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Full-Text Articles in Atmospheric Sciences

Initiation Criteria For The Onset Of Geomagnetic Substorms Based On Auroral Observations And Electrojet Current Signatures, Mayowa Michael Kayode-Adeoye Dec 2023

Initiation Criteria For The Onset Of Geomagnetic Substorms Based On Auroral Observations And Electrojet Current Signatures, Mayowa Michael Kayode-Adeoye

<strong> Theses and Dissertations </strong>

In recent years, several substorm onset criteria have been developed, either from auroral observations (many authors) or from auroral electrojet properties such as those described by (Forsyth et al., 2015; Maimaiti et al., 2019; Newell & Gjerloev, 2011; Partamies et al., 2011) The different criteria are being investigated using a low order physics model of the magnetosphere called WINDMI (Spencer et al., 2009) and inferences are being made in line with the WINDMI model. The model variables will be compared with the criteria for substorm onset proposed by examining the SML index.

The WINDMI model uses solar wind and IMF …


Effect Of Morphology And An Upstream Tall Building On A Street Canyon Flow, Haoran Du Jul 2023

Effect Of Morphology And An Upstream Tall Building On A Street Canyon Flow, Haoran Du

Electronic Thesis and Dissertation Repository

The effects of the morphological model and the existence of an upstream tall building on the turbulent street canyon flow and the overlying boundary layer are investigated in a wind tunnel, using Stereoscopic Particle Image Velocimetry (S-PIV) measurements. The velocity variances, Reynolds shear stress, and turbulent kinetic energy are found to be larger than in a similar idealized street canyon model. Increasing building height results in a decrease in vertical mass fluxes across the opening of the canyon, at least in the canyon portion directly downstream of the building. The interaction between the large-scale structures in the overlying boundary layer …


Identifying Particulate Matter Spatial Variation In The El Paso Del Norte Region Using Land-Use Regression Modeling And Data Obtained From A Network Of Low-Cost Sensors, Leonardo Demetrio Vazquez-Raygoza Dec 2022

Identifying Particulate Matter Spatial Variation In The El Paso Del Norte Region Using Land-Use Regression Modeling And Data Obtained From A Network Of Low-Cost Sensors, Leonardo Demetrio Vazquez-Raygoza

Open Access Theses & Dissertations

The emergence and rise in popularity of low-cost sensors for atmospheric observation aresetting a new precedent in identifying emission hotspots and providing high-resolution spatial and temporal data. Furthermore, low-cost sensors are becoming popular among institutions and the public, allowing community scientists to become more involved in air quality monitoring. However, concerns about the accuracy and precision of low-cost sensors have been questioned. Most recent research has focused on the utility of real-time monitoring and calibration requirements for these sensors. A low-cost monitoring project has deployed sensors in the El Paso del Norte region in low and high annual average daily …


Impact Of Climate Oscillations/Indices On Hydrological Variables In The Mississippi River Valley Alluvial Aquifer., Meena Raju May 2022

Impact Of Climate Oscillations/Indices On Hydrological Variables In The Mississippi River Valley Alluvial Aquifer., Meena Raju

Theses and Dissertations

The Mississippi River Valley Alluvial Aquifer (MRVAA) is one of the most productive agricultural regions in the United States. The main objectives of this research are to identify long term trends and change points in hydrological variables (streamflow and rainfall), to assess the relationship between hydrological variables, and to evaluate the influence of global climate indices on hydrological variables. Non-parametric tests, MMK and Pettitt’s tests were used to analyze trend and change points. PCC and Streamflow elasticity analysis were used to analyze the relationship between streamflow and rainfall and the sensitivity of streamflow to rainfall changes. PCC and MLR analysis …


Physical Investigation Of Downburst Winds And Applicability To Full Scale Events, Federico Canepa Feb 2022

Physical Investigation Of Downburst Winds And Applicability To Full Scale Events, Federico Canepa

