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- Alkali-silica reaction; confined concrete; crack orientation; mechanical properties degradation; rate of expansion;Siliceous and dolomitic limestones; Mitigation; Silica content; Rate of expansion; Concrete deterioration; ASR in field concrete (1)
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Articles 1 - 30 of 59
Full-Text Articles in Structural Materials
Stress Relaxation Cracking In 347h Austenitic Steel Weldments Under Various Heat Treatments: Experiments And Modeling, Yi Yang
Doctoral Dissertations
347H austenitic stainless steel exhibits exceptional creep and corrosion resistance, rendering it an exemplary candidate for pipeline materials, particularly in mid- to high-temperature working conditions. However, due to constraints in component dimensions, welding has been chosen as the preferred method for joining pipeline systems extensively employed in nuclear power plants, fossil fuel plants, and petrochemical companies. The welding process entails the accumulation of residual stress during the cooling stage, along with the introduction of microstructure evolution. Moreover, the residual stress field and microstructure continuously evolve under service conditions, thereby intensifying the susceptibility of crack initiation and propagation. The initial residual …
3d Experimental Studies Of Temperature And Crystallographic Effects On Creep And Strength In Rock Salt, Amirsalar Moslehy
3d Experimental Studies Of Temperature And Crystallographic Effects On Creep And Strength In Rock Salt, Amirsalar Moslehy
Doctoral Dissertations
Salt domes utilization as storage reservoirs in the energy sector has led to extensive studies on rock salt’s mechanical and geothermal behavior. These important facilities’ safety and serviceability rely on understanding rock salt’s compressive strength and creep behavior under various loading directions, water contents, in-situ stresses, and temperatures. Despite numerous studies on rock salt’s mechanical behavior in the literature, there are still many unanswered questions about rock salt’s behavior. This dissertation was aimed at utilizing state-of-the-art experimental techniques such as 3D synchrotron micro-computed tomography (SMT) and 3D x-ray diffraction (3DXRD) along with hundreds of compression and creep experiments to enhance …
Investigation Of Microstructure And Mechanical Behavior Of Novel Powder-Extruded Al-Ce-Mg Alloys, Mairym Vazquez
Investigation Of Microstructure And Mechanical Behavior Of Novel Powder-Extruded Al-Ce-Mg Alloys, Mairym Vazquez
Doctoral Dissertations
Pursuing advanced structural materials with enhanced performance, reduced weight, and lower costs is a constant endeavor in the aerospace and automotive industries. Conventional structural alloys, such as cast irons, carbon steels, and titanium alloys, have strength, weight, and cost limitations. Aluminum-based alloys, known for their lightweight and high strength, have gained popularity in these industries. This dissertation focuses on investigating microstructure and mechanical behavior of novel powder-extruded Al-Ce-Mg alloys as potential candidates for high-performance structural materials.
This research explores using powder extrusion, a well-established forging methodology in the steel industry, to produce Al-Ce-Mg alloys with improved properties and aims to …
A Study On Early Age Properties Of Concrete For Precast And 3d Printing, Debalina Ghosh
A Study On Early Age Properties Of Concrete For Precast And 3d Printing, Debalina Ghosh
Doctoral Dissertations
Concrete is the second-most consumed material, leading the global Portland cement production of 4.1 billion tons in 2020 and 5-8% of global Carbon dioxide (CO2) emission annually. As with any other material and practice, the construction industry is also ever-changing to meet market demand, evolving technology, and resource limitation. In the case of concrete construction, one of the main concerns is the lack of automation. In the last few decades, some new construction methods have risen to address this concern. Some of these economic and successful practices are precast construction, self-compacting concrete (SCC), and 3D printing of concrete(3DPC). …
Fabrication, Thermophysical, And Mechanical Properties Of Cermet And Cercer Fuel Composites For Nuclear Thermal Propulsion, Neal D. Gaffin
Fabrication, Thermophysical, And Mechanical Properties Of Cermet And Cercer Fuel Composites For Nuclear Thermal Propulsion, Neal D. Gaffin
Doctoral Dissertations
Nuclear thermal propulsion (NTP) utilizes nuclear fission to double the efficiency of
in-space propulsion systems compared with traditional combustion rocket systems.
