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Articles 1 - 12 of 12
Full-Text Articles in Engineering
Effects Of Feed And Draw Solution Temperature And Transmembrane Temperature Difference On The Rejection Of Trace Organic Contaminants By Forward Osmosis, Ming Xie, William E. Price, Long D. Nghiem, Menachem Elimelech
Effects Of Feed And Draw Solution Temperature And Transmembrane Temperature Difference On The Rejection Of Trace Organic Contaminants By Forward Osmosis, Ming Xie, William E. Price, Long D. Nghiem, Menachem Elimelech
William E. Price
The effects of feed and draw solution temperature and transmembrane temperature difference on the rejection of 12 trace organic contaminants (TrOCs) by two forward osmosis (FO) membranes were investigated. The membrane structure parameter (S) and the reverse salt (NaCl) flux selectivity (RSFS) were constant over the temperature range of 20-40 1C, suggesting that within this range, the solution temperature did not significantly influence the membrane polymeric structure. Draw solution properties, including diffusivity, viscosity, and osmotic pressure, played an important role in water and reverse salt (NaCl) flux behaviour and TrOC rejection. Pure water and salt (NaCl) permeability coefficients of the …
Coupling Granular Activated Carbon Adsorption With Membrane Bioreactor Treatment For Trace Organic Contaminant Removal: Breakthrough Behaviour Of Persistent And Hydrophilic Compounds, Luong N. Nguyen, Faisal I. Hai, William E. Price, Jinguo Kang, Long D. Nghiem
Coupling Granular Activated Carbon Adsorption With Membrane Bioreactor Treatment For Trace Organic Contaminant Removal: Breakthrough Behaviour Of Persistent And Hydrophilic Compounds, Luong N. Nguyen, Faisal I. Hai, William E. Price, Jinguo Kang, Long D. Nghiem
William E. Price
This study investigated the removal of trace organic contaminants by a combined membrane bioreactor - granular activated carbon (MBR-GAC) system over a period of 196 days. Of the 22 compounds investigated here, all six hydrophilic compounds with electron-withdrawing functional groups (i.e., metronidazole, carbamazepine, ketoprofen, naproxen, fenoprop and diclofenac) exhibited very low removal efficiency by MBR-only treatment. GAC post-treatment initially complemented MBR treatment very well; however, a compound-specific gradual deterioration of the removal of the above-mentioned problematic compounds was noted. While a 20% breakthrough of all four negatively charged compounds namely ketoprofen, naproxen, fenoprop and diclofenac occurred within 1000-3000 bed volumes …
Impact Of Chemical Cleaning On The Nanofiltration Of Pharmaceutically Active Compounds (Phacs): The Role Of Cleaning Temperature, Alexander Simon, William E. Price, Long D. Nghiem
Impact Of Chemical Cleaning On The Nanofiltration Of Pharmaceutically Active Compounds (Phacs): The Role Of Cleaning Temperature, Alexander Simon, William E. Price, Long D. Nghiem
William E. Price
This study investigated the impact of chemical cleaning on the physicochemical properties of a nanofiltration membrane and its subsequent separation efficiency of inorganic salts and two pharmaceutically active compounds (PhACs), sulfamethoxazole and carbamazepine. Chemical cleaning was simulated by immersing virgin membrane samples in aqueous citric acid, sodium hydroxide (NaOH), ethylenediaminetetraacetic-acid (EDTA) and sodium dodecyl sulphate (SDS) at various temperatures for 18 h. The cleaning temperature did not exert any discernible impact on the surface charge of the NF270 membrane selected in this study. However, high cleaning temperatures were shown to either amplify or reduce the impact of chemical cleaning on …
Predicting The Fate Of Emerging Trace Organic Contaminants Of Concern During Mbr Treatment Based On Their Molecular Properties, K C. Wijekoon, L D. Nghiem, F I. Hai, J Kang, W E. Price
Predicting The Fate Of Emerging Trace Organic Contaminants Of Concern During Mbr Treatment Based On Their Molecular Properties, K C. Wijekoon, L D. Nghiem, F I. Hai, J Kang, W E. Price
William E. Price
We demonstrate that the fate of emerging trace organic contaminants during membrane bioreactor (MBR) treatment can be qualitatively predicted by assessing their molecular properties. This work futher expands the qualitative framework for the prdiction of trace organic removal by MBR treatment reported in our recent study.
