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Potentially Massive And Global Non-Pyrogenic Production Of Condensed "Black" Carbon Through Biomass Oxidation, Aleksandar I. Goranov, Hongmei Chen, Jianshu Duan, Satish C. B. Myneni, Patrick G. Hatcher
Potentially Massive And Global Non-Pyrogenic Production Of Condensed "Black" Carbon Through Biomass Oxidation, Aleksandar I. Goranov, Hongmei Chen, Jianshu Duan, Satish C. B. Myneni, Patrick G. Hatcher
Chemistry & Biochemistry Faculty Publications
With the increased occurrences of wildfires worldwide, there has been an increase in scientific interest surrounding the chemistry of fire-derived "black" carbon (BC). Traditionally, wildfire research has assumed that condensed aromatic carbon (ConAC) is exclusively produced via combustion, and thus, ConAC is equated to BC. However, the lack of correlations between ConAC in soils or rivers and wildfire history suggests that ConAC may be produced non-pyrogenically. Here, we show quantitative evidence that this occurs during the oxidation of biomass with environmentally ubiquitous hydroxyl radicals. Pine wood boards exposed to iron nails and natural weather conditions for 12 years yielded a …
Direct Air Capture: Catalyzing A Carbon Negative Future, Tagg K. Lee
Direct Air Capture: Catalyzing A Carbon Negative Future, Tagg K. Lee
Civil and Environmental Engineering Publications
Direct Air Capture (DAC) technology has emerged as a promising means to address the escalating challenges of atmospheric carbon dioxide (CO2) levels and mitigate climate change. This paper provides an elementary overview of DAC, encompassing its underlying principles, technological advancements, and associated challenges. Point Source Carbon Capture is compared against Direct Air Capture with a solid or liquid sorbent, and physisorbents/chemisorbents are outlined. The past decade has seen a steep rise in the usage of chemical sorbents in particular, which are explored alongside their regeneration processes. This review provides an introductory explanation for the mechanisms of common DAC …
Characterization Of Biochar As A Carbon Regulator In Manure And Environmental Management Applications, Josephine Getz
Characterization Of Biochar As A Carbon Regulator In Manure And Environmental Management Applications, Josephine Getz
Doctoral
Biochar is a product of pyrolysis, which is the thermal decomposition of materials at elevated temperatures (300 - 900 °C) in an oxygen-limited atmosphere. Biochar has been recognized as a potentially vital tool to help reduce the climate change impact. It has been used in the agricultural sector as an addition to reduce greenhouse gas emissions in several animal husbandry settings. The application in the animal sector is an important point to reduce the overall amount of greenhouse gases released as this sector produces many greenhouse gases. Though not in every case a reduction of emissions was the result of …
Interactive Effects Of Hydrology And Fire Drive Differential Biogeochemical Legacies In Subtropical Wetlands, Andrea Nocentini, John S. Kominoski, Jay Sah
Interactive Effects Of Hydrology And Fire Drive Differential Biogeochemical Legacies In Subtropical Wetlands, Andrea Nocentini, John S. Kominoski, Jay Sah
All Faculty
Fire is an important component of many ecosystems, as it impacts biodiversity, biogeochemical cycles, and primary production. In wetlands, fire interacts with hydrologic regimes and other ecosystem characteristics to determine soil carbon (C) gains or losses and rates of nutrient cycling. However, how legacies of fire interact with wetland hydroperiod to affect soil chemistry is uncertain. We used the Florida Everglades as a model landscape to study how fire regimes, hydroperiod, and soil types collectively contribute to long-term C, nitrogen (N), and phosphorus (P) concentrations and stoichiometric mass ratios (C:N, C:P, N:P) in both short- and long-hydroperiod subtropical wetlands that …
Ecosystem-Scale Biogeochemical Fluxes From Three Bioenergy Crop Candidates: How Energy Sorghum Compares To Maize And Miscanthus, Caitlin E. Moore, Adam C. Von Haden, Mark B. Burnham, Ilsa B. Kantola, Christy D. Gibson, Bethany J. Blakely, Evan C. Dracup, Michael D. Masters, Wendy H. Yang, Evan H. Delucia, Carl J. Bernacchi