NTP systems are limited primarily by the fuel material choice, due to the extreme
conditions they will need to endure, including temperatures up to 3000 K, multiple
thermal cycles with rapid heating and cooling, exposure to hot flowing hydrogen,
large thermal gradients, and high neutron flux. Particle based fuels, namely ceramic-
metallic (cermet) and ceramic-ceramic (cercer) composites are both promising fuel
element material candidates for NTP. Given the high temperature nature, these
materials are difficult to fabricate and very …
Fundamental Understanding Of The Transient Melt Pool Dynamics, Solidification Kinetics And Build Texture In Spot-Melt Additive Manufacturing Of Ti-6al-4v, Rakesh Rajaram Kamath
Fundamental Understanding Of The Transient Melt Pool Dynamics, Solidification Kinetics And Build Texture In Spot-Melt Additive Manufacturing Of Ti-6al-4v, Rakesh Rajaram Kamath
Doctoral Dissertations
The overarching goal of this dissertation is to better understand the underlying process-structure relationships in play during the implementation of a spot melt strategy for metal additive manufacturing, which has become a popular alternative to the conventional raster melt strategy for site-specific microstructure control. In the first part of this dissertation, the effect of a spot melt strategy on the solidification texture, variant selection, phase fraction, and their variations along the build height of an E-PBF Ti-6Al-4V is investigated in comparison to a conventional linear melt strategy using high-energy synchrotron x-ray diffraction. In spite of the thermal excursions involved, the …
Effects Of Plastic Deformation From Ultrasonic Additive Manufacturing, Michael Pagan
Effects Of Plastic Deformation From Ultrasonic Additive Manufacturing, Michael Pagan
Doctoral Dissertations
Nuclear energy technology can be exponentially advanced using advanced manufacturing, which can drastically transform how materials, structures, and designs can be built. Ultrasonic Additive Manufacturing (UAM) represents one of the four main additive manufacturing methods, although it is also the newest. As UAM technology and applications develop, a fundamental understanding of the bonding mechanism is crucial to fully realize its potential. Currently UAM bonding is considered to occur through breaking down surface asperities and removing surface oxides. Plastic deformation occurs although its role is currently unclear. This research analyzes material configurations in a variety of geometries, with similar and dissimilar …
Interfacial Bonding Between Thermoset And Thermoplastic Polyurethane Reinforced Textile Grade Carbon Fiber: Structure Property Relationships, Surbhi Subhash Kore
Interfacial Bonding Between Thermoset And Thermoplastic Polyurethane Reinforced Textile Grade Carbon Fiber: Structure Property Relationships, Surbhi Subhash Kore
Doctoral Dissertations
The research work focused on examining the interfacial adhesion of unsized, epoxy, and urethane-sized textile grade carbon fiber (TCF) reinforced in different classes of polyurethane (PU) thermoplastic (TPU) and thermoset (TSU) polyurethane (PU) through the structure-property relationship. The Carbon Fiber Technology Facility (CFTF) at Oak Ridge National Laboratory (ORNL) has produced TCF to reduce the cost of commercial-grade carbon fiber. The first part of the research examined the fundamental relationships between (a) soft segment thermoplastic polyurethane (S-TPU), (b) hard segment thermoplastic polyurethane (H-TPU), (c) thermoset polyurethane (TSU) and TCF reinforcement’s molecular behavior at the interface using the surface and thermal …
Fundamentals Of Cavity Formation In Α-Fe And Fe-Cr Alloys, Yan-Ru Lin
Fundamentals Of Cavity Formation In Α-Fe And Fe-Cr Alloys, Yan-Ru Lin
Doctoral Dissertations
Ferritic-martensitic steels are attractive candidate materials for fusion and advanced fission reactors primarily due to their low swelling characteristic, attractive thermo-mechanical properties, and the potential for development of nanostructured ferritic alloys. However, significant discrepancies exist regarding the effect of solutes and irradiation temperature on cavity swelling under ion versus neutron irradiation conditions. Several mechanisms have been proposed that may affect cavity swelling, but no general theory or model has received complete acceptance to explain these phenomena.
