the ion microfield on the line broadening mechanism and also …

Dephasing Model For Spatially Extended Atomic States In Cyclotronlike Resonances, R E. Wagner, S Radovich, J Gillespie, Q Su, Rainer Grobe

Faculty publications – Physics

In recent work, the formation of ring-shaped electron distributions for hydrogen atoms in resonant static magnetic-laser fields has exclusively been associated with the impact of relativity. In this note we will generalize this statement and show that the nonlinearity associated with the nuclear binding force can trigger similarly shaped steady-state charge clouds in atoms under suitable conditions. The dephasing model, based on modeling the quantum-mechanical state by a classical ensemble of quasiparticles evolving with slightly different cyclotron periods, can recover features, in the two lowest-order resonances as well as the Coulomb-field-induced charge distributions.

Holographic Analysis Of Diffraction Structure Factors, S. Marchesini, N. Mannella, C. S. Fadley, M. A. Van Hove, J. J. Bucher, D. K. Shuh, L. Fabris, M. J. Press, M. W. West, Wayne C. Stolte, Z. Hussain

Chemistry and Biochemistry Faculty Research

We combine the theory of inside-source/inside-detector x-ray fluorescence holography and Kossel lines/x ray standing waves in kinematic approximation to directly obtain the phases of the diffraction structure factors. The influence of Kossel lines and standing waves on holography is also discussed. We obtain partial phase determination from experimental data obtaining the sign of the real part of the structure factor for several reciprocal lattice vectors of a vanadium crystal.

Non-Dipolar Electron Angular Distributions From Fixed-In-Space Molecules, Renaud Guillemin, Oliver Hemmers, Dennis W. Lindle, E. Shigemasa, K. Le Guen, D. Ceolin, C. Miron, N. Leclercq, P. Morin, Marc Simon, P. W. Langhoff

Environmental Studies Faculty Publications

The first indication of nondipole effects in the azimuthal dependence of photoelectron angular distributions emitted from fixed-in-space molecules is demonstrated in N₂. Comparison of the results with angular distributions observed for randomly oriented molecules and theoretical derivations for the nondipole correction first order in photon momentum suggests that higher orders will be needed to describe distributions measured in the molecular frame.

In-Situ X-Ray-Absorption Spectroscopy Study Of Hydrogen Absorption By Nickel-Magnesium Thin Films, B. Farangis, Ponnusamy Nachimuthu, T. J. Richardson, J. L. Slack, Rupert C. Perera, Eric M. Gullikson, Dennis W. Lindle, M. Rubin

Chemistry and Biochemistry Faculty Research

Structural and electronic properties of co-sputtered Ni-Mg thin films with varying Ni to Mg ratio were studied by in-situ x-ray absorption spectroscopy in the Ni L-edge and Mg K-edge regions. Co-deposition of the metals led to increased disorder and decreased coordination around Ni and Mg compared to pure metal films. Exposure of the metallic films to hydrogen resulted in formation of hydrides and increased disorder. The presence of hydrogen as a near neighbor around Mg caused a drastic reduction in the intensities of multiple scattering resonances at higher energies. The optical switching behavior and changes in the x-ray spectra varied …

Electric-Field-Induced Relativistic Larmor-Frequency Reduction, P Krekora, Q Su, Rainer Grobe

Faculty publications – Physics

Using the numerical solution to the time-dependent Dirac equation we show that the effect of relativity on the usual Larmor period for an electron in a magnetic field can be enhanced drastically if a suitably scaled and aligned static electric field is added to the interaction. This electric field does not change the electron's speed but leads to an elliptical spin precession due to relativity. This spin precession is accompanied by a position-dependent spin distribution.