The Fate Of Pharmaceuticals, Steroid Hormones, Phytoestrogens, Uv-Filters And Pesticides During Mbr Treatment, Kaushalya C. Wijekoon, Faisal I. Hai, Jinguo Kang, William E. Price, Wenshan Guo, Hao H. Ngo, Long D. Nghiem
The Fate Of Pharmaceuticals, Steroid Hormones, Phytoestrogens, Uv-Filters And Pesticides During Mbr Treatment, Kaushalya C. Wijekoon, Faisal I. Hai, Jinguo Kang, William E. Price, Wenshan Guo, Hao H. Ngo, Long D. Nghiem
William E. Price
This study examined the relationship between molecular properties and the fate of trace organic contaminants (TrOCs) in the aqueous and solid phases during wastewater treatment by MBR. A set of 29 TrOCs was selected to represent pharmaceuticals, steroid hormones, phytoestrogens, UV-filters and pesticides that occur ubiquitously in municipal wastewater. Both adsorption and biodegradation/transformation were found responsible for the removal of TrOCs by MBR treatment. A connection between biodegradation and molecular structure could be observed while adsorption was the dominant removal mechanism for the hydrophobic (logD > 3.2) compounds. Highly hydrophobic (logD > 3.2) but readily biodegradable compounds did not accumulate in sludge. …
Understanding The Factors Controlling The Removal Of Trace Organic Contaminants By White-Rot Fungi And Their Lignin Modifying Enzymes: A Critical Review, Shufan Yang, Faisal I. Hai, Long D. Nghiem, William E. Price, Felicity Roddick, Maria T. Moreira, Saleh F. Magram
Understanding The Factors Controlling The Removal Of Trace Organic Contaminants By White-Rot Fungi And Their Lignin Modifying Enzymes: A Critical Review, Shufan Yang, Faisal I. Hai, Long D. Nghiem, William E. Price, Felicity Roddick, Maria T. Moreira, Saleh F. Magram
William E. Price
White-rot fungi (WRF) and their lignin modifying enzymes (LME) can degrade a wide range of trace organic contaminants (TrOC), which are suspected to cause adverse health effects in humans and other biota. Recent studies have successfully applied either whole-cell WRF or their extracellular culture extract to remove TrOC from the aqueous phase. TrOC removal by a WRF system is dependent on a range of factors including molecular structure of the TrOC, fungal species and their specific LME, culture medium composition, and methods to enhance fungal degradation capacity; however, the specific relationships between these factors have not been systematically delineated. The …
Removal Of Trace Organic Contaminants By An Mbr Comprising A Mixed Culture Of Bacteria And White-Rot Fungi, Luong N. Nguyen, Faisal I. Hai, Shufan Yang, Jinguo Kang, Frederic D L Leusch, Felicity Roddick, William E. Price, Long D. Nghiem
Removal Of Trace Organic Contaminants By An Mbr Comprising A Mixed Culture Of Bacteria And White-Rot Fungi, Luong N. Nguyen, Faisal I. Hai, Shufan Yang, Jinguo Kang, Frederic D L Leusch, Felicity Roddick, William E. Price, Long D. Nghiem
William E. Price
The degradation of 30 trace organic contaminants (TrOC) by a white-rot fungus-augmented membrane bioreactor (MBR) was investigated. The results show that white-rot fungal enzyme (laccase), coupled with a redox mediator (1-hydroxy benzotriazole, HBT), could degrade TrOC that are resistant to bacterial degradation (e.g. diclofenac, triclosan, naproxen and atrazine) but achieved low removal of compounds (e.g. ibuprofen, gemfibrozil and amitriptyline) that are well removed by conventional activated sludge treatment. Overall, the fungus-augmented MBR showed better TrOC removal compared to a system containing conventional activated sludge. The major role of biodegradation in removal by the MBR was noted. Continuous mediator dosing to …
Effects Of Caustic Cleaning On Pore Size Of Nanofiltration Membranes And Their Rejection Of Trace Organic Chemicals, Alexander Simon, James A. Mcdonald, Stuart J. Khan, William E. Price, Long D. Nghiem
Effects Of Caustic Cleaning On Pore Size Of Nanofiltration Membranes And Their Rejection Of Trace Organic Chemicals, Alexander Simon, James A. Mcdonald, Stuart J. Khan, William E. Price, Long D. Nghiem
William E. Price
The aim of this study was to assess the impact of caustic cleaning on the rejection of three different trace organic chemical (TrOC) groups (i.e. neutral hydrophilic, neutral hydrophobic and negatively charged) by two nanofiltration (NF) membranes ‒ namely NF270 and NF90. Chemical cleaning was simulated by exposing virgin membrane samples to commercial caustic cleaning formulations as well as sodium hydroxide solutions containing analytical grade additives such as sodium dodecyl sulfate or ethylenediaminetetraacetic acid. The membrane average pore size before and after exposure to a commercially available caustic cleaning formulation was determined based on the pore transport model. The results …