To better understand the formation of cavities in ferritic steels, we have performed multi-temperature (400-550°C) single-beam and simultaneous dual-beam irradiations (ex-situ and in-situ) on …
Advanced Materials Design Using Application-Based Processing Techniques, Daniel S. Camarda
Advanced Materials Design Using Application-Based Processing Techniques, Daniel S. Camarda
Doctoral Dissertations
This dissertation pertains to generating advanced materials using application-based processing techniques. First, billets consisting of PTFE sintering powders are evaluated using Thermomechancal Analysis. It was found that both shape change and volume change are associated with enthalpic and entropic recoil, respectively. These phenomena, due to melting and stored energy during the powder compaction process, were found to be molecular weight dependent. Additionally, kinetics of the recovery and sintering process were found to be slower in blended specimens than pure samples. Next, the creation of graft copolymers by selectively grafting a second polymer to the amorphous fraction of a semi-crystalline polymer …
Development Of Density-Functional Tight-Binding Methods For Chemical Energy Science, Quan Vuong
Development Of Density-Functional Tight-Binding Methods For Chemical Energy Science, Quan Vuong
Doctoral Dissertations
Density-functional tight-binding (DFTB) method is an approximation to the popular first-principles density functional theory (DFT) method. Recently, DFTB has gained considerable visibility due to its inexpensive computational requirements that confer it the capability of sustaining long-timescale reactive molecular dynamics (MD) simulations while providing an explicit description of electronic structure at all time steps. This capability allows the description of bond formation and breaking processes, as well as charge polarization and charge transfer phenomena, with accuracy and transferability beyond comparable classical reactive force fields. It has thus been employed successfully in the simulation of many complex chemical processes. However, its applications …
Material Property Heterogeneity In Dimensional Lumber And Its Relationship To Mass Timber Performance, Fiona O'Donnell
Material Property Heterogeneity In Dimensional Lumber And Its Relationship To Mass Timber Performance, Fiona O'Donnell
Doctoral Dissertations
According to the Environmental Protection Agency, buildings account for 38% of the United States' carbon dioxide emissions, providing architects and structural engineers a unique opportunity to mitigate a significant factor driving climate change by implementing innovative and sustainable technology in infrastructure design. Wood and mass timber products are becoming an increasingly popular alternative building material due to their economic and environmental benefits. The natural growth of wood leads to highly heterogeneous material properties. Defects such as checks, knots, and localized slope of grain contribute to some of this variation; however, wood properties vary significantly even in clear wood. Using mass …
Harnessing The Mechanics Of Thin-Walled Metallic Structures: From Plate-Lattice Materials To Cold-Formed Steel Shear Walls, Fani Derveni
Harnessing The Mechanics Of Thin-Walled Metallic Structures: From Plate-Lattice Materials To Cold-Formed Steel Shear Walls, Fani Derveni
Doctoral Dissertations
Thin-walled structures have received a lot of interest during the last years due to their light weight, cost efficiency, and ease in fabrication and transportation, along with their high strength and stiffness. This dissertation focuses on the mechanical performance of thin-walled metallic structures from cold-formed steel shear walls and connections (PART I) to plate-lattice architected materials (PART II) via computational, experimental, and probabilistic methods. Cold-formed steel (CFS) shear walls subjected to seismic loads is the focus of PART I of this dissertation. An innovative three-dimensional shell finite element model of oriented strand board (OSB) sheathed CFS shear walls is introduced …
3d Printing Of Hybrid Architectures Via Core-Shell Material Extrusion Additive Manufacturing, Robert Cody Pack
3d Printing Of Hybrid Architectures Via Core-Shell Material Extrusion Additive Manufacturing, Robert Cody Pack
Doctoral Dissertations
Biological materials often employ hybrid architectures, such as the core-shell motif present in porcupine quills and plant stems, to achieve unique properties and performance. Drawing inspiration from these natural materials, a new method to fabricate lightweight and stiff core-shell architected filaments is reported. Specifically, a core-shell printhead conducive to printing highly loaded fiber-filled inks, as well as a new low-density syntactic foam ink, are utilized to 3D-print core-shell architectures consisting of a syntactic epoxy foam core surrounded by a stiff carbon fiber-reinforced epoxy composite shell. Effective printing of test specimens and structures with controlled geometry, composition, and architecture is demonstrated …
Microscopic And Image Processing Characterization Of Aggregates To Predict Asr Expansion Potential Of Concrete, Ammar Elfatih Abdelssamd Elhassan
Microscopic And Image Processing Characterization Of Aggregates To Predict Asr Expansion Potential Of Concrete, Ammar Elfatih Abdelssamd Elhassan
Doctoral Dissertations
Preventing ASR occurrence in new concrete structures requires reliable and quick methods to identify reactive aggregates and to evaluate proper mitigation alternatives. The current accelerated mortar-bar expansion tests (ASTM C 1260 or ASTM C1567) and the concrete prism expansion test (ASTM C 1293) have been reported to have several limitations. Assessment of the extend of ASR damage in existing affected structures requires more understanding on how ASR expansion and damage develop in field conditions such as under confinements and under relatively slow rate of ASR reaction.