Electronic Thesis and Dissertation Repository

Thunderstorm winds, i.e. downbursts, are cold descending currents originating from cumulonimbus clouds which, upon the impingement on the ground, spread radially with high intensities. The downdraft phase of the storm and the subsequent radial outflow that is formed can cause major issues for aviation and immense damages to ground-mounted structures. Thunderstorm winds present characteristics completely different from the stationary Gaussian synoptic winds, which largely affect the mid-latitude areas of the globe in the form of extra-tropical cyclones. Downbursts are very localized winds in both space and time. It follows that their statistical investigation, by means of classical full scale anemometric …


A Greenhouse Gas Emissions Inventory For Nebraska: Livestock And Coal Loom Large, Eric R. Holley, Adam Liska Jan 2022

A Greenhouse Gas Emissions Inventory For Nebraska: Livestock And Coal Loom Large, Eric R. Holley, Adam Liska

Adam Liska Papers

Mitigation of climate change requires the systematic identification and cataloging of emissions sources at city, state, and national levels. In this study, an inventory of annual greenhouse gas emissions from the state of Nebraska was created based on industry data, and emissions inventories were completed each year from 1990 to 2016. Nebraska’s net emissions were found to increase from 56.2 million metric tons of carbon dioxide equivalents (MMtCO2e) in 1990 to 87.4 MMtCO2e in 2016. Agriculture was found to be the sector with the most emissions (36 MMtCO2e) followed by electricity generation (21 MMtCO …


Data Fusion And Synergy Of Active And Passive Remote Sensing; An Application For Freeze Thaw Detections, Zahra Sharifnezhadazizi Jan 2022

Data Fusion And Synergy Of Active And Passive Remote Sensing; An Application For Freeze Thaw Detections, Zahra Sharifnezhadazizi

Dissertations and Theses

There has been a recent evolvement in the field of remote sensing after increase of number satellites and sensors data which could be fused to produce new data and products. These efforts are mainly focused on using of simultaneous observations from different platforms with different spatial and temporal resolutions. The research dissertation aims to enhance the synergy use of active and passive microwave observations and examine the results in detection land freeze and thaw (FT) predictions. Freeze thaw cycles particularly in high-latitude regions have a crucial role in many applications such as agriculture, biogeochemical transitions, hydrology and ecosystem studies. The …


Indoor Air Quality Through The Lens Of Outdoor Atmospheric Chemistry, Jonathan P.D. Abbatt, Douglas B. Collins Jan 2022

Indoor Air Quality Through The Lens Of Outdoor Atmospheric Chemistry, Jonathan P.D. Abbatt, Douglas B. Collins

Faculty Contributions to Books

Outdoor atmospheric chemistry and air quality have been the topic of research that intensified in earnest around the mid-20th century, while indoor air quality research has only been a key focus of chemical researchers over the last 30 years. Examining practices and approaches employed in the outdoor atmospheric chemistry research enterprise provides an additional viewpoint from which we can chart new paths to increase scientific understanding of indoor chemistry. This chapter explores our understanding of primary chemical sources, homogeneous and multiphase reactivity, gas-surface partitioning, and the coupling between the chemistry and dynamics of indoor air through the lens of …


Recent Advancements In Electrochemical Conversion Of Carbon Dioxide, Nandan Nag, Amit Kumar, Sumit Sharma, Sandeep Kumar, Amit K. Thakur Jan 2022

Recent Advancements In Electrochemical Conversion Of Carbon Dioxide, Nandan Nag, Amit Kumar, Sumit Sharma, Sandeep Kumar, Amit K. Thakur

Civil & Environmental Engineering Faculty Publications

Electrochemical reduction of carbon dioxide into eco-friendly and clean products is a promising approach to eradicate pollution. Although carbon dioxide emission is inhibited by the advent of renewable sources of energy, it is present in the atmosphere and needs to be cleaned. The reduction of carbon dioxide from atmospheric gases can be accomplished by its adsorption and subsequent transportation to electrolytic chambers, where it is reduced to hydrocarbons, organic acids or carbonates. This review focuses on developing a three compartment electrochemical cell to reduce carbon dioxide used as a catholyte. Various factors affecting the electrochemical reduction of carbon dioxide and …