Higher-Order Evaluation Of The Critical Temperature For Interacting Homogeneous Dilute Bose Gases, Frederico F. F. De Souza Cruz, Marcus Pinto, Rudnei O. Ramos, Paulo Sena

Dartmouth Scholarship

We use the nonperturbative linear δ expansion method to evaluate analytically the coefficients c1 and c''2 that appear in the expansion for the transition temperature for a dilute, homogeneous, three-dimensional Bose gas given by Tc=T0(1+c1an1/3+[c′2ln(an1/3)+c''2]a2n2/3+O(a3n)), where T0 is the result for an ideal gas, a is the s-wave scattering length, and n is the number density. In a previous work the same method has been used to evaluate c1 to order δ2 with the result c1=3.06. Here, we push the calculation to the next two orders obtaining c1=2.45 at order δ3 and c1=1.48 at order δ4. Analyzing the topology …

Photoexcitation Of A Dipole-Forbidden Resonance In Helium, B. Krassig, E. P. Kanter, S. H. Southworth, Renaud Guillemin, Oliver Hemmers, Dennis W. Lindle, R. Wehlitz, N. L. S. Martin

Environmental Studies Faculty Publications

We have observed photoexcitation of the dipole-forbidden 1s²¹S₀→2p²¹D₂ resonance in helium by measuring the nondipolar forward-backward asymmetry of photoelectron angular distributions in the 2ℓ2ℓ^′ autoionizing region. By exploiting the electric dipole-quadrupole interference in the excitation of both the 2s2p¹P₁ and 2p²¹D₂ levels, we have observed the quadrupole resonance in photoabsorption and extracted its Fano line shape parameters and the relative phase of the 1sEp and 1sEd continua. We find the quadrupole line profile index q₂ to be markedly different from theoretical expectations.

Nonlinear Dynamics Of Mode-Locking Optical Fiber Ring Lasers, Kristin M. Spaulding, Darryl H. Yong, Arnold D. Kim, J Nathan Kutz

All HMC Faculty Publications and Research

We consider a model of a mode-locked fiber ring laser for which the evolution of a propagating pulse in a birefringent optical fiber is periodically perturbed by rotation of the polarization state owing to the presence of a passive polarizer. The stable modes of operation of this laser that correspond to pulse trains with uniform amplitudes are fully classified. Four parameters, i.e., polarization, phase, amplitude, and chirp, are essential for an understanding of the resultant pulse-train uniformity. A reduced set of four coupled nonlinear differential equations that describe the leading-order pulse dynamics is found by use of the variational nature …

Coherent Vs Incoherent Interlayer Transport In Layered Metals, Gary L. Gard, J. Wosnitza, J. Hagel, J. S. Qualls, J. S. Brooks, E. Balthes, D. Schweitzer, J. A. Schlueter, U. Geiser, Javid Mohtasham, Rolf Walter Winter

Chemistry Faculty Publications and Presentations

The magnetic-field, temperature, and angular dependence of the interlayer magnetoresistance of two different quasi-two-dimensional (2D) organic superconductors is reported. For k -BEDT-TTF)₂I₃, where BEDTTTF is bisethylenedithio-tetrathiafulvalene, we find a well-resolved peak in the angle-dependent magnetoresistance at Q590°(field parallel to the layers). This clear-cut proof for the coherent nature of the interlayer transport is absent for β″–(BEDT-TTF)₂SF₅CH₂CF₂SO₃. This and the nonmetallic behavior of the magnetoresistance suggest an incoherent quasiparticle motion for the latter 2D metal.

Parity Violation In Neutron Resonances Of Palladium, D A. Smith, J D. Bowman, Bret E. Crawford, C A. Grossmann, T Haseyama, A Masaike, Y Matsuda, G E. Mitchell, S I. Penttila, N R. Roberson, S J. Seestrom, E I. Sharapov, Sharon L. Stephenson, V W. Yuan

Physics and Astronomy Faculty Publications

Parity violation in p-wave neutron resonances of the palladium isotopes 104, 105, 106, and 108 has been measured by transmission of a longitudinally polarized neutron beam through a natural palladium target. The measurements were performed at the pulsed spallation neutron source of Los Alamos Neutron Science Center. The rms weak interaction matrix elements and the corresponding spreading widths were determined for 104 Pd, 105 Pd, and 106 Pd

A Rf Discharge Cell For Saturated Absorption Spectroscopy Of Metastable Argon, C. I. Sukenik, H. C. Busch

Physics Faculty Publications

We have produced a rf discharge in 40Ar and used saturated absorption spectroscopy to offset lock a Ti:Sapphire laser to the absorption peak of the 43P243D3 cooling transition at 811 nm. We describe the procedure for fabrication of the cell and production of the discharge.