The significance of ASR expansion rate and bi-axial restrain on concrete degradation has been …
Process-Structure-Property Relationships In 3d-Printed Epoxy Composites Produced Via Material Extrusion Additive Manufacturing, Nadim S. Hmeidat
Process-Structure-Property Relationships In 3d-Printed Epoxy Composites Produced Via Material Extrusion Additive Manufacturing, Nadim S. Hmeidat
Doctoral Dissertations
Extrusion-based additive manufacturing (AM) technologies, such as direct ink writing (DIW), offer unique opportunities to create composite materials and novel multi-material architectures that are not feasible using other AM technologies. DIW is a novel 3D-printing approach in which viscoelastic inks, with favorable rheological properties, are extruded through fine nozzles and patterned in a filament form at room temperature.
Recent developments in DIW of polymer composites have led to expanding the range of materials used for printing, as well as introducing novel deposition strategies to control filler orientation and create improved functional/structural composite materials. Despite these substantial advancements, the successful and …
Discontinuous Recycled And Repurposed Carbon Fiber Reinforced Thermoplastic Organosheet Composites, Philip R. Barnett
Discontinuous Recycled And Repurposed Carbon Fiber Reinforced Thermoplastic Organosheet Composites, Philip R. Barnett
Doctoral Dissertations
There is a significant need for low cost, high volume composites in the automotive industry to aid in vehicle lightweighting and safety. The current state-of-the-art severely compromises the mechanical properties of composites to achieve cost and cycle time goals. In this dissertation, a novel composite format, termed discontinuous carbon fiber organosheets, using recycled and repurposed carbon fibers in a thermoplastic matrix is developed and studied. Unlike traditional composites, the long fiber length and rapid processing time yield mechanical properties and cycle times competitive with automotive metals.
Several studies were performed to characterize this new material format. First, samples were manufactured …
Development Of A Novel Casting Alloy Composed Of Aluminum And Cerium With Other Minor Additions, Zachary Cole Sims
Development Of A Novel Casting Alloy Composed Of Aluminum And Cerium With Other Minor Additions, Zachary Cole Sims
Doctoral Dissertations
Eutectic casting alloys of aluminum and cerium are a recent discovery and early research describes an alloy with great potential to meet the growing demand for a lightweight, economical, high specific strength material for use in high-temperature or extremely corrosive environments. The broad application of aluminum alloys across industry sectors is driven by their collection of balanced properties including economical cost, high specific strength, and flexibility of their production pathways. Additionally, their high corrosion resistance makes them a good choice for structural materials. Despite this, the push to use aluminum alloys in ever more extreme environments with higher temperatures, stresses, …
Design And Development Of Strong And Ductile Single Bcc Refractory High-Entropy Alloys For High-Temperature Applications, Chanho Lee
Doctoral Dissertations
The objectives of this proposed study are to (1) design and develop single BCC phase refractory high-entropy alloys (HEAs) for the high-temperature applications, (2) investigate the deformation mechanisms of refractory HEAs, (3) improve an integrated approach, coupling focused experiments and theoretical modeling, to design, discover, and develop HEAs, and (4) understand the alloy design-microstructure-property-performance links underlying the mechanical behavior of refractory HEA systems for gas-turbine applications
A traditional alloy system generally includes one or two principal elements that form the matrix with other additional elements, e.g., iron or aluminum alloys, to strengthen some specific properties, such as strength and corrosion …
Cracking And Earing Phenomenon In Deep-Drawn Stainless Steel Alloys: Role Of Transformation Kinetics, Microstructure, And Texture, Peijun Hou
Doctoral Dissertations
The enhancement of formability of advanced high-strength TRIP-assisted steel alloys is a challenging assignment for industrial application due to the cracking phenomenon. The critical factor governing the cracking behavior is residual-stress concentration resulting from the inhomogeneous plastic deformation and microstructural evolution during the forming processes. Martensitic phase transformation kinetics, constituent phases, and crystallographic texture in TRIP-assisted steel alloys are correlated to the microstructure evolution, resulting in phase-specific stress concentration. In the current study, we are aiming at understanding the fundamental mechanisms responsible for the cracking phenomenon and thus improving the formability of TRIP-assisted steel alloys. Four stainless steel (SS) alloys …
Finite Element Simulation Of Bonded And Mechanically Anchored Shear Interfaces Of Externally Applied Frp Sheets To Concrete And Wood-Concrete Composites, Alaa Al-Sammari
Finite Element Simulation Of Bonded And Mechanically Anchored Shear Interfaces Of Externally Applied Frp Sheets To Concrete And Wood-Concrete Composites, Alaa Al-Sammari
Doctoral Dissertations