Greenhouse Gas Emissions And Drought Projections For Nebraska, Adam Liska Oct 2021

Greenhouse Gas Emissions And Drought Projections For Nebraska, Adam Liska

Adam Liska Papers

This lecture will focus on three issues. The first is a presentation of data from the first greenhouse gas emissions inventory for the State of Nebraska, which will be published in the coming weeks. In 2016, emissions from beef cattle made up 23% of net state emissions, and coal for electricity made up 23.7% of net state emissions. The second issue to be addressed are the impacts of the 2012 drought on agriculture in Nebraska and the region. The drought of 2012 indicates that future droughts in the 21st century in the region can be a dominant influence on …


Unintended Consequences Of Air Cleaning Chemistry, Douglas B. Collins, Delphine K. Farmer Aug 2021

Unintended Consequences Of Air Cleaning Chemistry, Douglas B. Collins, Delphine K. Farmer

Faculty Journal Articles

Amplified interest in maintaining clean indoor air associated with the airborne transmission risks of SARS-CoV-2 have led to an expansion in the market for commercially available air cleaning systems. While the optimal way to mitigate indoor air pollutants or contaminants is to control (remove) the source, air cleaners are a tool for use when absolute source control is not possible. Interventions for indoor air quality management include physical removal of pollutants through ventilation or collection on filters and sorbent materials, along with chemically reactive processes that transform pollutants or seek to deactivate biological entities. This perspective intends to highlight the …


Do Secondary Cyclones Increase The Category Scale Of Atmospheric Rivers?, Edgar Sanchez Fausto Jun 2021

Do Secondary Cyclones Increase The Category Scale Of Atmospheric Rivers?, Edgar Sanchez Fausto

University Honors Theses

Atmospheric rivers (ARs) play a crucial role in delivering precipitation worldwide. This makes them an important phenomenon for water resource specialists to study. One such interest is to understand what mechanisms make ARs produce significant rainfall and associated hazards such as flooding. One possible mechanism is that AR duration or intensity may increase when it interacts with a secondary cyclone, either of which can increase the AR category scale. The purpose of this study is to determine whether AR and secondary cyclone interactions increase the category scale ARs. Out of 52 AR events analyzed, 32 events contained at least one …


Real-Time Pm10 Emission Rates From Paved Roads By Measurement Of Concentrations In The Vehicle's Wake Using On-Board Sensors Part 2. Comparison Of Scamper, Traker™, Flux Measurements, And Ap-42 Silt Sampling Under Controlled Conditions, Dennis R. Fitz, Kurt Bullimer, Vic Etyemezian, Hampden D. Kuhns, John A. Gillies, George Nikolich, David E. James, Rodney Langston, Russell S. Merle Jr. May 2021

Real-Time Pm10 Emission Rates From Paved Roads By Measurement Of Concentrations In The Vehicle's Wake Using On-Board Sensors Part 2. Comparison Of Scamper, Traker™, Flux Measurements, And Ap-42 Silt Sampling Under Controlled Conditions, Dennis R. Fitz, Kurt Bullimer, Vic Etyemezian, Hampden D. Kuhns, John A. Gillies, George Nikolich, David E. James, Rodney Langston, Russell S. Merle Jr.

Civil and Environmental Engineering and Construction Faculty Research

Representative soil was evenly applied to an 800-m section of road surface. The test area was of sufficient length to allow for measurement at constant speeds of up to 72 km hr−1. SCAMPER and TRAKER™ mobile measurement vehicles made repeated test runs while an instrumented tower measured upwind-downwind horizontal PM10 flux. AP-42 methods were used to collect silt samples and calculate PM10 emission factors. Both silt loadings and vehicle speeds were varied during the experiment. Street sweeping the as-found roadway showed an initial rise in PM10 emission rates. Both TRAKER and SCAMPER measured rapid decay of PM10 emission rates after …


Past The Tipping Point, But With Hope Of Return: How Creating A Geoengineering Compulsory Licensing Scheme Can Incentivize Innovation, Brooke Wilson Apr 2021

Past The Tipping Point, But With Hope Of Return: How Creating A Geoengineering Compulsory Licensing Scheme Can Incentivize Innovation, Brooke Wilson

Washington and Lee Journal of Civil Rights and Social Justice

This Note explores the patenting of geoengineering technologies and issues arising from the early stages of this high-risk, high-reward technology. This Note focuses on one possible solution to solving the issues surrounding the patenting of geoengineering technology: Creating a specialized compulsory licensing scheme.