Changes In Surface Properties And Separation Efficiency Of A Nanofiltration Membrane After Repeated Fouling And Chemical Cleaning Cycles, Alexander Simon, William E. Price, Long D. Nghiem
Changes In Surface Properties And Separation Efficiency Of A Nanofiltration Membrane After Repeated Fouling And Chemical Cleaning Cycles, Alexander Simon, William E. Price, Long D. Nghiem
William E. Price
The aim of this study was to evaluate the changes in membrane surface properties and solute separation by a nanofiltration membrane during repetitive membrane fouling and chemical cleaning. Secondary treated effluent and model fouling solutions containing humic acids, sodium alginate, or silica colloids were used to simulate membrane fouling. Chemical cleaning was carried out using a commercially available caustic cleaning formulation. Carbamazepine and sulfamethoxazole were selected to examine the filtration behaviour of neutral and negatively charged organic compounds, respectively. Results show that the impact of membrane fouling on solute rejection is governed by pore blocking, modification of the membrane surface …
Comparison Between Sequential And Simultaneous Application Of Activated Carbon With Membrane Bioreactor For Trace Organic Contaminant Removal, Luong N. Nguyen, Faisal I. Hai, Jinguo Kang, Long D. Nghiem, William E. Price, Wenshan Guo, Huu H. Ngo, Kuo-Lun Tung
Comparison Between Sequential And Simultaneous Application Of Activated Carbon With Membrane Bioreactor For Trace Organic Contaminant Removal, Luong N. Nguyen, Faisal I. Hai, Jinguo Kang, Long D. Nghiem, William E. Price, Wenshan Guo, Huu H. Ngo, Kuo-Lun Tung
William E. Price
The removal efficiency of 22 selected trace organic contaminants by sequential application of granular activated carbon (GAC) and simultaneous application of powdered activated carbon (PAC) with membrane bioreactor (MBR) was compared in this study. Both sequential application of GAC following MBR treatment (MBR–GAC) and simultaneous application of PAC within MBR (PAC–MBR) achieved improved removal (over 95%) of seven hydrophilic and biologically persistent compounds, which were less efficiently removed by MBR-only treatment (negligible to 70%). However, gradual breakthrough of these compounds occurred over an extended operation period. Charged compounds, particularly, fenoprop and diclofenac, demonstrated the fastest breakthrough (complete and 50–70%, in …
Removal Of N-Nitrosamines By An Aerobic Membrane Bioreactor, Kaushalya C. Wijekoon, Takahiro Fujioka, James A. Mcdonald, Stuart J. Khan, Faisal I. Hai, William E. Price, Long D. Nghiem
Removal Of N-Nitrosamines By An Aerobic Membrane Bioreactor, Kaushalya C. Wijekoon, Takahiro Fujioka, James A. Mcdonald, Stuart J. Khan, Faisal I. Hai, William E. Price, Long D. Nghiem
William E. Price
This study investigated the fate of eight N-nitrosamines during membrane bioreactor (MBR) treatment. The results suggest that biodegradation is mainly responsible for the removal of N-nitrosamines during MBR treatment. Other removal mechanisms were insignificant (e.g. adsorption to sludge) or not expected (e.g. photolysis and volatilization) given the experimental conditions and physicochemical properties of the N-nitrosamines studied here. N-nitrosamine removal efficiencies were from 24% to 94%, depending on their molecular properties. High removal of N-nitrosamines such as N-nitrosodimethylamine and N-nitrosodiethylamine could be explained by the presence of strong electron donating functional groups (EDG) in their structure. In contrast, N-nitrosomorpholine possessing the …
Influence Of Formulated Chemical Cleaning Reagents On The Surface Properties And Separation Efficiency Of Nanofiltration Membranes, Alexander Simon, William E. Price, Long D. Nghiem
Influence Of Formulated Chemical Cleaning Reagents On The Surface Properties And Separation Efficiency Of Nanofiltration Membranes, Alexander Simon, William E. Price, Long D. Nghiem
William E. Price
This study investigated the impact of two caustic and one acidic cleaning formulations (namely MC11, PC98, and MC3, respectively) on the properties and separation efficiency of three different nanofiltration (NF) membranes (namely NF270, NF90 and TFC-SR100). Overall, the impact of chemical cleaning on surface properties and rejection was membrane and cleaning reagent specific. It was driven mostly by conformational changes of the membrane polymeric active skin layer in response to an extreme caustic or acidic environment and to a certain extent by the adsorption of cleaning additives (e.g., surfactants and chelating reagents). The influence of chemical cleaning on the membrane …