Composite construction is prevalent in advanced structural systems where components of different materials are combined in the same structure to improve the performance of strong and economic structural sections. Maintaining continuity between the different structural components to produce monolithic structural behavior is challenging because of differences in the mechanical properties of these materials in terms of stiffness, strength, and ductility. The different components of the composite section are typically joined using adhesives and/or mechanical anchors to produce partial or full composite action. This dissertation discusses two types of shear interfaces intended to result in structural composite behavior. The first type …
Northeastern Species In Hybrid Cross Laminated Timber, Hamid Kaboli
Northeastern Species In Hybrid Cross Laminated Timber, Hamid Kaboli
Doctoral Dissertations
Known in the building industry throughout the world, Cross Laminated Timber (CLT) is a massive timber building material with outstanding structural, fire, and seismic properties. CLT is a cost-competitive, sustainable construction material is a good candidate as a substitute material for concrete, masonry, and steel, in mid-rise and high-rise buildings. CLT is perpendicular layers of dimensional lumbers usually laminated together and forming a massive structural panel. This dissertation explores the viability of utilizing Massachusetts grown Eastern Hemlock and Eastern White Pine in CLT panels as pure or in conjunction with other high-value wood products. 59% of Massachusetts’ lands are covered …
Engineering Next Generation Anisotropic Materials And Composites, Nihal Kanbargi
Engineering Next Generation Anisotropic Materials And Composites, Nihal Kanbargi
Doctoral Dissertations
Polymer-based composite systems have been developed for a wide variety of applications ranging from aerospace to electronics. My work has focused on the structure-process-property relationships of anisotropic polymeric materials and composites, aimed primarily for structural applications. Anisotropic materials such as fibers have superior mechanical properties along the axial direction and this property can be exploited to engineer exceptionally strong and light materials. In the first chapter, we discuss the physics of degradation of Poly(p-phenylene-2,6-benzobisoxazole) (PBO) fibers. PBO, a fiber of extraordinary tensile modulus and strength has been found to degrade rapidly under moderate conditions of humidity and heat. Solid-state NMR …
Computational Studies Of Structure–Function Relationships Of Supported And Unsupported Metal Nanoclusters, Hongbo Shi
Computational Studies Of Structure–Function Relationships Of Supported And Unsupported Metal Nanoclusters, Hongbo Shi
Doctoral Dissertations
Fuel cells have been demonstrated to be promising power generation devices to address the current global energy and environmental challenges. One of the many barriers to commercialization is the cost of precious catalysts needed to achieve sufficient power output. Platinum-based materials play an important role as electrocatalysts in energy conversion technologies. In order to improve catalytic efficiency and facilitate rational design and development of new catalysts, structure–function relationships that underpin catalytic activity must be understood at a fundamental level. First, we present a systematic analysis of CO adsorption on Pt nanoclusters in the 0.2-1.5 nm size range with the aim …
Fabrication Of Functional Nano-Structured Materials And Devices Using Supercritical Fluids, Shengkai Li
Fabrication Of Functional Nano-Structured Materials And Devices Using Supercritical Fluids, Shengkai Li
Doctoral Dissertations
Nano-structured materials possess unconventional properties and enable miniaturization of devices. However, fabrications of such materials and devices are challenging and in many cases cumbersome, and development of nanofabrication techniques are essential to realizing novel designs and commercializing scientific ideas. Supercritical fluids possess a unique combination of gas-like diffusion properties and liquid-like dissolution power, and are suitable reaction media for fabricating materials at the nanometer scale. This dissertation focuses on developing supercritical fluids-related techniques for fast and large-scale fabrication of novel composite materials and devices. Using supercritical fluid deposition (SFD) technique, cobalt thin films were deposited on a variety of substrates, …
First-Principles Study Of Point Defect Behavior At Interfaces And In-Plane Strain Fields, Jianqi Xi
First-Principles Study Of Point Defect Behavior At Interfaces And In-Plane Strain Fields, Jianqi Xi
Doctoral Dissertations
Interfaces in solid materials are the so-called boundaries, separating crystals with the same structure and chemistry but different orientations, e.g. grain boundaries (GBs), different stacking sequences, e.g. stacking faults (SFs), or crystals with different structures and/or chemistries as well as orientations, e.g. the interface between substrate and thin film. In this study, first-principles calculations are used to investigate the defect behavior at different interfaces and in-plane strain fields, such as stacking fault (SF) in silicon carbide (SiC), in-plane strain field near interfaces in potassium tantalate (KTaO3), and grain boundary in ceria (CeO2).