Atmospheric Measurements With Unmanned Aerial Systems (Uas), Marcelo I. Guzman Nov 2020

Atmospheric Measurements With Unmanned Aerial Systems (Uas), Marcelo I. Guzman

Chemistry Faculty Publications

This Special Issue provides the first literature collection focused on the development and implementation of unmanned aircraft systems (UAS) and their integration with sensors for atmospheric measurements on Earth. The research covered in the Special Issue combines chemical, physical, and meteorological measurements performed in field campaigns as well as conceptual and laboratory work. Useful examples for the development of platforms and autonomous systems for environmental studies are provided, which demonstrate how careful the operation of sensors aboard UAS must be to gather information for remote sensing in the atmosphere. The work serves as a key collection of articles to introduce …


Climate Change And Market-Based Insurance Feedbacks, Eric R. Holley, Adam Liska, Cory Walters, Geoffrey C. Friesen, Michael Hayes, Max J. Rudolph, Donald A. Wilhite Aug 2020

Climate Change And Market-Based Insurance Feedbacks, Eric R. Holley, Adam Liska, Cory Walters, Geoffrey C. Friesen, Michael Hayes, Max J. Rudolph, Donald A. Wilhite

Adam Liska Papers

Climatic events have accounted for 91% of $1.05 trillion in insured costs for global catastrophic events from 1980 to 2016. Costs are driven by socio-economic development and increased frequency and severity of climatic disasters driven by climate change. Government policies to reduce systemic risk (e.g., cap-and-trade, carbon tax) have been a predominant approach for mitigation and adaptation. Alternatively, market-based incentives for climate change adaptation and mitigation already operate via the insurance industry to lessen impacts on society. Insurance feedbacks include changes in 1) premiums and insurance policies, 2) non-coverage, and 3) policy making and litigation. Alongside government policies, insurance feedbacks …


Development Of Novel Instrumentation And Methods To Investigate The Composition And Phase Partitioning Of Semivolatile And Intermediately Volatile Organic Compounds In Atmospheric Organic Aerosol, Claire Fortenberry May 2020

Development Of Novel Instrumentation And Methods To Investigate The Composition And Phase Partitioning Of Semivolatile And Intermediately Volatile Organic Compounds In Atmospheric Organic Aerosol, Claire Fortenberry

McKelvey School of Engineering Theses & Dissertations

Atmospheric particulate matter (PM) is ubiquitous in both indoor and outdoor air and is generally detrimental to human health. PM composed of particles with aerodynamic diameters less than 2.5 um (PM2.5) are related to adverse health outcomes including heart disease and respiratory disease. Fundamentally, particle physical properties such as size and hygroscopicity are dictated by chemical composition, which can be highly complex, particularly for organic aerosol (OA). In both outdoor and indoor air, OA is composed substantially of intermediately volatile and semivolatile organic compounds (I/SVOCs), which exist in both gas and particle phases under typical atmospheric conditions. The distribution of …


Surface Reservoirs Dominate Dynamic Gas-Surface Partitioning Of Many Indoor Air Constituents, Chen Wang, Douglas B. Collins, Caleb Arata, Allen H. Goldstein, James M. Mattila, Delphine K. Farmer, Laura Ampollini, Peter F. Decarlo, Atila Novoselac, Marina E. Vance, William W. Nazaroff, Jonathan P.D. Abbatt Feb 2020

Surface Reservoirs Dominate Dynamic Gas-Surface Partitioning Of Many Indoor Air Constituents, Chen Wang, Douglas B. Collins, Caleb Arata, Allen H. Goldstein, James M. Mattila, Delphine K. Farmer, Laura Ampollini, Peter F. Decarlo, Atila Novoselac, Marina E. Vance, William W. Nazaroff, Jonathan P.D. Abbatt

