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Full-Text Articles in Physical Sciences and Mathematics
Retrieving Photorecombination Cross Sections Of Atoms From High-Order Harmonic Spectra, Shinichiro Minemoto, Toshihito Umegaki, Yuichiro Oguchi, Toru Morishita, Anh-Thu Le, Shinichi Watanabe, Hirofumi Sakai
Retrieving Photorecombination Cross Sections Of Atoms From High-Order Harmonic Spectra, Shinichiro Minemoto, Toshihito Umegaki, Yuichiro Oguchi, Toru Morishita, Anh-Thu Le, Shinichi Watanabe, Hirofumi Sakai
Physics Faculty Research & Creative Works
We observe high-order harmonic spectra generated from a thin atomic medium, Ar, Kr, and Xe, by intense 800-nm and 1300-nm femtosecond pulses. A clear signature of a single-atom response is observed in the harmonic spectra. Especially in the case of Ar, a Cooper minimum, reflecting the electronic structure of the atom, is observed in the harmonic spectra. We successfully extract the photorecombination cross sections of the atoms in the field-free condition with the help of an accurate recolliding electron wave packet. The present protocol paves the way for exploring ultrafast imaging of molecular dynamics with attosecond resolution.
Spin- And Fine-Structure-Resolved Ionization Of Krypton, S. Bellm, J. Lower, R. P. Mceachran, E. Weigold, Ciarán Ryan-Anderson, Don H. Madison
Spin- And Fine-Structure-Resolved Ionization Of Krypton, S. Bellm, J. Lower, R. P. Mceachran, E. Weigold, Ciarán Ryan-Anderson, Don H. Madison
Physics Faculty Research & Creative Works
The influence of exchange, correlation, and relativistic effects in the ionization of heavy-target atoms can be sensitively probed by kinematically complete studies involving spin-polarized electrons, in particular when the fine structure of the residual ion is resolved. We present spin asymmetries, triple differential cross sections, and branching ratios for the ionization, by 127.5-eV and 114.3-eV electrons, of ground-state krypton atoms leading to the Kr+ 4s 2S1/2, 4p5 2P1/2, and 4p5 2P3/2 states. In order to untangle contributions from different physical effects, the experimental results are compared to those from distorted-wave Born approximation calculations (non- and semirelativistic) in which bound-state and …
Large-Angle Electron Diffraction Structure In Laser-Induced Rescattering From Rare Gases, D. Ray, B. Ulrich, I. Bocharova, C. Maharjan, P. Ranitovic, B. Gramkow, M. Magrakvelidze, S. De, I. V. Litvinyuk, Anh-Thu Le, Toru Morishita, C. D. Lin, G. G. Paulus, C. L. Cocke
Large-Angle Electron Diffraction Structure In Laser-Induced Rescattering From Rare Gases, D. Ray, B. Ulrich, I. Bocharova, C. Maharjan, P. Ranitovic, B. Gramkow, M. Magrakvelidze, S. De, I. V. Litvinyuk, Anh-Thu Le, Toru Morishita, C. D. Lin, G. G. Paulus, C. L. Cocke
Physics Faculty Research & Creative Works
We have measured full momentum images of electrons rescattered from Xe, Kr, and Ar following the liberation of the electrons from these atoms by short, intense laser pulses. At high momenta the spectra show angular structure (diffraction) which is very target dependent and in good agreement with calculated differential cross sections for the scattering of free electrons from the corresponding ionic cores.