Ecosystem-Scale Biogeochemical Fluxes From Three Bioenergy Crop Candidates: How Energy Sorghum Compares To Maize And Miscanthus, Caitlin E. Moore, Adam C. Von Haden, Mark B. Burnham, Ilsa B. Kantola, Christy D. Gibson, Bethany J. Blakely, Evan C. Dracup, Michael D. Masters, Wendy H. Yang, Evan H. Delucia, Carl J. Bernacchi
United States Department of Agriculture-Agricultural Research Service / University of Nebraska-Lincoln: Faculty Publications
Perennial crops have been the focus of bioenergy research and development for their sustainability benefits associated with high soil carbon (C) and reduced nitrogen (N) requirements. However, perennial crops mature over several years and their sustainability benefits can be negated through land reversion. A photoperiod-sensitive energy sorghum (Sorghum bicolor) may provide an annual crop alternative more ecologically sustainable than maize (Zea mays) that can more easily integrate into crop rotations than perennials, such as miscanthus (Miscanthus × giganteus). This study presents an ecosystem-scale comparison of C, N, water and energy fluxes from energy sorghum, maize and miscanthus during a typical …
Biofuels From Crop Residue Can Reduce Soil Carbon And Increase Co2 Emissions, Adam J. Liska, Haishun Yang, Maribeth Milner, Steve Goddard, Humberto Blanco-Canqui, Matthew P. Pelton, Xiao X. Fang, Haitao Zhu, Andrew E. Suyker
Biofuels From Crop Residue Can Reduce Soil Carbon And Increase Co2 Emissions, Adam J. Liska, Haishun Yang, Maribeth Milner, Steve Goddard, Humberto Blanco-Canqui, Matthew P. Pelton, Xiao X. Fang, Haitao Zhu, Andrew E. Suyker
Adam Liska Papers
Removal of corn residue for biofuels can decrease soil organic carbon(SOC) and increase CO2 emissions because residue C in biofuels is oxidized to CO2 at a faster rate than when added to soil. Net CO2 emissions from residue removal are not adequately characterized in biofuel life cycle assessment (LCA). Here we used a model to estimate CO2 emissions from corn residue removal across the US Corn Belt at 580 million geospatial cells. To test the SOC model, we compared estimated daily CO2 emissions from corn residue and soil with CO2 emissions measured using eddy covariance, …
Effects Of Activated Carbon Surface Chemistry Modification On The Adsorption Of Mercury From Aqueous Solution, Emily K. Faulconer
Effects Of Activated Carbon Surface Chemistry Modification On The Adsorption Of Mercury From Aqueous Solution, Emily K. Faulconer
Publications
Mercury (Hg), a naturally occurring element, is toxic and can lead to negative health impacts for humans and ecosystems. Activated carbon adsorption is effective in treating Hg-laden aqueous effluent for safe discharge. Two modifications of commercially available activated carbon were investigated: iron impregnation to allow for magnetic sorbent recapture and wet chemical oxidation to enhance aqueous Hg capture. The modified carbons were characterized by nitrogen adsorption-desorption, XRD, pHpzc, vibrating sample magnetometry, elemental analysis, and total acidity titration. The 3:1 C:Fe magnetic powdered activated carbon (MPAC) retained a high surface area of 790 m2 /g and was 95% magnetically recoverable, with …
Litter-Carbon Dynamics: The Importance Of Decomposition, Accretion, And Sequestration In Understanding Ecosystem Carbon Cycling, Amy Kochsiek
School of Biological Sciences: Dissertations, Theses, and Student Research
The atmospheric CO2 concentration has been increasing since the industrial revolution. A proposed mitigation strategy is sequestering carbon (C) in terrestrial ecosystems, either in plant biomass or soil organic matter. The litter-C pool is the second largest C pool in agroecosystems post-harvest, and the amount of litter-C loss has been correlated with ecosystem respiration. Yet, the potential importance of the litter pool as one of the major C pools in a system is relatively unknown. We do, however, know that the size of the litter pool can be affected by increases or decreases in both litter-C production and decomposition, …