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Full-Text Articles in Physical Sciences and Mathematics
Lattice Thermal Conductivity Of Quartz At High Pressure And Temperature From The Boltzmann Transport Equation, Xue Xiong, Eugene J. Ragasa, Aleksandr V. Chernatynskiy, Dawei Tang, Simon R. Phillpot
Lattice Thermal Conductivity Of Quartz At High Pressure And Temperature From The Boltzmann Transport Equation, Xue Xiong, Eugene J. Ragasa, Aleksandr V. Chernatynskiy, Dawei Tang, Simon R. Phillpot
Physics Faculty Research & Creative Works
The thermal conductivities along the basal and hexagonal directions of α-quartz silica, the low-temperature form of crystalline SiO2, are predicted from the solution of the Boltzmann transport equation combined with the van Beest, Kramer, and van Santen potential for the temperature up to 900 K and the pressure as high as 4 GPa. The thermal conductivities at atmospheric pressure, which show a negative and nonlinear dependence on temperature, are in reasonable agreement with the experimental data. The influence of pressure on thermal conductivity is positive and linear. The pressure (P) and temperature (T) dependences of the thermal conductivity …
Impact Of Anharmonicity On The Vibrational Entropy And Specific Heat Of Uo₂, M. S. Bryan, J. W. L. Pang, B. C. Larson, Aleksandr V. Chernatynskiy, D. L. Abernathy, K. Gofryk, M. E. Manley, For Full List Of Authors, See Publisher's Website.
Impact Of Anharmonicity On The Vibrational Entropy And Specific Heat Of Uo₂, M. S. Bryan, J. W. L. Pang, B. C. Larson, Aleksandr V. Chernatynskiy, D. L. Abernathy, K. Gofryk, M. E. Manley, For Full List Of Authors, See Publisher's Website.
Physics Faculty Research & Creative Works
The impact of anharmonicity on the vibrational entropy and heat capacity of UO2 has been investigated from 10 to 1200 K using inelastic neutron-scattering measurements of the phonon density of states (PDOS). Small changes in the PDOS are observed from 10 to 295 K, with more noticeable changes appearing in the 750- and 1200-K data. The specific heat determined from the PDOS measurements is in agreement with macroscopic specific heat measurements, and the overall impact of nondilation anharmonicity on the specific heat has been shown to be less than 2%. An analysis of the phonon measurements shows that the softening …