Faculty Journal Articles

Human health is affected by indoor air quality. One distinctive aspect of the indoor environment is its very large surface area that acts as a poorly characterized sink and source of gas-phase chemicals. In this work, air-surface interactions of 19 common indoor air contaminants with diverse properties and sources were monitored in a house using fast-response, on-line mass spectrometric and spectroscopic methods. Enhanced-ventilation experiments demonstrate that most of the contaminants reside in the surface reservoirs and not, as expected, in the gas phase. They participate in rapid air-surface partitioning that is much faster than air exchange. Phase distribution calculations are …


The Fluxnet2015 Dataset And The Oneflux Processing Pipeline For Eddy Covariance Data, Gilberto Pastorello, Timothy Arkebauer, Dave P. Billesbach, Anatoly Gitelson, Adam Liska, Andrew Suyker, Elizabeth Walter-Shea, More Than 200 Other Jan 2020

The Fluxnet2015 Dataset And The Oneflux Processing Pipeline For Eddy Covariance Data, Gilberto Pastorello, Timothy Arkebauer, Dave P. Billesbach, Anatoly Gitelson, Adam Liska, Andrew Suyker, Elizabeth Walter-Shea, More Than 200 Other

Adam Liska Papers

The FLUXNET2015 dataset provides ecosystem-scale data on CO2, water, and energy exchange between the biosphere and the atmosphere, and other meteorological and biological measurements, from 212 sites around the globe (over 1500 site-years, up to and including year 2014). These sites, independently managed and operated, voluntarily contributed their data to create global datasets. Data were quality controlled and processed using uniform methods, to improve consistency and intercomparability across sites. The dataset is already being used in a number of applications, including ecophysiology studies, remote sensing studies, and development of ecosystem and Earth system models. FLUXNET2015 includes derived-data products, such as …


Using A Balloon-Launched Unmanned Glider To Validate Real-Time Wrf Modeling, Travis J. Schuyler, S. M. Iman Gohari, Gary Pundsack, Donald Berchoff, Marcelo I. Guzman Apr 2019

Using A Balloon-Launched Unmanned Glider To Validate Real-Time Wrf Modeling, Travis J. Schuyler, S. M. Iman Gohari, Gary Pundsack, Donald Berchoff, Marcelo I. Guzman

Chemistry Faculty Publications

The use of small unmanned aerial systems (sUAS) for meteorological measurements has expanded significantly in recent years. SUAS are efficient platforms for collecting data with high resolution in both space and time, providing opportunities for enhanced atmospheric sampling. Furthermore, advances in mesoscale weather research and forecasting (WRF) modeling and graphical processing unit (GPU) computing have enabled high resolution weather modeling. In this manuscript, a balloon-launched unmanned glider, complete with a suite of sensors to measure atmospheric temperature, pressure, and relative humidity, is deployed for validation of real-time weather models. This work demonstrates the usefulness of sUAS for validating and improving …


Daily And Seasonal Variability Of Offshore Wind Power On The Central California Coast And Statewide Demand, Matthew Douglas Kehrli Apr 2019

Daily And Seasonal Variability Of Offshore Wind Power On The Central California Coast And Statewide Demand, Matthew Douglas Kehrli

Physics

No abstract provided.


The Effects Of Reactant Concentration And Air Flow Rate In The Consumption Of Dissolved O2 During The Photochemistry Of Aqueous Pyruvic Acid, Alexis J. Eugene, Marcelo I. Guzman Mar 2019

The Effects Of Reactant Concentration And Air Flow Rate In The Consumption Of Dissolved O2 During The Photochemistry Of Aqueous Pyruvic Acid, Alexis J. Eugene, Marcelo I. Guzman