Stark Shifts And Transition Probabilities In The Ne Ii Spectrum, Stevan Djenize, Vladimir Milosavljevic, Milan S. Dimitrijevic

Articles

Stark shifts (d) and transition probabilities of the spontaneous emission (Einstein's A values) of forty two singly charged neon ( ) ion spectral lines have been measured in a linear, low pressure, pulsed arc at 35 300 K electron temperature and 1.83 10 ²³ m ^-3 electron density. Transition probabilities have been obtained using the relative line intensity ratio (RLIR) method. Stark shift values have also been calculated, using the semiclassical perturbation formalism (SCPF). The measured and calculated shift values and the measured A values have been compared to the existing data taken from available data sources.

Specification Of Jecp/Sp: Stereographic Projection With An Application For Specimen Orientation Adjustment Using Tem Holders, Xingzhong Li

Nebraska Center for Materials and Nanoscience: Faculty Publications

1. Purpose of the program 2. Graphic user interface and program design 3. Crystallographic principle and implementation 4. System requirement 5. Installation and user instruction 6. How to contact the author 7. References

1. Purpose of the program JECP/SP is a computer program in Java Electron Crystallography Package. JECP is developed for quantitative electron diffraction and image processing, the package is designed and written by Dr. XingZhong Li. JECP/SP provides the all necessary functions of stereographic projection for regular application and furthermore it can be used to minimized the difficulties encountered when tilting highly beam-sensitive, or small-grain-size specimens with known …

Exploring The Limits Of The Dipole Approximation With Angle-Resolved Electron Time-Of-Flight Spectrometry, Sierra Laidman, Monica Pangilinan, Renaud Guillemin, Sung Woo Yu, Gunnar Ohrwall, Dennis W. Lindle, Oliver Hemmers

Environmental Studies Faculty Publications

Understanding the electronic structure of atoms and molecules is fundamental in determining their basic properties as well as the interactions that occur with different particles such as light. One such interaction is single photoionization; a process in which a photon collides with an atom or molecule and an electron with a certain kinetic energy is emitted, leaving behind a residual ion. Theoretical models of electronic structures use the dipole approximation to simplify x-ray interactions by assuming that the electromagnetic field of the radiation, expressed as a Taylor-series expansion, can be simplified by using only the first term. It has been …

The Effect Of Phase Separation On Charge Ordering State In La12xcaxmno3 (X ¼ 1/2, 2/3, And 3/4), H. D. Zhou, G. Li, S. J. Feng, Y. Liu, T. Qian, Xiaojuan Fan, X. G. Li

Physics Faculty Research

The magnetic phase separation characteristics are found in manganese perovskite La_1/3Ca_2/3MnO₃ by electron spin resonance (ESR) and magnetization measurements. An extra resonance signal observed in ESR spectra just above the charge ordering (CO) temperature T_CO provides strong evidence for the existence of ferromagnetic (FM) clusters near the CO state. The investigation of the resistivity of La_1-xCa_xMnO₃ (x=1/2, 2/3, and 3/4) in different magnetic fields up to 14 T shows that the effect of magnetic fields on CO state decreases with increasing x. Our results indicate that the percolative characteristics …

Jecp/Ed Manual, Xingzhong Li

Nebraska Center for Materials and Nanoscience: Faculty Publications

JECP/ED is a Java program with graphic interface for simulating electron diffraction pattern. It is designed and written by Dr. Xingzhong in University of Nebraska- Lincoln. This is verision 12-2002. It can be used for simulating electron diffraction zone pattern(ZOLZ with/without FOLZ), it allows to select zone axis, high voltage, sample thickness in the simulation, optional to show index, intensity and Laue center, featureed with manuniplating the pattern with slightly tilting, 360 degree rotation, zoom. The diffraction intensity is calculated on the basis of the kinematical theory. The program is extended to simulate electron diffraction with a precession of incident …