Results show that the …
Experimental And Computational Investigation Of High Entropy Alloys For Elevated-Temperature Applications, Haoyan Diao
Experimental And Computational Investigation Of High Entropy Alloys For Elevated-Temperature Applications, Haoyan Diao
Doctoral Dissertations
To create and design novel structural materials with enhanced creep-resistance, fundamental studies have been conducted on high-entropy alloys (HEAs), using (1) thermodynamic calculations, (2) mechanical tests, (3) neutron diffraction, (4) characterization techniques, and (5) crystal-plasticity finite-element modeling (CPFEM), to explore future candidates for next-generation power plants.
All the constituent binary and ternary systems of the Al-Cr-Cu-Fe-Mn-Ni and Al-Co-Cr- Fe-Ni systems were thermodynamically modeled within the whole composition range. Comparisons between the calculated phase diagrams and literature data are in good agreement. The AlxCrCuFeMnNi HEAs have disordered [face-centered-cubic (FCC) + body-centered-cubic (BCC)] crystal structures. Excessive alloying of the Al …
Microstructure Control And Correlation To Creep Properties In Grade 91 Steel Weldment After Thermo-Mechanical Treatments And An Fe-30cr-3al Alloy Strengthened By Fe2nb Laves Phase, Benjamin Allen Shassere
Microstructure Control And Correlation To Creep Properties In Grade 91 Steel Weldment After Thermo-Mechanical Treatments And An Fe-30cr-3al Alloy Strengthened By Fe2nb Laves Phase, Benjamin Allen Shassere
Doctoral Dissertations
Type IV cracking in weldments of steel pipes after creep deformation is a concern in modern fossil-fueled power plants. Two possible methods for minimizing or eliminating Type IV cracking will be discussed. The first method alters the initial microstructure of typical Grade 91 steel base metal before welding, while the second provides baseline microstructure characteristics and creep performance of a new alloy that is strengthened by the intermetallic Fe2Nb Laves phase. The initial microstructure of the Grade 91 steel can be controlled by Thermo-Mechanical Treatments, which aids in precipitation of fine (5-10 nm) MX particles in austenite before transformation to …
Structure And Properties Of Cnt Yarns And Cnt/Cnf Reinforced Pan-Based Carbon Fibers, Nitilaksha Phalaxayya Hiremath
Structure And Properties Of Cnt Yarns And Cnt/Cnf Reinforced Pan-Based Carbon Fibers, Nitilaksha Phalaxayya Hiremath
Doctoral Dissertations
There is continuing effort to enhance the strength and modulus of carbon fibers by various combinations of materials and processing. Carbon fibers are produced from various precursors, and the strength of the CFs are directly related to the type of precursor used to make them. Carbon Nanotubes (CNTs) have received a great deal of attention due to their unique structure and properties. Major focus of this research is on the evaluation of processing, structure and properties of CNT based yarns and composite fibers.
High strength and low cost carbon fibers (CFs) are needed for today’s applicatio ns. A low cost …
Nanoscience At Interfaces And Surfaces: From Jamming To Electrode Texturing, Mengmeng Cui
Nanoscience At Interfaces And Surfaces: From Jamming To Electrode Texturing, Mengmeng Cui
Doctoral Dissertations
This dissertation focuses on the nanoparticle self-assembly on the liquid/liquid interface and the nanomaterial modification on surface. The self-assembly of nanoparticles at the liquid/liquid interface was utilized to trap non-equilibrium morphology when the nanoparticles reach jamming state. The dynamics of jammed systems were further studied by X-ray photon correlation spectroscopy. For the surface part, the nanomaterials were modified on the electrodes to improve the performance of microbial electrosynthesis. Also, a novel and simple method was developed to prepare nanomaterials including nanoparticle surfactants and carbon nanotubes (CNTs).