Chemistry Faculty Publications

The sunlight photochemistry of the organic chromophore pyruvic acid (PA) in water generates ketyl and acetyl radicals that contribute to the production and processing of atmospheric aerosols. The photochemical mechanism is highly sensitive to dissolved oxygen content, [O2(aq)], among other environmental conditions. Thus, herein we investigate the photolysis (λ ≥ 305 nm) of 10–200 mM PA at pH 1.0 in water covering the relevant range 0 ≤ [O2(aq)] ≤ 1.3 mM. The rapid consumption of dissolved oxygen by the intermediate photolytic radicals is monitored in real time with a dissolved oxygen electrode. …


Modeled And Measured Ecosystem Respiration In Maize–Soybean Systems Over 10 Years, Ming Zhan, Adam Liska, Anthony Nguy-Robertson, Andrew E. Suyker, Matthew P. Pelton, Haishun Yang Jan 2019

Modeled And Measured Ecosystem Respiration In Maize–Soybean Systems Over 10 Years, Ming Zhan, Adam Liska, Anthony Nguy-Robertson, Andrew E. Suyker, Matthew P. Pelton, Haishun Yang

Adam Liska Papers

Crop residue is an abundant resource for the potential production of biofuels, but a better understanding of its use on net carbon emissions must be developed to mitigate climate change. This analysis combines two established crop growth models (Hybrid-Maize and SoySim) with a simple soil and crop residue respiration model to estimate daily ecosystem respiration (ERe) from maize and soybean; ERe was estimated to be the sum of CO2 emissions from the oxidation of the growing crop, crop residue, and soil organic carbon (SOC). Model-estimated CO2 fluxes from irrigated continuous maize and irrigated maize–soybean cropping systems in eastern …


Water, Energy, And Carbon Footprints Of Bioethanol From The U.S. And Brazil, Mesfin Mekonnen, Thiago L. Romanelli, Chittaranjan Ray, Arjen Y. Hoekstra, Adam Liska, Christopher M. U. Neale Nov 2018

Water, Energy, And Carbon Footprints Of Bioethanol From The U.S. And Brazil, Mesfin Mekonnen, Thiago L. Romanelli, Chittaranjan Ray, Arjen Y. Hoekstra, Adam Liska, Christopher M. U. Neale

Adam Liska Papers

Driven by biofuel policies, which aim to reduce greenhouse gas (GHG) emissions and increase domestic energy supply, global production and consumption of bioethanol have doubled between 2007 and 2016, with rapid growth in corn-based bioethanol in the U.S. and sugar cane-based bioethanol in Brazil. Advances in crop yields, energy use efficiency in fertilizer production, biomass-to-ethanol conversion rates, and energy efficiency in ethanol production have improved the energy balance and GHG emission reduction potential of bioethanol. In the current study, the water, energy, and carbon footprints of bioethanol from corn in the U.S. and sugar cane in Brazil were assessed. The …


Development Of The Nebraska Department Of Transportation Winter Severity Index, Mark R. Anderson, Behzad Esmaeili, Curtis L. Walker, Dylan Steinkruger, Sogand Hasanzadeh, Pouya Gholizadeh, Bac Dao Jun 2018

Development Of The Nebraska Department Of Transportation Winter Severity Index, Mark R. Anderson, Behzad Esmaeili, Curtis L. Walker, Dylan Steinkruger, Sogand Hasanzadeh, Pouya Gholizadeh, Bac Dao

Nebraska Department of Transportation: Research Reports

Adverse weather conditions are responsible for millions of vehicular crashes, thousands of vehicular deaths and billions of dollars in economic and congestion costs. Many transportation agencies utilize a performance or mobility metric to assess how well they are maintaining road access. This research focuses on the development of a winter severity index for the State of Nebraska (NEWINS). NEWINS is an event-driven index that was derived for the Nebraska Department of Transportation (NDOT) and its districts across the state. The NEWINS framework includes a categorical storm classification framework and climatological aspect to capture atmospheric conditions more accurately across the diverse …


Adam J. Liska: Curriculum Vitae, Adam Liska May 2018

Adam J. Liska: Curriculum Vitae, Adam Liska

Adam Liska Papers

Associate Professor, George Dempster Smith Chair of Industrial Ecology, Departments of Biological Systems Engineering and Agronomy & Horticulture, University of Nebraska-Lincoln 236 L.W. Chase Hall, Lincoln, NE 68583-0726, Ph: (402) 472-8744, e-mail: aliska2@unl.edu