Atomic Hydrogen Cleaning Of Inp(100): Electron Yield And Surface Morphology Of Negative Electron Affinity Activated Surfaces, M. A. Hafez, H. E. Elsayed-Ali

Electrical & Computer Engineering Faculty Publications

Atomic hydrogen cleaning of the InP(100) surface has been investigated using quantitative reflection high-energy electron diffraction. The quantum efficiency of the surface when activated to negative electron affinity was correlated with surface morphology. The electron diffraction patterns showed that hydrogen cleaning is effective in removing surface contaminants, leaving a clean, ordered, and (2×4)-reconstructed surface. After activation to negative electron affinity, a quantum efficiency of ∼6% was produced in response to photoactivation at 632 nm. Secondary electron emission from the hydrogen-cleaned InP(100)-(2×4) surface was measured and correlated to the quantum efficiency. The morphology of the vicinal InP(100) surface was investigated using …

Acceleration Element For Femtosecond Electron Pulse Compression, Bao-Liang Qian, Hani E. Elsayed-Ali

Electrical & Computer Engineering Faculty Publications

An acceleration element is proposed for compressing the electron pulse duration in a femtosecond photoelectron gun. The element is a compact metal cavity with curved-shaped walls. An external voltage is applied to the cavity where a special electric field forms in such a way that the slow electrons in the electron pulse front are accelerated more than the fast electrons, and consequently the electron pulse duration will be compressed. The distribution of the electric field inside the acceleration cavity is analyzed for the geometry of the cavity. The electron dynamics in this acceleration cavity is also investigated numerically. Numerical results …

Electron Pulse Broadening Due To Space Charge Effects In A Photoelectron Gun For Electron Diffraction And Streak Camera Systems, Bao-Liang Qian, Hani E. Elsayed-Ali

Electrical & Computer Engineering Faculty Publications

The electron pulse broadening and energy spread, caused by space charge effects, in a photoelectron gun are studied analytically using a fluid model. The model is applicable in both the photocathode-to-mesh region and the postanode electron drift region. It is found that space charge effects in the photocathode-to-mesh region are generally unimportant even for subpicosecond pulses. However, because of the long drift distance, electron pulse broadening due to space charge effects in the drift region is usually significant and could be much larger than the initial electron pulse duration for a subpicosecond electron pulse. Space charge effects can also lead …

Neutron Resonance Spectroscopy Of 104pd, 105pd, And 110pd, J D. Bowman, D A. Smith, Bret E. Crawford, T Haseyama, C A. Grossmann, A Masaike, Y Matsuda, G E. Mitchell, S I. Penttila, N R. Roberson, S J. Seestrom, E I. Sharapov, Sharon L. Stephenson, V W. Yuan, A M. Sukhovoj

Physics and Astronomy Faculty Publications

We have measured neutron resonances in the palladium isotopes 104, 105, and 110 for neutron energies from 1 to 2100 eV. Many new p-wave resonances have been observed. Their neutron widths and, in several cases, the radiative widths were measured. The average level spacings and the s-wave and p-wave neutron strength functions were determined. The time-of-flight method was used for both neutron total cross section measurements and total (n,γ) reaction yield measurements at the pulsed spallation neutron source of Los Alamos Neutron Science Center. Well established resonance spectroscopy for these isotopes is essential for the analysis of parity violation data …

Phase And Absorption Gratings For Electrons, Hong Gao, Glen Gronniger, Daniel Friemund, Alex Cronin

Department of Physics and Astronomy: Faculty Publications

We report the experimental realization of phase and absorption gratings for electrons. Phase gratings made with standing waves of light with a periodicity of 266 nm are used to diffract 380 eV electrons [1]. Material gratings of 100 and 200 nm periodicity are used to diffract 500 eV electrons. We are exploring the possibility to use these gratings for low energy electron interferometry.