Ph.D. 2003 Biology (magna cum laude), Max Planck Institute of Molecular Cell Biology & Genetics, Technische Universität Dresden, Dresden, Germany


A Comparative Study Characterizing Traffic Related Air Pollutant Concentrations At Near-Road Communities In El Paso, Texas, Adan Rangel Jan 2018

A Comparative Study Characterizing Traffic Related Air Pollutant Concentrations At Near-Road Communities In El Paso, Texas, Adan Rangel

Open Access Theses & Dissertations

Numerous scientific studies have demonstrated the influence of traffic related air pollution at near-road communities and the associated health risks for these populations. This study uses on-site air quality monitors to characterize air pollutants at near-road schools in El Paso, TX to understand children's exposure to traffic-related air pollutants. Ambient air monitoring stations were installed at Coldwell Elementary, Bliss Elementary, and a residential house located in close proximity to major inter-state roadways. In this study, air quality data for PM2.5, PM10, NO2, and O3 was collected over a period of nine weeks in Fall 2018. The spatial and temporal variability …


Wildfire Emissions In The Context Of Global Change And The Implications For Mercury Pollution, Aditya Kumar Jan 2018

Wildfire Emissions In The Context Of Global Change And The Implications For Mercury Pollution, Aditya Kumar

Dissertations, Master's Theses and Master's Reports

Wildfires are episodic disturbances that exert a significant influence on the Earth system. They emit substantial amounts of atmospheric pollutants, which can impact atmospheric chemistry/composition and the Earth’s climate at the global and regional scales. This work presents a collection of studies aimed at better estimating wildfire emissions of atmospheric pollutants, quantifying their impacts on remote ecosystems and determining the implications of 2000s-2050s global environmental change (land use/land cover, climate) for wildfire emissions following the Intergovernmental Panel on Climate Change (IPCC) A1B socioeconomic scenario.

A global fire emissions model is developed to compile global wildfire emission inventories for major atmospheric …


Unmanned Aerial Systems For Monitoring Trace Tropospheric Gases, Travis J. Schuyler, Marcelo I. Guzman Oct 2017

Unmanned Aerial Systems For Monitoring Trace Tropospheric Gases, Travis J. Schuyler, Marcelo I. Guzman

Chemistry Faculty Publications

The emission of greenhouse gases (GHGs) has changed the composition of the atmosphere during the Anthropocene. Accurately documenting the sources and magnitude of GHGs emission is an important undertaking for discriminating the contributions of different processes to radiative forcing. Currently there is no mobile platform that is able to quantify trace gases at altitudes(UASs) can be deployed on-site in minutes and can support the payloads necessary to quantify trace gases. Therefore, current efforts combine the use of UASs available on the civilian market with inexpensively designed analytical systems for monitoring atmospheric trace gases. In this context, this perspective introduces the …


Oxidation Of Substituted Catechols At The Air-Water Interface: Production Of Carboxylic Acids, Quinones, And Polyphenols, Elizabeth A. Pillar, Marcelo I. Guzman Apr 2017

Oxidation Of Substituted Catechols At The Air-Water Interface: Production Of Carboxylic Acids, Quinones, And Polyphenols, Elizabeth A. Pillar, Marcelo I. Guzman

Chemistry Faculty Publications

Anthropogenic activities contribute benzene, toluene, and anisole to the environment, which in the atmosphere are converted into the respective phenols, cresols, and methoxyphenols by fast gas-phase reaction with hydroxyl radicals (HO(•)). Further processing of the latter species by HO(•) decreases their vapor pressure as a second hydroxyl group is incorporated to accelerate their oxidative aging at interfaces and in aqueous particles. This work shows how catechol, pyrogallol, 3-methylcatechol, 4-methylcatechol, and 3-methoxycatechol (all proxies for oxygenated aromatics derived from benzene, toluene, and anisole) react at the air-water interface with increasing O3(g) during τc ≈ 1 μs contact time and contrasts their …